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Junhao Lin

Publications and source records attributed to Junhao Lin.

At least 19 recordsLinked to original sources

Odd spin symmetry and anisotropy switching in p-wave magnet CeNiAsO

Odd-parity magnets, complementary to altermagnets, exhibit unique properties such as high efficiency in charge-spin conversion and compatibility with conventional superconductivity, of critical importance in the pursuit of energy-efficient spintronics and topological superconductors for quantum computation. For even-parity d-wave and g-wave altermagnets, the magnetic structure, spin-split band structure and physical properties are currently under intensive study. On the contrary, while hundreds of odd-parity magnets and the promising properties have been predicted in theory, experimental studies are scarce. Specifically, the magnetic structure and transport properties of candidates NiI2 and Ga3Ru4Al12 have been reported, yet the characteristic band structure and particularly the odd-parity spin symmetry remain elusive. Here we demonstrate experimentally the deterministic p-wave spin symmetry and resistance anisotropy switching for the prototype odd-parity magnet, CeNiAsO. Angle-resolved photoemission spectroscopy (ARPES) reveals two cleaved terminations with distinct surface band structure. By compensating the polar surface, we achieve intrinsic bulk band structure, for which the spin splitting can be well described by the p-wave magnetic structure through first-principles calculation. The bulk spin polarization measured by spin-resolved ARPES exhibits symmetry with only one degenerate plane, fingerprint of p-wave magnetism. We further demonstrate giant resistance anisotropy and switching between high-resistance and low-resistance states through modest field-induced domain selection, highlighting its potential for antiferromagnetic spin memory devices. The structural similarity between CeNiAsO and 1111-type Fe-based superconductors stimulates further exploration on the interplay between p-wave magnetism, superconductivity and band topology.

cond-mat.str-el

Discovery of d-orbital order in Tb2CoAl4Ge2

Orbital order describes a quantum state where occupied orbitals line up in a periodic pattern. While orbital physics plays a fundamental and universal role in strongly correlated electron systems, the existence and particularly the band structure fingerprint of orbital order remain a long-standing mystery. Here, we report the discovery of rare earth 5d-orbital order developed by the surface states of intermetallic compound Tb2CoAl4Ge2. Angle-resolved photoemission spectroscopy reveals characteristic nematic features like Fermi surface deformation and band split. These experimental observations can be described by a ferro-orbital order term in the mean-field Hamiltonian. The structural and magnetic origin of such order is excluded by systematic high-resolution neutron powder diffraction and scanning tunnelling microscopy measurements. Our results provide strong evidence for a pure surface orbital order scenario avoiding complications from structural distortion as in colossal magnetoresistance manganites, magnetic order as in iron-based superconductors, and charge transfer p-orbital order in cuprates.

cond-mat.str-el

When the Strongest Teacher Is Not the Best Teacher: Student-Centric Answer Selection

LLM training increasingly relies on teacher-generated supervision, from synthetic responses to reasoning traces and tool-use demonstrations. Current practice often chooses the highest-performing teacher to generate student training data, implicitly treating teacher test performance as a proxy for teaching quality. We show that this assumption can fail: even when multiple teachers provide correct answers to the same question, the answer from the strongest teacher is not necessarily the best supervision for a given student. To address this gap, we propose Student-Centric Answer Sampling (SCAS), a framework that selects from verified teacher-generated answers according to their estimated student-centric learning cost. Motivated by a token-wise gradient decomposition, we derive an efficient forward-only proxy for this cost and use it to guide answer selection during training. Experiments across 30 teacher models, 6 student base models, and 6 tasks show that SCAS consistently improves student performance, suggesting that effective distillation should prioritize supervision matched to the current student rather than teacher strength alone.

cs.LG

Superconductivity and Electronic Structures of Nickelate Thin Film Superstructures

Ruddlesden-Popper (RP) nickelates have emerged as a crucial platform for exploring the mechanisms of high-temperature superconductivity. However, the Fermi surface topology required for superconductivity remains elusive. Here, beyond the superconducting pure bilayer (2222) phase, we report the thin film growth and ambient-pressure superconductivity of monolayer-bilayer (1212) and bilayer-trilayer (2323) superstructures, together with the absence of superconductivity in monolayer-trilayer (1313) superstructure, under identical compressive epitaxial strain. The onset superconducting transition temperatures range from 46 to 50 K, exceeding the McMillan limit. Angle-resolved photoemission spectroscopy reveals key Fermi surface differences in these atomically-engineered structures. In superconducting 1212 and 2222 films, a dispersive hole-like band ($\gamma^{\mathrm{II}}$) forms an underlying Fermi pocket, surrounding the Brillouin zone corner. In contrast, the top of the flat band ($\gamma^{\mathrm{III}}$) is observed ~70 meV below $E_\text{F}$ in the non-superconducting 1313 films. Particularly, the superconducting 2323 films host both $\gamma^{\mathrm{II}}$ and $\gamma^{\mathrm{III}}$ bands. The polarization dependence of the $\gamma$ bands reveals their Ni $d_{z^2}$ origin. Our findings expand the family of ambient-pressure nickelate superconductors and establish a connection between structural configuration, electronic structure, and the emergence of superconductivity in nickelates.

cond-mat.supr-con

Signatures of unconventional superconductivity near reentrant and fractional quantum anomalous Hall insulators

Two-dimensional moir\'e Chern bands provide an exceptional platform for exploring a variety of many-body quantum phases at zero magnetic field within a lattice system. One particular intriguing possibility is that flat Chern bands can, in principle, support exotic superconducting phases together with fractional topological phases. Here, we report the observation of integer and fractional quantum anomalous Hall effects, the reentrant quantum anomalous Hall effect, and superconductivity within the first moir\'e Chern band of twisted bilayer MoTe2. The superconducting phase emerges from a normal state exhibiting anomalous Hall effects. Our results present the first example of superconductivity emerging within a flat Chern band that simultaneously hosts fractional quantum anomalous effects, a phenomenon never observed in any other systems. Our work expands the understanding of emergent quantum phenomena in moir\'e Chern bands, and offers a nearly ideal platform for engineering Majorana and parafermion zero modes in gate-controlled hybrid devices.

cond-mat.mes-hall

Angle-resolved photoemission spectroscopy of superconducting (La,Pr)3Ni2O7/SrLaAlO4 heterostructures

Ruddlesden-Popper bilayer nickelate thin film superconductors discovered under ambient pressure enable vast possibilities for investigating electronic structures of the superconducting state. Here, we report angle-resolved photoemission spectroscopy (ARPES) measurements of 1, 2, and 3 unit-cell epitaxial La2.85Pr0.15Ni2O7 films grown on SrLaAlO4 substates, through pure-oxygen in situ sample transportation. Evidence obtained using photons with distinct probing depths shows that conduction is localized primarily at the first unit cell near the interface. Scanning transmission electron microscopy (STEM), together with energy-dispersive X-ray spectroscopy (EDS) and electron energy loss spectroscopy (EELS), indicates that interfacial Sr diffusion and pronounced p-d hybridization gradient may collectively account for the interfacial confinement of conduction. Fermi surface maps reveal hole doping compared to non-superconducting ambient-pressure bulk crystals. Measurements of dispersive band structures suggest the contributions from both Ni dx2-y2 and dz2 orbitals at the Fermi level. Density functional theory (DFT) + U calculations capture qualitative features of the ARPES results, consistent with a hole-doped scenario. These findings constrain theoretical models of the superconducting mechanism and suggest potential for enhancing superconductivity in nickelates under ambient pressure.

cond-mat.supr-con

Correlated electronic structures and unconventional superconductivity in bilayer nickelate heterostructures

The recent discovery of ambient-pressure superconductivity in thin-film bilayer nickelates opens new possibilities for investigating electronic structures in this new class of high-transition temperature $T_C$ superconductors. Here, we construct a realistic multi-orbital Hubbard model for the thin-film system, by integrating ab initio calculations with scanning transmission electron microscopy (STEM) measurements, which reveal a higher-symmetry lattice. The interaction parameters are calculated with the constrained random phase approximation (cRPA). Density functional theory (DFT) plus cluster dynamical mean-field theory (CDMFT) calculations, with cRPA calculated on-site Coulomb repulsive $U$ and experimentally measured electron filling $n$, quantitatively reproduces Fermi surfaces from angle-resolved photoemission spectroscopy (ARPES) experiments. The distinct Fermi surface topology from simple DFT+$U$ results features the indispensable role of correlation effects. Based upon the correlated electronic structures, A modified random-phase-approximation (RPA) approach yields a pronounced $s^{\pm}$-wave pairing instability, due to the strong spin fluctuations originated from Fermi surface nesting between bands with predominantly $d_{z^{2}}$ characters. Our findings highlight the quantitative effectiveness of the DFT+cRPA+CDMFT approach that precisely determines correlated electronic structure parameters without fine-tuning. The revealed intermediate correlation effect may explain the same order-of-magnitude onset $T_C$ observed both in pressured bulk and strained thin film bilayer nickelates.

cond-mat.str-el

Crystal-symmetry-paired spin-valley locking in a layered room-temperature antiferromagnet

Recent theoretical efforts predicted a type of unconventional antiferromagnet characterized by the crystal symmetry C (rotation or mirror), which connects antiferromagnetic sublattices in real space and simultaneously couples spin and momentum in reciprocal space. This results in a unique C-paired spin-valley locking (SVL) and corresponding novel properties such as piezomagnetism and noncollinear spin current even without spin-orbit coupling. However, the unconventional antiferromagnets reported thus far are not layered materials, limiting their potential in spintronic applications. Additionally, they do not meet the necessary symmetry requirements for nonrelativistic spin current. Here, we report the realization of C-paired SVL in a layered room-temperature antiferromagnetic compound, Rb1-{\delta}V2Te2O. Spin resolved photoemission measurements directly demonstrate the opposite spin splitting between C-paired valleys. Quasi-particle interference patterns reveal the suppression of inter-valley scattering due to the spin selection rules, as a direct consequence of C-paired SVL. All these experiments are well consistent with the results obtained from first-principles calculations. Our observations represent the first realization of layered antiferromagnets with C-paired SVL, enabling both the advantages of layered materials and possible control through crystal symmetry manipulation. These results hold significant promise and broad implications for advancements in magnetism, electronics, and information technology.

cond-mat.str-el

Gigantic-oxidative atomic-layer-by-layer epitaxy for artificially designed complex oxides

In designing material functionalities for transition metal oxides, lattice structure and d-orbital occupancy are key determinants. However, the modulation of these two factors is inherently limited by the need to balance thermodynamic stability, growth kinetics, and stoichiometry precision, particularly for metastable phases. We introduce a methodology, namely the gigantic-oxidative atomic-layer-by-layer epitaxy (GOALL-Epitaxy), enhancing oxidation power 3-4 orders of magnitude beyond conventional pulsed laser deposition (PLD) and oxide molecular beam epitaxy (OMBE), while ensuring atomic-layer-by-layer growth of designed complex structures. Thermodynamic stability is markedly augmented with stronger oxidation at elevated temperatures, whereas growth kinetics is sustained by laser ablation at lower temperatures. We demonstrate the accurate growth of complex nickelates and cuprates, especially an artificially designed structure with alternating single and double NiO2 layers possessing distinct nominal d-orbital occupancy, as a parent of high-temperature superconductor. The GOALL-Epitaxy enables material discovery within the vastly broadened growth parameter space.

cond-mat.str-el

ViDSOD-100: A New Dataset and a Baseline Model for RGB-D Video Salient Object Detection

With the rapid development of depth sensor, more and more RGB-D videos could be obtained. Identifying the foreground in RGB-D videos is a fundamental and important task. However, the existing salient object detection (SOD) works only focus on either static RGB-D images or RGB videos, ignoring the collaborating of RGB-D and video information. In this paper, we first collect a new annotated RGB-D video SOD (ViDSOD-100) dataset, which contains 100 videos within a total of 9,362 frames, acquired from diverse natural scenes. All the frames in each video are manually annotated to a high-quality saliency annotation. Moreover, we propose a new baseline model, named attentive triple-fusion network (ATF-Net), for RGB-D video salient object detection. Our method aggregates the appearance information from an input RGB image, spatio-temporal information from an estimated motion map, and the geometry information from the depth map by devising three modality-specific branches and a multi-modality integration branch. The modality-specific branches extract the representation of different inputs, while the multi-modality integration branch combines the multi-level modality-specific features by introducing the encoder feature aggregation (MEA) modules and decoder feature aggregation (MDA) modules. The experimental findings conducted on both our newly introduced ViDSOD-100 dataset and the well-established DAVSOD dataset highlight the superior performance of the proposed ATF-Net. This performance enhancement is demonstrated both quantitatively and qualitatively, surpassing the capabilities of current state-of-the-art techniques across various domains, including RGB-D saliency detection, video saliency detection, and video object segmentation. Our data and our code are available at github.com/jhl-Det/RGBD_Video_SOD.

cs.CV

On the price of exact truthfulness in incentive-compatible online learning with bandit feedback: A regret lower bound for WSU-UX

In one view of the classical game of prediction with expert advice with binary outcomes, in each round, each expert maintains an adversarially chosen belief and honestly reports this belief. We consider a recently introduced, strategic variant of this problem with selfish (reputation-seeking) experts, where each expert strategically reports in order to maximize their expected future reputation based on their belief. In this work, our goal is to design an algorithm for the selfish experts problem that is incentive-compatible (IC, or \emph{truthful}), meaning each expert's best strategy is to report truthfully, while also ensuring the algorithm enjoys sublinear regret with respect to the expert with the best belief. Freeman et al. (2020) recently studied this problem in the full information and bandit settings and obtained truthful, no-regret algorithms by leveraging prior work on wagering mechanisms. While their results under full information match the minimax rate for the classical ("honest experts") problem, the best-known regret for their bandit algorithm WSU-UX is $O(T^{2/3})$, which does not match the minimax rate for the classical ("honest bandits") setting. It was unclear whether the higher regret was an artifact of their analysis or a limitation of WSU-UX. We show, via explicit construction of loss sequences, that the algorithm suffers a worst-case $\Omega(T^{2/3})$ lower bound. Left open is the possibility that a different IC algorithm obtains $O(\sqrt{T})$ regret. Yet, WSU-UX was a natural choice for such an algorithm owing to the limited design room for IC algorithms in this setting.

cs.LG

Anomalous exchange bias effect in ferromagnetic VI3 flakes

The exchange bias (EB) effect, pivotal in magnetic data storage and sensing devices, has been observed not only in interfacial regions but also in intrinsic ferromagnetic materials. Here, we've uncovered a robust and stable exchange bias effect within the layered van der Waals (vdW) ferromagnet VI3 employing magnetic circular dichroism microscopy. At 10 K, we observed a significant exchange field of approximately 0.1 T, accompanied by random shifts (positive or negative relative to zero magnetic field) after zero-field cooling. Notably, this effect is effectively controllable after field cooling, with shift direction opposing the applied magnetic field. The presence of strong magnetic anisotropic energy within VI3 results in larger coercivity-bound magnetic domains. These domains dictate the neighboring ferromagnetic alignment and induce shifts in the hysteresis loop. Our study not only contributes to comprehending fundamental nanoscale magnetic interactions but also sheds light on emergent phenomena within layered van der Waals magnets.

cond-mat.mtrl-sci

Shifting More Attention to Breast Lesion Segmentation in Ultrasound Videos

Breast lesion segmentation in ultrasound (US) videos is essential for diagnosing and treating axillary lymph node metastasis. However, the lack of a well-established and large-scale ultrasound video dataset with high-quality annotations has posed a persistent challenge for the research community. To overcome this issue, we meticulously curated a US video breast lesion segmentation dataset comprising 572 videos and 34,300 annotated frames, covering a wide range of realistic clinical scenarios. Furthermore, we propose a novel frequency and localization feature aggregation network (FLA-Net) that learns temporal features from the frequency domain and predicts additional lesion location positions to assist with breast lesion segmentation. We also devise a localization-based contrastive loss to reduce the lesion location distance between neighboring video frames within the same video and enlarge the location distances between frames from different ultrasound videos. Our experiments on our annotated dataset and two public video polyp segmentation datasets demonstrate that our proposed FLA-Net achieves state-of-the-art performance in breast lesion segmentation in US videos and video polyp segmentation while significantly reducing time and space complexity. Our model and dataset are available at https://github.com/jhl-Det/FLA-Net.

eess.IV

Ferromagnetic Superconductivity in Two-dimensional Niobium Diselenide

The co-existence of ferromagnetism and superconductivity becomes possible through unconventional pairing in the superconducting state. Such materials are exceedingly rare in solid-state systems but are promising platforms to explore topological phases, such as Majorana bound states. Theoretical investigations date back to the late 1950s, but only a few systems have so far been experimentally identified as potential hosts. Here, we show that atomically-thin niobium diselenide (NbSe$_2$) intercalated with dilute cobalt atoms spontaneously displays ferromagnetism below the superconducting transition temperature ($T_c$). We elucidate the origin of this phase by constructing a magnetic tunnel junction that consists of cobalt and cobalt-doped niobium diselenide (Co-NbSe$_2$) as the two ferromagnetic electrodes, with an ultra-thin boron nitride as the tunnelling barrier. At a temperature well below $T_c$, the tunnelling magnetoresistance shows a bistable state, suggesting a ferromagnetic order in Co-NbSe$_2$. We propose a RKKY exchange coupling mechanism based on the spin-triplet superconducting order parameter to mediate such ferromagnetism. We further perform non-local lateral spin valve measurements to confirm the origin of the ferromagnetism. The observation of Hanle precession signals show spin diffusion length up to micrometres below Tc, demonstrating an intrinsic spin-triplet nature in superconducting NbSe$_2$. Our discovery of superconductivity-mediated ferromagnetism opens the door to an alternative design of ferromagnetic superconductors

cond-mat.supr-con

Intrinsic Magnetic Topological Materials

Topological states of matter possess bulk electronic structures categorized by topological invariants and edge/surface states due to the bulk-boundary correspondence. Topological materials hold great potential in the development of dissipationless spintronics, information storage, and quantum computation, particularly if combined with magnetic order intrinsically or extrinsically. Here, we review the recent progress in the exploration of intrinsic magnetic topological materials, including but not limited to magnetic topological insulators, magnetic topological metals, and magnetic Weyl semimetals. We pay special attention to their characteristic band features such as the gap of topological surface state, gapped Dirac cone induced by magnetization (either bulk or surface), Weyl nodal point/line, and Fermi arc, as well as the exotic transport responses resulting from such band features. We conclude with a brief envision for experimental explorations of new physics or effects by incorporating other orders in intrinsic magnetic topological materials.

cond-mat.mes-hall

On the topological surface states of the intrinsic magnetic topological insulator Mn-Bi-Te family

We review recent progress in the electronic structure study of intrinsic magnetic topological insulators (MnBi$_2$Te$_4$)(Bi$_2$Te$_3$)$_n$ ($n=0,1,2,3$) family. Specifically, we focus on the ubiquitously (nearly) gapless behavior of the topological surface state Dirac cone observed by photoemission spectroscopy, even though a large Dirac gap is expected because of surface ferromagnetic order. The dichotomy between experiment and theory concerning this gap behavior is perhaps the most critical and puzzling question in this frontier. We discuss various proposals accounting for the lack of magnetic effect on the topological surface state Dirac cone, which are mainly categorized into two pictures, magnetic reconfiguration, and topological surface state redistribution. Band engineering towards opening a magnetic gap of topological surface states provides great opportunities to realize quantized topological transport and axion electrodynamics at higher temperatures.

cond-mat.mes-hall

Strain tunability of perpendicular magnetic anisotropy in van der Waals ferromagnets VI3

Layered ferromagnets with high coercivity have special applications in nanoscale memory elements in electronic circuits, such as data storage. Therefore, searching for new hard ferromagnets and effectively tuning or enhancing the coercivity are the hottest topics in layered magnets today. Here, we report a strain tunability of perpendicular magnetic anisotropy in van der Waals (vdW) ferromagnets VI3 using magnetic circular dichroism measurements. For an unstrained flake, the M-H curve shows a rectangular-shaped hysteresis loop with perpendicular magnetic anisotropy and a large coercivity (up to 1.775 T at 10 K). Furthermore, the coercivity can be enhanced to a maximum of 2.6 T at 10 K under a 2.9% in-plane tensile strain. Our DFT calculations show that the magnetic anisotropy energy (MAE) can be dramatically increased after applying an in-plain tensile strain, which contributes to the enhancement of coercivity in the VI3 flake. Meanwhile, the strain tunability on the coercivity of CrI3, with a similar crystal structure, is limited. The main reason is the strong spin-orbital coupling in V3+ in VI6 octahedra in comparison with that in Cr3+. The strain tunability of coercivity in VI3 flakes highlights its potential for integration into vdW heterostructures, paving the way toward nanoscale spintronic devices and applications in the future.

cond-mat.mtrl-sci

Realization of Practical Eightfold Fermions and Fourfold van Hove Singularity in TaCo$_2$Te$_2$

Space groups describing the symmetry of lattice structure allow the emergence of fermionic quasiparticles with various degeneracy in the band structure. Theoretical efforts have predicted many materials hosting fermions with the highest degeneracy, i.e., eightfold fermions, yet lacking experimental realization. Here, we explore the band degeneracies in TaCo$_2$Te$_2$ crystals. Through systematic experimental and theoretical analyses, we establish TaCo$_2$Te$_2$ as a nonsymmorphic crystal with negligible spin-orbit coupling (SOC) and long-range magnetic order. These critical properties guarantee the first realization of practical eightfold fermions and fourfold van Hove singularity, as directly observed by photoemission spectroscopy. TaCo$_2$Te$_2$ serves as a topological quantum critical platform, which can be tuned into various magnetic, topologically trivial, and nontrivial phases by adding strain, magnetic field, or SOC. The latter is demonstrated by our first-principles calculations, which show that enhancing SOC in TaCo$_2$Te$_2$ will promote the experimental observation of bulk hourglass fermions. Our results establish TaCo$_2$Te$_2$ as a unique platform to explore states of matter intertwining magnetism, correlation, symmetry, and band topology.

cond-mat.str-el