arXiv subjects

Junwei Liu

Publications and source records attributed to Junwei Liu.

At least 55 records · Page 3Linked to original sources

arXiv2025

Ferroelastic Altermagnetism

Synergizing altermagnetism and other ferroic orders, such as ferroelectric switchable altermagnetism [Phys. Rev. Lett. 134, 106801 (2025) and ibid. 106802 (2025)], offers an effective route to achieve nonvolatile switching of altermagnetic spin splitting. In this work, by synergizing altermagnetism and ferroelasticity, we propose the concept of ferroelastic altermagnets in which the ferroelastic crystal reorientation can drive multistate nonvolatile switching of the altermagnetic spin splitting via altermagnetoelastic effect. Using monolayers RuF4 and CuF2 as material candidates, we demonstrate 2-state and 3-state altermagnetic spin splitting switching as driven by ferroelastic strain states. Transport calculation shows that multistate spin conductivities can be ferroelastically encoded in an ferroelastic altermagnet, thus suggesting the potential of ferroelastic altermagnetic as nonvolatile nanomechanical spin switches. The proposed concept of ferroelastic altermagnetism enriches the emerging landscape of multiferroic altermagnetism, paving a way towards altermagnetic-based straintronic device applications.

cond-mat.mtrl-sci↗

arXiv2025

Tunable altermagnetism via inter-chain engineering in parallelassembled atomic chains

Altermagnetism has recently drawn considerable attention in three- and twodimensional materials. Here, we extend this concept to quasi-one-dimensional (Q1D) monolayers assembled from single-atomic magnetic chains. Through systematically examining nine types of structures, two stacking orders, and intra-/inter-chain magnetic couplings, we identify four out of thirty promising structural prototypes for hosting altermagnetism, which yields 192 potential monolayer materials. We further confirm eight thermodynamically stable Q1D monolayers via high-throughput calculations. Using symmetry analysis and first-principles calculations, we find that the existence of altermagnetism is determined by the type of inter-chain magnetic coupling and predict three intrinsic altermagnets,$CrBr_3$,$VBr_3$,$MnBr_3$,due to their ferromagnetic inter-chain couplings and five extrinsic ones,$CrF_3$,$CrCl_3$,$CrI_3$,$FeCl_3$and $CoTe_3$, ascribed to their neglectable or antiferromagnetic inter-chain couplings. Moreover, the inter-chain magnetic coupling here is highly tunable by manipulating the inter-chain spacing, leading to experimentally feasible transitions between altermagnetic and nodal-line semiconducting states. In addition, applying external electric fields can further modulate the spin splitting. Our findings establish a highly tunable family of Q1D altermagnets, offering fundamental insights into the intricate relationship between geometry, electronic structure, and magnetism.These discoveries hold significant promises for experimental realization and future spintronic applications.

cond-mat.mtrl-sci↗

arXiv2025

Cryogenic in-memory computing using magnetic topological insulators

Machine learning algorithms have been proven effective for essential quantum computation tasks such as quantum error correction and quantum control. Efficient hardware implementation of these algorithms at cryogenic temperatures is essential. Here, we utilize magnetic topological insulators as memristors (termed magnetic topological memristors) and introduce a cryogenic in-memory computing scheme based on the coexistence of the chiral edge state and the topological surface state. The memristive switching and reading of the giant anomalous Hall effect exhibit high energy efficiency, high stability, and low stochasticity. We achieve high accuracy in a proof-of-concept classification task using four magnetic topological memristors. Furthermore, our algorithm-level and circuit-level simulations of large-scale neural networks demonstrate software-level accuracy and lower energy consumption for image recognition and quantum state preparation compared with existing magnetic memristor and CMOS technologies. Our results not only showcase a new application of chiral edge states but also may inspire further topological quantum physics-based novel computing schemes.

cond-mat.mes-hall↗

arXiv2025

Chemical design of monolayer altermagnets

The crystal-symmetry-paired spin-momentum locking (CSML) arisen from the intrinsic crystal symmetry connecting different magnetic sublattices in altermagnets enables many exotic spintronics properties such as unconventional piezomagnetism and noncollinear spin current. However, the shortage of monolayer altermagnets restricts further exploration of dimensionally confined phenomena and applications of nanostructured devices. Here, we propose general chemical design principles inspired by sublattice symmetry of layered altermagnet V$_2$(Se,Te)$_2$O through symmetry-preserving structural modification and valence-adaptive chemical substitutions. In total, we construct 2600 candidates across four structural frameworks, M$_2$A$_2$B$_{1,0}$ and their Janus derivatives. High-throughput calculations identify 670 potential altermagnets with Néel-ordered ground states, among which 91 ones exhibiting CSML Dirac cones that enable spin-polarized ultra-fast transport. These materials also feature different ground-state magnetic orderings and demonstrate diverse electronic behaviors, ranging from semiconductors, metals, half-metals, to Dirac semimetals. This work not only reveals abundant monolayer altermagnets, but also establishes a rational principle for their design, opening gates for exploration of confined magnetism and spintronics in atomically thin systems.

cond-mat.mtrl-sci↗

arXiv2025

Photoswitchable exceptional points derived from bound states in the continuum

Bound states in the continuum (BICs) and exceptional points (EPs), as two distinct physical singularities represented by complex frequencies in non-Hermitian systems, have garnered significant attention and clear definitions in their respective fields in recent years. They share overlapping applications in areas such as high-sensitivity sensing and laser emission. However, the transition between the two, inspired by these intersections, remains largely unexplored. In this work, we reveal the transition process in a non-Hermitian two-mode system, evolving from one bound singularity to a two-dimensional exceptional ring, where the EP is the coalescent state of the quasi-Friedrich-Wintgen (FW)-BIC. This phenomenon is experimentally validated through pored dielectric metasurfaces in terahertz band. Furthermore, external pumping induced photocarriers as the dissipative perturbation, facilitates the breaking of degeneracy in the complex eigenfrequency and enables dynamic EP switching. Finally, we experimentally demonstrate a switchable terahertz beam deflection driven by the phase singularities of the EP. These findings are instrumental in advancing the development of compact devices for sensing and wavefront control within non-Hermitian systems.

physics.optics↗

arXiv2025

Discovery of a large magnetic nonlinear Hall effect in an altermagnet

Since Edwin Halls groundbreaking discovery of the Hall effect in 1879, magnetism, spin, and quantization have been expanding the scope of Hall effects, continuously driving transformative progress in science and technology. Among them, the latest nonlinear Hall effect (NLHE), where longitudinal electric field tunes quantum geometry to generate nonlinear Hall voltage, attracts wide attention as a sensitive probe of topological phases across a wide range of materials. Here, we report a new Hall effect member: the magnetic nonlinear Hall effect (MNLHE), characterized by a quadratic Hall conductivity dependence on magnetic field, rather than electric field as in NLHE. This finding relies on an altermagnet, Mn5Si3 thin film, whose alternating-sign Berry curvatures ensure higher-order MNLHE clearly distinguishable from the first-order anomalous Hall effect. The observed quadratic dependence originates from chiral next-nearest-neighbor hopping processes that acquire magnetic-exchange-driven Zeeman energies and Haldane-like chiral flux phases. Remarkably, this MNLHE is non-analytic, as reversing the magnetic field flips the alternating spin-splitting bands and reverses the hopping chirality, which is absent in traditional NLHE. Beyond offering a distinctive transport fingerprint for altermagnet Mn5Si3 thin film, this MNLHE is large and unsaturated up to 60 T, providing opportunities for pulsed high-field sensing technologies in both fundamental researches and engineering applications.

cond-mat.mtrl-sci↗

arXiv2025

Catalogue of $C$-paired spin-momentum locking in antiferromagnetic systems

Antiferromagnetic materials (AFMs) have been gaining lots of attentions due to its great potential in spintronics devices and the recently discovered novel spin structure in the momentum space, i.e., $C$-paired spin-valley or spin-momentum locking (CSVL/CSML), where spins and valleys/momenta are locked to each other due to the crystal symmetry guaranteeing zero magnetization. Here, we systematically studied CSMLs and proposed a general theory and algorithm using little co-group and coset representatives, which reveals that 12 elementary kinds of CSMLs, determined by the geometric relation of spins and valleys and the essential symmetry guaranteeing zero magnetization, are sufficient to fully represent all possible CSMLs. By combining the proposed algorithm and high-throughput first-principles calculations, we predicted 38 magnetic point groups and identified 142 experimentally verified AFMs that can realize CSML. Besides predicting new materials, our theory can naturally reveal underlying mechanisms of CSMLs' responses to external fields. As an example, two qualitatively different types of piezomagnetism via occupation imbalance or spin tilting were predicted in RbV$_2$Te$_2$O. The algorithm and conclusions can be directly extended to the locking between valley/momentum and any other pseudo-vector degree of freedom, e.g., Berry curvature, as exemplified in RbV$_2$Te$_2$O and the new proposed piezo-Hall effect, where a strain can induce a non-zero anomalous Hall conductance. In addition, the proposed concept and methodology can be straightforwardly applied to other symmetry groups, such as spin group.

cond-mat.mtrl-sci↗

arXiv2025

Room temperature observation of the anomalous in-plane Hall effect in epitaxial thin films of a Weyl ferromagnet

Topologically nontrivial electronic states can give rise to novel anomalous Hall effects. The potential appearance of these effects at room temperature holds promise for their application in magnetic sensing, spintronics, and energy harvesting technology. The anomalous in-plane Hall effect (IPHE) is predicted to arise in topological magnetic materials when an external magnetic field is applied within the sample plane. Because of stringent symmetry requirements, the conclusive detection of the anomalous IPHE induced by topological electronic states remains challenging, and the study of anomalous Hall effects is often confined to cryogenic conditions. Combining molecular beam epitaxy of the kagome metal Fe$_3$Sn with measurements of the electric Hall effect and theoretical calculations, we propose and experimentally demonstrate that the interplay of the kagome lattice motif with spin-orbit coupling and canted ferromagnetism with large exchange interactions gives rise to the anomalous IPHE at room temperature that is induced by topological Weyl points in the electronic band structure. Synthesizing a topological heterostructure including layers of Fe$_3$Sn and ferromagnetic CoFeB, we further show the enhancement of the anomalous IPHE through the magnetic stray field of the CoFeB layer. Our work establishes a design paradigm for topological magnets and heterostructures to discover and control novel anomalous Hall effects toward their use in technological applications.

cond-mat.mes-hall↗

arXiv2024

Global Estimation of Building-Integrated Facade and Rooftop Photovoltaic Potential by Integrating 3D Building Footprint and Spatio-Temporal Datasets

This research tackles the challenges of estimating Building-Integrated Photovoltaics (BIPV) potential across various temporal and spatial scales, accounting for different geographical climates and urban morphology. We introduce a holistic methodology for evaluating BIPV potential, integrating 3D building footprint models with diverse meteorological data sources to account for dynamic shadow effects. The approach enables the assessment of PV potential on facades and rooftops at different levels-individual buildings, urban blocks, and cities globally. Through an analysis of 120 typical cities, we highlight the importance of 3D building forms, cityscape morphology, and geographic positioning in measuring BIPV potential at various levels. In particular, our simulation study reveals that among cities with optimal facade PV performance, the average ratio of facade PV potential to rooftop PV potential is approximately 68.2%. Additionally, approximately 17.5% of the analyzed samples demonstrate even higher facade PV potentials compared to rooftop installations. This finding underscores the strategic value of incorporating facade PV applications into urban sustainable energy systems.

cs.IR↗

arXiv2024

Ubiquitous van der Waals altermagnetism with sliding/moire ferroelectricity

According to the recent studies on sliding/moire ferroelectricity, most 2D van der Waals nonferroelectric monolayers can become ferroelectric via multilayer stacking. In this paper we propose that similar strategy can be used to induce desirable van der Waals altermagnetism with symmetry-compensated collinear magnetic orders and non-relativistic spin splitting. Our first-principles calculations show the pervasive co-existence of sliding ferroelectricity and altermagnetism in a series of magnetic multilayers with anti-parallel stacking configurations. Upon a twist angle in bilayers, moire ferroelectricity can be combined with altermagnetism, while some untwisted bilayers exhibit pseudo-altermagnetism with zero net magnetizations and non-relativistic spin splittings coupled with sliding ferroelectricity. Our study significantly expands the scope of altermagnetism, and its combination with sliding/moire ferroelectricity brings in new physics as well as promising applications, which should stimulate further experimental efforts.

cond-mat.mtrl-sci↗

arXiv2024

Large-scale simulations of vortex Majorana zero modes in topological crystalline insulators

Topological crystalline insulators are known to support multiple Majorana zero modes (MZMs) at a single vortex, their hybridization is forbidden by a magnetic mirror symmetry $M_T$. Due to the limited energy resolution of scanning tunneling microscopes and the very small energy spacing of trivial bound states, it remains challenging to directly probe and demonstrate the existence of multiple MZMs. In this work, we propose to demonstrate the existence of MZMs by studying the hybridization of multiple MZMs in a symmetry breaking field. The different responses of trivial bound states and MZMs can be inferred from their spatial distribution in the vortex. However, the theoretical simulations are very demanding since it requires an extremely large system in real space. By utilizing the kernel polynomial method, we can efficiently simulate large lattices with over $10^8$ orbitals to compute the local density of states which bridges the gap between theoretical studies based on minimal models and experimental measurements. We show that the spatial distribution of MZMs and trivial vortex bound states indeed differs drastically in tilted magnetic fields. The zero-bias peak elongates when the magnetic field preserves $M_T$, while it splits when $M_T$ is broken, giving rise to an anisotropic magnetic response. Since the bulk of SnTe are metallic, we also study the robustness of MZMs against the bulk states, and clarify when can the MZMs produce a pronounced anisotropic magnetic response.

cond-mat.supr-con↗

arXiv2024

All-Electrical Layer-Spintronics in Altermagnetic Bilayer

Electrical manipulation of spin-polarized current is highly desirable yet tremendously challenging in developing ultracompact spintronic device technology. Here we propose a scheme to realize the all-electrical manipulation of spin-polarized current in an altermagnetic bilayer. Such a bilayer system can host layer-spin locking, in which one layer hosts a spin-polarized current while the other layer hosts a current with opposite spin polarization. An out-of-plane electric field breaks the layer degeneracy, leading to a gate-tunable spin-polarized current whose polarization can be fully reversed upon flipping the polarity of the electric field. Using first-principles calculations, we show that CrS bilayer with C-type antiferromagnetic exchange interaction exhibits a hidden layer-spin locking mechanism that enables the spin polarization of the transport current to be electrically manipulated via the layer degree of freedom. We demonstrate that sign-reversible spin polarization as high as 87% can be achieved at room temperature. This work presents the pioneering concept of layer-spintronics which synergizes altermagnetism and bilayer stacking to achieve efficient electrical control of spin.

cond-mat.mes-hall↗

arXiv2024

Robust Coulomb Gap and Varied-temperature Study of Epitaxial 1T'-WSe$_2$ Monolayers

The transition metal dichalcogenides (TMDCs) with a 1T' structural phase are predicted to be two-dimensional topological insulators at zero temperature. Although the quantized edge conductance of 1T'-WTe$_2$ has been confirmed to survive up to 100 K, this temperature is still relatively low for industrial applications. Addressing the limited studies on temperature effects in 1T'-TMDCs, our research focuses on the electronic and crystal properties of the epitaxial 1T'-WSe$_2$ monolayers grown on bilayer graphene (BLG) and SrTiO$_3$(100) substrates at various temperatures. For the 1T'-WSe$_2$ grown on BLG, we observed a significant thermal expansion effect on its band structures with a thermal expansion coefficient of $\sim$60$\times$10$^{-6}$ K$^{-1}$. In contrast, the 1T'-WSe$_2$ grown on SrTiO$_3$(100) exhibits minimal changes with varied temperatures due to the enhanced strain exerted by the substrate. Besides, A significant Coulomb gap (CG) was observed pinned at the Fermi level in the angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling spectroscopy (STS). The CG was founded to decrease with increasing temperatures, and can persist up to 200 K for 1T'-WSe$_2$/BLG, consistent with our Monte Carlo simulations. The robustness of the CG and the positive fundamental gap endow the epitaxial 1T'-WSe$_2$ monolayers with huge potential for realizing the quantum spin Hall devices.

cond-mat.mes-hall↗

arXiv2024

Light-induced percolative topological phase transition in type-II Weyl semimetal WTe2

We report on an ultrafast terahertz free-carrier dynamic study of a photo-excited WTe2 thin film. In the photo-excited state, we observe a metastable electronic state featuring negative differential terahertz photoconductivity and reduced scattering rate. Detailed electrodynamics analysis and first-principal calculation attribute it to light-induced topological phase transition, reducing density of states near the Fermi level. Furthermore, the emergence of an unconventional temporal isosbestic point marks a dynamic universality, strongly suggesting a percolative interaction between the two topologically distinct phases.

cond-mat.mtrl-sci↗

arXiv2024

Crystal-symmetry-paired spin-valley locking in a layered room-temperature antiferromagnet

Recent theoretical efforts predicted a type of unconventional antiferromagnet characterized by the crystal symmetry C (rotation or mirror), which connects antiferromagnetic sublattices in real space and simultaneously couples spin and momentum in reciprocal space. This results in a unique C-paired spin-valley locking (SVL) and corresponding novel properties such as piezomagnetism and noncollinear spin current even without spin-orbit coupling. However, the unconventional antiferromagnets reported thus far are not layered materials, limiting their potential in spintronic applications. Additionally, they do not meet the necessary symmetry requirements for nonrelativistic spin current. Here, we report the realization of C-paired SVL in a layered room-temperature antiferromagnetic compound, Rb1-δV2Te2O. Spin resolved photoemission measurements directly demonstrate the opposite spin splitting between C-paired valleys. Quasi-particle interference patterns reveal the suppression of inter-valley scattering due to the spin selection rules, as a direct consequence of C-paired SVL. All these experiments are well consistent with the results obtained from first-principles calculations. Our observations represent the first realization of layered antiferromagnets with C-paired SVL, enabling both the advantages of layered materials and possible control through crystal symmetry manipulation. These results hold significant promise and broad implications for advancements in magnetism, electronics, and information technology.

cond-mat.str-el↗

arXiv2024

Observation of surface Fermi arcs in altermagnetic Weyl semimetal CrSb

As a special type of collinear antiferromagnetism (AFM), altermagnetism has garnered significant research interest recently. Altermagnets exhibit broken parity-time symmetry and zero net magnetization in real space, leading to substantial band splitting in momentum space even in the absence of spin-orbit coupling. Meanwhile, parity-time symmetry breaking always induce nontrivial band topology such as Weyl nodes. While Weyl semimetal states and nodal lines have been theoretically proposed in altermagnets, rare reports of experimental observation have been made up to this point. Using ARPES and first-principles calculations, we systematically studied the electronic structure of the room-temperature altermagnet candidate CrSb. At generic locations in momentum space, we clearly observed band spin splitting. Furthermore, we identified discrete surface Fermi arcs on the (100) cleaved side surface close to the Fermi level originating from bulk band topology. Our results imply that CrSb contains interesting nontrivial topological Weyl physics, in addition to being an excellent room temperature altermagnet.

cond-mat.mtrl-sci↗

arXiv2024

A Refer-and-Ground Multimodal Large Language Model for Biomedicine

With the rapid development of multimodal large language models (MLLMs), especially their capabilities in visual chat through refer and ground functionalities, their significance is increasingly recognized. However, the biomedical field currently exhibits a substantial gap in this area, primarily due to the absence of a dedicated refer and ground dataset for biomedical images. To address this challenge, we devised the Med-GRIT-270k dataset. It comprises 270k question-and-answer pairs and spans eight distinct medical imaging modalities. Most importantly, it is the first dedicated to the biomedical domain and integrating refer and ground conversations. The key idea is to sample large-scale biomedical image-mask pairs from medical segmentation datasets and generate instruction datasets from text using chatGPT. Additionally, we introduce a Refer-and-Ground Multimodal Large Language Model for Biomedicine (BiRD) by using this dataset and multi-task instruction learning. Extensive experiments have corroborated the efficacy of the Med-GRIT-270k dataset and the multi-modal, fine-grained interactive capabilities of the BiRD model. This holds significant reference value for the exploration and development of intelligent biomedical assistants.

cs.CV↗

arXiv2024

STALL+: Boosting LLM-based Repository-level Code Completion with Static Analysis

Repository-level code completion is challenging as it involves complicated contexts from multiple files in the repository. To date, researchers have proposed two technical categories to enhance LLM-based repository-level code completion, i.e., retrieval-augmented generation (RAG) and static analysis integration. This work performs the first study on the static analysis integration in LLM-based repository-level code completion by investigating both the effectiveness and efficiency of static analysis integration strategies across different phases of code completion. We first implement a framework STALL+, which supports an extendable and customizable integration of multiple static analysis strategies into the complete pipeline of LLM-based repository-level code completion; and based on STALL+, we perform extensive experiments by including different code LLMs on the latest repository-level code completion benchmark CrossCodeEval. Our findings show that integrating file-level dependencies in prompting phase performs the best while the integration in post-processing phase performs the worse. Additionally, we observe different improvements from static analysis between dynamic languages and static languages, i.e., the best combination is prompting-phase with decoding-phase integration for Java while the best combination is prompting-phase with post-processing-phase integration for Python given the limitations of statically analyzing dynamic languages. Additionally, we find the complementarity between RAG and static analysis integration as well as their cost-effectiveness after combination.

cs.SE↗