arXiv subjects

Justin M. Shaw

Publications and source records attributed to Justin M. Shaw.

At least 19 recordsLinked to original sources

arXiv2025

How to Measure and Model Light-Induced Spin Transfer

Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To date, ultrafast spin transfer has predominantly been explained in terms of the initial and final states available for laser excitation. Here, by comparing the measured and calculated dynamics across the entire $M$-edges of two very similar Heusler compounds, $Co_2MnGa$ and $Co_2MnGe$ as well as a sample of elemental Co, we find that simply accounting for the initial and final electron states available for laser excitation cannot alone explain the experimental observations. The influence of spin lifetimes must also be included, due to the shifting of the Fermi level upon replacing Ga with Ge, or the presence of crystalline disorder. This explains why the ordered $L2_1$ phase of $Co_2MnGa$ demonstrates strong laser-induced magnetic signal enhancements across the entire Co-edge, while similar enhancements were not observed in partially disordered $Co_2MnGe$. Although intra-site spin-transfers were expected in the minority channel in pure Co due to the presence of many more available states in the minority channel above the Fermi level, no such signal was observed due to very short few-femtosecond spin lifetimes in a metal. Finally, we identify key regions in the magnetic asymmetry where a transiently enhanced signal could be misinterpreted as a light-induced spin-transfer signature.

cond-mat.mtrl-sci↗

arXiv2024

Uncovering the Timescales of Spin Reorientation in $TbMn_{6}Sn_{6}$

Kagome ferrimagnets are of fundamental interest because of their tunable magnetic, electronic and topological properties, with potential applications for quantum-enabled technologies and spintronics. Here we present the first direct measurement of the intrinsic timescale of the spin reorientation transition in the Kagome ferrimagnet $TbMn_{6}Sn_{6}$. This material exhibits a magnetic phase transition near room temperature, where spins remain collinear while the total magnetic moment rotates from out-of-plane to in-plane. This reorientation has been attributed to the competing anisotropies of Tb and Mn, whose magnetic moments have very different temperature dependencies. By probing at the Mn M-edge using high harmonic extreme ultraviolet pulses, we measure reorientation timescales between 6 and 18 ps, depending on the laser excitation fluence. Our model of the magnetization dynamics shows that this timescale is consistent with a spin reorientation driven by very large anisotropy energies, on meV energy scales. Our model also predicts a possibility of a 180$^{\circ}$ reorientation of the out-of-plane moment, that could facilitate optically controlled magnetization switching between very stable ground states, for applications in spintronics or data storage.

cond-mat.mtrl-sci↗

arXiv2024

Element-specific and high-bandwidth ferromagnetic resonance spectroscopy with a coherent, extreme ultraviolet (EUV) source

We applied a tabletop, ultrafast, high-harmonic generation (HHG) source to measure the element-specific ferromagnetic resonance (FMR) in ultra-thin magnetic alloys and multilayers on an opaque Si substrate. We demonstrate a continuous wave bandwidth of 62 GHz, with promise to extend to 100 GHz or higher. This laboratory-scale instrument detects the FMR using ultrafast, extreme ultraviolet (EUV) light, with photon energies spanning the M-edges of most relevant magnetic elements. An RF frequency comb generator is used to produce a microwave excitation that is intrinsically synchronized to the EUV pulses with a timing jitter of 1.1 ps or better. We apply this system to measure the dynamics in a multilayer system as well as Ni-Fe and Co-Fe alloys. Since this instrument operates in reflection-mode, it is a milestone toward measuring and imaging the dynamics of the magnetic state and spin transport of active devices on arbitrary and opaque substrates. The higher bandwidth also enables measurements of materials with high magnetic anisotropy, as well as ferrimagnets, antiferromagnets, and short-wavelength (high wavevector) spinwaves in nanostructures or nanodevices. Furthermore, the coherence and short wavelength of the EUV will enable extending these studies using dynamic nanoscale lensless imaging techniques such as coherent diffractive imaging, ptychography, and holography.

cond-mat.mtrl-sci↗

arXiv2023

Evidence of extreme domain wall speeds under ultrafast optical excitation

Time-resolved ultrafast EUV magnetic scattering was used to test a recent prediction of >10 km/s domain wall speeds by optically exciting a magnetic sample with a nanoscale labyrinthine domain pattern. Ultrafast distortion of the diffraction pattern was observed at markedly different timescales compared to the magnetization quenching. The diffraction pattern distortion shows a threshold-dependence with laser fluence, not seen for magnetization quenching, consistent with a picture of domain wall motion with pinning sites. Supported by simulations, we show that a speed of $\approx$ 66 km/s for highly curved domain walls can explain the experimental data. While our data agree with the prediction of extreme, non-equilibrium wall speeds locally, it differs from the details of the theory, suggesting that additional mechanisms are required to fully understand these effects.

cond-mat.mes-hall↗

arXiv2022

Brillouin Light Scattering from Quantized Spin Waves in Nanowires with Antisymmetric Exchange Interactions

Antisymmetric exchange interactions lead to non-reciprocal spin-wave propagation. As a result, spin waves confined in a nanostructure are not standing waves; they have a time-dependent phase, because counter-propagating waves of the same frequency have different wavelengths. We report on a Brillouin light scattering (BLS) study of confined spin waves in Co/Pt nanowires with strong Dzyaloshinskii-Moriya interactions (DMI). Spin-wave quantization in narrow ($\lesssim 200$ nm width) wires dramatically reduces the frequency shift between BLS Stokes and anti-Stokes lines associated with the scattering of light incident transverse to the nanowires. In contrast, the BLS frequency shift associated with the scattering of spin waves propagating along the nanowire length is independent of nanowire width. A model that considers the chiral nature of modes captures this physics and predicts a dramatic reduction in frequency shift of light scattered from higher energy spin waves in narrow wires, which is confirmed by our experiments.

cond-mat.mes-hall↗

arXiv2022

Ultrafast perturbation of magnetic domains by optical pumping in a ferromagnetic multilayer

Ultrafast optical pumping of spatially nonuniform magnetic textures is known to induce far-from-equilibrium spin transport effects. Here, we use ultrafast x-ray diffraction with unprecedented dynamic range to study the laser-induced dynamics of labyrinth domain networks in ferromagnetic CoFe/Ni multilayers. We detected azimuthally isotropic, odd order, magnetic diffraction rings up to 5th order. The amplitudes of all three diffraction rings quench to different degrees within 1.6 ps. In addition, all three of the detected diffraction rings both broaden by 15% and radially contract by 6% during the quench process. We are able to rigorously quantify a 31% ultrafast broadening of the domain walls via Fourier analysis of the order-dependent quenching of the three detected diffraction rings. The broadening of the diffraction rings is interpreted as a reduction in the domain coherence length, but the shift in the ring radius, while unambiguous in its occurrence, remains unexplained. In particular, we demonstrate that a radial shift explained by domain wall broadening can be ruled out. With the unprecedented dynamic range of our data, our results provide convincing evidence that labyrinth domain structures are spatially perturbed at ultrafast speeds under far-from-equilibrium conditions, albeit the mechanism inducing the perturbations remains yet to be clarified.

cond-mat.mes-hall↗

arXiv2022

Engineering of Heterostructure Pt/Co/AlOx for the enhancement of Dyzaloshinskii-Moria interaction

The interfacial Dyzaloshinskii-Moria interaction (DMI) helps to stabilize chiral domain walls and magnetic skyrmions, which will facilitate new magnetic memories and spintronics logic devices. The study of interfacial DMI in perpendicularly magnetized structurally asymmetric heavy metal (HM) / ferromagnetic (FM) multilayer systems is of high importance due to the formation of chiral magnetic textures in the presence of DMI. Here, we report the impact of the cobalt oxidation at the cobalt -aluminum oxide interface in Pt/Co/AlOx trilayer structure on the DMI by varying the post-growth annealing time and Aluminum thickness. For quantifying DMI, we employed magneto-optical imaging of asymmetric domain wall expansion, hysteresis loop shift, and spin-wave spectroscopy techniques. We further correlated the Cobalt oxidation with low-temperature Hall effect measurements and X-ray photoelectron spectroscopy. Our results emphasize the characterization of magnetic films for MRAM technologies semiconductor temperature process window, where magnetic interaction will be critical for device performance.

cond-mat.mtrl-sci↗

arXiv2022

Tuning of the Dzyaloshinskii-Moriya Interaction by He$^+$ ion irradiation

We studied the impact of He$^+$ irradiation on the Dzyaloshinskii-Moriya interaction (DMI) in Ta/Co20Fe60B20/Pt/MgO samples. We found that irradiation with of 40 keV He$^+$ ions increases DMI by approximately 20% for fluences up to 2$\cdot$10$\rm{^{16}}$ $\rm{ions/cm}^2$ before it decreases for higher fluence values. In contrast, the interfacial anisotropy shows a distinctly different fluence dependence. To better understand the impact of the ion irradiation on the Ta and Pt interfaces with the Co20Fe60B20 layer, we carried out Monte-Carlo simulations, which showed an expected increase of disorder at the interfaces. A moderate increase in disorder can increase the total number of triplets for the three-site exchange mechanism and can consequently increase the DMI. Our results demonstrate that the DMI can be locally engineered at the nanometer scale, providing a highly promising approach to advance skyrmion-based memories.

cond-mat.mtrl-sci↗

arXiv2022

Simultaneous measurement of the exchange parameter and saturation magnetization using propagating spin waves

The exchange interaction in ferromagnetic ultra-thin films is a critical parameter in magnetization-based storage and logic devices, yet the accurate measurement of it remains a challenge. While a variety of approaches are currently used to determine the exchange parameter, each has its limitations, and good agreement among them has not been achieved. To date, neutron scattering, magnetometry, Brillouin light scattering, spin-torque ferromagnetic resonance spectroscopy, and Kerr microscopy have all been used to determine the exchange parameter. Here we present a novel method that exploits the wavevector selectivity of Brillouin light scattering to measure the spin wave dispersion in both the backward volume and Damon-Eshbach orientations. The exchange, saturation magnetization, and magnetic thickness are then determined by a simultaneous fit of both dispersion branches with general spin wave theory without any prior knowledge of the thickness of a magnetic "dead layer". In this work, we demonstrate the strength of this technique for ultrathin metallic films, typical of those commonly used in industrial applications for magnetic random-access memory.

cond-mat.mtrl-sci↗

arXiv2022

Megahertz-rate Ultrafast X-ray Scattering and Holographic Imaging at the European XFEL

The advent of X-ray free-electron lasers (XFELs) has revolutionized fundamental science, from atomic to condensed matter physics, from chemistry to biology, giving researchers access to X-rays with unprecedented brightness, coherence, and pulse duration. All XFEL facilities built until recently provided X-ray pulses at a relatively low repetition rate, with limited data statistics. Here, we present the results from the first megahertz repetition rate X-ray scattering experiments at the Spectroscopy and Coherent Scattering (SCS) instrument of the European XFEL. We illustrate the experimental capabilities that the SCS instrument offers, resulting from the operation at MHz repetition rates and the availability of the novel DSSC 2D imaging detector. Time-resolved magnetic X-ray scattering and holographic imaging experiments in solid state samples were chosen as representative, providing an ideal test-bed for operation at megahertz rates. Our results are relevant and applicable to any other non-destructive XFEL experiments in the soft X-ray range.

cond-mat.mes-hall↗

arXiv2021

Symmetry-dependent ultrafast manipulation of nanoscale magnetic domains

Symmetry is a powerful concept in physics, but its applicability to far-from-equilibrium states is still being understood. Recent attention has focused on how far-from-equilibrium states lead to spontaneous symmetry breaking. Conversely, ultrafast optical pumping can be used to drastically change the energy landscape and quench the magnetic order parameter in magnetic systems. Here, we find a distinct symmetry-dependent ultrafast behaviour by use of ultrafast x-ray scattering from magnetic patterns with varying degrees of isotropic and anisotropic symmetry. After pumping with an optical laser, the scattered intensity reveals a radial shift exclusive to the isotropic component and exhibits a faster recovery time from quenching for the anisotropic component. These features arise even when both symmetry components are concurrently measured, suggesting a correspondence between the excitation and the magnetic order symmetry. Our results underline the importance of symmetry as a critical variable to manipulate the magnetic order in the ultrafast regime.

cond-mat.mes-hall↗

arXiv2021

Skyrmions in synthetic antiferromagnets and their nucleation via electrical current and ultrafast laser illumination

Magnetic skyrmions are topological spin textures that hold great promise as nanoscale information carriers in non-volatile memory and logic devices. While room-temperature magnetic skyrmions and their current-induced manipulation were recently demonstrated, the stray field resulting from their finite magnetization as well as their topological charge limit their minimum size and reliable motion in tracks. Antiferromagnetic (AF) skyrmions allow these limitations to be lifted owing to their vanishing magnetization and net zero topological charge, promising room-temperature, ultrasmall skyrmions, fast dynamics, and insensitivity to external magnetic fields. While room-temperature AF spin textures have been recently demonstrated, the observation and controlled nucleation of AF skyrmions operable at room temperature in industry-compatible synthetic antiferromagnetic (SAF) material systems is still lacking. Here we demonstrate that isolated skyrmions can be stabilized at zero field and room temperature in a fully compensated SAF. Using X-ray microscopy techniques, we are able to observe the skyrmions in the different SAF layers and demonstrate their antiparallel alignment. The results are substantiated by micromagnetic simulations and analytical models using experimental parameters, which confirm the chiral SAF skyrmion spin texture and allow the identification of the physical mechanisms that control the SAF skyrmion size and stability. We also demonstrate the local nucleation of SAF skyrmions via local current injection as well as ultrafast laser excitations at zero field. These results will enable the utilization of SAF skyrmions in skyrmion-based devices.

cond-mat.mtrl-sci↗

arXiv2021

Strong coupling of Fe-Co alloy with ultralow damping to superconducting co-planar waveguide resonators

We report on the strong coupling between a metallic ferromagnetic Fe75Co25 thin film patterned element and a range of superconducting Nb half-wavelength co-planar waveguide (CPW) resonators. By varying the volume of the ferromagnet we demonstrate that the coupling rate scales linearly with the square root of the number of spins and achieve a coupling rate over 700 MHz, approaching the ultrastrong coupling regime. Experiments varying the center conductor width while maintaining constant magnetic volume verify that decreasing the center conductor width increases coupling and cooperativity. Our results show that the frequency dependence of the coupling rate is linear with the fundamental and higher order odd harmonics of the CPW, but with differing efficiencies. The results show promise for scaling planar superconducting resonator/magnetic hybrid systems to smaller dimensions.

cond-mat.other↗

arXiv2020

Nonlinear losses in magnon transport due to four-magnon scattering

We report on the impact of nonlinear four-magnon scattering on magnon transport in microstructured Co25Fe75 waveguides with low magnetic damping. We determine the magnon propagation length with microfocused Brillouin light scattering over a broad range of excitation powers and detect a decrease of the attenuation length at high powers. This is consistent with the onset of nonlinear four-magnon scattering. Hence, it is critical to stay in the linear regime, when deriving damping parameters from the magnon propagation length. Otherwise, the intrinsic nonlinearity of magnetization dynamics may lead to a misinterpretation of magnon propagation lengths and, thus, to incorrect values of the magnetic damping of the system.

cond-mat.mtrl-sci↗

arXiv2019

High Spin-Wave Propagation Length Consistent with Low Damping in a Metallic Ferromagnet

We report ultra-low intrinsic magnetic damping in Co$_{\text{25}}$Fe$_{\text{75}}$ heterostructures, reaching the low $10^{-4}$ regime at room temperature. By using a broadband ferromagnetic resonance technique, we extracted the dynamic magnetic properties of several Co$_{\text{25}}$Fe$_{\text{75}}$-based heterostructures with varying ferromagnetic layer thickness. By estimating the eddy current contribution to damping, measuring radiative damping and spin pumping effects, we found the intrinsic damping of a 26\,nm thick sample to be $$α_{\mathrm{0}} \lesssim 3.18\times10^{-4}$. Furthermore, using Brillouin light scattering microscopy we measured spin-wave propagation lengths of up to $(21\pm1)\,\mathrm{μm}$ in a 26 nm thick Co$_{\text{25}}$Fe$_{\text{75}}$ heterostructure at room temperature, which is in excellent agreement with the measured damping.

cond-mat.mtrl-sci↗

arXiv2019

Correlation between the Dzyaloshinskii-Moriya interaction and the orbital angular momentum at an oxide / ferromagnet interface

We report on the Dzyaloshinskii-Moriya (DMI) interaction at the interface between a ferromagnet and an oxide. We demonstrate experimentally that oxides can give rise to DMI. By comparison of systems comprised of Pt/Co90Fe10/Oxide and Cu/Co90Fe10/Oxide, we also show how oxidation of one interface can enhance and add to the total DMI of that generated by the Pt interface. This is due to the fact that the DMI on both interfaces promotes left-handed chirality. Finally, by use of ferromagnetic resonance spectroscopy, we show that the DMI and the spectroscopic splitting factor, which is a measure of the orbital momentum, are correlated. This indicates the importance of hybridization and charge transfer at the oxide interface for the DMI.

cond-mat.mtrl-sci↗

arXiv2019

Magnetoelasticity of $\mathrm{Co_{25}}\mathrm{Fe_{75}}$ thin films

We investigate the magnetoelastic properties of $\mathrm{Co_{25}}\mathrm{Fe_{75}}$ and $\mathrm{Co_{10}}\mathrm{Fe_{90}}$ thin films by measuring the mechanical properties of a doubly clamped string resonator covered with multi-layer stacks containing these films. For the magnetostrictive constants we find $λ_{\mathrm{Co_{25}}\mathrm{Fe_{75}}}=(-20.68\pm0.25)\times10^{-6}$ and $λ_{\mathrm{Co_{10}}\mathrm{Fe_{90}}}=(-9.80\pm0.12)\times10^{-6}$ at room temperature. In stark contrast to the positive magnetostriction previously found in bulk CoFe crystals. $\mathrm{Co_{25}}\mathrm{Fe_{75}}$ thin films unite low damping and sizable magnetostriction and are thus a prime candidate for micromechanical magnonic applications, such as sensors and hybrid phonon-magnon systems.

cond-mat.mes-hall↗

arXiv2019

Near-Unity Spin Hall Ratio in Ni$_x$Cu$_{1-x}$ Alloys

We report a large spin Hall effect in the 3$d$ transition metal alloy Ni$_x$Cu$_{1-x}$ for $x\in\left\{ 0.3,0.75\right\} $, detected via the ferromagnetic resonance of a Permalloy (Py = Ni$_{80}$Fe$_{20}$) film deposited in a bilayer with the alloy. A thickness series at $x$ = 0.6, for which the alloy is paramagnetic at room temperature, allows us to determine the spin Hall ratio $θ_{\rm{SH}}\approx1$, spin diffusion length $λ_{\rm{s}}$, spin mixing conductance $G_{\uparrow\downarrow}$, and damping $α_{\rm{SML}}$ due to spin memory loss . We compare our results with similar experiments on Py/Pt bilayers measured using the same method. Ab initio band structure calculations with disorder and spin-orbit coupling suggest an intrinsic spin Hall effect in Ni$_x$Cu$_{1-x}$ alloys, although the experiments here cannot distinguish between extrinsic and intrinsic mechanisms.

cond-mat.mes-hall↗