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K. E. Gray

Publications and source records attributed to K. E. Gray.

32 records · Page 2Linked to original sources

Persistence of Strong Electron Coupling to a Narrow Boson Spectrum in Overdoped BiSrCaCuO (Bi2212) Tunneling Data

A d-wave, Eliashberg analysis of break junction and STM tunneling spectra on BiSrCaCuO (Bi2212) reveals that a spectral dip feature is directly linked to strong electronic coupling to a narrow boson spectrum, evidenced by a large peak in the boson spectral weight. The tunneling dip feature remains robust in the overdoped regime of Bi2212 with bulk Tc values of 56 K-62 K. This is contrary to recent optical conductivity measurements of the self-energy that suggest the narrow boson spectrum disappears in overdoped Bi2212 and therefore cannot be essential for the pairing mechanism. The discrepancy is resolved by considering the way each technique probes the electron self-energy, in particular, the unique sensitivity of tunneling to the off-diagonal or pairing part of the self-energy.

cond-mat.supr-con↗

Full Bulk Spin Polarization and Intrinsic Tunnel Barriers at the Surface of Layered Manganites

Transmission of information using the spin of the electron as well as its charge requires a high degree of spin polarization at surfaces. At surfaces however this degree of polarization can be quenched by competing interactions. Using a combination of surface sensitive x-ray and tunneling probes, we show for the quasi-two-dimensional bilayer manganites that the outermost Mn-O bilayer, alone, is affected: it is a 1-nm thick insulator that exhibits no long-range ferromagnetic order while the next bilayer displays the full spin polarization of the bulk. Such an abrupt localization of the surface effects is due to the two-dimensional nature of the layered manganite while the loss of ferromagnetism is attributed to weakened double exchange in the reconstructed surface bilayer and a resultant antiferromagnetic phase. The creation of a well-defined surface insulator demonstrates the ability to naturally self-assemble two of the most demanding components of an ideal magnetic tunnel junction.

cond-mat.str-el↗

Single Junction and Intrinsic Josephson Junction Tunneling Spectroscopies of Bi2Sr2CaCu2O8+d

Tunneling spectroscopy measurements are reported on optimally-doped and overdoped Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ single crystals. A novel point contact method is used to obtain superconductor-insulator-normal metal (SIN) and SIS break junctions as well as intrinsic Josephson junctions (IJJ) from nanoscale crystals. Three junction types are obtained on the same crystal to compare the quasiparticle peaks and higher bias dip/hump structures which have also been found in other surface probes such as scanning tunneling spectroscopy and angle-resolved photoemission spectroscopy. However, our IJJ quasiparticle spectra consistently reveal very sharp conductance peaks and no higher bias dip structures. The IJJ conductance peak voltage divided by the number of junctions in the stack consistently leads to a significant underestimate of $Δ$ when compared to the single junction values. The comparison of the three methods suggests that the markedly different characteristics of IJJ are a consequence of nonequilibrium effects and are not intrinsic quasiparticle features.

cond-mat.supr-con↗

Retention of Two-Band Superconductivity in Highly Carbon-Doped MgB2

Tunneling data on MgB_{1.8}C_{0.2} show a reduction in the energy gap of the pi-bands by a factor of two from undoped MgB2 that is consistent with the Tc reduction, but inconsistent with the expectations of the dirty limit. Dirty-limit theory for undoped MgB2 predicts a single gap about three times larger than measured and a reduced Tc comparable to that measured. Our heavily-doped samples exhibit a uniform dispersion of C suggestive of significantly enhanced scattering, and we conclude that the retention of two-band superconductivity in these samples is caused by a selective suppression of interband scattering.

cond-mat.supr-con↗

Probing the Phase Diagram of Bi2Sr2CaCu2O8+d with Tunneling Spectroscopy

Tunneling measurements are performed on Ca-rich single crystals of Bi2Sr2CaCu2O8+d (Bi2212), with various oxygen doping levels, using a novel point contact method. At 4.2 K, SIN and SIS tunnel junctions are obtained with well-defined quasiparticle peaks, robust dip and hump features and in some cases Josephson currents. The doping dependence of tunneling conductances of Ca-rich Bi2212 are analyzed and compared to stoichiometric Bi2212. A similar profile of energy gap vs. doping concentration is found although the Ca-rich samples have a slighly smaller optimum Tc and therefore smaller gap values for any doping level. The evolution of tunneling conductance peak height to background ratios with hole concentration are compared. For a given doping level, the Ca-rich spectra showed more broadened features compared to the stoichiometric counterparts, most likely due to increased disorder from the excess Ca. Comparison of the dip and hump features has provided some potential insights into their origins.

cond-mat.supr-con↗

Break-Junction Tunneling on MgB_2

Tunneling data on magnesium diboride, MgB_2, are reviewed with a particular focus on superconductor-insulator-superconductor (SIS) junctions formed by a break-junction method. The collective tunneling literature reveals two distinct energy scales, a large gap, Delta_L~7.2 meV, close to the expected BCS value, and a small gap, Delta_S~2.4 meV. The SIS break junctions show clearly that the small gap closes near the bulk critical temperature, T_c=39 K. The SIS spectra allow proximity effects to be ruled out as the cause for the small gap and therefore make a strong case that MgB_2 is a coupled, two-band superconductor. While the break junctions sometimes reveal parallel contributions to the conductance from both bands, it is more often found that Delta_S dominates the spectra. In these cases, a subtle feature is observed near Delta_S+Delta_L that is reminiscent of strong-coupling effects. This feature is consistent with quasiparticle scattering contributions to the interband coupling which provides an important insight into the nature of two-band superconductivity in MgB_2.

cond-mat.supr-con↗

Evidence for Two-Band Superconductivity from Break Junction Tunneling on MgB2

Superconductor-insulator-superconductor tunnel junctions have been fabricated on MgB2 that display Josephson and quasiparticle currents. These junctions exhibit a gap magnitude, Delta~2.5 meV, that is considerably smaller than the BCS value, but which clearly and reproducibly closes near the bulk Tc. In conjunction with fits of the conductance spectra, these results are interpreted as direct evidence of two-band superconductivity.

cond-mat.supr-con↗

Correlation of Tunneling Spectra in Bi2Sr2CaCu2O(8+delta) with the Resonance Spin Excitation

New break-junction tunneling data are reported in Bi2Sr2CaCu2O(8+delta) over a wide range of hole concentration from underdoped (Tc = 74 K) to optimal doped (Tc = 95 K) to overdoped (Tc = 48 K). The conductances exhibit sharp dips at a voltage, Omega/e, measured with respect to the superconducting gap. Clear trends are found such that the dip strength is maximum at optimal doping and that Omega scales as 4.9 kTc over the entire doping range. These features link the dip to the resonance spin excitation and suggest quasiparticle interactions with this mode are important for superconductivity.

cond-mat.supr-con↗

Energy Gap from Tunneling and Metallic Sharvin Contacts onto MgB2: Evidence for a Weakened Surface Layer

Point-contact tunnel junctions using a Au tip on sintered MgB2 pellets reveal a sharp superconducting energy gap that is confirmed by subsequent metallic Sharvin contacts made on the same sample. The peak in the tunneling conductance and the Sharvin contact conductance follow the BCS form, but the gap values of 4.3 meV are less than the weak-coupling BCS value of 5.9 meV for the bulk Tc of 39 K. The low value of Delta compared to the BCS value for the bulk Tc is possibly due to chemical reactions at the surface.

cond-mat.supr-con↗

Tunneling Spectroscopy of Tl2Ba2CuO6

New results from tunneling spectroscopies on near optimally-doped single crystals of Tl_{2}Ba_{2}CuO_{6} (Tl-2201) junctions are presented. The superconductor-insulator-normal metal (SIN) tunnel junctions are obtained using the point-contact technique with a Au tip. The tunneling conductances reproducibly show a sharp cusp-like subgap, prominent quasiparticle peaks with a consistent asymmetry, and weakly decreasing backgrounds. A rigorous analysis of the SIN tunneling data is performed using two different models for the $d_{x^{2}-y^{2}}$ (d-wave) density of states (DOS). Based on these and earlier results, the tunneling DOS of Tl-2201 have exhibited the most reproducible data that are consistent with a d-wave gap symmetry. We show that the dip feature at $2Δ$ that is clearly seen in SIN tunneling data of Bi_{2}Sr_{2}CaCu_{2}O_{8+δ} is also present in Tl-2201, but at a weaker level. The gap values for crystals with a bulk T_c = 86 K are in the range of 19-25 meV.

cond-mat.supr-con↗

Direct Imaging of the First Order Spin Flop Transition in the Layered Manganite La1.4Sr1.6Mn2O7

Magnetic field induced transitions in the antiferromagnetic layered manganite La1.4Sr1.6Mn2O7 were studied using magnetization measurements and a high-resolution magneto-optical imaging technique. We report the first direct observation of the formation of ferromagnetic domains appearing at the first order spin-flop transition. The magnetization process proceeds through nucleation of polarized domains at crystal defect sites and not by domain wall motion. A small magnetic hysteresis is caused by the nucleation and annihilation of domains in the mixed state. These results establish a direct link betweeen the magnetic structure on the atomic scale as seen in neutron scattering and the macroscopic properties of the sample as seen in magnetization and conductivity measurements.

cond-mat↗

Evidence for a Purely Double-Exchange Mechanism for the Anisotropic Conductivities in Layered La-Sr-Mn-O Single Crystals Below TC

Experimental evidence supports the double-exchange (DE) mechanism for both in-plane and c-axis conductivity in the colossal-magnetoresistive (CMR) layered manganite La1.4Sr1.6Mn2O7. Below TC, the data determine both the DE and antiferromagnetic (AF) superexchange between bilayers. These agree with recent spin-wave data, such that the ratio of intra- to inter-bilayer DE constants is very close to the spin-independent conductance anisotropy of ~300. The conductivity is shown to be proportional to the square of the measured magnetization over a wide range of fields and for temperatures below the in-plane ferromagnetic ordering temperature, TC. This dependence is shown to be consistent with DE coupling and earlier zero-field studies of La1.2Sr1.8Mn2O7 near TC, which used neutron scattering for the local magnetization. A mixed AF and spin-flop state (similar to the intermediate state of type-I superconductors) is a rigorous prediction of the data and modeling.

cond-mat↗

Predominantly Superconducting Origin of Large Energy Gaps in Underdoped Bi2Sr2CaCu2O8-d from Tunneling Spectroscopy

New tunneling data are reported in underdoped Bi2Sr2CaCu2O8-d using superconductor-insulator-superconductor break junctions. Energy gaps, Delta, of 51+2, 54+2 and 57+3 meV are observed for three crystals with Tc=77, 74, and 70 K respectively. These energy gaps are nearly three times larger than for overdoped crystals with similar Tc. Detailed examination of tunneling spectra over a wide doping range from underdoped to overdoped, including the Josephson IcRn product, indicate that these energy gaps are predominantly of superconducting origin.

cond-mat.supr-con↗

Neutron scattering investigation of magnetic bilayer correlations in $La_{1.2}Sr_{1.8}Mn_2O_7$

Neutron scattering investigations of the paramagnetic correlations in the layered manganite La$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$, which exhibits colossal magnetoresistance above the Curie transition at T$_C$ = 112 K, show that spins in neighboring layers within each bilayer are strongly canted at an average angle that is dependent on both the magnetic field and temperature, as predicted by de Gennes. The in-plane correlation length does not diverge at T$_C$, although the magnetic Bragg intensity obeys critical scaling below T$_C$, with the same temperature dependence as the zero-field electrical conductance.

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