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K. G. Leach

Publications and source records attributed to K. G. Leach.

At least 55 records · Page 3Linked to original sources

Benchmarking $^{136}$Xe Neutrinoless $ββ$ Decay Matrix Element Calculations with the $^{138}{\rm Ba}(p,t)$ Reaction

We used a high-resolution magnetic spectrograph to study neutron pair-correlated $0^+$ states in $^{136}$Ba, produced via the $^{138}{\rm Ba}(p,t)$ reaction. In conjunction with state-of-the-art shell model calculations, these data benchmark part of the dominant Gamow-Teller component of the nuclear matrix element (NME) for $^{136}$Xe neutrinoless double beta ($0νββ$) decay. We demonstrate for the first time an evaluation of part of a $0νββ$ decay NME by use of an experimental observable, presenting a new avenue of approach for more accurate calculations of $0νββ$ decay matrix elements.

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Mass Measurements of Neutron-Rich Gallium Isotopes Refine Production of Nuclei of the First r-Process Abundance Peak in Neutron Star Merger Calculations

We report mass measurements of neutron-rich Ga isotopes $^{80-85}$Ga with TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The measurements determine the masses of $^{80-83}$Ga in good agreement with previous measurements. The masses of $^{84}$Ga and $^{85}$Ga were measured for the first time. Uncertainties between $25-48$ keV were reached. The new mass values reduce the nuclear uncertainties associated with the production of A $\approx$ 84 isotopes by the \emph{r}-process for astrophysical conditions that might be consistent with a binary neutron star (BNS) merger producing a blue kilonova. Our nucleosynthesis simulations confirm that BNS merger may contribute to the first abundance peak under moderate neutron-rich conditions with electron fractions $Y_e=0.35-0.38$.

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Reflectivity and PDE of VUV4 Hamamatsu SiPMs in Liquid Xenon

Understanding reflective properties of materials and photodetection efficiency (PDE) of photodetectors is important for optimizing energy resolution and sensitivity of the next generation neutrinoless double beta decay, direct detection dark matter, and neutrino oscillation experiments that will use noble liquid gases, such as nEXO, DARWIN, DarkSide-20k, and DUNE. Little information is currently available about reflectivity and PDE in liquid noble gases, because such measurements are difficult to conduct in a cryogenic environment and at short enough wavelengths. Here we report a measurement of specular reflectivity and relative PDE of Hamamatsu VUV4 silicon photomultipliers (SiPMs) with 50 micrometer micro-cells conducted with xenon scintillation light (~175 nm) in liquid xenon. The specular reflectivity at 15 deg. incidence of three samples of VUV4 SiPMs is found to be 30.4+/-1.4%, 28.6+/-1.3%, and 28.0+/-1.3%, respectively. The PDE at normal incidence differs by +/-8% (standard deviation) among the three devices. The angular dependence of the reflectivity and PDE was also measured for one of the SiPMs. Both the reflectivity and PDE decrease as the angle of incidence increases. This is the first measurement of an angular dependence of PDE and reflectivity of a SiPM in liquid xenon.

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Detailed spectroscopy of $^{46}$Ca: A study of the $β^-$ decay of $^{46}$K

We report on high-statistics data from the $β^-$ decay of the $^{46}$K $J^π$ = 2$^-$ ground state taken with the GRIFFIN spectrometer located at the TRIUMF-ISAC facility. In total, 199 $γ$ rays and 42 excited states were placed in the level scheme, and from the observed $β$ feeding and angular correlations of pairs of cascading $γ$ rays, it was possible to assign spins and parities to excited states and determine mixing ratios for selected $γ$ rays. The level structure of $^{46}$Ca is compared to theoretical predictions from a microscopic valence-space Hamiltonian derived from two- (NN) and three-nucleon (3N) forces. These calculations are in reasonable agreement with the experimental data and indicate that the protons in this region are not as inert as would be expected for semi-magic nuclei.

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Reflectance of Silicon Photomultipliers at Vacuum Ultraviolet Wavelengths

Characterization of the vacuum ultraviolet (VUV) reflectance of silicon photomultipliers (SiPMs) is important for large-scale SiPM-based photodetector systems. We report the angular dependence of the specular reflectance in a vacuum of SiPMs manufactured by Fondazionc Bruno Kessler (FBK) and Hamamatsu Photonics K.K. (HPK) over wavelengths ranging from 120 nm to 280 nm. Refractive index and extinction coefficient of the thin silicon-dioxide film deposited on the surface of the FBK SiPMs are derived from reflectance data of a FBK silicon wafer with the same deposited oxide film as SiPMs. The diffuse reflectance of SiPMs is also measured at 193 nm. We use the VUV spectral dependence of the optical constants to predict the reflectance of the FBK silicon wafer and FBK SiPMs in liquid xenon.

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Measurements of electron transport in liquid and gas Xenon using a laser-driven photocathode

Measurements of electron drift properties in liquid and gaseous xenon are reported. The electrons are generated by the photoelectric effect in a semi-transparent gold photocathode driven in transmission mode with a pulsed ultraviolet laser. The charges drift and diffuse in a small chamber at various electric fields and a fixed drift distance of 2.0 cm. At an electric field of 0.5 kV/cm, the measured drift velocities and corresponding temperature coefficients respectively are $1.97 \pm 0.04$ mm/$μ$s and $(-0.69\pm0.05)$\%/K for liquid xenon, and $1.42 \pm 0.03$ mm/$μ$s and $(+0.11\pm0.01)$\%/K for gaseous xenon at 1.5 bar. In addition, we measure longitudinal diffusion coefficients of $25.7 \pm 4.6$ cm$^2$/s and $149 \pm 23$ cm$^2$/s, for liquid and gas, respectively. The quantum efficiency of the gold photocathode is studied at the photon energy of 4.73 eV in liquid and gaseous xenon, and vacuum. These charge transport properties and the behavior of photocathodes in a xenon environment are important in designing and calibrating future large scale noble liquid detectors.

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Simulation of charge readout with segmented tiles in nEXO

nEXO is a proposed experiment to search for the neutrino-less double beta decay ($0νββ$) of $^{136}$Xe in a tonne-scale liquid xenon time projection chamber (TPC). The nEXO TPC will be equipped with charge collection tiles to form the anode. In this work, the charge reconstruction performance of this anode design is studied with a dedicated simulation package. A multi-variate method and a deep neural network are developed to distinguish simulated $0νββ$ signals from backgrounds arising from trace levels of natural radioactivity in the detector materials. These simulations indicate that the nEXO TPC with charge-collection tiles shows promising capability to discriminate the $0νββ$ signal from backgrounds. The estimated half-life sensitivity for $0νββ$ decay is improved by $\sim$20$~(32)\%$ with the multi-variate~(deep neural network) methods considered here, relative to the sensitivity estimated in the nEXO pre-conceptual design report.

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Direct observation of proton emission in 11Be

The elusive $β^-\text{p}^+$ decay was observed in $^{11}$Be by directly measuring the emitted protons and their energy distribution for the first time with the prototype Active Target Time Projection Chamber (pAT-TPC) in an experiment performed at ISAC-TRIUMF. The measured $β^-\text{p}^+$ branching ratio is orders of magnitude larger than any previous theoretical model predicted. This can be explained by the presence of a narrow resonance in $^{11}$B above the proton separation energy.

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Isospin symmetry in $B(E2)$ values: Coulomb excitation study of ${}^{21}$Mg

The $T_z$~=~$-\frac{3}{2}$ nucleus ${}^{21}$Mg has been studied by Coulomb excitation on ${}^{196}$Pt and ${}^{110}$Pd targets. A 205.6(1)-keV $γ$-ray transition resulting from the Coulomb excitation of the $\frac{5}{2}^+$ ground state to the first excited $\frac{1}{2}^+$ state in ${}^{21}$Mg was observed for the first time. Coulomb excitation cross-section measurements with both targets and a measurement of the half-life of the $\frac{1}{2}^+$ state yield an adopted value of $B(E2;\frac{5}{2}^+\rightarrow\frac{1}{2}^+)$~=~13.3(4)~W.u. A new excited state at 1672(1)~keV with tentative $\frac{9}{2}^+$ assignment was also identified in ${}^{21}$Mg. This work demonstrates large difference of the $B(E2;\frac{5}{2}^+\rightarrow\frac{1}{2}^+)$ values between $T$~=~$\frac{3}{2}$, $A$~=~21 mirror nuclei. The difference is investigated in the shell-model framework employing both isospin conserving and breaking USD interactions and using modern \textsl{ab initio} nuclear structure calculations, which have recently become applicable in the $sd$ shell.

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The GRIFFIN Facility for Decay-Spectroscopy Studies at TRIUMF-ISAC

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new high-efficiency $γ$-ray spectrometer designed for use in decay spectroscopy experiments with low-energy radioactive ion beams provided by TRIUMF's Isotope Separator and Accelerator (ISAC-I) facility. GRIFFIN is composed of sixteen Compton-suppressed large-volume clover-type high-purity germanium (HPGe) $γ$-ray detectors combined with a suite of ancillary detection systems and coupled to a custom digital data acquisition system. The infrastructure and detectors of the spectrometer as well as the performance characteristics and the analysis techniques applied to the experimental data are described.

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High-resolution (p,t) reaction measurements as spectroscopic tests of {\it ab-initio} theory in the mid $pf$-shell

Detailed spectroscopic measurements of excited states in $^{50}$Cr and $^{62}$Zn were performed using 24~MeV (p,t) transfer reactions on $^{52}$Cr and $^{64}$Zn, respectively. In total, forty-five states in $^{50}$Cr and sixty-seven states in $^{62}$Zn were observed up to excitation energies of 5.5~MeV, including several previously unobserved states. These experimental results are compared to {\it ab-initio} shell-model calculations using chiral effective field theory ($χ$-EFT) with the valence-space in-medium similarity renormalization group (VS-IMSRG) method. This comparison demonstrates good agreement in the level orderings with these new theoretical methods, albeit with a slight over binding in the calculations. This work is part of a continued push to benchmark {\it ab-initio} theoretical techniques to nuclear structure data in $0^+\rightarrow0^+$ superallowed Fermi $β$ decay systems.

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Dawning of the N=32 shell closure seen through precision mass measurements of neutron-rich titanium isotopes

A precision mass investigation of the neutron-rich titanium isotopes $^{51-55}$Ti was performed at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The range of the measurements covers the $N=32$ shell closure and the overall uncertainties of the $^{52-55}$Ti mass values were significantly reduced. Our results confirm the existence of a weak shell effect at $N=32$, establishing the abrupt onset of this shell closure. Our data were compared with state-of-the-art \textit{ab-initio} shell model calculations which, despite very successfully describing where the $N=32$ shell gap is strong, overpredict its strength and extent in titanium and heavier isotones. These measurements also represent the first scientific results of TITAN using the newly commissioned Multiple-Reflection Time-of-Flight Mass Spectrometer (MR-TOF-MS), substantiated by independent measurements from TITAN's Penning trap mass spectrometer.

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High-precision $Q_{EC}$-value measurement of the superallowed $β^+$ emitter $^{22}$Mg and an evaluation of the $A=22$ isobaric triplet

A direct $Q_{EC}$-value measurement of the superallowed $β^+$ emitter $^{22}$Mg was performed using TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The direct ground-state to ground-state atomic mass difference between $^{22}$Mg and $^{22}$Na was determined to be $Q_{EC}=4781.40(22)$~keV, representing the most precise single measurement of this quantity to date. In a continued push towards calculating superallowed isospin-symmetry-breaking (ISB) corrections from first principles, ab-initio shell-model calculations of the $A=22$ IMME are also presented for the first time using the valence-space in-medium similarity renormalization group formalism. With particular starting two- and three-nucleon forces, this approach demonstrates a level of agreement with the experimental data that suggests reliable ab-initio calculations of superallowed ISB corrections are now possible.

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High-Precision Half-life Measurement for the Superallowed Fermi $β^+$ Emitter $^{22}$Mg

A high-precision half-life measurement for the superallowed Fermi $β^+$ emitter $^{22}$Mg was performed at the TRIUMF-ISAC facility using a 4$π$ proportional gas counter. The result of $T_{1/2} = 3.87400 \pm 0.00079$ s is a factor of 3 more precise than the previously adopted world average and resolves a discrepancy between the two previously published $^{22}$Mg half-life measurements.

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Precision mass measurements of $^{125-127}$Cd isotopes and isomers approaching the $N=82$ closed shell

We present the results of precision mass measurements of neutron-rich cadmium isotopes. These nuclei approach the $N=82$ closed neutron shell and are important to nuclear structure as they lie near doubly-magic $^{132}$Sn on the chart of nuclides. Of particular note is the clear identification of the ground state mass in $^{127}$Cd along with the isomeric state. We show that the ground state identified in a previous mass measurement which dominates the mass value in the Atomic Mass Evaluation is an isomeric state. In addition to $^{127/m}$Cd, we present other cadmium masses measured ($^{125/m}$Cd and $^{126}$Cd) in a recent TITAN experiment at TRIUMF. Finally, we compare our measurements to new \emph{ab initio} shell-model calculations and comment on the state of the field in the $N=82$ region.

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A Novel Transparent Charged Particle Detector for the CPET Upgrade at TITAN

The detection of an electron bunch exiting a strong magnetic field can prove challenging due to the small mass of the electron. If placed too far from a solenoid's entrance, a detector outside the magnetic field will be too small to reliably intersect with the exiting electron beam because the light electrons will follow the diverging magnetic field outside the solenoid. The TITAN group at TRIUMF in Vancouver, Canada, has made use of advances in the practice and precision of photochemical machining (PCM) to create a new kind of charge collecting detector called the "mesh detector." The TITAN mesh detector was used to solve the problem of trapped electron detection in the new Cooler PEnning Trap (CPET) currently under development at TITAN. This thin array of wires etched out of a copper plate is a novel, low profile, charge agnostic detector that can be made effectively transparent or opaque at the user's discretion.

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Precision mass measurements of magnesium isotopes and implications on the validity of the Isobaric Mass Multiplet Equation

If the mass excess of neutron-deficient nuclei and their neutron-rich mirror partners are both known, it can be shown that deviations of the Isobaric Mass Multiplet Equation (IMME) in the form of a cubic term can be probed. Such a cubic term was probed by using the atomic mass of neutron-rich magnesium isotopes measured using the TITAN Penning trap and the recently measured proton-separation energies of $^{29}$Cl and $^{30}$Ar. The atomic mass of $^{27}$Mg was found to be within 1.6$σ$ of the value stated in the Atomic Mass Evaluation. The atomic masses of $^{28,29}$Mg were measured to be both within 1$σ$, while being 8 and 34 times more precise, respectively. Using the $^{29}$Mg mass excess and previous measurements of $^{29}$Cl we uncovered a cubic coefficient of $d$ = 28(7) keV, which is the largest known cubic coefficient of the IMME. This departure, however, could also be caused by experimental data with unknown systematic errors. Hence there is a need to confirm the mass excess of $^{28}$S and the one-neutron separation energy of $^{29}$Cl, which have both come from a single measurement. Finally, our results were compared to ab initio calculations from the valence-space in-medium similarity renormalization group, resulting in a good agreement.

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Electroweak Decay Studies of Highly Charged Radioactive Ions with TITAN at TRIUMF

Several modes of electroweak radioactive decay require an interaction between the nucleus and bound electrons within the constituent atom. Thus, the probabilities of the respective decays are not only influenced by the structure of the initial and final states in the nucleus, but can also depend strongly on the atomic charge. Conditions suitable for the partial or complete ionization of these rare isotopes occur naturally in hot, dense astrophysical environments, but can also be artificially generated in the laboratory to selectively block certain radioactive decay modes. Direct experimental studies on such scenarios are extremely difficult due to the laboratory conditions required to generate and store radioactive ions at high charge states. A new electron-beam ion trap (EBIT) decay setup with the TITAN experiment at TRIUMF has successfully demonstrated such techniques for performing spectroscopy on the radioactive decay of highly charged ions.

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