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K. H. Bennemann

Publications and source records attributed to K. H. Bennemann.

At least 19 recordsLinked to original sources

On Ultrafast Spin Dynamics: Spin Dependent Fast Response of Hot Electrons, of Band--Structure

Different energy shifts for majority and minority electrons occur. Thus, for example in case of (laser) excited ferromagnetic metals majority and minority electrons may respond differently in time during closing the exchange splitting. Spin flip transitions of the hot electrons due to electron interactions cause quasi hybridization of the spin split states. This is also the case in itinerant ferromagnetic metals due to hopping between sites having magnetic moments pointing in direction of the magnetization (+) and opposite direction (-) and with energy levels $\varepsilon^+_{iσ}$ and $\varepsilon^-_{iσ}$. For energetic reasons the molecular field acts asymmetrically on the spins of the electrons and on spin flip transitions and thus causes different lifetimes of minority and majority electrons and spin dependent electron energy shifts. Quite general minority hot electrons in spin split states may respond faster than majority electrons at non--equilibrium. The molecular field acting on the spins delays spin flip transitions $\uparrow \rightarrow \downarrow$ and thus a response of the hot majority electrons and their energy levels. The closing of the exchange splitting in the electron spectrum of ferromagnetic transition and rare--earth metals, ferromagnetic semiconductors, spin split quantum well states in thin ferromagnetic films, etc. will reflect this. The time and spin dependent energy shifts of electrons at non--equilibrium may cause interesting behavior, in particular of magnetic tunnel junctions, spin currents etc.. In ferromagnets the moment reversal lifetime of (local) magnetic moments parallel to the global magnetization is larger than of moments pointing in opposite direction.

cond-mat.mes-hall↗

Photoinduced Phase Transitions

Optically induced ultrafast electronic excitations with sufficiently long lifetimes may cause strong effects on phase transitions like structural and nonmetal to metal ones. Examples are transitions diamond to graphite, graphite to graphene, non-metal to metal, solid to liquid and vapor to liquid, solid. A spectacular case is photo-induced water condensation. These non-equilibrium transitions are an ultrafast response, on a few hundred fs-time scale, to the fast electronic excitations. The energy of the photons is converted into electronic one via electronic excitations changing the cohesive energy. This changes the chemical potential controlling the phase transition. In view of the advances in laser optics photon induced transitions are expected to become an active area in non-equilibrium physics and phase transition dynamics. Conservation laws like energy or angular momentum conservation control the time during which the transitions occur. Since the photon induced effects result largely from weakening or strenghtening of the bonding between the atoms or molecules transitions like solid/liquid etc. can be shifted in both directions. Photoinduced transitions will be discussed from an unified point of view.

cond-mat.mtrl-sci↗

Magnetic Nanostructures

Characteristic results of magnetism in small particles and thin films are presented. As a consequence of the reduced atomic coordination in small clusters and thin films the electronic states and density of states modify. Thus magnetic moments and magnetization are affected. In tunnel junctions interplay of magnetism, spin currents and superconductivity are of particular interest. Results are given for single transition metal clusters, cluster ensembles, thin films and tunnel systems. Interesting behavior of tunnel currents and currents induced by Aharonov-Bohm effect into mesoscopic rings etc. are discussed.

cond-mat.mes-hall↗

Two-dimensional Heisenberg antiferromagnet in a transverse field

We investigate the magnetic reorientation in a two-dimensional anisotropic antiferromagnet due to a transverse magnetic field. Using a many-body Green's function approach, we show that the magnetization component perpendicular to the applied field (and along the easy-axis of the antiferromagnet) initially increases with increasing field strength. We show that this unexpected result arises from the suppression of quantum and thermal fluctuations in the antiferromagnet. Above the Néel temperature, this effect leads to a reappearance of a magnetic moment along the easy-axis.

cond-mat.str-el↗

Response theory for time-resolved second-harmonic generation and two-photon photoemission

A unified response theory for the time-resolved nonlinear light generation and two-photon photoemission (2PPE) from metal surfaces is presented. The theory allows to describe the dependence of the nonlinear optical response and the photoelectron yield, respectively, on the time dependence of the exciting light field. Quantum-mechanical interference effects affect the results significantly. Contributions to 2PPE due to the optical nonlinearity of the surface region are derived and shown to be relevant close to a plasmon resonance. The interplay between pulse shape, relaxation times of excited electrons, and band structure is analyzed directly in the time domain. While our theory works for arbitrary pulse shapes, we mainly focus on the case of two pulses of the same mean frequency. Difficulties in extracting relaxation rates from pump-probe experiments are discussed, for example due to the effect of detuning of intermediate states on the interference. The theory also allows to determine the range of validity of the optical Bloch equations and of semiclassical rate equations, respectively. Finally, we discuss how collective plasma excitations affect the nonlinear optical response and 2PPE.

cond-mat↗

Magnetic relaxation and dipole-coupling-induced magnetization in nanostructured thin films during growth: A cluster Monte Carlo study

For growing inhomogeneous thin films with an island nanostructure similar as observed in experiment, we determine the nonequilibrium and equilibrium remanent magnetization. The single-island magnetic anisotropy, the dipole coupling, and the exchange interaction between magnetic islands are taken into account within a micromagnetic model. A cluster Monte Carlo method is developed which includes coherent magnetization changes of connected islands. This causes a fast relaxation towards equilibrium for irregularly connected systems. We analyse the transition from dipole coupled islands at low coverages to a strongly connected ferromagnetic film at high coverages during film growth. For coverages below the percolation threshold, the dipole interaction induces a collective magnetic order with ordering temperatures of 1 - 10 K for the assumed model parameters. Anisotropy causes blocking temperatures of 10 - 100 K and thus pronounced nonequilibrium effects. The dipole coupling leads to a somewhat slower magnetic relaxation.

cond-mat.stat-mech↗

Renormalization of the elementary excitations in hole- and electron-doped cuprates due to spin fluctuations

Extending our previous studies we present results for the doping-, momentum-, frequency-, and temperature- dependence of the kink-like change of the quasiparticle velocity resulting from the coupling to spin fluctuations. In the nodal direction a kink is found in both the normal and superconducting state while in the antinodal direction a kink occurs only below $T_c$ due to the opening of the superconducting gap. A pronounced kink is obtained only for hole-doped, but not for electron-doped cuprates and is characteristically different from what is expected due to electron-phonon interaction. We further demonstrate that the kink structure is intimately connected to the resonance peak seen in inelastic neutron scattering. Our results suggest similar effects in other unconventional superconductors like ${Sr}_2{RuO}_4$.

cond-mat.supr-con↗

Theory for the optimal control of time-averaged quantities in open quantum systems

We present variational theory for optimal control over a finite time interval in quantum systems with relaxation. The corresponding Euler-Lagrange equations determining the optimal control field are derived. In our theory the optimal control field fulfills a high order differential equation, which we solve analytically for some limiting cases. We determine quantitatively how relaxation effects limit the control of the system. The theory is applied to open two level quantum systems. An approximate analytical solution for the level occupations in terms of the applied fields is presented. Different other applications are discussed.

quant-ph↗

Electronic theory for the normal state spin dynamics in Sr$_2$RuO$_4$: anisotropy due to spin-orbit coupling

Using a three-band Hubbard Hamiltonian we calculate within the random-phase-approximation the spin susceptibility, $χ({\bf q},ω)$, and NMR spin-lattice relaxation rate, 1/T$_1$, in the normal state of the triplet superconductor Sr$_2$RuO$_4$ and obtain quantitative agreement with experimental data. Most importantly, we find that due to spin-orbit coupling the out-of-plane component of the spin susceptibility $χ^{zz}$ becomes at low temperatures two times larger than the in-plane one. As a consequence strong incommensurate antiferromagnetic fluctuations of the quasi-one-dimensional $xz$- and $yz$-bands point into the $z$-direction. Our results provide further evidence for the importance of spin fluctuations for triplet superconductivity in Sr$_2$RuO$_4$.

cond-mat.supr-con↗

Phase diagram of underdoped cuprate superconductors: effect of Cooper-pair phase fluctuations

In underdoped cuprates fluctuations of the phase of the superconducting order parameter play a role due to the small superfluid density. We consider the effects of phase fluctuations assuming the exchange of spin fluctuations to be the predominant pairing interaction. Spin fluctuations are treated in the fluctuation-exchange approximation, while phase fluctuations are included by Berezinskii-Kosterlitz-Thouless theory. We calculate the stiffness against phase fluctuations, ns(omega)/m*, as a function of doping, temperature, and frequency, taking its renormalization by phase fluctuations into account. The results are compared with recent measurements of the high-frequency conductivity. Furthermore, we obtain the temperature T*, where the density of states at the Fermi energy starts to be suppressed, the temperature Tc*, where Cooper pairs form, and the superconducting transition temperature Tc, where their phase becomes coherent. We find a crossover from a phase-fluctuation-dominated regime with Tc proportinal to ns for underdoped cuprates to a BCS-like regime for overdoped materials.

cond-mat.supr-con↗

Theory for phonon-induced superconductivity in MgB$_2$

We analyze superonductivity in MgB$_2$ observed below $T_c=39$ K resulting from electron-phonon coupling involving a mode at $\hbar ω_1 = 24$ meV and most importantly the in-plane B-B $E_{2g}$ vibration at $\hbar ω_2=67$ meV. The quasiparticles originating from $π$- and $σ$-states couple strongly to the low-frequency mode and the $E_{2g}$-vibrations respectively. Using two-band Eliashberg theory, $λ_π = 1.4$ and $λ_σ = 0.7$, we calculate the gap functions $Δ^{i}(ω,0)$ ($i=π$, $σ$). Our results provide an explanation of recent tunneling experiments. We get $H^{ab}_{c_2}/H^{c}_{c_2} \approx 3.9$.

cond-mat.supr-con↗

Model study for the nonequlibrium magnetic domain structure during the growth of nanostructured ultrathin films

The nonequilibrium magnetic domain structure of growing ultrathin ferromagnetic films with a realistic atomic structure is studied as a function of coverage and temperature. We apply a kinetic Monte Carlo method to a micromagnetic model describing the transition from superparamagnetic islands at low coverages to a closed ferromagnetic film. The magnetic relaxation and the island growth happen simultaneously. Near the percolation threshold a metastable magnetic domain structure is obtained with an average domain area ranging between the area of individual magnetic islands and the area of the large domains observed for thicker ferromagnetic films. We conclude that this micro-domain structure is controlled and stabilized by the nonuniform atomic nanostructure of the ultrathin film, causing a random interaction between magnetic islands with varying sizes and shapes. The average domain area and domain roughness are determined. A maximum of the domain area and a minimum of the domain roughness are obtained as a function of the temperature.

cond-mat.dis-nn↗

Analysis of the elementary excitations in high-T_c cuprates: explanation of the new energy scale observed by ARPES

Using the Hubbard Hamiltonian we analyze the energy- and momentum-dependence of the elementary excitations in high-T$_c$ superconductors resulting from the coupling to spin fluctuations. As a result of the energy dependence of the self-energy $Σ({\bf k}, ω)$, characteristic features occur in the spectral density explaining the 'kink' in recent ARPES experiments. We present results for the spectral density $A({\bf k}, ω)$ resulting from the crossover from Im $Σ({\bf k}, ω)\propto ω$ to Im $Σ({\bf k}, ω)\propto ω^2$, for the feedback of superconductivity on the excitations, and for the superconducting order parameter $Δ({\bf k}, ω)$. These results relate also to inelastic neutron scattering and tunneling experiments and shed important light on the essential ingredients a theory of the elementary excitations in the cuprates must contain.

cond-mat.supr-con↗

Electronic theory for superconductivity in Sr$_2$RuO$_4$: triplet pairing due to spin-fluctuation exchange

Using a two-dimensional Hubbard Hamiltonian for the three electronic bands crossing the Fermi level in Sr$_2$RuO$_4$ we calculate the band structure and spin susceptibility $χ({\bf q}, ω)$ in quantitative agreement with nuclear magnetic resonance (NMR) and inelastic neutron scattering (INS) experiments. The susceptibility has two peaks at {\bf Q}$_i = (2π/3, 2π/3)$ due to the nesting Fermi surface properties and at {\bf q}$_i = (0.6π, 0)$ due to the tendency towards ferromagnetism. Applying spin-fluctuation exchange theory as in layered cuprates we determine from $χ({\bf q}, ω)$, electronic dispersions, and Fermi surface topology that superconductivity in Sr$_2$RuO$_4$ consists of triplet pairing. Combining the Fermi surface topology and the results for $χ({\bf q}, ω)$ we can exclude $s-$ and $d-$wave symmetry for the superconducting order parameter. Furthermore, within our analysis and approximations we find that $f$-wave symmetry is slightly favored over p-wave symmetry due to the nesting properties of the Fermi surface.

cond-mat.supr-con↗

Time-dependent energy absorption changes during ultrafast lattice deformation

The ultrafast time-dependence of the energy absorption of covalent solids upon excitation with femtosecond laser pulses is theoretically analyzed. We use a microscopic theory to describe laser induced structural changes and their influence on the electronic properties. We show that from the time evolution of the energy absorbed by the system important information on the electronic and atomic structure during ultrafast phase transitions can be gained. Our results reflect how structural changes affect the capability of the system to absorb external energy.

cond-mat.mtrl-sci↗

Theory for the ultrafast ablation of graphite films

The physical mechanisms for damage formation in graphite films induced by femtosecond laser pulses are analyzed using a microscopic electronic theory. We describe the nonequilibrium dynamics of electrons and lattice by performing molecular dynamics simulations on time-dependent potential energy surfaces. We show that graphite has the unique property of exhibiting two distinct laser induced structural instabilities. For high absorbed energies (> 3.3 eV/atom) we find nonequilibrium melting followed by fast evaporation. For low intensities above the damage threshold (> 2.0 eV/atom) ablation occurs via removal of intact graphite sheets.

cond-mat.mtrl-sci↗

Analysis of the resonance peak and magnetic coherence seen in inelastic neutron scattering of cuprate superconductors: a consistent picture with tunneling and conductivity data

Assuming the exchange of antiferromagnetic spin fluctuations as the Cooper pairing mechanism we calculate the doping dependence of the resonance peak seen in inelastic neutron scattering and the magnetic coherence effect. Most importantly, we find that the resonance peak in the magnetic susceptibility, ${Im}χ({\bf q},ω)$, appears {\it only} in the superconducting state, that it scales with $T_c$, and that magnetic coherence is a result of a d-wave order parameter. We further analyze the structure of ${Im}χ$ below $T_c$, the position of the peak at $ω_{res}$ and the consequences for photoemission, tunneling spectroscopy and the optical conductivity.

cond-mat.supr-con↗

Theory for Electron-Doped Cuprate Superconductors: d-wave symmetry order parameter

Using as a model the Hubbard Hamiltonian we determine various basic properties of electron-doped cuprate superconductors like ${Nd}_{2-x}{Ce}_{x}{CuO}_{4}$ and ${Pr}_{2-x}{Ce}_{x}{CuO}_{4}$ for a spin-fluctuation-induced pairing mechanism. Most importantly we find a narrow range of superconductivity and like for hole-doped cuprates $d_{x^{2}-y^{2}}$ - symmetry for the superconducting order parameter. The superconducting transition temperatures $T_{c}(x)$ for various electron doping concentrations $x$ are calculated to be much smaller than for hole-doped cuprates due to the different Fermi surface and a flat band well below the Fermi level. Lattice disorder may sensitively distort the symmetry $d_{x^{2}-y^{2}}$ via electron-phonon interaction.

cond-mat.supr-con↗