arXiv subjects

K. Hashimoto

Publications and source records attributed to K. Hashimoto.

At least 37 records · Page 2Linked to original sources

arXiv2023

Anisotropic Enhancement of Lower Critical Field in Ultraclean Crystals of Spin-Triplet Superconductor UTe2

The paramagnetic spin-triplet superconductor UTe$_2$ has attracted significant attention because of its exotic superconducting properties including an extremely high upper critical field and possible chiral superconducting states. Recently, ultraclean single crystals of UTe$_2$ have become available, and thus measurements on these crystals are crucial to elucidate the intrinsic superconducting properties. Here, we report the thermodynamic critical field $H_{\rm c}$, the lower critical field $H_{\rm c1}$, and the upper critical field $H_{\rm c2}$ at low fields of these high-quality single crystals. From the comparison of the anisotropies in $H_{\rm c1}$ and $H_{\rm c2}$, we find that the experimental $H_{\rm c1}$ values with the magnetic field along $b$- and $c$-axes are anomalously enhanced, showing unusual low-temperature upturns. We propose an effect of the strong Ising-like ferromagnetic fluctuations on the vortex line energy as the origin of the anisotropic enhancement of $H_{\rm c1}$.

cond-mat.supr-con↗

arXiv2022

Bulk evidence of anisotropic $s$-wave pairing with no sign change in the kagome superconductor CsV$_3$Sb$_5$

The recently discovered kagome superconductors $A$V$_3$Sb$_5$ ($A$ = K, Rb, Cs) possess a unique band structure with van Hove singularities and Dirac dispersions, in which unusual charge-density-wave (CDW) orders with time-reversal and rotational symmetry breaking have been reported. One of the most crucial unresolved issues is identifying the symmetry of the superconductivity that develops inside the CDW phase. Theory predicts a variety of unconventional superconducting symmetries, including exotic states with chiral and topological properties accompanied by a sign-changing superconducting gap. Experimentally, however, the phase information on the superconducting gap in $A$V$_3$Sb$_5$ is still lacking. Here we report the electron irradiation effects in CsV$_3$Sb$_5$ using introduced impurities as a phase-sensitive probe of superconductivity. Our magnetic penetration depth measurements reveal that with increasing impurities, a highly anisotropic fully-gapped state changes gradually to an isotropic full-gap state without passing through a nodal state. Furthermore, transport measurements under high pressure show that the double superconducting dome in the pressure-temperature phase diagram survives against sufficient impurities. These results are strong bulk evidence that CsV$_3$Sb$_5$ is a non-chiral, anisotropic $s$-wave superconductor with no sign change both at ambient and high pressure, which provides a clue to understanding the relationship between CDW and superconductivity in kagome superconductors.

cond-mat.supr-con↗

arXiv2022

Pure nematic quantum critical point accompanied by a superconducting dome

When a symmetry-breaking phase of matter is suppressed to a quantum critical point (QCP) at absolute zero, quantum-mechanical fluctuations proliferate. Such fluctuations can lead to unconventional superconductivity, as evidenced by the superconducting domes often found near magnetic QCPs in correlated materials. However, it remains unclear whether this superconductivity mechanism holds for QCPs of the electronic nematic phase, characterized by rotational symmetry breaking. Here, we demonstrate from systematic elastoresistivity measurements that nonmagnetic FeSe$_{1-x}$Te$_{x}$ exhibits an electronic nematic QCP showing diverging nematic susceptibility. This finding establishes two nematic QCPs in FeSe-based superconductors with contrasting accompanying phase diagrams. In FeSe$_{1-x}$Te$_{x}$, a superconducting dome is centered at the QCP, whereas FeSe$_{1-x}$S$_{x}$ shows no QCP-associated enhancement of superconductivity. We find that this difference is related to the relative strength of nematic and spin fluctuations. Our results in FeSe$_{1-x}$Te$_{x}$ present the first case in support of the superconducting dome being associated with the pure nematic QCP.

cond-mat.supr-con↗

arXiv2022

Chiral superconductivity in UTe2 probed by anisotropic low-energy excitations

Chiral spin-triplet superconductivity is a topologically nontrivial pairing state with broken time-reversal symmetry, which can host Majorana quasiparticles. The recently discovered heavy-fermion superconductor UTe$_2$ exhibits peculiar properties of spin-triplet pairing, and the possible chiral state has been actively discussed. However, the symmetry and nodal structure of its order parameter in the bulk, which determine the Majorana surface states, remains controversial. Here we focus on the number and positions of superconducting gap nodes in the ground state of UTe$_2$. Our magnetic penetration depth measurements for three field orientations in the Meissner state reveal the power-law temperature dependence with exponents nearly equal to 2 or less than 2, which excludes single-component spin-triplet states. The anisotropy of low-energy quasiparticle excitations indicates multiple point nodes near the $k_y$- and $k_z$-axes, evidencing that the order parameter has multiple components in a chiral complex form. We find that most consistent is a chiral $B_{3u}+iA_u$ non-unitary state, which provides fundamentals of the topological properties in UTe$_2$.

cond-mat.supr-con↗

arXiv2021

Thermodynamic evidence for field-angle dependent Majorana gap in a Kitaev spin liquid

The exactly-solvable Kitaev model of two-dimensional honeycomb magnet leads to a quantum spin liquid (QSL) characterized by Majorana fermions, relevant for fault-tolerant topological quantum computations. In the high-field paramagnetic state of $α$-RuCl3, half-integer quantization of thermal Hall conductivity has been reported as a signature of edge current, but the bulk nature of this state remains elusive. Here, from high-resolution heat capacity measurements under in-plane field rotation, we find strongly angle-dependent low-energy excitations in bulk $α$-RuCl3. The excitation gap has a sextuple node structure, and the gap amplitude increases with field, exactly as expected for itinerant Majorana fermions in the Kitaev model. Our thermodynamic results are fully linked with the transport quantization properties, providing the first demonstration of the bulk-edge correspondence in a Kitaev QSL. Moreover, at higher fields where the quantum thermal Hall effect vanishes, we find the possible emergence of a novel nematic QSL state with two-fold rotational symmetry.

cond-mat.str-el↗

arXiv2021

Tuning the Parity Mixing of Singlet-Septet Pairing in a Half-Heusler Superconductor

In superconductors, electrons with spin ${s=1/2}$ form Cooper pairs whose spin structure is usually singlet (${S=0}$) or triplet (${S=1}$). When the electronic structure near the Fermi level is characterized by fermions with angular momentum ${j=3/2}$ due to strong spin-orbit interactions, novel pairing states such as even-parity quintet (${J=2}$) and odd-parity septet (${J=3}$) states become allowed. Prime candidates for such exotic states are half-Heusler superconductors, which exhibit unconventional superconducting properties, but their pairing nature remains unsettled. Here we show that the superconductivity in the noncentrosymmetric half-Heusler LuPdBi can be consistently described by the admixture of isotropic even-parity singlet and anisotropic odd-parity septet pairing, whose ratio can be tuned by electron irradiation. From magnetotransport and penetration depth measurements, we find that carrier concentrations and impurity scattering both increase with irradiation, resulting in a nonmonotonic change of the superconducting gap structure. Our findings shed new light on our fundamental understanding of unconventional superconducting states in topological materials.

cond-mat.supr-con↗

arXiv2021

Resistively-detected NMR lineshapes in a local filling $ν< 1$ quantum Hall breakdown

Resistively-detected NMR (RDNMR) is a unique characterization method enabling highly-sensitive NMR detection for a single quantum nanostructure, such as a quantum point contact (QPC). In many studies, we use dynamic nuclear polarization and RDNMR detection in a quantum Hall breakdown regime of a local QPC filling factor of 1 ($ν_{\rm{qpc}} = 1$). However, the lineshapes of RDNMR signal are proved to be complicated and still not fully understood yet. Here, we systematically polarize the nuclear spins by current-pumping from the close vicinity of $ν_{\rm{qpc}} = 1$ conductance plateau all the way down to pinch-off point, providing a clear evidence that the spin-flip scattering between two edge channels at the lowest Landau level still occurs in the constriction even when it is close to the pinch off point ($G \approx 10^{-2}$ $2e^{2}/h$). The collected RDNMR spectra reveal two sets of distinguished features. First, in a strong to intermediate tunneling regime, we observe an ordinary resistance dip lineshape but interestingly its transition frequency follows a snake-like pattern, an indicative of spatial modulation of electron density in the QPC. Second, in a weak tunneling regime, the spectrum turns into a dispersive lineshape which we interpret due to the build up of two sets of nuclear spin polarization that are in contact with different electron spin polarization.

cond-mat.mes-hall↗

arXiv2021

Thermodynamic Signatures of Diagonal Nematicity in RbFe$_2$As$_2$ Superconductor

Electronic nematic states with broken rotational symmetry often emerge in correlated materials. In most iron-based superconductors, the nematic anisotropy is oriented in the Fe-Fe direction of the iron square lattice. Recently, a novel type of nematicity along the diagonal Fe-As direction has been suggested in heavily hole-doped $A$Fe$_2$As$_2$ ($A=$ Rb or Cs). However, the transport studies focusing on the fluctuations of such nematicity have provided controversial results regarding the presence of diagonal nematic order. Here we report high-resolution heat capacity measurements under in-plane field rotation in RbFe$_2$As$_2$. While the temperature dependence of specific heat shows no discernible anomaly associated with the nematic transition, the field-angle dependence of specific heat near the superconducting transition (at $\sim 2.8$ K) reveals clear two-fold oscillations within the plane, providing thermodynamic evidence for the diagonal nematicity. Moreover, we find that Mössbauer spectroscopy sensitively probes the nematic transition at $\sim 50$ K with no evidence of static magnetism. These results imply that the diagonal nematicity in RbFe$_2$As$_2$ has a unique mechanism involving charge degrees of freedom, having unusual thermodynamic properties of the transition.

cond-mat.supr-con↗

arXiv2021

Strongly correlated superconductivity in a copper-based metal-organic framework with a perfect kagome lattice

Metal-organic frameworks (MOFs), which are self-assemblies of metal ions and organic ligands, provide a tunable platform to search a new state of matter. A two-dimensional (2D) perfect kagome lattice, whose geometrical frustration is a key to realizing quantum spin liquids, has been formed in the $π$-${d}$ conjugated 2D MOF [Cu$_{3}$(C$_{6}$S$_{6}$)]$_{n}$ (Cu-BHT). The recent discovery of its superconductivity with a critical temperature $T_{\rm c}$ of 0.25\,kelvin raises fundamental questions about the nature of electron pairing. Here, we show that Cu-BHT is a strongly correlated unconventional superconductor with extremely low superfluid density. A nonexponential temperature dependence of superfluid density is observed, indicating the possible presence of superconducting gap nodes. The magnitude of superfluid density is much smaller than those in conventional superconductors, and follows the Uemura's relation of strongly correlated superconductors. These results imply that the unconventional superconductivity in Cu-BHT originates from electron correlations related to spin fluctuations of kagome lattice.

cond-mat.str-el↗

arXiv2020

Measurement of $J/ψ$ at forward and backward rapidity in $p$+$p$, $p$$+A$l, $p$$+A$u, and $^3$He+Au collisions at $\sqrt{s_{_{NN}}}=200~{\rm GeV}$

Charmonium is a valuable probe in heavy-ion collisions to study the properties of the quark gluon plasma, and is also an interesting probe in small collision systems to study cold nuclear matter effects, which are also present in large collision systems. With the recent observations of collective behavior of produced particles in small system collisions, measurements of the modification of charmonium in small systems have become increasingly relevant. We present the results of $J/ψ$ measurements at forward and backward rapidity in various small collision systems, $p$$+$$p$, $p$$+$Al, $p$$+$Au and $^3$He$+$Au, at $\sqrt{s_{_{NN}}}$=200 GeV. The results are presented in the form of the observable $R_{AB}$, the nuclear modification factor, a measure of the ratio of the $J/ψ$ invariant yield compared to the scaled yield in $p$$+$$p$ collisions. We examine the rapidity, transverse momentum, and collision centrality dependence of nuclear effects on $J/ψ$ production with different projectile sizes $p$ and $^3$He, and different target sizes Al and Au. The modification is found to be strongly dependent on the target size, but to be very similar for $p$$+$Au and $^{3}$He$+$Au. However, for 0%--20% central collisions at backward rapidity, the modification for $^{3}$He$+$Au is found to be smaller than that for $p$$+$Au, with a mean fit to the ratio of $0.89\pm0.03$(stat)${\pm}0.08$(syst), possibly indicating final state effects due to the larger projectile size.

hep-ex↗

arXiv2019

Probing breakdown of topological protection: Filling-factor-dependent evolution of robust quantum Hall incompressible phases

The integer quantum Hall (QH) effects characterized by topologically quantized and nondissipative transport are caused by an electrically insulating incompressible phase that prevents backscattering between chiral metallic channels. We probed the incompressible area susceptible to the breakdown of topological protection using a scanning gate technique incorporating nonequilibrium transport. The obtained pattern revealed the filling-factor ($ν$)-dependent evolution of the microscopic incompressible structures located along the edge and in the bulk region. We found that these specific structures, respectively attributed to the incompressible edge strip and bulk localization, show good agreement in terms of $ν$-dependent evolution with a calculation of the equilibrium QH incompressible phases, indicating the robustness of the QH incompressible phases under the nonequilibrium condition. Further, we found that the $ν$ dependency of the incompressible patterns is, in turn, destroyed by a large imposed current during the deep QH effect breakdown. These results demonstrate the ability of our method to image the microscopic transport properties of a topological two-dimensional system.

cond-mat.mes-hall↗

arXiv2019

Multi-particle azimuthal correlations for extracting event-by-event elliptic and triangular flow in Au$+$Au collisions at $\sqrt{s_{_{NN}}}=200$ GeV

We present measurements of elliptic and triangular azimuthal anisotropy of charged particles detected at forward rapidity $1<|η|<3$ in Au$+$Au collisions at $\sqrt{s_{_{NN}}}=200$ GeV, as a function of centrality. The multiparticle cumulant technique is used to obtain the elliptic flow coefficients $v_2\{2\}$, $v_2\{4\}$, $v_2\{6\}$, and $v_2\{8\}$, and triangular flow coefficients $v_3\{2\}$ and $v_3\{4\}$. Using the small-variance limit, we estimate the mean and variance of the event-by-event $v_2$ distribution from $v_2\{2\}$ and $v_2\{4\}$. In a complementary analysis, we also use a folding procedure to study the distributions of $v_2$ and $v_3$ directly, extracting both the mean and variance. Implications for initial geometrical fluctuations and their translation into the final state momentum distributions are discussed.

nucl-ex↗

arXiv2018

Pseudorapidity dependence of particle production and elliptic flow in asymmetric nuclear collisions of $p$$+$Al, $p$$+$Au, $d$$+$Au, and $^{3}$He$+$Au at $\sqrt{s_{_{NN}}}=200$ GeV

Asymmetric nuclear collisions of $p$$+$Al, $p$$+$Au, $d$$+$Au, and $^{3}$He$+$Au at $\sqrt{s_{_{NN}}}=200$ GeV provide an excellent laboratory for understanding particle production, as well as exploring interactions among these particles after their initial creation in the collision. We present measurements of charged hadron production $dN_{\rm ch}/dη$ in all such collision systems over a broad pseudorapidity range and as a function of collision multiplicity. A simple wounded quark model is remarkably successful at describing the full data set. We also measure the elliptic flow $v_{2}$ over a similarly broad pseudorapidity range. These measurements provide key constraints on models of particle emission and their translation into flow.

nucl-ex↗

arXiv2018

Measurements of mass-dependent azimuthal anisotropy in central $p$$+$Au, $d$$+$Au, and $^3$He$+$Au collisions at $\sqrt{s_{_{NN}}}=200$ GeV

We present measurements of the transverse-momentum dependence of elliptic flow $v_2$ for identified pions and (anti)protons at midrapidity ($|η|<0.35$), in 0%--5% central $p$$+$Au and $^3$He$+$Au collisions at $\sqrt{s_{_{NN}}}=200$ GeV. When taken together with previously published measurements in $d$$+$Au collisions at $\sqrt{s_{_{NN}}}=200$ GeV, the results cover a broad range of small-collision-system multiplicities and intrinsic initial geometries. We observe a clear mass-dependent splitting of $v_2(p_{T})$ in $d$$+$Au and $^3$He$+$Au collisions, just as in large nucleus-nucleus ($A$$+$$A$) collisions, and a smaller splitting in $p$$+$Au collisions. Both hydrodynamic and transport model calculations successfully describe the data at low $p_T$ ($< 1.5$ GeV/$c$), but fail to describe various features at higher $p_T$. In all systems, the $v_2$ values follow an approximate quark-number scaling as a function of the hadron transverse kinetic energy per constituent quark($KE_T/n_q$), which was also seen previously in $A$$+$$A$ collisions.

nucl-ex↗

arXiv2017

Crystallization and vitrification of electrons in a glass-forming charge liquid

Charge ordering (CO) is a phenomenon in which electrons in solids crystallize into a periodic pattern of charge-rich and charge-poor sites owing to strong electron correlations. This usually results in long-range order. In geometrically frustrated systems, however, a glassy electronic state without long-range CO has been observed. We found that a charge-ordered organic material with an isosceles triangular lattice shows charge dynamics associated with crystallization and vitrification of electrons, which can be understood in the context of an energy landscape arising from the degeneracy of various CO patterns. The dynamics suggest that the same nucleation and growth processes that characterize conventional glass-forming liquids guide the crystallization of electrons. These similarities may provide insight into our understanding of the liquid-glass transition.

cond-mat.str-el↗

arXiv2017

Dimer-Mott and charge-ordered insulating states in the quasi-one-dimensional organic conductors $δ'_{P}$- and $δ'_{C}$-(BPDT-TTF)$_2$ICl$_2$

We investigated the electronic states of the quasi-one-dimensional organic conductors $δ'_{P}$-(BPDT-TTF)$_2$ICl$_2$ and $δ'_{C}$-(BPDT-TTF)$_2$ICl$_2$, both of which are insulating at room temperature owing to strong electron correlations. Through measurements of electrical resistivity, optical conductivity, and magnetic susceptibility, as well as band-structure calculations, we have revealed that the two materials possess completely different ground states, even though they have the same chemical composition and stacking configuration of the donor molecules. We have found that the $δ_P'$-type salt with an effective half-filled band behaves as a dimer-Mott (DM) insulator and exhibits a nonmagnetic transition at 25 K, whereas the $δ'_C$-type salt with a 3/4-filled band shows a charge ordering (CO) transition just above room temperature and becomes nonmagnetic below 20 K. The optical spectra of the $δ_P'$-type salt are composed of two characteristic bands due to intra- and interdimer charge transfers, supporting the DM insulating behavior arising from the strong on-site Coulomb interaction. By contrast, in the $δ'_C$-type salt, a single band characterizing the formation of CO arising from the off-site Coulomb interactions is observed. Upon lowering the temperature, the shape of the optical spectra in the $δ_C'$-type salt becomes asymmetric and shifts to much lower frequencies, suggesting the emergence of domain-wall excitations with fractional charges expected in a one-dimensional CO chain. The temperature dependence of the magnetic susceptibility of the $δ_P'$-type salt is well described by a 2D spin-1/2 Heisenberg AFM model on an anisotropic square lattice in the dimerized picture, while in the $δ_C'$-type salt, it can be explained by a 2D spin-1/2 Heisenberg AFM model on an anisotropic honeycomb lattice formed in the CO state.

cond-mat.str-el↗

arXiv2017

Quantum-disordered state of magnetic and electric dipoles in a hydrogen-bonded Mott system

Strongly enhanced quantum fluctuations often lead to a rich variety of quantum-disordered states. A representative case is liquid helium, in which zero-point vibrations of the helium atoms prevent its solidification at low temperatures. A similar behaviour is found for the internal degrees of freedom in electrons. Among the most prominent is a quantum spin liquid (QSL), in which localized spins are highly correlated but fluctuate even at absolute zero. Recently, a coupling of spins with other degrees of freedom has been proposed as an innovative approach to generate even more fascinating QSLs such as orbital--spin liquids. However, such ideas are limited to the internal degrees of freedom in electrons. Here, we demonstrate that a coupling of localized spins with the zero-point motion of hydrogen atoms (proton fluctuations) in a hydrogen-bonded organic Mott insulator provides a new class of QSLs. We find that a divergent dielectric behaviour towards a hydrogen-bond order is suppressed by the quantum proton fluctuations, resulting in a quantum paraelectric (QPE) state. Furthermore, our thermal-transport measurements reveal that a QSL state with gapless spin excitations rapidly emerges upon entering the QPE state. These findings indicate that the quantum proton fluctuations give rise to a novel QSL --- a quantum-disordered state of magnetic and electric dipoles --- through the coupling between the electron and proton degrees of freedom.

cond-mat.str-el↗

arXiv2017

Measurements of double-helicity asymmetries in inclusive $J/ψ$ production in longitudinally polarized $p+p$ collisions at $\sqrt{s}=510$ GeV

We report the double helicity asymmetry, $A_{LL}^{J/ψ}$, in inclusive $J/ψ$ production at forward rapidity as a function of transverse momentum $p_T$ and rapidity $|y|$. The data analyzed were taken during $\sqrt{s}=510$ GeV longitudinally polarized $p$$+$$p$ collisions at the Relativistic Heavy Ion Collider (RHIC) in the 2013 run using the PHENIX detector. At this collision energy, $J/ψ$ particles are predominantly produced through gluon-gluon scatterings, thus $A_{LL}^{J/ψ}$ is sensitive to the gluon polarization inside the proton. We measured $A_{LL}^{J/ψ}$ by detecting the decay daughter muon pairs $μ^+ μ^-$ within the PHENIX muon spectrometers in the rapidity range $1.2<|y|<2.2$. In this kinematic range, we measured the $A_{LL}^{J/ψ}$ to be $0.012 \pm 0.010$~(stat)~$\pm$~$0.003$(syst). The $A_{LL}^{J/ψ}$ can be expressed to be proportional to the product of the gluon polarization distributions at two distinct ranges of Bjorken $x$: one at moderate range $x \approx 0.05$ where recent RHIC data of jet and $π^0$ double helicity spin asymmetries have shown evidence for significant gluon polarization, and the other one covering the poorly known small-$x$ region $x \approx 2\times 10^{-3}$. Thus our new results could be used to further constrain the gluon polarization for $x< 0.05$.

hep-ex↗