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K. I. Kugel

Publications and source records attributed to K. I. Kugel.

At least 37 records · Page 2Linked to original sources

Thermodynamics of symmetric spin--orbital model: One- and two-dimensional cases

The specific heat and susceptibilities for the two- and one-dimensional spin--orbital models are calculated in the framework of a spherically symmetric self-consistent approach at different temperatures and relations between the parameters of the system. It is shown that even in the absence of the long-range spin and orbital order, the system exhibits the features in the behavior of thermodynamic characteristics, which are typical of those manifesting themselves at phase transitions. Such features are attributed to the quantum entanglement of the coupled spin and orbital degrees of freedom.

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Observation of sub-kelvin superconductivity in Cd$_3$As$_2$ thin films

We report the first experimental observation of superconductivity in Cd$_3$As$_2$ thin films without application of external pressure. Surface studies suggest that the observed transport characteristics are related to the polycrystalline continuous part of investigated films with homogeneous distribution of elements and the Cd-to-As ratio close to stoichiometric Cd$_3$As$_2$. The latter is also supported by Raman spectra of the studied films, which are similar to those of Cd$_3$As$_2$ single crystals. The formation of superconducting phase in films under study is confirmed by the characteristic behavior of temperature and magnetic field dependence of samples resistances, as well as by the presence of pronounced zero-resistance plateaux in $dV/dI$ characteristics. The corresponding $H_c-T_c$ plots reveal a clearly pronounced linear behavior within the intermediate temperature range, similar to that observed for bulk Cd$_3$As$_2$ and Bi$_2$Se$_3$ films under pressure, suggesting the possibility of nontrivial pairing in the films under investigation. We discuss a possible role of sample inhomogeneities and crystal strains in the observed phenomena.

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Spin-valley half-metal in systems with Fermi surface nesting

Half-metals have fully spin polarized charge carriers at the Fermi surface. Such polarization usually occurs due to strong electron--electron correlations. Recently [Phys. Rev. Lett. {\bf{119}}, 107601 (2017)], we have demonstrated theoretically that adding (or removing) electrons to systems with Fermi surface nesting also stabilizes the half-metallic states even in the weak-coupling regime. In the absence of doping, the ground state of the system is a spin or charge density wave, formed by four nested bands. Each of these bands is characterized by charge (electron/hole) and spin (up/down) labels. Only two of these bands accumulate charge carriers introduced by doping, forming a half-metallic two-valley Fermi surface. Analysis demonstrates that two types of such half-metallicity can be stabilized. The first type corresponds to the full spin polarization of the electrons and holes at the Fermi surface. The second type, with antiparallel spins in electron-like and hole-like valleys, is referred to as a "spin-valley half-metal" and corresponds to the complete polarization with respect to the spin-valley operator. We analyze spin and spin-valley currents and possible superconductivity in these systems. We show that spin or spin-valley currents can flow in both half-metallic phases.

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Collective magnetic response of inhomogeneous nanoisland FeNi films around the percolation transition

By using superconducting quantum interference device (SQUID) magnetometry we investigated anisotropic high-field (H < 7 T) low-temperature (10 K) magnetization response of inhomogeneous nanoisland FeNi films grown by rf sputtering deposition on Sitall (TiO2) glass substrates. In the grown FeNi films, the FeNi layer nominal thickness varied from 0.6 to 2.5 nm, across the percolation transition at the d_c=1.8 nm. We discovered that, beyond conventional spin-magnetism of Fe21Ni79 permalloy, the extracted out-of-plane magnetization response of the nanoisland FeNi films is not saturated in the range of investigated magnetic fields and exhibits paramagnetic-like behavior. We found that the anomalous out-of-plane magnetization response exhibits an escalating slope with increase in the nominal film thickness from 0.6 to 1.1 nm, however, it decreases with further increase in the film thickness, and then practically vanishes on approaching the FeNi film percolation threshold. At the same time, the in-plane response demonstrates saturation behavior above 1.5-2 T, competing with anomalously large diamagnetic-like response, which becomes pronounced at high magnetic fields. It is possible that the supported-metal interaction leads to the creation of a thin charge-transfer (CT) layer and a Schottky barrier at the FeNi film/Sitall (TiO2) interface. Then, in the system with nanoscale circular domains, the observed anomalous paramagnetic-like magnetization response can be associated with a large orbital moment of the localized electrons. The observed magnetization response is determined by the interplay between the paramagnetic- and diamagnetic-like contributions.

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Quantum phase transitions and the degree of nonidentity in the system with two different species of vector bosons

We address the system with two species of vector bosons in an optical lattice. In addition to the the standard parameters characterizing such a system, we are dealing here with the "degree of atomic nonidentity", manifesting itself in the difference of tunneling amplitudes and on-site Coulomb interactions. We obtain a cascade of quantum phase transitions occurring with the increase in the degree of atomic nonidentity. In particular, we show that the phase diagram for strongly distinct atoms is qualitatively different from that for (nearly) identical atoms considered earlier. The resulting phase diagrams evolve from the images similar to the "J. Miró-like paintings" to "K. Malewicz-like" ones.

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Magnetic and magnetotransport properties of Bi$_2$Se$_3$ thin films doped by Eu

Structural, magnetic and magnetotransport properties of (Bi$_{1-x}$Eu$_x$)$_2$Se$_3$ thin films have been studied experimentally as a function of Eu content. The films were synthesized by MBE. It is demonstrated that Eu distribution is not uniform, it enter quint-layers forming inside them plain (pancake-like) areas containing Eu atoms, which sizes and concentration increase with the growth of Eu content. Positive magnetoresistance related to the weak antilocalization was observed up to 15K. The antilocalization was not followed by weak localization as theory predicts for nontrivial topological states. Surprisingly, the features of antilocalization were seen even at Eu content $x$ $=$ 0.21. With the increase of Eu content the transition to ferromagnetic state occurs at $x$ about 0.1 and with the Curie temperature $\approx$ 8K, that rises up to 64K for $x$ $=$ 0.21. At temperatures above 1-2 K, the dephasing length is proportional to $T^{-1/2}$ indicating the dominant contribution of inelastic $e-e$ scattering into electron phase breaking. However, at low temperatures the dephasing length saturates, that could be due to the scattering on magnetic ions.

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Magnetic phase diagram and quantum phase transitions in a two-species boson model

We analyze the possible types of ordering in a boson--fermion model. The Hamiltonian is inherently related to the Bose--Hubbard model for vector two-species bosons in optical lattices. We show that such model can be reduced to the Kugel--Khomskii type spin--pseudospin model, but in contrast to the usual version of the latter model, we are dealing here with the case of spin $S=1$ and pseudospin $1/2$. We show that the interplay of spin and pseudospin degrees of freedom leads to a rather nontrivial magnetic phase diagram including the spin-nematic configurations. Tuning the spin-channel interaction parameter $U_s$ gives rise to quantum phase transitions. We find that the ground state of the system always has the pseudospin domain structure. On the other hand, the sign change of $U_s$ switches the spin arrangement of the ground state within domains from ferro- to aniferromagnetic one. Finally, we revisit the spin (pseudospin)-1/2 Kugel--Khomskii model and see the inverse picture of phase transitions.

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Spin-valley half-metal as a prospective material for spin-valley-tronics

Half-metallicity (full spin polarization of the Fermi surface) usually occurs in strongly correlated electron systems. We demonstrate that doping a spin-density wave insulator in the weak-coupling regime may also stabilize half-metallic states. The undoped spin-density wave is formed by four nested bands [i.e., each band is characterized by charge (electron/hole) and spin (up/down) labels]. Of these four bands only two accumulate the doped carriers, forming a half-metallic two-valley Fermi surface. Depending on parameters, the spin polarizations of the electron-like and hole-like valleys may be (i) parallel or (ii) antiparallel. The Fermi surface of (i) is fully spin-polarized (similar to usual half-metals). Case (ii), referred to as "a spin-valley half-metal", corresponds to complete polarization with respect to the spin-valley operator. The properties of these states are discussed.

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Magnetic field effects in electron systems with imperfect nesting

We analyze the effects of an applied magnetic field on the phase diagram of a weakly-correlated electron system with imperfect nesting. The Hamiltonian under study describes two bands: electron and hole ones. Both bands have spherical Fermi surfaces, whose radii are slightly mismatched due to doping. These types of models are often used in the analysis of magnetic states in chromium and its alloys, superconducting iron pnictides, AA-type bilayer graphene, borides, etc. At zero magnetic field, the uniform ground state of the system turns out to be unstable against electronic phase separation. The applied magnetic field affects the phase diagram in several ways. In particular, the Zeeman term stabilizes new antiferromagnetic phases. It also significantly shifts the boundaries of inhomogeneous (phase-separated) states. At sufficiently high fields, the Landau quantization gives rise to oscillations of the order parameters and of the Néel temperature as a function of the magnetic field.

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Floquet spectrum and driven conductance in Dirac materials: Effects of Landau-Zener-Stückelberg-Majorana interferometry

Using the Landau-Zener-Stückelberg-Majorana-type (LZSM) semiclassical approach, we study both graphene and a thin film of a Weyl semimetal subjected to a strong AC electromagnetic field. The spectrum of quasi energies in the Weyl semimetal turns out to be similar to that of a graphene sheet. Earlier it has been predicted qualitatively that the transport properties of strongly-irradiated graphene oscillate as a function of the radiation intensity [S.V. Syzranov et al., Phys. Rev. B 88, 241112 (2013)]. Here we obtain rigorous quantitative results for a driven linear conductance of graphene and a thin film of a Weyl semimetal. The exact quantitative structure of oscillations exhibits two contributions. The first one is a manifestation of the Ramsauer-Townsend effect, while the second contribution is a consequence of the LZSM interference defining the spectrum of quasienergies.

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Role of local geometry in spin and orbital structure of transition metal compounds

We analyze the role of local geometry in the spin and orbital interaction in transition metal compounds with orbital degeneracy. We stress that the tendency observed for the most studied case (transition metals in O$_6$ octahedra with one common oxygen -- common corner of neighboring octahedra and with $\sim 180^{\circ}$ metal--oxygen--metal bonds), that ferro-orbital ordering renders antiferro-spin coupling, and, {\it vice versa}, antiferro-orbitals give ferro-spin ordering, is not valid in general case, in particular for octahedra with common edge and with $\sim 90^{\circ}$ M--O--M bonds. Special attention is paid to the ``third case'', neighboring octahedra with common face (three common oxygens) -- the case practically not considered until now, although there are many real systems with this geometry. Interestingly enough, the spin--orbital exchange in this case turns out to be to be simpler and more symmetric than in the first two cases. We also consider, which form the effective exchange takes for different geometries in case of strong spin--orbit coupling.

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Anomalous Hall effect in a 2D magnetic semiconductor hetereostructure: Evidence of Berry phase effects in the hopping-transport regime

The temperature and magnetic field dependences of the anomalous Hall effect (AHE) are studied in Mn delta-doped semiconductor heterostructures with a two-dimensional hole gas in a quantum well interacting with the Mn layer. The analysis of experimental data reveals four distinct temperature ranges differing in the behavior of AHE. The Mn layer induces an inhomogeneity of the hole gas leading to an interplay between the hopping and drift conductivities. It is shown that at sufficiently low temperatures, hopping conductivity favors the mechanisms of AHE related to the geometric (Berry-Pancharatnam) phase.

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Effects of anisotropy and disorder on the conductivity of Weyl semimetals

We study dc conductivity of a Weyl semimetal with uniaxial anisotropy (Fermi velocity ratio $ξ= v_\bot/v_\parallel\neq1$) considering the scattering of charge carriers by a wide class of impurity potentials, both short- and long-range. We obtain the ratio of transverse and longitudinal (with respect to the anisotropy axis) conductivities as a function of both $ξ$ and temperature. We find that the transverse and longitudinal conductivities exhibit different temperature dependence in the case of short-range disorder. For general long-range disorder, the temperature dependence ($\sim T^4$) of the conductivity turns out to be insensitive of the anisotropy in the limits of strong ($ξ\gg$ and $\ll1$) and weak ($ξ\approx1$) anisotropy.

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Spin--orbital interaction for face-sharing octahedra: Realization of a highly symmetric SU(4) model

Specific features of orbital and spin structure of transition metal compounds in the case of the face-sharing MO$_6$ octahedra are analyzed. In this geometry, we consider the form of the spin--orbital Hamiltonian for transition metal ions with double ($e_g^σ$) or triple ($t_{2g}$) orbital degeneracy. Trigonal distortions typical of the structures with face-sharing octahedra lead to splitting of $t_{2g}$ orbitals into an $a_{1g}$ singlet and $e_g^π$ doublet. For both doublets ($e_g^σ$ and $e_g^π$), in the case of one electron or hole per site, we arrive at a symmetric model with the orbital and spin interaction of the Heisenberg type and the Hamiltonian of unexpectedly high symmetry: SU(4). Thus, many real materials with this geometry can serve as a testing ground for checking the prediction of this interesting theoretical model. We also compare general trends in spin--orbital ("Kugel--Khomskii") exchange interaction for three typical situations: those of MO$_6$ octahedra with common corner, common edge, and the present case of common face, which has not been considered yet.

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Resonant indirect exchange via remote 2D channel

We apply the previously developed theory of the resonant indirect exchange interaction to explain the ferromagnetic properties of the hybrid heterostructure consisting of a InGaAs-based quantum well (QW) sandwiched between GaAs barriers with a remote Mn delta-layer. The experimentally obtained dependence of the Curie temperature on the QW depth exhibits a maximum related to the region of resonant indirect exchange. We suggest the theoretical explanantion and a fit to this dependence as a result of the two contributions to ferromagnetism - the intralayer contribution and the resonant exchange contribution provided by the QW.

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Intrinsic arrested nanoscale phase separation near a topological Lifshitz transition in strongly correlated two-band metals

The arrested nanoscale phase separation in a two-band Hubbard model for strongly correlated charge carriers is shown to occur in a particular range in vicinity of the topological Lifshitz transition, where the Fermi energy crosses the bottom of the narrow band and a new sheet of the Fermi surface related to the charge carriers of the second band comes into play. We determine the phase separation diagram of this two-band Hubbard model as a function of two variables, the charge carrier density and the energy shift between the chemical potential and the bottom of the second band. In this phase diagram, we first determine a line of quantum critical points for the Lifshitz transition and find criteria for the electronic phase separation resulting in an inhomogeneous charge distribution. Finally, we identify the critical point in presence of a variable long-range Coulomb interaction where the scale invariance of the coexisting phases with different charge densities appears. We argue that this point is relevant for the regime of scale invariance of the nanoscale phase separation in cuprates like it was first observed in La$_2$CuO$_{4.1}$.

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Elementary Excitations in the Symmetric Spin--Orbital Model

Possible types of elementary excitations in the symmetric spin-orbital model on the a square lattice are analyzed using a spherically symmetric self-consistent approach. The excitation spectra are calculated. The behavior of the corresponding correlation functions depending on the temperature and parameters of the model is studied. A schematic phase diagram is plotted. It is shown that the thermodynamics of the system is mainly determined by elementary excitations with the entangled spin and orbital degrees of freedom.

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Optical evidence of quantum rotor orbital excitations in orthorhombic manganites

In magnetic compounds with Jahn-Teller (JT) ions (such as Mn3+ or Cu2+), the ordering of the electron or hole orbitals is associated with cooperative lattice distortions. There the role of JT effect, although widely recognised, is still elusive in the ground state properties. We suggest that, in these materials, there exist elementary excitations whose energy spectrum is described in terms of the total angular momentum eigenstates and is quantised as in quantum rotors found in JT centers. We observed features originating from these excitations in the optical spectra of a model compound LaMnO3 using ellipsometry technique. They appear clearly as narrow sidebands accompanying the electron transition between the JT split orbitals on neighbouring Mn3+ ions, strongly influenced by anisotropic spin correlations. We present these results together with new experimental data on photoluminescence and its kinetics found in LaMnO3, which lend additional support to the ellipsometry implying the existence of the quantum rotor orbital excitations. We note that the discovered elementary excitations of quantum rotors may play an important role in many unusual properties observed in these materials upon doping, such as high-temperature superconductivity and colossal magnetoresistance.

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