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K. Nomura

Publications and source records attributed to K. Nomura.

At least 73 records · Page 4Linked to original sources

Site-specific $^{13}$C NMR study on locally distorted triangular lattice of organic conductor $κ$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$

To verify the effect of geometrical frustration, we artificially distort the triangular lattice of quasi-two-dimensional organic conductor $κ$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ [BEDT-TTF: bis(ethylenedithio)terathiofulvalene] by analogous-molecular substitution and apply $^{13}$C NMR of bulk and substituted sites, electric conductivity, and static magnetic susceptibility measurements. The results indicate that the magnetic characteristics of the substituted sample are quantitatively similar to those of the pure sample. Moreover the magnetic characteristics at the substituted sites are also the same as in the bulk. These results suggest that the observed magnetic properties may not be due to the geometrical frustration but the importance of disorder.

cond-mat.str-el↗

Shape coexistence in the microscopically guided interacting boson model

Shape coexistence has been a subject of great interest in nuclear physics for many decades. In the context of the nuclear shell model, intruder excitations may give rise to remarkably low-lying excited $0^+$ states associated with different intrinsic shapes. In heavy open-shell nuclei, the dimension of the shell-model configuration space that includes such intruder excitations becomes exceedingly large, thus requiring a drastic truncation scheme. Such a framework has been provided by the interacting boson model (IBM). In this article we address the phenomenon of shape coexistence and its relevant spectroscopy from the point of view of the IBM. A special focus is placed on the method developed recently which makes use of the link between the IBM and the self-consistent mean-field approach based on the nuclear energy density functional. The method is extended to deal with various intruder configurations associated with different equilibrium shapes. We assess the predictive power of the method and suggest possible improvements and extensions, by considering illustrative examples in the neutron-deficient Pb region, where shape coexistence has been experimentally studied.

nucl-th↗

Spectroscopy of quadrupole and octupole states in rare-earth nuclei from a Gogny force

Collective quadrupole and octupole states are described in a series of Sm and Gd isotopes within the framework of the interacting boson model (IBM), whose Hamiltonian parameters are deduced from mean field calculations with the Gogny energy density functional. The link between both frameworks is the ($β_2β_3$) potential energy surface computed within the Hartree-Fock-Bogoliubov framework in the case of the Gogny force. The diagonalization of the IBM Hamiltonian provides excitation energies and transition strengths of an assorted set of states including both positive and negative parity states. The resultant spectroscopic properties are compared with the available experimental data and also with the results of the configuration mixing calculations with the Gogny force within the generator coordinate method (GCM). The structure of excited $0^{+}$ states and its connection with double octupole phonons is also addressed. The model is shown to describe the empirical trend of the low-energy quadrupole and octupole collective structure fairly well, and turns out to be consistent with GCM results obtained with the Gogny force.

nucl-th↗

Evolution of E2 transition strength in deformed hafnium isotopes from new measurements on $^{172}$Hf, $^{174}$Hf, and $^{176}$Hf

The available data for E2 transition strengths in the region between neutron-deficient Hf and Pt isotopes are far from complete. More and precise data are needed to enhance the picture of structure evolution in this region and to test state-of-the-art nuclear models. In a simple model, the maximum collectivity is expected at the middle of the major shell. However, for actual nuclei, this picture may no longer be the case, and one should use a more realistic nuclear-structure model. We address this point by studying the spectroscopy of Hf. We remeasure the 2^+_1 half-lives of 172,174,176Hf, for which there is some disagreement in the literature. The main goal is to measure, for the first time, the half-lives of higher-lying states of the rotational band. The new results are compared to a theoretical calculation for absolute transition strengths. The half-lives were measured using γ-γand conversion-electron-γdelayed coincidences with the fast timing method. For the determination of half-lives in the picosecond region, the generalized centroid difference method was applied. For the theoretical calculation of the spectroscopic properties, the interacting boson model is employed, whose Hamiltonian is determined based on microscopic energy-density functional calculations. The measured 2^+_1 half-lives disagree with results from earlier γ-γfast timing measurements, but are in agreement with data from Coulomb excitation experiments and other methods. Half-lives of the 4^+_1 and 6^+_1 states were measured, as well as a lower limit for the 8^+_1 states. We show the importance of the mass-dependence of effective boson charge in the description of E2 transition rates in chains of nuclei. It encourages further studies of the microscopic origin of this mass dependence. New data on transition rates in nuclei from neighboring isotopic chains could support these studies.

nucl-ex↗

Microscopic description of octupole shape-phase transitions in light actinides and rare-earth nuclei

A systematic analysis of low-lying quadrupole and octupole collective states is presented, based on the microscopic energy density functional framework. By mapping the deformation constrained self-consistent axially symmetric mean-field energy surfaces onto the equivalent Hamiltonian of the $sdf$ interacting boson model (IBM), that is, onto the energy expectation value in the boson condensate state, the Hamiltonian parameters are determined. The study is based on the global relativistic energy density functional DD-PC1. The resulting IBM Hamiltonian is used to calculate excitation spectra and transition rates for the positive- and negative-parity collective states in four isotopic chains characteristic for two regions of octupole deformation and collectivity: Th, Ra, Sm and Ba. Consistent with the empirical trend, the microscopic calculation based on the systematics of $β_{2}$-$β_{3}$ energy maps, the resulting low-lying negative-parity bands and transition rates show evidence of a shape transition between stable octupole deformation and octupole vibrations characteristic for $β_{3}$-soft potentials.

nucl-th↗

Bulk topological insulators as inborn spintronics detectors

Detection and manipulation of electrons' spins are key prerequisites for spin-based electronics or spintronics. This is usually achieved by contacting ferromagnets with metals or semiconductors, in which the relaxation of spins due to spin-orbit coupling limits both the efficiency and the length scale. In topological insulator materials, on the contrary, the spin-orbit coupling is so strong that the spin direction uniquely determines the current direction, which allows us to conceive a whole new scheme for spin detection and manipulation. Nevertheless, even the most basic process, the spin injection into a topological insulator from a ferromagnet, has not yet been demonstrated. Here we report successful spin injection into the surface states of topological insulators by using a spin pumping technique. By measuring the voltage that shows up across the samples as a result of spin pumping, we demonstrate that a spin-electricity conversion effect takes place in the surface states of bulk-insulating topological insulators Bi1.5Sb0.5Te1.7Se1.3 and Sn-doped Bi2Te2Se. In this process, due to the two-dimensional nature of the surface state, there is no spin current along the perpendicular direction. Hence, the mechanism of this phenomenon is different from the inverse spin Hall effect and even predicts perfect conversion between spin and electricity at room temperature. The present results reveal a great advantage of topological insulators as inborn spintronics devices.

cond-mat.mtrl-sci↗

Evidence for shape coexistence in $^{98}$Mo

A $γγ$ angular correlation experiment has been performed to investigate the low-energy states of the nucleus $^{98}$Mo. The new data, including spin assignments, multipole mixing ratios and lifetimes reveal evidence for shape coexistence and mixing in $^{98}$Mo, arising from a proton intruder configuration. This result is reproduced by a theoretical calculation within the proton-neutron interacting boson model with configuration mixing, based on microscopic energy density functional theory. The microscopic calculation indicates the importance of the proton particle-hole excitation across the Z=40 sub-shell closure and the subsequent mixing between spherical vibrational and the $γ$-soft equilibrium shapes in $^{98}$Mo.

nucl-ex↗

Microscopic analysis of the octupole phase transition in Th isotopes

A shape phase transition between stable octupole deformation and octupole vibrations in Th nuclei is analyzed in a microscopic framework based on nuclear density functional theory. The relativistic functional DD-PC1 is used to calculate axially-symmetric quadrupole-octupole constrained energy surfaces. Observables related to order parameters are computed using an interacting-boson Hamiltonian, with parameters determined by mapping the microscopic energy surfaces to the expectation value of the Hamiltonian in the boson condensate. The systematics of constrained energy surfaces and low-energy excitation spectra point to the occurrence of a phase transition between octupole-deformed shapes and shapes characterized by octupole-soft potentials.

nucl-th↗

Mixed Orbital Ground States of Fe2+ in Prussian Blues

We report on the mixed-orbital ground state compounds analogous to the mixed-valence ones. Orbital doublet and singlet ground states of the Fe2+ ion displayed in Moessbauer spectra of the Prussian blue analogues AyFe3-y[Co(CN)6]2xH2O (y<1) are interconverting to each other as temperature changes for A = K, Na. Relative weight of orbital singlet ground states increases with lowering temperature. In the alcali-free cobalticyanides, the Moessbauer spectra are dominated by quadrupole-splt doublets of the same origin with a large splitting characteristic of the Fe2+ species coordinated by two (at least) oxygen atoms of water molecules in cis-configuration. Single type octahedral coordination of Fe2+ is isolated in A-filled cobalticyanides for A=Rb, Cs to be characterized by the narrower quadrupole spectrum associated with the orbital doublet ground states. Ionic exchange of K for Cs in KFe[Co(CN)6]H2O results in predominance of the orbital singlet, i.e., in enhanced anisotropy of the Fe2+ valence electrons. We found hence that the Fe2+ charge distribution can be modified together with crystal size at the step of synthesis owing to distortion isomerism.

cond-mat.mtrl-sci↗

Shape evolution and the role of intruder configurations in Hg isotopes within the interacting boson model based on a Gogny energy density functional

The interacting boson model with configuration mixing, with parameters derived from the self-consistent mean-field calculation employing the microscopic Gogny energy density functional, is applied to the systematic analysis of the low-lying structure in Hg isotopes. Excitation energies, electromagnetic transition rates, deformation properties, and ground-state properties of the $^{172-204}$Hg nuclei are obtained by mapping the microscopic deformation energy surface onto the equivalent IBM Hamiltonian in the boson condensate. These results point to the overall systematic trend of the transition from the near spherical vibrational state in lower-mass Hg nuclei close to $^{172}$Hg, onset of intruder prolate configuration as well as the manifest prolate-oblate shape coexistence around the mid-shell nucleus $^{184}$Hg, weakly oblate deformed structure beyond $^{190}$Hg up to the spherical vibrational structure toward the near semi-magic nucleus $^{204}$Hg, as observed experimentally. The quality of the present method in the description of the complex shape dynamics in Hg isotopes is examined.

nucl-th↗

Shape coexistence in Lead isotopes in the interacting boson model with Gogny energy density functional

We investigate the emergence and evolution of shape coexistence in the neutron-deficient Lead isotopes within the interacting boson model (IBM) plus configuration mixing with microscopic input based on the Gogny energy density functional (EDF). The microscopic potential energy surface obtained from the constrained self-consistent Hartree-Fock-Bogoliubov method employing the Gogny-D1M EDF is mapped onto the coherent-state expectation value of the configuration-mixing IBM Hamiltonian. In this way, the parameters of the IBM Hamiltonian are fixed for each of the three relevant configurations (spherical, prolate and oblate) associated to the mean field minima. Subsequent diagonalization of the Hamiltonian provides the excitation energy of the low-lying states and transition strengths among them. The model predictions for the $0^{+}$ level energies and evolving shape coexistence in the considered Lead chain are consistent both with experiment and with the indications of the Gogny-EDF energy surfaces.

nucl-th↗

Robust Regularity in γ-Soft Nuclei and its Microscopic Realization

γ-softness in atomic nuclei is investigated in the framework of energy density functionals. By mapping constrained microscopic energy surfaces for a set of representative non-axial medium-heavy and heavy nuclei to a Hamiltonian of the proton-neutron interacting boson model (IBM-2) containing up to three-body interactions, low-lying collective spectra and transition rates are calculated. Observables are analyzed that distinguish between the two limiting geometrical pictures of non-axial nuclei: the rigid-triaxial rotor and the γ-unstable rotor. It is shown that neither of these pictures is realized in actual nuclei, and that a microscopic description leads to results that are almost exactly in between the two geometrical limits. This finding points to the optimal choice of the IBM Hamiltonian for γ-soft nuclei.

nucl-th↗

Collective structural evolution in neutron-rich Yb, Hf, W, Os and Pt isotopes

An interacting boson model Hamiltonian determined from Hartree-Fock-Bogoliubov calculations with the new microscopic Gogny energy density functional D1M, is applied to the spectroscopic analysis of neutron-rich Yb, Hf, W, Os and Pt isotopes with mass $A\sim 180-200$. Excitation energies and transition rates for the relevant low-lying quadrupole collective states are calculated by this method. Transitions from prolate to oblate ground-state shapes are analyzed as a function of neutron number $N$ in a given isotopic chain by calculating excitation energies, $B$(E2) ratios, and correlation energies in the ground state. It is shown that such transitions tend to occur more rapidly for the isotopes with lower proton number $Z$, when departing from the proton shell closure Z=82. The triaxial degrees of freedom turn out to play an important role in describing the considered mass region. Predicted low-lying spectra for the neutron-rich exotic Hf and Yb isotopes are presented. The approximations used in the model and the possibilities to refine its predictive power are addressed.

nucl-th↗

Quadrupole Collective Dynamics from Energy Density Functionals: Collective Hamiltonian and the Interacting Boson Model

Microscopic energy density functionals (EDF) have become a standard tool for nuclear structure calculations, providing an accurate global description of nuclear ground states and collective excitations. For spectroscopic applications this framework has to be extended to account for collective correlations related to restoration of symmetries broken by the static mean field, and for fluctuations of collective variables. In this work we compare two approaches to five-dimensional quadrupole dynamics: the collective Hamiltonian for quadrupole vibrations and rotations, and the Interacting Boson Model. The two models are compared in a study of the evolution of non-axial shapes in Pt isotopes. Starting from the binding energy surfaces of $^{192,194,196}$Pt, calculated with a microscopic energy density functional, we analyze the resulting low-energy collective spectra obtained from the collective Hamiltonian, and the corresponding IBM-2 Hamiltonian. The calculated excitation spectra and transition probabilities for the ground-state bands and the $γ$-vibration bands are compared to the corresponding sequences of experimental states.

nucl-th↗

Spectroscopic calculations of the low-lying structure in exotic Os and W isotopes

Structural evolution in neutron-rich Os and W isotopes is investigated in terms of the Interacting Boson Model (IBM) Hamiltonian determined by (constrained) Hartree-Fock-Bogoliubov (HFB) calculations with the Gogny-D1S Energy Density Functional (EDF). The interaction strengths of the IBM Hamiltonian are produced by mapping the potential energy surface (PES) of the Gogny-EDF with quadrupole degrees of freedom onto the corresponding PES of the IBM system. We examine the prolate-to-oblate shape/phase transition which is predicted to take place in this region as a function of neutron number $N$ within the considered Os and W isotopic chains. The onset of this transition is found to be more rapid compared to the neighboring Pt isotopes. The calculations also allow prediction of spectroscopic variables (excited state energies and reduced transition probabilities) which are presented for the neutron-rich $^{192,194,196}$W nuclei, for which there is only very limited experimental data available to date.

nucl-th↗

Structural evolution in Pt isotopes with the Interacting Boson Model Hamiltonian derived from the Gogny Energy Density Functional

Spectroscopic calculations are carried out, for the description of the shape/phase transition in Pt nuclei in terms of the Interacting Boson Model (IBM) Hamiltonian derived from (constrained) Hartree-Fock-Bogoliubov (HFB) calculations with the finite range and density dependent Gogny-D1S Energy Density Functional. Assuming that the many-nucleon driven dynamics of nuclear surface deformation can be simulated by effective bosonic degrees of freedom, the Gogny-D1S potential energy surface (PES) with quadrupole degrees of freedom is mapped onto the corresponding PES of the IBM. Using this mapping procedure, the parameters of the IBM Hamiltonian, relevant to the low-lying quadrupole collective states, are derived as functions of the number of valence nucleons. Merits of both Gogny-HFB and IBM approaches are utilized so that the spectra and the wave functions in the laboratory system are calculated precisely. The experimental low-lying spectra of both ground-state and side-band levels are well reproduced. From the systematics of the calculated spectra and the reduced E2 transition probabilities $B$(E2), the prolate-to-oblate shape/phase transition is shown to take place quite smoothly as a function of neutron number $N$ in the considered Pt isotopic chain, for which the $γ$-softness plays an essential role. All these spectroscopic observables behave consistently with the relevant PESs and the derived parameters of the IBM Hamiltonian as functions of $N$. Spectroscopic predictions are also made for those nuclei which do not have enough experimental E2 data.

nucl-th↗

Spin-Orbit Interaction Enhanced Fractional Quantum Hall States in the Second Landau Level

We study the fractional quantum Hall effect at filling fractions 7/3 and 5/2 in the presence of the spin-orbit interaction, using the exact diagonalization method and the density matrix renormalization group (DMRG) method in a spherical geometry. Trial wave functions at these fillings are the Laughlin state and the Moore-Reed-Pfaffian state. The ground state excitation energy gaps and pair-correlation functions at fractional filling factor 7/3 and 5/2 in the second Landau level are calculated. We find that the spin-orbit interaction stabilizes the fractional quantum Hall states.

cond-mat.str-el↗

Manganite charge and orbitally ordered and disordered states probed by Fe substitution into Mn site in LnBaMn1.96Fe0.04O5, LnBaMn1.96Fe0.04O6 and LnBaMn1.96Fe0.04O5.5 (Ln=Y, Gd, Sm, Nd, Pr, La)

The layered manganese oxides LnBaMn1.96Fe0.04Oy (Ln=Y, Gd, Sm, Nd, Pr, La) have been synthesized for y=5, 5.5 and 6. In the oxygen-saturated state (y=6) they exhibit the charge and orbital order at ambient temperature for Ln=Y, Gd, Sm, but unordered eg-electronic system for Ln=La,Pr,Nd. Fourfold increase of quadrupole splitting was observed owing to the charge and orbital ordering. This is in agreement with the jumplike increase in distortion of the reduced perovskite-like cell for the charge and orbitally ordered manganites compared to the unordered ones. Substitution of 2 percents of Mn by Fe suppresses the temperatures of structural and magnetic transitions by 20 to 50 K. Parameters of the crystal lattices and the room-temperature Mössbauer spectra were studied on forty samples whose structures were refined within five symmetry groups: P4/mmm, P4/nmm, Pm-3m, Icma and P2/m. Overwhelming majority of the Fe species are undifferentiated in the Mössbauer spectra for most of the samples. Such the single-component spectra in the two-site structures are explained by the preference of Fe towards the site of Mn(III) and by the segmentation of the charge and orbitally ordered domains.

cond-mat.str-el↗