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K. Pomorski

Publications and source records attributed to K. Pomorski.

At least 19 recordsLinked to original sources

From Superfluid Coherence to High-$K$ Fragment Channels at Nuclear Scission

The origin of fission-fragment spin remains unresolved. For $^{236}$U fission, we combine deformation-dependent finite-temperature pairing with a multidimensional scission-spectrum analysis. Near the pairing-quenching boundary, pair breaking exposes near-Fermi high-$\Omega$ intruder orbitals and opens high-$K$ channels. The resulting maximum spectroscopic capacities range from a few to more than a dozen units of $\hbar$. Rapid neck rupture acts as a non-adiabatic projection freeze-out, where pairing serves as a dynamical gate: its critical attenuation does not generate angular momentum but allows existing high-$K$ projections to be retained diabatically as local fragment-$K$ components while total angular momentum remains conserved.

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Sensitivity of Isotopic Fission Yields in Actinides to the Macroscopic Liquid-Drop Model: LSD vs ISOLDA

The impact of the macroscopic liquid-drop prescription on isotope-resolved fission-fragment yields in the actinide region is assessed by comparing two alternative parameterizations: the Lublin--Strasbourg Drop (LSD) model and the ISOscalar Liquid Drop Approximation (ISOLDA). The two prescriptions differ primarily in the treatment of isospin dependence in the volume and surface terms; in ISOLDA, an explicit dependence on the isospin square $T(T+1)$, where $T=|N-Z|/2$, is introduced in both coefficients. Using an identical set of fragment-yield observables and the same experimental reference (fission of $^{250}$Cf$^*$ at low and high energies), the propagation of the macroscopic-energy choice into the predicted yields is quantified in terms of (i) the location of the most probable post-neutron isotopes along elemental chains, (ii) the widths and asymmetries of the isotopic distributions, and (iii) the population of neighboring nuclides on the distribution tails. A comparable description of the gross properties of the isotopic yield pattern is obtained with both prescriptions, particularly for light and intermediate fragments, where peak positions and near-maximum curvatures are reproduced similarly. The most discriminating differences are found for heavy-fragment chains, for which the ridge location and isotopic centroids are rendered more sensitive to macroscopic isospin terms. Overall, a closer average agreement with the evaluated data is obtained with LSD, while the LSD--ISOLDA spread is shown to provide a practical estimate of the macroscopic-model uncertainty in isotope-resolved yields.

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Comparative Study of Langevin and Random Walk Models for Nuclear Fission in the Overdamped Regime

We present a comparative study of Langevin dynamics and a Metropolis random walk model applied to thermal neutron-induced fission of $^{229}$Th, $^{235}$U, $^{239}$Pu, $^{245}$Cm, $^{249}$Cf, and $^{255}$Fm. Both methods are implemented within an identical four-dimensional Fourier-over-Spheroid framework, using potential energy surfaces derived from the macroscopic-microscopic model. We show that the Metropolis walk corresponds to the overdamped limit of the Langevin equations and confirm this correspondence numerically by Langevin calculations performed in the strongly damped regime and with quantum corrections to the random force switched off. Under these conditions, the two approaches produce essentially identical mass distributions for the lighter actinides. Systematic deviations develop for the heavier actinides, where the Langevin dynamics yields a non-negligible symmetric fission component absent in the random walk results. We trace this difference to the kinematic structure of the Metropolis sampling and to the residual inertial dynamics retained in the Langevin framework. A parallel comparison of Langevin calculations with and without the quantum-corrected effective temperature $T^*$ isolates the contribution of zero-point fluctuations and suggests that their standard phenomenological treatment may overestimate their impact in certain cases. Both approaches qualitatively reproduce the asymmetric peak positions and their systematic evolution across the actinide chain, while a common quantitative limitation -- the narrowness of the predicted distributions -- points to the role of higher-dimensional deformation modes not included in the present parametrization.

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Survival of Pairing Correlations and Shell Effects at Scission in Finite-Temperature Nuclear Fission: Implications for Odd-Even Staggering

We investigate the finite-temperature evolution of microscopic free-energy corrections in nuclear fission, focusing on pairing and shell effects near scission. The analysis is based on a finite-temperature BCS treatment combined with the Strutinsky method and is performed for representative deformation points along the fission path. Both pairing and shell contributions exhibit regular thermal attenuation, but their deformation dependencies differ substantially. In particular, pairing remains strongly deformation-dependent in the scission region, and its free-energy contribution differs markedly between the constant and surface-dependent pairing-strength prescriptions. The shell correction near scission is also significant at low temperature and is progressively suppressed with increasing excitation energy. These results support the interpretation of odd-even staggering in fragment charge yields as a manifestation of pairing correlations surviving into the strongly deformed pre-scission configuration. They also show that pairing and shell effects should be treated separately in finite-temperature dynamical calculations, with distinct deformation- and temperature-dependent attenuation laws.

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Isotope-Resolved Ba and Xe Yields in Actinide Fission and Correlated Heavy--Light Fragment Systematics

Isotope-resolved post-neutron fission yields in the Ba and Xe chains are calculated and benchmarked against evaluated reference data, with emphasis on element-resolved isotopic chains $Y(N_f)$ at fixed fragment charge $Z$ and on the consistency of heavy--light fragment correlations. Calculations are performed within a four-dimensional (4D) Langevin framework employing Fourier-over-Spheroid shape parametrization. The benchmark covers spontaneous fission of selected Cm and Cf isotopes (including $^{244,246}$Cm and $^{250}$Cf) as well as neutron-induced fission at thermal and 14-MeV energies for representative actinides in the Th--Pu region (including $^{229}$Th, $^{235}$U, $^{239}$Pu, and $^{249}$Cf). The dominant neutron-number maxima are reproduced for a large fraction of the isotopic chains considered, indicating that the mean charge partition and the average neutron content of the main fission channels are described consistently. A systematic residual discrepancy is observed in the isotopic widths: the calculated yields often fall off too rapidly on the distribution tails, producing distributions that are narrower than the evaluated data, most notably for heavy-fragment chains.

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Static Fission Properties of Even-Even Actinides within the Warsaw Macroscopic-Microscopic Model Using Fourier-over-Spheroid Parameterization

A systematic study of fission barrier heights and static properties of even-even actinide nuclei from Th to Cf has been performed within the Warsaw macroscopic-microscopic model using the five-dimensional Fourier-over-Spheroid (FoS) shape parameterization. The use of a large deformation grid, containing about $1.3\times10^{8}$ points for each nucleus, allows for a refined and numerically complete exploration of the potential energy landscape without dividing the configuration space into subregions or applying interpolation. Barrier heights, extracted via the Immersion Water Flow method, show good agreement with empirical evaluations (including the new IAEA RIPL-4 dataset) with mean deviations below 1 MeV. Special attention is given to the long-debated third, hyperdeformed minimum. For Th isotopes, a shallow but distinct third well appears, whereas it's absent in heavier actinides (U, Pu).

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Search for shape-isomers in the Pt-Hg-Pb region

Potential energy surfaces of nine even-even isotopes of Pt, Hg, and Pb around $^{186}$Pt are evaluated within a macroscopic-microscopic model based on the Lublin-Strasbourg-Drop macroscopic energy and the microscopic energy obtained using the Yukawa-folded mean-field potential to establish the Strutinski shell corrections and the pairing correlation energy through the BCS approach with a monopole pairing force. The rapidly converging Fourier-over-Spheroid shape parametrization is used to describe nuclear deformations. The stability of the identified shape isomeric states with respect to non-axial and higher-order deformations is investigated. It is also found that in the description of non-axial deformations special attention needs to be devoted to the orientation of the triaxial shape. For the example of the $^{186}$Hg nucleus, where three prolate shape-isomeric states are found, it is shown that the potential energy surface obtained in our model is close to the one obtained in the Hartree-Fock-Bogoliubov theory with the Gogny energy-density functional.

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Towards a unified description of isotopic fragment properties in spontaneous and fusion-induced fission within a 4D dynamical Langevin model

Spontaneous fission of 252Cf and fusion-induced fission of 250Cf are investigated within a multi-dimensional Langevin model. The potential-energy surface is calculated in the macroscopic-microscopic LSD+Yukawa-folded approach using the four-dimensional Fourier-over-Spheroid shape parametrization. The dynamical evolution described by the Langevin equation is coupled to neutron evaporation, thereby allowing for the possibility of multi-chance fission. Charge equilibration and excitation-energy sharing between the fragments emerging at scission are evaluated, and their de-excitation is finally computed. The correlation between various observables, particularly the isotopic properties of the fragments, is discussed and compared with the experiment whenever available. The theoretical predictions are generally in good agreement with the data.

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Fission Fragment Mass and Kinetic Energy Yields of Fermium Isotopes

A rapidly converging 4-dimensional Fourier shape parametrization is used to model the fission process of heavy nuclei. Potential energy landscapes are computed within the macroscopic-microscopic approach, on top of which the multi-dimensional Langevin equation is solved to describe the fission dynamics. Charge equilibration at scission and de-excitation by neutron evaporation of the primary fragments after scission is investigated. The model describes various observables, including fission-fragment mass, charge, and kinetic energy yields, as well as post-scission neutron multiplicities and, most importantly, their correlations, which are crucial to unravel the complexity of the fission process. The parameters of the dynamical model were tuned to reproduce experimental data obtained from thermal neutron-induced fission of $^{235}$U, which allows us to discuss the transition from asymmetric to symmetric fission along the Fm isotopic chain.

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Fourier-over-Spheroid shape parametrization applied to nuclear fission dynamics

We propose a new, rapidly convergent, the so-called Fourier over Spheroid (FoS), shape parametrization to model fission of heavy nuclei. Four collective coordinates are used to characterize the shape of the fissioning system, being its elongation, left-right asymmetry, neck size, and non-axiality. The potential energy landscape is computed within the macroscopic-microscopic approach, on the top of which the multi-dimensional Langevin equation is solved to describe the dynamics. Charge equilibration at scission and de-excitation of the primary fragments after scission are further considered. The model gives access to a wide variety of observables, including fission fragments mass, charge, and kinetic energy yields, fragment mean N/Z and post-scission neutron multiplicities, and importantly, their correlations. The latter are crucial to unravel the complexity of the fission process. The parameters of the model were tuned to reproduce experimental observation from thermal neutron-induced fission of 235U, and next used to discuss the transition from the asymmetric to symmetric fission along the Fm isotopic chain.

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Potential energy surfaces and fission fragment mass yields of even-even superheavy nuclei

Potential energy surfaces and fission barriers of superheavy nuclei are analyzed in the macroscopic-microscopic model. The Lublin-Strasbourg Drop (LSD) is used to obtain the macroscopic part of the energy, whereas the shell and pairing energy corrections are evaluated using the Yukawa-folded potential. A standard flooding technique has been used to determine the barrier heights. It was shown the Fourier shape parametrization containing only three deformation parameters reproduces well the nuclear shapes of nuclei on their way to fission. In addition, the non-axial degree of freedom is taken into account to describe better the form of nuclei around the ground state and in the saddles region. Apart from the symmetric fission valley, a new very asymmetric fission mode is predicted in most superheavy nuclei. The fission fragment mass distributions of considered nuclei are obtained by solving the 3D Langevin equations.

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Fission Fragment Mass and Total Kinetic Energy Distributions of Spontaneously Fissioning Plutonium Isotopes

The fission-fragment mass and total kinetic energy (TKE) distributions are evaluated in a quantum mechanical framework using elongation, mass asymmetry, neck degree of freedom as the relevant collective parameters in the Fourier shape parametrization recently developed by us. The potential energy surfaces (PES) are calculated within the macroscopic-microscopic model based on the Lublin-Strasbourg Drop (LSD), the Yukawa-folded (YF) single-particle potential and a monopole pairing force. The PES are presented and analysed in detail for even-even Plutonium isotopes with $A=236 -246$. They reveal deep asymmetric valleys. The fission-fragment mass and TKE distributions are obtained from the ground state of a collective Hamiltonian computed within the Born-Oppenheimer approximation, in the WKB approach by introducing a neck-dependent fission probability. The calculated mass and total kinetic energydistributions are found in good agreement with the data.

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On the stability of super-heavy nuclei

The potential-energy surfaces of an extended set of heavy and super-heavy even-even nuclei with $92 \le Z \le 126$ and isospins $40 \le N-Z \le 74$ are evaluated within the recently developed Fourier shape parametrization. Ground-state and decay properties are studied for 324 different even-even isotopes in a four-dimensional deformation space, defined by non-axiality, quadrupole, octupole, and hexadecapole degrees of freedom. Nuclear deformation energies are evaluated in the framework of the macroscopic-microscopic approach, with the Lublin-Strasbourg-Drop model and a Yukawa-folded mean-field potential. The evolution of the ground-state equilibrium shape (and possible isomeric, metastable states) is studied as a function of $Z$ and $N$. Alpha-decay $Q$-values and half-lives, as well as fission-barrier heights, are deduced. In order to understand the transition from asymmetric to symmetric fission along the Fm isotopic chain, the properties of all identified fission paths are investigated. Good agreement is found with experimental data wherever available. New interesting features about the population of different fission modes for nuclei beyond Fm are predicted.

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On spontaneous fission and alpha-decay half-lives of atomic nuclei

It is shown, that the Gamow-like model with only one adjustable parameter - radius constant is able to reproduce well the alpha-decay half-lives for all even-even nuclei with the proton number larger than 50. The systematics for odd-A and odd-odd isotopes can be also well described when ones introduces an additional hindrance factor. Similar model based on the W. J. Swiatecki idea from 1955 is developed to reproduce the spontaneous fission half-lives of transactinide nuclei. The achieved accuracy of reproduction of the data is better than that obtained in more advanced theories.

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Beta decay of 252Cf on the way to scission from the exit point

Upon increasing significantly the nuclear elongation, the beta-decay energy grows. This paper investigates within a simple yet partly microscopic approach, the transition rate of the beta decay of the 252Cf nucleus on the way to scission from the exit point for a spontaneous fission process. A rather crude classical approximation is made for the corresponding damped collective motion assumed to be one dimensional. Given these assumptions, we only aim in this paper at providing the order of magnitudes of such a phenomenon. At each deformation the energy available for beta decay, is determined from such a dynamical treatment. Then, for a given elongation, transition rates for the allowed (Fermi) beta decay are calculated from pair correlated wave functions obtained within a macroscopic-microscopic approach and then integrated over the time corresponding to the whole descent from exit to scission. The results are presented as a function of the damping factor (inverse of the characteristic damping time) in use in our classical dynamical approach. For instance, in the case of a descent time from the exit to the scission points of about $10^{- 20}$ second, one finds a total rate of beta decay corresponding roughly to 20 events per year and per milligram of 252Cf. The inclusion of pairing correlations does not affect much these results.

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Spontaneous fission half-lives of nuclei in a phenomenological model

A simple phenomenological model, based on the Świ{\c a}tecki idea for evaluation of the spontaneous fission half-lives is proposed. The model contains only one adjustable parameter fixed to the data for even-even nuclei and two additional hindrance factors to the life-times, which give the effect of odd particles. A good agreement with the experimental data for all fissioning nuclei is achieved.

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A Particle number conserving shell-correction method

The shell correction method is revisited. Contrary to the traditional Strutinsky method, the shell energy is evaluated by an averaging over the number of particles and not over the single-particle energies, which is more consistent with the definition of the macroscopic energy. In addition, the smooth background is subtracted before averaging the sum of single-particle energies, which significantly improves the plateau condition and allows to apply the method also for nuclei close to the proton or neutron drip lines. A significant difference between the shell correction energy obtained with the traditional and the new method is found in particular for highly degenerated single-particle spectra (as i.e. in magic nuclei) while for deformed nuclei (where the degeneracy is lifted to a large extent) both estimates are close, except in the region of super or hyper-deformed states.

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On electronic shells surrounding charged insulated metallic clusters

We determine the wavefunctions of electrons bound to a positively charged mesoscopic metallic cluster covered by an insulating surface layer. The radius of the metal core and the thickness of the insulating surface layer are of the order of a couple of angstroems. We study in particular the electromagnetic decay of externally located electrons into unoccupied internally located states which exhibits a resonance behaviour. This resonance structure has the consequence that the lifetime of the `mesoscopic atoms' may vary by up to 6 orders of magnitude depending on the values of the parameters (from sec to years).

cond-mat.mes-hall