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K. Shimada

Publications and source records attributed to K. Shimada.

At least 55 records · Page 3Linked to original sources

Out-of-plane momentum and symmetry dependent superconducting gap in Ba0.6K0.4Fe2As2

The three-dimensional band structure and superconducting gap of Ba0.6K0.4Fe2As2 are studied with high-resolution angle-resolved photoemission spectroscopy. In contrast to previous results, we have identified three hole-like Fermi surfaces near the zone center with sizable out-of-plane or kz dispersion. The superconducting gap on certain Fermi surface shows significant kz-dependence. Moreover, we found that the superconducting gap sizes are different at the same Fermi momentum for two bands with different spatial symmetries (one odd, one even). Our results provide further information on the rich superconducting gap structure in iron pnictides, and a distinct test for theories.

cond-mat.supr-con↗

Surface and bulk electronic structures of LaOFeAs studied by angle resolved photoemission spectroscopy

The electronic structure of LaOFeAs, a parent compound of iron-arsenic superconductors, is studied by angleresolved photoemission spectroscopy. By examining its dependence on photon energy, polarization, sodium dosing and the counting of Fermi surface volume, both the bulk and the surface contributions are identified. We find that a bulk band moves toward high binding energies below structural transition, and shifts smoothly across the spin density wave transition by about 25 meV. Our data suggest the band reconstruction may play a crucial role in the spin density wave transition, and the structural transition is driven by the short range magnetic order. For the surface states, both the LaO-terminated and FeAs-terminated components are revealed. Certain small band shifts are verified for the FeAs-terminated surface states in the spin density wave state, which is a reflection of the bulk electronic structure reconstruction. Moreover, sharp quasiparticle peaks quickly rise at low temperatures, indicating of drastic reduction of the scattering rate. A kink structure in one of the surface band is shown to be possibly related to the electron-phonon interactions.

cond-mat.supr-con↗

Strong correlation and massive spectral-weight redistribution induced spin density wave in a-Fe1.06Te

The electronic structure of a-Fe1.06Te is studied with angle-resolved photoemission spectroscopy. We show that there is substantial spectral weight around Gamma and X, and lineshapes are intrinsically incoherent in the paramagnetic state. The magnetic transition is characterized by a massive spectral-weight transfer over an energy range as large as the band width, which even exhibits a hysteresis loop that marks the strong first order transition. Coherent quasiparticles emerge in the magnetically ordered state due to decreased spin fluctuations, which account for the change of transport properties from insulating behavior to metallic behavior. Our observation demonstrates that Fe1.06Te distinguishes itself from other iron-based systems with more local characters and much stronger interactions among different degrees of freedom, and how a spin density wave is formed in the presence of strong correlation.

cond-mat.supr-con↗

Electronic structure reconstruction: the driving force behind the magnetic and structural transitions in NaFeAs

The electronic structure of NaFeAs is studied with angle resolved photoemission spectroscopy on high quality single crystals. Large portions of the band structure start to shift around the structural transition temperature, and smoothly evolve as the temperature lowers through the spin density wave transition. Moreover, band folding due to magnetic order emerges around structural transition. Our observation provides direct evidence that the structural and magnetic transitions share the same origin, and are both driven by the electronic structure reconstruction in Fe-based superconductors, instead of Fermi surface nesting.

cond-mat.supr-con↗

Precision measurement of the electric quadrupole moment of 31Al and determination of the effective proton charge in the sd-shell

he electric quadrupole coupling constant of the 31Al ground state is measured to be nu_Q = |eQV_{zz}/h| = 2196(21)kHz using two different beta-NMR (Nuclear Magnetic Resonance) techniques. For the first time, a direct comparison is made between the continuous rf technique and the adiabatic fast passage method. The obtained coupling constants of both methods are in excellent agreement with each other and a precise value for the quadrupole moment of 31Al has been deduced: |Q(31Al)| = 134.0(16) mb. Comparison of this value with large-scale shell-model calculations in the sd and sdpf valence spaces suggests that the 31Al ground state is dominated by normal sd-shell configurations with a possible small contribution of intruder states. The obtained value for |Q(31Al)| and a compilation of measured quadrupole moments of odd-Z even-N isotopes in comparison with shell-model calculations shows that the proton effective charge e_p=1.1 e provides a much better description of the nuclear properties in the sd-shell than the adopted value e_p=1.3 e.

nucl-ex↗

Measurement of electron correlations in LixCoO2 (x=0.0 - 0.35) using 59Co nuclear magnetic resonance and nuclear quadrupole resonance techniques

CoO2 is the parent compound for the superconductor NaxCoO2\cdot1.3H2O and was widely believed to be a Mott insulator. We performed 59Co nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) studies on LixCoO2 (x = 0.35, 0.25, 0.12, and 0.0) to uncover the electronic state and spin correlations in this series of compounds which was recently obtained through electrochemical de-intercalation of Li from pristine LiCoO2. We find that although the antiferromagnetic spin correlations systematically increase with decreasing Li-content (x), the end member, CoO2 is a non-correlated metal that well satisfies the Korringa relation for a Fermi liquid. Thus, CoO2 is not simply located at the limit of x->0 for AxCoO2 (A = Li, Na) compounds. The disappearance of the electron correlations in CoO2 is due to the three dimensionality of the compound which is in contrast to the highly two dimensional structure of AxCoO2.

cond-mat.supr-con↗

Two superconducting gaps in LaFeAsO0.92F0.08 revealed by 75As nuclear quadrupole resonance

We report $^{75}$As nuclear quadrupole resonance (NQR) studies on superconducting oxypnictide LaFeAsO$_{0.92}$F$_{0.08}$ ($T_{\rm c}$ = 23 K). The temperature dependence of the spin lattice relaxation rate (1/$T_1$) decreases below $T_{\rm c}$ without a coherence (Hebel-Slichter) peak and shows a temperature dependence that is not simple power-law nor exponential. We show that the result can be understood in terms of two superconducting gaps of either $d$- or ${\pm}s$-wave symmetry, with the larger gap $Δ_1\sim 4 k_{\rm B}T_{\rm c}$ and the smaller one $Δ_2 \sim 1.5 k_{\rm B}T_{\rm c}$. Our result suggests that the multiple-gaps feature is universal in the oxypnictides superconductors, which is probably associated with the multiple electronic bands structure in this new class of materials. We also find that 1/$T_1T$ above $T_{\rm c}$ increases with decreasing temperature, which suggests weak magnetic fluctuations in the normal state.

cond-mat.supr-con↗

Primary role of the barely occupied states in the charge density wave formation of NbSe2

NbSe2 is a prototypical charge-density-wave (CDW) material, whose mechanism remains mysterious so far. With angle resolved photoemission spectroscopy, we mapped out the CDW gap and recovered the long-lost nesting condition over a large broken-honeycomb region in the Brillouin zone, which consists of six saddle band point regions with high density of states (DOS), and large regions away from Fermi surface with negligible DOS at the Fermi energy. We show that the major contributions to the CDW come from these barely occupied states rather than the saddle band points. Our findings not only resolve a long standing puzzle, but also overthrow the conventional wisdom that CDW is dominated by regions with high DOS.

cond-mat.str-el↗

Ground-state electric quadrupole moment of 31Al

Ground-state electric quadrupole moment of 31Al (I =5/2+, T_1/2 = 644(25) ms) has been measured by means of the beta-NMR spectroscopy using a spin-polarized 31Al beam produced in the projectile fragmentation reaction. The obtained Q moment, |Q_exp(31Al)| = 112(32)emb, are in agreement with conventional shell model calculations within the sd valence space. Previous result on the magnetic moment also supports the validity of the sd model in this isotope, and thus it is concluded that 31Al is located outside of the island of inversion.

nucl-ex↗

Correlation effects of exchange splitting and coexistence of spin-density-wave and superconductivity in single crystalline Sr1-xKxFe2As2

The nature of spin-density wave and its relation with superconductivity are crucial issues in the newly discovered Fe-based high temperature superconductors. Particularly it is unclear whether the superconducting phase and spin density wave (SDW) are truly exclusive from each other as suggested by certain experiments. With angle resolved photoemission spectroscopy, we here report exchange splittings of the band structures in Sr1-xKxFe2As2 (x=0,0.1,0.2), and the non-rigid-band behaviors of the splitting. Our data on single crystalline superconducting samples unambiguously prove that SDW and superconductivity could coexist in iron-pnictides.

cond-mat.supr-con↗

An Isotopic Fingerprint of Electron-Phonon Coupling in High-Tc Cuprates

Angle-resolved photoemission spectroscopy with low-energy tunable photons along the nodal direction of oxygen isotope substituted Bi2Sr2CaCu2O8+delta reveals a distinct oxygen isotope shift near the electron-boson coupling "kink" in the electronic dispersion. The magnitude (a few meV) and direction of the kink shift are as expected due to the measured isotopic shift of phonon frequency, which are also in agreement with theoretical expectations. This demonstrates the participation of the phonons as dominant players, as well as pinpointing the most relevant of the phonon branches.

cond-mat.supr-con↗

Electronic structure and exotic exchange splitting in spin-density-wave states of BaFe$_2$As$_2$

The magnetic properties in the parent compounds are often intimately related to the microscopic mechanism of superconductivity. Here we report the first direct measurements on the electronic structure of a parent compound of the newly discovered iron-based superconductor, BaFe$_2$As$_2$, which provides a foundation for further studies. We show that the energy of the spin density wave (SDW) in BaFe$_2$As$_2$ is lowered through exotic exchange splitting of the band structure, rather than Fermi surface nesting of itinerant electrons. This clearly demonstrates that a metallic SDW state could be solely induced by interactions of local magnetic moments, resembling the nature of antiferromagnetic order in cuprate parent compounds.

cond-mat.supr-con↗

Novel electronic structure induced by a highly strained oxide interface with incommensurate crystal fields

The misfit oxide, Bi$_{2}$Ba$_{1.3}$K$_{0.6}$Co$_{2.1}$O$_{y}$, made of alternating rocksalt-structured [BiO/BaO] layers and hexagonal CoO$_{2}$ layers, was studied by angle-resolved photoemission spectroscopy. Detailed electronic structure of such a highly strained oxide interfaces is revealed for the first time. We found that under the two incommensurate crystal fields, electrons are confined within individual sides of the interface, and scattered by umklapp scattering of the crystal field from the other side. In addition, the high strain on the rocksalt layer raises its chemical potential and induces large charge transfer to the CoO$_{2}$ layer. Furthermore, a novel interface effects, the interfacial enhancement of electron-phonon interactions, is discovered. Our findings of these electronic properties lay a foundation for designing future functional oxide interfaces.

cond-mat.str-el↗

Doping-insensitive density-of-states suppression in polycrystalline iron-based superconductor SmO$_{1-x}$F$_{x}$FeAs

We investigated the temperature dependence of the density-of-states in the iron-based superconductor SmO_1-xF_xFeAs (x=0, 0.12, 0.15, 0.2) with high resolution angle-integrated photoemission spectroscopy. The density-of-states suppression is observed with decreasing temperature in all samples, revealing two characteristic energy scales (10meV and 80meV). However, no obvious doping dependence is observed. We argue that the 10meV suppression is due to an anomalously doping-independent normal state pseudogap, which becomes the superconducting gap once in the superconducting state; and alert the possibility that the 80meV-scale suppression might be an artifact of the polycrystalline samples.

cond-mat.supr-con↗

Electronic Structures of Fe$_{3-x}V$_x$Si Probed by Photoemission Spectroscopy

The electronic structures of the Heusler type compounds Fe$_{3-x}V$_x$Si in the concentration range between x = 0 and x = 1 have been probed by photoemission spectroscopy (PES). The observed shift of Si 2p core- level and the main valence band structres indicate a chemical potential shift to higher energy with increasing x. It is also clarified that the density of state at Fermi edge is owing to the collaboration of V 3d and Fe 3d derived states. Besides the decrease of the spectral intensity near Fermi edge with increasing x suggests the formation of pseudo gap at large x.

cond-mat.mtrl-sci↗

Superconducting coherence peak in the electronic excitations of a single layer cuprate superconductor $Bi_2 Sr_{1.6} La_{0.4} Cu O_{6+δ}$

Angle resolved photoemission spectroscopy study is reported on a high quality optimally doped Bi2Sr1.6La0.4CuO6+delta high Tc superconductor. In the antinodal region with maximal d-wave gap, the symbolic superconducting coherence peak, which has been widely observed in multi-CuO2-layer cuprate superconductors, is unambiguously observed in a single layer system. The associated peak-dip separation is just about 19 meV, which is much smaller than its counterparts in multi-layered compounds, but correlates with the energy scales of spin excitations in single layer cuprates.

cond-mat.supr-con↗

Electronic Structure of Charge- and Spin-controlled Sr_{1-(x+y)}La_{x+y}Ti_{1-x}Cr_{x}O_{3}

We present the electronic structure of Sr_{1-(x+y)}La_{x+y}Ti_{1-x}Cr_{x}O_{3} investigated by high-resolution photoemission spectroscopy. In the vicinity of Fermi level, it was found that the electronic structure were composed of a Cr 3d local state with the t_{2g}^{3} configuration and a Ti 3d itinerant state. The energy levels of these Cr and Ti 3d states are well interpreted by the difference of the charge-transfer energy of both ions. The spectral weight of the Cr 3d state is completely proportional to the spin concentration x irrespective of the carrier concentration y, indicating that the spin density can be controlled by x as desired. In contrast, the spectral weight of the Ti 3d state is not proportional to y, depending on the amount of Cr doping.

cond-mat.str-el↗

Bulk and surface-sensitive high-resolution photoemission study of Mott-Hubbard systems SrVO$_3$ and CaVO$_3$

We study the electronic structure of Mott-Hubbard systems SrVO$_{3}$ and CaVO$_3$ with bulk and surface-sensitive high-resolution photoemission spectroscopy (PES), using a VUV laser, synchrotron radiation and a discharge lamp ($hν$ = 7 - 21 eV). A systematic suppression of the density of states (DOS) within $\sim$ 0.2 eV of the Fermi level ($E_F$) is found on decreasing photon energy i.e. on increasing bulk sensitivity. The coherent band in SrVO$_{3}$ and CaVO$_3$ is shown to consist of surface and bulk derived features, separated in energy. The stronger distortion on surface of CaVO$_{3}$ compared to SrVO$_{3}$ leads to higher surface metallicity in the coherent DOS at $E_F$, consistent with recent theory.

cond-mat.str-el↗