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K. Watanabe

Publications and source records attributed to K. Watanabe.

At least 307 records · Page 17Linked to original sources

Many-particle effects in the cyclotron resonance of encapsulated monolayer graphene

We study the infrared cyclotron resonance of high mobility monolayer graphene encapsulated in hexagonal boron nitride, and simultaneously observe several narrow resonance lines due to interband Landau level transitions. By holding the magnetic field strength, $B$, constant while tuning the carrier density, $n$, we find the transition energies show a pronounced non-monotonic dependence on the Landau level filling factor, $ν\propto n/B$. This constitutes direct evidence that electron-electron interactions contribute to the Landau level transition energies in graphene, beyond the single-particle picture. Additionally, a splitting occurs in transitions to or from the lowest Landau level, which is interpreted as a Dirac mass arising from coupling of the graphene and boron nitride lattices.

cond-mat.mes-hall↗

Shape anisotropy revisited in single-digit nanometer magnetic tunnel junctions

Nanoscale magnetic tunnel junction plays a pivotal role in magnetoresistive random access memories. Successful implementation depends on a simultaneous achievement of low switching current for the magnetization switching by spin-transfer torque and high thermal stability, along with a continuous reduction of junction size. Perpendicular-easy-axis CoFeB/MgO stacks possessing interfacial anisotropy have paved the way down to 20-nm scale, below which a new approach needs to be explored. Here we show magnetic tunnel junctions that satisfy the requirements at ultrafine scale by revisiting shape anisotropy, which is a classical part of magnetic anisotropy but has not been fully utilized in the current perpendicular systems. Magnetization switching solely driven by current is achieved for junctions smaller than 10 nm where sufficient thermal stability is provided by shape anisotropy without adopting new material systems. This work is expected to push forward the development of magnetic tunnel junctions towards single-digit-nm-scale nano-magnetics/spintronics.

physics.app-ph↗

Even denominator fractional quantum Hall states at an isospin transition in monolayer graphene

Magnetic fields quench the kinetic energy of two dimensional electrons, confining them to highly degenerate Landau levels. In the absence of disorder, the ground state at partial Landau level filling is determined only by Coulomb interactions, leading to a variety of correlation-driven phenomena. Here, we realize a quantum Hall analog of the Neél-to-valence bond solid transition within the spin- and sublattice- degenerate monolayer graphene zero energy Landau level by experimentally controlling substrate-induced sublattice symmetry breaking. The transition is marked by unusual isospin transitions in odd denominator fractional quantum Hall states for filling factors $ν$ near charge neutrality, and the unexpected appearance of incompressible even denominator fractional quantum Hall states at $ν=\pm1/2$ and $\pm1/4$ associated with pairing between composite fermions on different carbon sublattices.

cond-mat.str-el↗

Optical spectroscopy of excited exciton states in MoS2 monolayers in van der Waals heterostructures

The optical properties of MoS2 monolayers are dominated by excitons, but for spectrally broad optical transitions in monolayers exfoliated directly onto SiO2 substrates detailed information on excited exciton states is inaccessible. Encapsulation in hexagonal boron nitride (hBN) allows approaching the homogenous exciton linewidth, but interferences in the van der Waals heterostructures make direct comparison between transitions in optical spectra with different oscillator strength more challenging. Here we reveal in reflectivity and in photoluminescence excitation spectroscopy the presence of excited states of the A-exciton in MoS2 monolayers encapsulated in hBN layers of calibrated thickness, allowing to extrapolate an exciton binding energy of about 220 meV. We theoretically reproduce the energy separations and oscillator strengths measured in reflectivity by combining the exciton resonances calculated for a screened two-dimensional Coulomb potential with transfer matrix calculations of the reflectivity for the van der Waals structure. Our analysis shows a very different evolution of the exciton oscillator strength with principal quantum number for the screened Coulomb potential as compared to the ideal two-dimensional hydrogen model.

cond-mat.mtrl-sci↗

Out-of-plane heat transfer in van der Waals stacks: electron-hyperbolic phonon coupling

Van der Waals heterostructures have emerged as promising building blocks that offer access to new physics, novel device functionalities, and superior electrical and optoelectronic properties. Applications such as thermal management, photodetection, light emission, data communication, high-speed electronics and light harvesting require a thorough understanding of (nanoscale) heat flow. Here, using time-resolved photocurrent measurements we identify an efficient out-of-plane energy transfer channel, where charge carriers in graphene couple to hyperbolic phonon polaritons in the encapsulating layered material. This hyperbolic cooling is particularly efficient, giving picosecond cooling times, for hexagonal BN, where the high-momentum hyperbolic phonon polaritons enable efficient near-field energy transfer. We study this heat transfer mechanism through distinct control knobs to vary carrier density and lattice temperature, and find excellent agreement with theory without any adjustable parameters. These insights may lead to the ability to control heat flow in van der Waals heterostructures.

cond-mat.mes-hall↗

Tunneling Devices with Perpendicular Magnetic Anisotropy Electrodes on Atomically Thin van der Waals Heterostructures

We report the fabrication of perpendicular ferromagnetic electrodes for tunneling devices consist of van der Waals heterostructure. We found MgO/Co/Pt films on Hexagonal BN shows perpendicular magnetic anisotropy (PMA) with the easy axis perpendicular to the substrate. Vacuum annealing enhances the perpendicular anisotropy. The easy axis along the perpendicular direction persists up to room temperature with the Pt layer thickness ranges from 1.5 to 5 nm. We employed the PMA electrodes to construct tunneling devices on graphene and monolayer WSe2, where spin injection characteristics and field effect transistor behavior were demonstrated without strong Schottky barrier formation.

cond-mat.mes-hall↗

Approaching quantum anomalous Hall effect in proximity-coupled YIG/graphene/h-BN sandwich structure

Quantum anomalous Hall state is expected to emerge in Dirac electron systems such as graphene under both sufficiently strong exchange and spin-orbit interactions. In pristine graphene, neither interaction exists; however, both interactions can be acquired by coupling graphene to a magnetic insulator (MI) as revealed by the anomalous Hall effect. Here, we show enhanced magnetic proximity coupling by sandwiching graphene between a ferrimagnetic insulator yttrium iron garnet (YIG) and hexagonal-boron nitride (h-BN) which also serves as a top gate dielectric. By sweeping the top-gate voltage, we observe Fermi level-dependent anomalous Hall conductance. As the Dirac point is approached from both electron and hole sides, the anomalous Hall conductance reaches 1/4 of the quantum anomalous Hall conductance 2e2/h. The exchange coupling strength is determined to be as high as 27 meV from the transition temperature of the induced magnetic phase. YIG/graphene/h-BN is an excellent heterostructure for demonstrating proximity-induced interactions in two-dimensional electron systems.

cond-mat.mes-hall↗

Dynamic band structure tuning of graphene moiré superlattices with pressure

Heterostructures of atomically-thin materials have attracted significant interest owing to their ability to host novel electronic properties fundamentally distinct from their constituent layers. In the case of graphene on boron nitride, the closely-matched lattices yield a moiré superlattice that modifies the graphene electron dispersion and opens gaps both at the primary Dirac point (DP) and the moiré-induced secondary Dirac point (SDP) in the valence band. While significant effort has focused on controlling the superlattice period via the rotational stacking order, the role played by the magnitude of the interlayer coupling has received comparatively little attention. Here, we modify the interaction between graphene and boron nitride by tuning their separation with hydrostatic pressure. We observe a dramatic enhancement of the DP gap with increasing pressure, but little change in the SDP gap. Our surprising results identify the critical role played by atomic-scale structural deformations of the graphene lattice and reveal new opportunities for band structure engineering in van der Waals heterostructures.

cond-mat.mes-hall↗

Manipulation and steering of hyperbolic surface polaritons in hexagonal boron nitride

Hexagonal boron nitride (hBN) is a natural hyperbolic material that supports both volume-confined hyperbolic polaritons (HPs) and sidewall-confined hyperbolic surface polaritons (HSPs). In this work, we demonstrate effective excitation, control and steering of HSPs in hBN through engineering the geometry and orientation of hBN sidewalls. By combining infrared (IR) nano-imaging and numerical simulations, we investigate the reflection, transmission and scattering of HSPs at the hBN corners with various apex angles. We show that the sidewall-confined nature of HSPs enables a high degree of control over their propagation by designing the geometry of hBN nanostructures.

cond-mat.mes-hall↗

Superballistic flow of viscous electron fluid through graphene constrictions

Electron-electron (e-e) collisions can impact transport in a variety of surprising and sometimes counterintuitive ways. Despite strong interest, experiments on the subject proved challenging because of the simultaneous presence of different scattering mechanisms that suppress or obscure consequences of e-e scattering. Only recently, sufficiently clean electron systems with transport dominated by e-e collisions have become available, showing behavior characteristic of highly viscous fluids. Here we study electron transport through graphene constrictions and show that their conductance below 150 K increases with increasing temperature, in stark contrast to the metallic character of doped graphene. Notably, the measured conductance exceeds the maximum conductance possible for free electrons. This anomalous behavior is attributed to collective movement of interacting electrons, which 'shields' individual carriers from momentum loss at sample boundaries. The measurements allow us to identify the conductance contribution arising due to electron viscosity and determine its temperature dependence. Besides fundamental interest, our work shows that viscous effects can facilitate high-mobility transport at elevated temperatures, a potentially useful behavior for designing graphene-based devices.

cond-mat.mes-hall↗

Short-range test of the universality of gravitational constant $G$ at the millimeter scale using a digital image sensor

The composition dependence of gravitational constant $G$ is measured at the millimeter scale to test the weak equivalence principle, which may be violated at short range through new Yukawa interactions such as the dilaton exchange force. A torsion balance on a turning table with two identical tungsten targets surrounded by two different attractor materials (copper and aluminum) is used to measure gravitational torque by means of digital measurements of a position sensor. Values of the ratios $\tilde{G}_{Al-W}/\tilde{G}_{Cu-W} -1$ and $\tilde{G}_{Cu-W}/G_{N} -1$ were $(0.9 \pm 1.1_{\mathrm{sta}} \pm 4.8_{\mathrm{sys}}) \times 10^{-2}$ and $ (0.2 \pm 0.9_{\mathrm{sta}} \pm 2.1_{\mathrm{sys}}) \times 10^{-2}$ , respectively; these were obtained at a center to center separation of 1.7 cm and surface to surface separation of 4.5 mm between target and attractor, which is consistent with the universality of $G$. A weak equivalence principle (WEP) violation parameter of $η_{Al-Cu}(r\sim 1\: \mathrm{cm})=(0.9 \pm 1.1_{\mathrm{sta}} \pm 4.9_{\mathrm{sys}}) \times 10^{-2} $ at the shortest range of around 1 cm was also obtained.

gr-qc↗

Analysis of solar gamma rays and solar neutrons detected on March 7th and September 25th of 2011 by Ground Level Neutron Telescopes, SEDA-FIB and FERMI-LAT

At the 33rd ICRC, we reported the possible detection of solar gamma rays by a ground level detector and later re-examined this event. On March 7, 2011, the solar neutron telescope (SNT) located at Mt. Sierra Negra, Mexico (4,600 m) observed enhancements of the counting rate from 19:49 to 20:02 UT and from 20:50 to 21:01 UT. The statistical significance was 9.7sigma and 8.5sigma, respectively. This paper discusses the possibility of using this mountain detector to detect solar gamma rays. In association with this event, the solar neutron detector SEDA-FIB onboard the International Space Station has also detected solar neutrons with a statistical significance of 7.5sigma. The FERMI-LAT detector also observed high-energy gamma rays from this flare with a statistical significance of 6.7sigma. We thus attempted to make a unified model to explain this data. In this paper, we report on another candidate for solar gamma rays detected on September 25th, 2011 by the SNT located in Tibet (4,300 m) from 04:37 to 04:47 UT with a statistical significance of 8.0sigma (by the Li-Ma method).

astro-ph.HE↗

Direct measurement of discrete valley and orbital quantum numbers in a multicomponent quantum Hall system

Strongly interacting two dimensional electron systems (2DESs) host a complex landscape of broken symmetry states. The possible ground states are further expanded by internal degrees of freedom such as spin or valley-isospin. While direct probes of spin in 2DESs were demonstrated two decades ago, the valley quantum number has only been probed indirectly in semiconductor quantum wells, graphene mono- and bilayers, and transition-metal dichalcogenides. Here, we present the first direct experimental measurement of valley polarization in a two dimensional electron system, effected via the direct mapping of the valley quantum number onto the layer polarization in bilayer graphene at high magnetic fields. We find that the layer polarization evolves in discrete steps across 32 electric field-tuned phase transitions between states of different valley, spin, and orbital polarization. Our data can be fit by a model that captures both single particle and interaction induced orbital, valley, and spin anisotropies, providing the most complete model of this complex system to date. Among the newly discovered phases are theoretically unanticipated orbitally polarized states stabilized by skew interlayer hopping. The resulting roadmap to symmetry breaking in bilayer graphene paves the way for deterministic engineering of fractional quantum Hall states, while our layer-resolved technique is readily extendable to other two dimensional materials where layer polarization maps to the valley or spin quantum numbers, providing an essential direct probe that is a prerequisite for manipulating these new quantum degrees of freedom.

cond-mat.mes-hall↗

Even denominator fractional quantum Hall state in bilayer graphene

The multi-component nature of bilayer graphene (BLG), together with the ability to controllably tune between the various ground state orders, makes it a rich system in which to explore interaction driven phenomena. In the fractional quantum Hall effect (FQHE) regime, the unique Landau level spectrum of BLG is anticipated to support a non-Abelian even-denominator state that is tunable by both electric and magnetic fields. However, observation of this state, which is anticipated to be stronger than in conventional systems, has been conspicuously difficult. Here we report transport measurements of a robust even denominator FQHE in high-mobility, dual gated BLG devices. We confirm that the stability of the energy gap can be sensitively tuned and map the phase diagram. Our results establish BLG as a dynamic new platform to study topological ground states with possible non-Abelian excitations.

cond-mat.mes-hall↗

In-plane Propagation of Light in Transition Metal Dichalcogenide Monolayers: Optical Selection Rules

The optical selection rules for inter-band transitions in WSe2, WS2 and MoSe2 transition metal dichalcogenide monolayers are investigated by polarization-resolved photoluminescence experiments with a signal collection from the sample edge. These measurements reveal a strong polarization-dependence of the emission lines. We see clear signatures of the emitted light with the electric field oriented perpendicular to the monolayer plane, corresponding to an inter-band optical transition forbidden at normal incidence used in standard optical spectroscopy measurements. The experimental results are in agreement with the optical selection rules deduced from group theory analysis, highlighting the key role played by the different symmetries of the conduction and valence bands split by the spin-orbit interaction. These studies yield a direct determination on the bright-dark exciton splitting, for which we measure 40 $\pm 1$ meV and 55 $\pm 2$ meV for WSe2 and WS2 monolayer, respectively.

cond-mat.mtrl-sci↗

Sub-bandgap voltage electroluminescence and magneto-oscillations in a WSe2 light-emitting van der Waals heterostructure

We report on experimental investigations of an electrically driven WSe2 based light-emitting van der Waals heterostructure. We observe a threshold voltage for electroluminescence significantly lower than the corresponding single particle band gap of monolayer WSe2. This observation can be interpreted by considering the Coulomb interaction and a tunneling process involving excitons, well beyond the picture of independent charge carriers. An applied magnetic field reveals pronounced magneto-oscillations in the electroluminescence of the free exciton emission intensity with a 1/B-periodicity. This effect is ascribed to a modulation of the tunneling probability resulting from the Landau quantization in the graphene electrodes. A sharp feature in the differential conductance indicates that the Fermi level is pinned and allows for an estimation of the acceptor binding energy.

cond-mat.mes-hall↗

Contact-less characterizations of encapsulated graphene p-n junctions

Accessing intrinsic properties of a graphene device can be hindered by the influence of contact electrodes. Here, we capacitively couple graphene devices to superconducting resonant circuits and observe clear changes in the resonance- frequency and -widths originating from the internal charge dynamics of graphene. This allows us to extract the density of states and charge relaxation resistance in graphene p-n junctions without the need of electrical contacts. The presented characterizations pave a fast, sensitive and non-invasive measurement of graphene nanocircuits.

cond-mat.mes-hall↗

Excitonic linewidth approaching the homogeneous limit in MoS2 based van der Waals heterostructures : accessing spin-valley dynamics

The strong light matter interaction and the valley selective optical selection rules make monolayer (ML) MoS2 an exciting 2D material for fundamental physics and optoelectronics applications. But so far optical transition linewidths even at low temperature are typically as large as a few tens of meV and contain homogenous and inhomogeneous contributions. This prevented in-depth studies, in contrast to the better-characterized ML materials MoSe2 and WSe2. In this work we show that encapsulation of ML MoS2 in hexagonal boron nitride can efficiently suppress the inhomogeneous contribution to the exciton linewidth, as we measure in photoluminescence and reflectivity a FWHM down to 2 meV at T = 4K. This indicates that surface protection and substrate flatness are key ingredients for obtaining stable, high quality samples. Among the new possibilities offered by the well-defined optical transitions we measure the homogeneous broadening induced by the interaction with phonons in temperature dependent experiments. We uncover new information on spin and valley physics and present the rotation of valley coherence in applied magnetic fields perpendicular to the ML.

cond-mat.mtrl-sci↗