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Kenji Watanabe

Publications and source records attributed to Kenji Watanabe.

At least 271 records · Page 15Linked to original sources

Pre-Patterned Superconducting Contacts for Clean Superconductor-Topological Material Interfaces Enabling Long-Range Josephson Coupling

Phase-coherent superconducting proximity in topological materials requires clean superconductor-topological material (SC-TM) interfaces, yet conventional top-contact fabrication often degrades them through oxidation, polymer residue, and process-induced disorder. Here we introduce a pre-patterned superconducting bottom-contact architecture in which MoRe/Au electrodes are defined before van der Waals crystal transfer, thereby avoiding on-flake lithography after transfer. In WTe2- and Bi1.5Sb0.5Te1.7Se1.3-based Josephson junctions, this architecture yields systematically larger I_c R_N and longer-ranged coupling than conventional top contacts. Cross-sectional STEM/EDS reveals atomically abrupt, chemically well-separated interfaces. These results establish pre-patterned SC-TM contacts as a practical route to reproducible, micrometer-scale Josephson platforms in van der Waals topological materials.

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Electrically controllable valence-conduction band reversals in helical trilayer graphene

In moiré graphene systems, electronic interactions lift spin and valley degeneracies, leading to symmetry-broken ground states. In helical trilayer graphene (HTG), we uncover a distinct interaction-driven mechanism in which the roles of sublattice-polarized valence and conduction bands are cyclically reversed. Using scanning nano-SQUID magnetometry, we detect a series of sharp magnetic signatures consistent with seesaw-like transitions, where occupied and unoccupied valence and conduction bands interchange repeatedly with doping, accompanied by a novel form of magnetic hysteresis. These transitions occur entirely within metallic regimes and leave only weak fingerprints in transport measurements. Self-consistent Hartree-Fock calculations reveal that interactions reorganize all eight low-energy flat bands, driving abrupt changes in orbital magnetization. Our results establish HTG as the first system where electronic interactions provide doping-controlled access to all three internal degrees of freedom - spin, valley, and sublattice - introducing a new class of correlated phase transitions.

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Programmable, Spontaneous Superlattice Memory in a Monolayer Topological Insulator

Memory is a foundational concept across disciplines, from neurobiology and electronics to artificial intelligence and quantum gravity. In materials, memory effects typically arise from ferroic orders, such as ferroelectricity and ferromagnetism, where information is stored in charge or spin degrees of freedom. Here, we report a surprising discovery of a nonvolatile superlattice memory effect in monolayer TaIrTe4, a dual quantum spin Hall insulator, where information is encoded through sharply contrasting lattice periodicities. In particular, in a pristine monolayer, we observe the spontaneous emergence of a long-period superlattice that can be programmed ON and OFF in a nonvolatile manner by electrostatic tuning of low-energy electronic states. This switching toggles the system between two structural configurations with unit cell areas differing by nearly two orders of magnitude. Mechanistically, our results reveal two independent and distinct instabilities, one in the lattice and the other in the QSH electrons, which are coupled, leading to electrostatic control of lattice configurations with nonvolatile memory. This finding is enabled by combining linear and nonlinear transport measurements, Raman spectroscopy, and scanning tunneling microscopy, which probe complementary aspects of the underlying orders. Remarkably, this nonvolatile memory effect stabilizes a spontaneous superlattice with a periodicity on the few-nanometer scale that remains robust across a wide doping range, persists over days, and survives above 70 K. Combined with the QSH topology, this stability offers a promising route to nonvolatile memory control of topological flat bands and their filling enabled quantum states. Our preliminary data indeed show the emergence of new insulating states at fractional superlattice fillings, which can be clearly switched ON and OFF together with the superlattice.

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Polarization-Aligned, Spectrally Consistent Quantum Emitters in As-Exfoliated Carbon-Doped Hexagonal Boron Nitride

Solid-state quantum emitters constitute an essential building blocks of integrated quantum photonic circuits. Among potential emitter platforms, hexagonal boron nitride (hBN) hosts single-photon emitters in an atomically thin lattice amenable to photonic integration. However, multi-step fabrication approaches, limited defect specificity, and poor emission wavelength repeatability limit the performance of hBN quantum light sources relative to established solid-state architectures. Developing methods to induce emitters that are both suitable for planar photonic devices and that exhibit consistent optical properties remains a key objective. In this work, we identify quantum emitters in as-exfoliated carbon-doped hBN that exhibit both stable and repeatable emission energies together with polarization-aligned dipoles. Owing to the high lattice crystallinity, these single-photon light sources demonstrate exceptional spectral stability with a standard deviation of 7 $μ$eV. The emission energy is reproducible and confined within a narrow range of 2.2825 ${\pm}$ 0.0042 eV. Notably, consistent dipole alignment for absorption and emission polarization suggests that the intrinsic defects are of the same nature. The color centers are observed in as-exfoliated hBN without any post-treatment, significantly facilitating further interfacing with planar photonic structures. These reproducible, polarization-aligned quantum emitters in as-exfoliated hBN provide a versatile platform for scalable integration, offering a pathway toward a broad range of quantum technologies.

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Coexisting Massive and Massless Dirac Fermions in Moire'-Reconstructed Bilayer Graphene

We report the emergence of massless Dirac fermions in moiré-reconstructed bands of bilayer graphene (BLG) aligned with hexagonal boron nitride (hBN). Magnetotransport measurements reveal that while the primary BLG band retains a parabolic dispersion with a Berry phase of $2π$, the moiré-induced secondary bands at $n/n_0 = \pm 4$ host chiral massless quasiparticles with a Berry phase $π$ and a Fermi velocity $v_m \approx 3.6 \times 10^5 \mathrm{m s^{-1}}$. This transition from massive to massless carriers arises from topological band reconstruction driven by the hBN moiré potential. Our results demonstrate that moiré engineering in BLG/hBN offers a powerful route to tune band topology and realize coexisting Dirac and massive fermions within a single crystalline platform.

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Observation of a Reconstructed Chern Insulator in Twisted Bilayer MoTe2

Twisted bilayer MoTe2 is a prototypical moire material in which long-wavelength superlattices amplify electron correlations, enabling a wealth of emergent quantum phases. To date, experimental efforts have focused primarily on small twist angles (typically smaller than 4deg ), whereas the larger-angle regime-where moire bands become more dispersive and correlations are reduced-has remained largely unexplored. Here we chart the topological phase space of tMoTe2 at a relatively large twist angle of approximately 4.54deg, accessing a moderately correlated regime with enhanced bandwidth. In contrast to small-angle devices that predominantly host fractional quantum anomalous Hall or spin Hall responses, we uncover multiple Chern-insulating states with C = 1 at moire fillings v = -1, -0.53 and -1/2. Strikingly, at v = -2/3 a magnetic field induces a fractional Chern insulator accompanied by an insulator-metal transition. Our results broaden the topological phase diagram of tMoTe2 and establish large-angle moire superlattices as a versatile platform for engineering robust topological states beyond the strong-correlation limit.

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Interlayer exciton condensates between second Landau level orbitals in double bilayer graphene

We present Coulomb-drag measurements on a heterostructure comprising two Bernal-stacked bilayer graphene (BLG) sheets separated by a 2.5 nm hexagonal boron nitride (hBN) spacer in the quantum Hall (QH) regime. Using top and bottom gate control, together with an interlayer bias, we independently tune the two BLG layers into either the lowest (N = 0) or second (N = 1) Landau level (LL) orbital and probe their interlayer QH states. When both layers occupy the N = 0 orbital, we observe both interlayer exciton condensates (ECs) at integer total filling and interlayer fractional QH states, echoing the results in double monolayer graphene. In contrast to previous studies, however, when both BLG layers occupy the N = 1 orbital, we also observe quantized drag signals, signifying an interlayer exciton condensate formed between the second LLs. By tuning the layer degree of freedom, we find that this N = 1 EC state arises only when the N = 1 wavefunction in each BLG is polarized toward the hBN interface to maximize the interlayer Coulomb interaction.

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Observation of two-component exciton condensates in an excitonic insulator

Macroscopic quantum coherence emerges when bosons condense into a Bose-Einstein condensate (BEC). First observed as a single-component superfluid in helium, BECs later emerged in ultracold atomic gases at nanokelvin temperatures as weakly interacting quantum fluids, which can also host multicomponent spinor condensates with rich internal degrees of freedom. Excitons provide a promising solid-state platform for BECs that can combine strong interactions, electrical tunability, high transition temperatures, and multicomponent order. Yet, conclusive evidence for condensation has remained elusive. Here, we report evidence of two-component exciton BECs in MoSe2/hBN/WSe2 electron-hole bilayers by directly probing the spin susceptibility of constituent electrons and holes. This heterostructure hosts equilibrium exciton fluids with four spin-valley flavors. Using magneto-optical spectroscopy in a dilution refrigerator, we reveal three exciton condensate phases with distinct flavor polarizations. At zero magnetic field, the many-body ground state is a coherent superposition of two simultaneously condensed intravalley exciton flavors. Under a magnetic field, the intravalley exciton condensate first switches to a two-component intervalley exciton condensate via a first-order quantum phase transition at a weak critical field, and then turns into a fully-polarized single-component condensate at high fields. The two-component condensates persist up to ~1.8 K. Our results establish van der Waals electron-hole bilayers as a versatile platform for exploring strongly interacting, multicomponent exciton BECs.

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Magnetic-field-induced superconductivity in hexalayer rhombohedral graphene

In conventional superconductors, superconductivity is generally suppressed by external magnetic fields due to spin-singlet pairing. Here, we report signatures of in-plane-magnetic-field-induced superconductivity in hexalayer rhombohedral graphene and reveal electric-field control of its depairing behavior. With the application of a small in-plane magnetic field $B_{\parallel}$, a superconducting state emerges within a narrow band along a phase boundary. Its properties evolve continuously with increasing $B_{\parallel}$: the superconducting region progressively shifts toward higher electric field as the $B_{\parallel}$ increases and the transition temperature rises with increasing $B_{\parallel}$. Remarkably, the superconducting state remains robust under $B_{\parallel}$ up to 14 T, far exceeding the conventional Pauli limit. Quantum oscillation measurements further reveal that the superconductivity emerges from nematic Fermi surface reconstruction. These results suggest a spin-polarized superconducting states with unconventional origins.

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Crystallizing electrons with artificially patterned lattices

Wigner crystals are typically confined to ultralow temperatures where thermal motion is frozen out. Moiré superlattices in twisted two-dimensional materials have extended their stability to higher temperatures and densities, but rely on delicate stacking that fixes the lattice geometry and limits tunability. Here we demonstrate a lithographic approach that bypasses these constraints. Using high-resolution nanofabrication, we pattern a nanoscale triangular lattice directly into a graphene gate integrated with a monolayer MoSe2 semiconductor. This engineered potential landscape localizes electrons into generalized Wigner crystal states that persist up to 15 K and densities of 2X10^12 cm-2, representing an order of magnitude improvement over pristine monolayer MoSe2. Gate-voltage control allows real-time switching between stable and unstable crystalline states, with the latter exhibiting stochastic telegraph noise from nearly degenerate configurations. This work demonstrates the ability of this platform to transform Wigner crystals from fragile, static phases into reconfigurable quantum matter.

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Selective braiding of different anyons in the even-denominator fractional quantum Hall effect

Even-denominator quantum Hall states can host several types of anyons with distinct exchange statistics. Depending on the anyon type, exchanging two quasiparticles can impart a phase to the many-body wave function or even transform it into a different state. Here, we realize a gate-tunable Fabry-Pérot interferometer with an embedded antidot that provides local control over the number of anyons within the interference loop. By independently tuning the magnetic field, carrier densities across the device, and the antidot potential, we access regimes in which localized anyons form reproducibly and measure the associated statistical phases $e^{i θ_\mathrm{braid}}$. We resolve braiding phases of $θ_{\mathrm{braid}}=π$ and $θ_{\mathrm{braid}}=\fracπ{2}$, which we attribute to $e/2$ quasiparticles encircling either $e/2$ or $e/4$ quasiparticles, respectively. We further observe switching between different anyon occupancies of the antidot over time, directly resolving individual anyon tunnelling events into the interference loop. Similar behavior occurs at filling factor one third. Our work addresses one of the two key challenges in observing non-Abelian braiding, which requires control of both localized and interfering anyon types.

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Controlled localization of anyons in a graphene quantum Hall interferometer

Exchange statistics are a fundamental principle of quantum mechanics, dictating the symmetry of identical particle wavefunctions and thereby enabling emergent phenomena of many-body quantum states. The exchange-induced unitary transformation of both abelian and non-abelian anyonic wavefunctions can be probed using electronic fractional quantum Hall (FQH) interferometers, where quasiparticles propagating along the interfering FQH edge braid with those localized within the interferometer. Here, we add a gate-controlled dot/anti-dot in the center of a bilayer graphene FQH interferometer cavity to tune the number of enclosed anyons. We observe hundreds of controlled phase slips in the diagonal conductance across the interferometer for both abelian and non-abelian states, consistent with discrete changes in the localized quasiparticle population. For abelian anyons, the observed phase slips agree with the theoretically expected value. At half filling, our results suggest the interfering edge carries charge $|e^*/e| = 1/2$ abelian excitations, whereas charge $|e^*/e| = 1/4$ putative non-abelian anyons remain localized in the interferometer cavity. Controlling the population of localized $e/4$ anyons in an interferometer marks a significant milestone towards observing their non-local exchange statistics and building a fault tolerant topological qubit based on non-abelian anyon manipulation.

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Probing Quantum Anomalous Hall States in Twisted Bilayer WSe2 via Attractive Polaron Spectroscopy

Moiré superlattices in semiconductors exhibit a rich variety of interaction-induced topological states, including quantum anomalous Hall (QAH) effects. A recent study hinted that twisted WSe2 homobilayer (tWSe2) could host a QAH state but lacked direct evidence of ferromagnetism, a key hallmark of this phase. Here, we report the first direct evidence of QAH states in tWSe2 with spontaneous ferromagnetism. Specifically, we employ polarization-resolved attractive polaron spectroscopy on a dual-gated, 2 degree tWSe2 and observe direct signatures of spontaneous time-reversal symmetry breaking at hole filling ν= 1. Together with a Chern number measurement via Streda formula analysis, we identify this magnetized state as a topological state, characterized by C = 1. Furthermore, we demonstrate that these topological and magnetic properties are tunable via a finite displacement field, between a QAH ferromagnetic state and an antiferromagnetic state. Our findings position tWSe2 as a highly versatile, stable, and optically addressable platform for investigating topological order and strong correlations in two-dimensional landscapes.

cond-mat.str-el↗

Intrinsic magnetization of the superconducting condensate in Fe(Te,Se)

A spin-polarized superconducting condensate generates a net magnetization with measurable signatures. We present evidence for an intrinsic magnetic field in mesoscopic Fe(Te,Se) rings. The intrinsic field, encoded in the phase of superconducting quantum oscillations, scales linearly with the DC bias current, and its orientation exhibits an anomalous dependence on polarity and magnitude of the applied current. The magnetoresistance displays a dual flux-quantization effect with respect to the external magnetic field and the DC current. A minimal model incorporating Rashba coupling with an effective anisotropic out-of-plane interaction accounts for the experimental observations. These results provide evidence for spin-polarized superconductivity at the device scale and open new opportunities for superconducting spintronic and quantum information platforms.

cond-mat.supr-con↗

Interaction-driven quantum phase transitions between topological and crystalline orders of electrons

Topological and crystalline orders of electrons both benefit from enhanced Coulomb interactions in partially filled Landau levels. In bilayer graphene (BLG), the competition between fractional quantum Hall liquids and electronic crystals can be tuned electrostatically. Applying a displacement field leads to Landau-level crossings, where the interaction potential is strongly modified due to changes in the orbital wave functions. Here, we leverage this control to investigate phase transitions between topological and crystalline orders at constant filling factors in the lowest Landau level of BLG. Using transport measurements in high-quality hBN-encapsulated devices, we study transitions as a function of displacement field near crossings of $N=0$ and $N=1$ orbitals. The enhanced Landau-level mixing near the crossing stabilizes electronic crystals at all fractional fillings, including a resistive state at $ν= \frac{1}{3}$ and a reentrant integer quantum Hall state at $ν= \frac{7}{3}$. On the $N=0$ side, the activation energies of the crystal and fractional quantum Hall liquid vanish smoothly and symmetrically at the transition, while the $N=1$ transitions out of the crystal appear discontinuous. Additionally, we observe quantized plateaus forming near the crystal transition at half filling of the $N=0$ levels, suggesting a paired composite fermion state stabilized by Landau level mixing.

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Systematic study of superconductivity in few-layer $T_d$-MoTe$_2$

We present a systematic investigation of superconductivity in a topological superconductor candidate $T_{\rm d}$-MoTe$_2$ in the few-layer limit. By examining multiple mechanically exfoliated samples with different thicknesses, substrates and crystal qualities, we quantitatively correlate superconducting temperature ($T_c$) with disorder, carrier density, carrier type and mobility. By integrating these experimental findings with first-principles calculations, we reveal the relationship between the band structure and superconductivity in this material. Notably, in 2 L samples we access a highly hole-doped regime that has not been systematically explored in previous experiments, providing a complementary perspective to earlier studies. In this regime, we demonstrate that superconductivity can be realized in a manner consistent with a conventional phonon-mediated $s_{(++)}$-wave pairing.

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Superconductivity and Ferroelectric Orbital Magnetism in Semimetallic Rhombohedral Hexalayer Graphene

Rhombohedral multilayer graphene has emerged as a promising platform for exploring correlated and topological quantum phases, enabled by its Berry-curvature-bearing flat bands. While prior work has focused on separated conduction and valence bands, we probe the extensive semimetallic regime of rhombohedral hexalayer graphene. We survey a rich phase diagram dominated by flavor-symmetry breaking and reveal an electric-field-driven band inversion by fermiology. Near this inversion, we observe two superconducting-like states confined to regions with coexisting electron and hole Fermi surfaces, suggesting a possible dual-carrier origin. In addition, we identify a ferroelectric orbital magnet that undergoes sharp switching under unipolar electric fields, signaling spontaneous electric polarization. Unlike previously reported multiferroicity near zero electric field, this new state exhibits magnetic hysteresis reversible by electric field, consistent with a phenomenological model of coupled electric and magnetic polarization. Our work elucidates the correlated semimetal regime in rhombohedral graphene and underscores its potential to host diverse quantum phases.

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Layer-polarized Transport via Gate-defined 1D and 0D PN Junctions in Double Bilayer Graphene

We fabricate twisted double bilayer graphene devices with zero twist angle and a set of local top and bottom gates aligned perpendicularly to each other. A 1D PN junction can be electrostatically defined when the gate voltages applied to the top gates are the same but different on the bottom gates. Resistance peaks are observed at finite doping instead of at the charge neutrality points, exhibiting an unconventional broken-cross shape that arises from layer polarization of the P and N region, which can be further enhanced with finite magnetic fields. A 0D point junction (PJ) can be electrostatically defined by applying different gate voltages to the top and bottom gates, such that the P and N sides of the device are connected at a single point in the center of the device. As finite magnetic field B increases, the quantum Hall (QH) states are selectively brought into contact or away from each other depending on their layer polarization, leading to unconventional quantum oscillations which characterize the layer-polarized band-crossing. Our work provides new insights into understanding band-structure evolution and layer polarization in twisted bilayers and paves the way for new device functionality based on manipulating layer-polarized electronic states.

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