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Kento Sasaki

Publications and source records attributed to Kento Sasaki.

At least 37 records · Page 2Linked to original sources

Systematic investigation of dynamic nuclear polarization with boron vacancy in hexagonal boron nitride

Dynamic nuclear polarization (DNP) using the boron vacancy ($\mathrm{V_B^-}$) in hexagonal boron nitride (hBN) has gained increasing attention. Understanding this DNP requires systematically investigating the optically detected magnetic resonance (ODMR) spectra and developing a model that quantitatively describes its behavior. Here, we measure the ODMR spectra of $\mathrm{V_B^-}$ in $\mathrm{h}^{10}\mathrm{B}^{15}\mathrm{N}$ over a wide magnetic field range, including the ground state level anti-crossing (GSLAC), and compare them with the results of the Lindblad-based simulation that considers a single electron spin and three neighboring $^{15}\mathrm{N}$ nuclear spins. Our simulation successfully reproduces the experimental spectra, including the vicinity of GSLAC. It can explain the overall behavior of the magnetic field dependence of the nuclear spin polarization estimated using the Lorentzian fitting of the spectra. Despite such qualitative agreement, we also demonstrate that the fitting methods cannot give accurate polarizations. Finally, we discuss that symmetry-induced mechanisms of $\mathrm{V_B^-}$ limit the maximum polarization. Our study is an essential step toward a quantitative understanding of DNP using defects in hBN and its quantum applications.

cond-mat.mes-hall↗

One-D-Piece: Image Tokenizer Meets Quality-Controllable Compression

Current image tokenization methods require a large number of tokens to capture the information contained within images. Although the amount of information varies across images, most image tokenizers only support fixed-length tokenization, leading to inefficiency in token allocation. In this study, we introduce One-D-Piece, a discrete image tokenizer designed for variable-length tokenization, achieving quality-controllable mechanism. To enable variable compression rate, we introduce a simple but effective regularization mechanism named "Tail Token Drop" into discrete one-dimensional image tokenizers. This method encourages critical information to concentrate at the head of the token sequence, enabling support of variadic tokenization, while preserving state-of-the-art reconstruction quality. We evaluate our tokenizer across multiple reconstruction quality metrics and find that it delivers significantly better perceptual quality than existing quality-controllable compression methods, including JPEG and WebP, at smaller byte sizes. Furthermore, we assess our tokenizer on various downstream computer vision tasks, including image classification, object detection, semantic segmentation, and depth estimation, confirming its adaptability to numerous applications compared to other variable-rate methods. Our approach demonstrates the versatility of variable-length discrete image tokenization, establishing a new paradigm in both compression efficiency and reconstruction performance. Finally, we validate the effectiveness of tail token drop via detailed analysis of tokenizers.

cs.CV↗

Wideband wide-field imaging of spin-wave propagation using diamond quantum sensors

Imaging spin-wave propagation in magnetic materials in a wide frequency range is crucial for understanding and applying spin-wave dynamics. Recently, nitrogen-vacancy (NV) centers in diamond have attracted attention as sensors capable of quantitatively measuring the amplitude and phase of coherent spin waves. However, the conventional sensing protocol has been limited to detecting spin waves whose frequencies match the resonance frequency of the NV spins. We demonstrate that by utilizing the AC Zeeman effect, it is possible to image spin waves propagating in a yttrium iron garnet (YIG) thin film over a wide frequency range up to a maximum detuning of 567 MHz without changing the external magnetic field. Our results expand the applicability of NV centers for spin-wave sensing and pave the way for quantitative investigations of the dynamics in various magnetic materials, such as metallic ferromagnets and van der Waals magnets.

cond-mat.mes-hall↗

Systematic characterization of nanoscale $h$-BN quantum sensor spots created by helium-ion microscopy

The nanosized boron vacancy ($V_\mathrm{B}^-$) defect spot in hexagonal boron nitride ($h$-BN) is promising for a local magnetic field quantum sensor. One of its advantages is that a helium-ion microscope can make a spot at any location in an $h$-BN flake with nanometer accuracy. In this study, we investigate the properties of the created nanosized $V_\mathrm{B}^-$ defect spots by systematically varying three conditions: the helium-ion dose, the thickness of the $h$-BN flakes, and the substrate on which the $h$-BN flakes are attached. The physical background of the results obtained is successfully interpreted using Monte Carlo calculations. From the findings obtained here, a guideline for their optimal creation conditions is obtained to maximize its performance as a quantum sensor concerning sensitivity and localization.

cond-mat.mes-hall↗

Observation of chiral domain walls in an octupole-ordered antiferromagnet

Spin chirality in antiferromagnets offers new opportunities for spintronics. The kagome antiferromagnet Mn3Sn is a paradigmatic material in which the antiferromagnetic order parameter can be detected and controlled by electrical means. However, direct investigation of the magnetic texture of Mn3Sn has been challenging because of the tiny moment hosted in its magnetic octupole, hindering further clarification of this unique material. Here, we address this issue by observing the stray magnetic field from Mn3Sn using a diamond quantum scanning magnetometer. The spatially-resolved intrinsic domains and domain walls in a high-quality single-crystalline Mn3Sn film quantitatively reveal the polarization angle of the magnetic octupole in the kagome plane, the domain's local magnetization, the domain wall's width and chirality, and the octupole order in domain walls. Our nanoscale investigation of Mn3Sn, a powerful complement to macroscopic measurements, paves the road for developing chiral antiferromagnetism and its potential for spintronic applications.

cond-mat.mtrl-sci↗

Heron-Bench: A Benchmark for Evaluating Vision Language Models in Japanese

Vision Language Models (VLMs) have undergone a rapid evolution, giving rise to significant advancements in the realm of multimodal understanding tasks. However, the majority of these models are trained and evaluated on English-centric datasets, leaving a gap in the development and evaluation of VLMs for other languages, such as Japanese. This gap can be attributed to the lack of methodologies for constructing VLMs and the absence of benchmarks to accurately measure their performance. To address this issue, we introduce a novel benchmark, Japanese Heron-Bench, for evaluating Japanese capabilities of VLMs. The Japanese Heron-Bench consists of a variety of imagequestion answer pairs tailored to the Japanese context. Additionally, we present a baseline Japanese VLM that has been trained with Japanese visual instruction tuning datasets. Our Heron-Bench reveals the strengths and limitations of the proposed VLM across various ability dimensions. Furthermore, we clarify the capability gap between strong closed models like GPT-4V and the baseline model, providing valuable insights for future research in this domain. We release the benchmark dataset and training code to facilitate further developments in Japanese VLM research.

cs.CV↗

Demonstration of highly-sensitive wideband microwave sensing using ensemble nitrogen-vacancy centers

Microwave magnetometry is essential for the advancement of microwave technologies. We demonstrate a broadband microwave sensing protocol using the AC Zeeman effect with ensemble nitrogen-vacancy (NV) centers in diamond. A widefield microscope can visualize the frequency characteristics of the microwave resonator and the spatial distribution of off-resonant microwave amplitude. Furthermore, by combining this method with dynamical decoupling, we achieve the microwave amplitude sensitivity of $5.2 \, \mathrm{μT} / \sqrt{\mathrm{Hz}}$, which is 7.7 times better than $40.2 \, \mathrm{μT} / \sqrt{\mathrm{Hz}}$ obtained using the protocol in previous research over a sensing volume of $2.77 \, \mathrm{μm} \times 2.77 \, \mathrm{μm} \times 30 \, \mathrm{nm}$. Our achievement is a concrete step in adapting ensemble NV centers for wideband and widefield microwave imaging.

quant-ph↗

Wide-field quantitative magnetic imaging of superconducting vortices using perfectly aligned quantum sensors

Various techniques have been applied to visualize superconducting vortices, providing clues to their electromagnetic response. Here, we present a wide-field, quantitative imaging of the stray field of the vortices in a superconducting thin film using perfectly aligned diamond quantum sensors. Our analysis, which mitigates the influence of the sensor inhomogeneities, visualizes the magnetic flux of single vortices in YBa$_2$Cu$_3$O$_{7-δ}$ with an accuracy of $\pm10~\%$. The obtained vortex shape is consistent with the theoretical model, and penetration depth and its temperature dependence agree with previous studies, proving our technique's accuracy and broad applicability. This wide-field imaging, which in principle works even under extreme conditions, allows the characterization of various superconductors.

cond-mat.supr-con↗

Nitrogen isotope effects on boron vacancy quantum sensors in hexagonal boron nitride

There has been growing interest in studying hexagonal boron nitride (hBN) for quantum technologies. Here, we investigate nitrogen isotope effects on boron vacancy (V$_\text{B}$) defects, one of the candidates for quantum sensors, in $^{15}$N isotopically enriched hBN synthesized using a metathesis reaction. The Raman shifts are scaled with the reduced mass, consistent with previous work on boron isotope enrichment. We obtain nitrogen isotopic composition-dependent magnetic resonance spectra of V$_\text{B}$ defects and determine the magnitude of the hyperfine interaction parameter of $^{15}$N spin to be 64 MHz. Our investigation provides a design policy for hBNs for quantum sensing.

quant-ph↗

Suppression of Pulsed Dynamic Nuclear Polarization by Many-Body Spin Dynamics

We study a mechanism by which nuclear hyperpolarization due to the polarization transfer from a microwave-pulse-controlled electron spin is suppressed. From analytical and numerical calculations of the unitary dynamics of multiple nuclear spins, we uncover that, combined with the formation of the dark state within a cluster of nuclei, coherent higher-order nuclear spin dynamics impose limits on the efficiency of the polarization transfer even in the absence of mundane depolarization processes such as nuclear spin diffusion and relaxation. Furthermore, we show that the influence of the dark state can be partly mitigated by introducing a disentangling operation. Our analysis is applied to the nuclear polarizations observed in $^{13}$C nuclei coupled with a single nitrogen-vacancy center in diamond [Science 374, 1474 (2021) by J. Randall et al.]. Our work sheds light on collective engineering of nuclear spins as well as future designs of pulsed dynamic nuclear polarization protocols.

quant-ph↗

Optical-power-dependent splitting of magnetic resonance in nitrogen-vacancy centers in diamond

Nitrogen-vacancy (NV) centers in diamonds are a powerful tool for accurate magnetic field measurements. The key is precisely estimating the field-dependent splitting width of the optically detected magnetic resonance (ODMR) spectra of the NV centers. In this study, we investigate the optical power dependence of the ODMR spectra using NV ensemble in nanodiamonds (NDs) and a single-crystal bulk diamond. We find that the splitting width exponentially decays and is saturated as the optical power increases. Comparison between NDs and a bulk sample shows that while the decay amplitude is sample-dependent, the optical power at which the decay saturates is almost sample-independent. We propose that this unexpected phenomenon is an intrinsic property of the NV center due to non-axisymmetry deformation or impurities. Our finding indicates that diamonds with less deformation are advantageous for accurate magnetic field measurements.

cond-mat.mes-hall↗

Magnetic field imaging by hBN quantum sensor nanoarray

Placing a sensor close to the target at the nano-level is a central challenge in quantum sensing. We demonstrate high-spatial-resolution magnetic field imaging with a boron vacancy (V$_\text{B}^-$) defects array in hexagonal boron nitride with a few 10 nm thickness. V$_\text{B}^-$ sensor spots with a size of (100 nm)$^2$ are arranged periodically with nanoscale precision using a helium ion microscope and attached tightly to a gold wire. The sensor array allows us to visualize the magnetic field induced by the current in the wire with a spatial resolution beyond the diffraction limit. Each sensor exhibits a practical sensitivity of $73.6~μ\text{T/Hz}^{0.5}$, suitable for quantum materials research. Our technique of arranging V$_\text{B}^-$ quantum sensors periodically and tightly on measurement targets will maximize their potential.

cond-mat.mes-hall↗

Demonstration of geometric diabatic control of quantum states

Geometric effects can play a pivotal role in streamlining quantum manipulation. We demonstrate a geometric diabatic control, that is, perfect tunneling between spin states in a diamond by a quadratic sweep of a driving field. The field sweep speed for the perfect tunneling is determined by the geometric amplitude factor and can be tuned arbitrarily. Our results are obtained by testing a quadratic version of Berry's twisted Landau-Zener model. This geometric tuning is robust over a wide parameter range. Our work provides a basis for quantum control in various systems, including condensed matter physics, quantum computation, and nuclear magnetic resonance.

quant-ph↗

Frequency-tunable magnetic field sensing using continuous-wave optically detected magnetic resonance with nitrogen-vacancy centers in diamond

The nitrogen-vacancy (NV) center is a promising candidate to realize practical quantum sensors with high sensitivity and high spatial resolution, even at room temperature and atmospheric pressure. In conventional high-frequency AC magnetometry with NV centers, the setup requires a pulse sequence with an appropriate time synchronization and strong microwave power. To avoid these practical difficulties, AC magnetic field sensing using continuous-wave opticallydetected magnetic resonance (CW-ODMR) was recently demonstrated. That previous study utilized radio frequency (RF) dressed states generated by the coherent interaction between the electron spin of the NV center and the RF wave. However, the drawback of this method is that the detectable frequency of the AC magnetic fields is fixed. Here, we propose and demonstrate frequency-tunable magnetic field sensing based on CW-ODMR. In the new sensing scheme, we obtain RF double-dressed states by irradiation with a RF field at two different frequencies. One creates the RF dressed states and changes the frequency of the target AC field. The other is a target AC field that induces a change in the CW-ODMR spectrum by generating the RF double-dressed states through coherent interaction with the RF dressed states. The sensitivity of our method is estimated to be comparable to or even higher than that of the conventional method based on a RF field with a single frequency. The estimated bandwidth is 7.45 MHz, higher than that of the conventional method using the RF dressed states. Our frequency-tunable magnetic field sensor based on CW-ODMR paves the way for new applications in diamond devices.

quant-ph↗

Lock-in thermography using diamond quantum sensors

Precise measurement of temperature distribution and thermal behavior in microscopic regions is critical in many research fields. We demonstrate lock-in thermography using nitrogen-vacancy centers in diamond nanoparticles. We successfully visualize thermal diffusion in glass coverslip and Teflon with micrometer resolution and deduce their thermal diffusivity. By spreading diamond nanoparticles over the sample surface, temperature variation can be measured directly without any physical contact, such as lead wires, making it possible to visualize the micrometer-scale thermal behavior of various materials.

physics.app-ph↗

Machine-learning-enhanced quantum sensors for accurate magnetic field imaging

Local detection of magnetic fields is crucial for characterizing nano- and micro-materials and has been implemented using various scanning techniques or even diamond quantum sensors. Diamond nanoparticles (nanodiamonds) offer an attractive opportunity to chieve high spatial resolution because they can easily be close to the target within a few 10 nm simply by attaching them to its surface. A physical model for such a randomly oriented nanodiamond ensemble (NDE) is available, but the complexity of actual experimental conditions still limits the accuracy of deducing magnetic fields. Here, we demonstrate magnetic field imaging with high accuracy of 1.8 $μ$T combining NDE and machine learning without any physical models. We also discover the field direction dependence of the NDE signal, suggesting the potential application for vector magnetometry and improvement of the existing model. Our method further enriches the performance of NDE to achieve the accuracy to visualize mesoscopic current and magnetism in atomic-layer materials and to expand the applicability in arbitrarily shaped materials, including living organisms. This achievement will bridge machine learning and quantum sensing for accurate measurements.

quant-ph↗

Detection and control of single proton spins in a thin layer of diamond grown by chemical vapor deposition

We report detection and coherent control of a single proton nuclear spin using an electronic spin of the nitrogen-vacancy (NV) center in diamond as a quantum sensor. In addition to determining the NV-proton hyperfine parameters by employing multipulse sequences, we polarize and coherently rotate the single proton spin, and detect an induced free precession. Observation of free induction decays is an essential ingredient for high resolution proton nuclear magnetic resonance, and the present work extends it to the atomic scale. We also discuss the origin of the proton as incorporation during chemical vapor deposition growth, which provides an opportunity to use protons in diamond as built-in quantum memories coupled with the NV center.

quant-ph↗

Spin coherence and depths of single nitrogen-vacancy centers created by ion implantation into diamond via screening masks

We characterize single nitrogen-vacancy (NV) centers created by 10-keV N+ ion implantation into diamond via thin SiO$_2$ layers working as screening masks. Despite the relatively high acceleration energy compared with standard ones (< 5 keV) used to create near-surface NV centers, the screening masks modify the distribution of N$^+$ ions to be peaked at the diamond surface [Ito et al., Appl. Phys. Lett. 110, 213105 (2017)]. We examine the relation between coherence times of the NV electronic spins and their depths, demonstrating that a large portion of NV centers are located within 10 nm from the surface, consistent with Monte Carlo simulations. The effect of the surface on the NV spin coherence time is evaluated through noise spectroscopy, surface topography, and X-ray photoelectron spectroscopy.

quant-ph↗