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Kevin F. MacDonald

Publications and source records attributed to Kevin F. MacDonald.

At least 19 recordsLinked to original sources

Improving Optical Metrology by Engineering the Target Environment

Measurements of positional coordinates and dimensions - whether by human vision or optical instrumentation - are fundamental to safety, industrial productivity, manufacturing quality/accuracy, and scientific discovery. The ultimate precision of such measurements is governed by the Fisher information conveyed from an object to a detector through the optical field, and strategies for enhancing measurement performance often focus on reducing detector noise and/or refining estimation algorithms. Building on the emerging understanding of Fisher information as a physical quantity that propagates through space in a wave-like fashion, we demonstrate that substantial gains in precision can also be made by engineering the electromagnetic environment of a measurement target to optimise the generation and transmission of Fisher information. Using nanowire position metrology based on light scattering at a wavelength {\lambda} = 640 nm as an architype system, we achieve a multifold enhancement in localisation precision, reaching beyond {\lambda}/10,000. Our results establish target environment engineering as a powerful and broadly applicable strategy for advancing measurement and sensing performance across platforms ranging from optical characterisation of micro- and nano-objects to microwave radars and optical LiDAR navigation systems.

physics.optics

Resolving Complex Subwavelength Grating Structures Using Topologically Structured Light

It has been seen recently that when probing a nanoscale object to determine, for example, size or position via light scattering, significant advantage in measurement precision can be gained from exploiting phase singularities in a topologically structured incident light field. Here, we demonstrate that this advantage, derived from the dependence of scattered intensity profiles on strong local (subwavelength-scale) intensity and phase variations in the incident field, can be extended towards imaging applications: Analysis of scattering patterns from arbitrary binary gratings under superoscillatory illumination successfully resolves feature sizes down to ~{\lambda}/7 in single-shot measurements (a factor of 1.4x smaller than is achieved with plane wave illumination), and ~{\lambda}/10.5 in positionally-displaced multi-shot measurements (which yields no improvement in the plane wave case). Interestingly, there are circumstances in which more complex objects are better resolved than simple structures, because interference effects increase the information content of their scattering patterns.

physics.optics

Electron-beam-controlled volatile nanomechanical bistability

Bistability in nanomechanical resonators can be exploited for sensing, signal processing, and memory applications due to its potential for switching and high sensitivity to external stimuli. External vibration can be used to drive a doubly-clamped nanowire into the nonlinear regime of bistable oscillation. Here, we experimentally demonstrate that the bistable oscillation of such a nonlinear nanomechanical resonator can be controlled, switched and read by an electron beam.

physics.app-ph

Control of nanomechanical resonances by an electron beam

The sensitivity of mechanical resonators to physical quantities such as acceleration, pressure, mass and temperature enables them to underpin sensing and metrology applications. Here, we observe that the resonance frequency of a nanomechanical resonator depends strongly on charging. We show that repulsion between an electron beam and charge accumulated on a nanomechanical cantilever yields a stiffening that increases its resonance frequency, providing a mechanism for controlling resonators and sensing charge. For a cantilever of microscale length and nanoscale cross-section interacting with the electron beam of a scanning electron microscope, we observe a resonance shift on the order of 1% per nanocoulomb.

physics.app-ph

Controlling the Flow of Information in Optical Metrology

Optical metrology has progressed beyond the Abbe-Rayleigh limit, unlocking (sub)atomic precision by leveraging nonlinear phenomena, statistical accumulation, and AI estimators trained on measurand variations. Here, we show that Fisher information, which defines the fundamental precision limit, can be viewed as a physical entity that propagates through space, and we derive a wave equation for sensitivity fields describing its flow, which can resonate, diffract, and interfere. We reveal how material composition, geometry, and environmental design dictate where information is generated and how it travels, analogous to antennas and metasurfaces sculpting electromagnetic energy. Plasmonic and dielectric resonances enhance information flow, while gratings and near-field structures reshape radiation patterns. This perspective reframes metrology as a discipline in which resolution can be engineered by tailoring information sources and flow for applications in atomic-scale diagnostics and beyond, including optimisation of Light Detection and Ranging (LiDAR), remote sensing, and radar technologies.

physics.optics

Localization of nanoscale objects with light singularities

Unprecedented atomic-scale measurement resolution has recently been demonstrated in single-shot optical localization metrology based on deep-learning analyses of diffraction patterns of topologically structured light scattered from objects. Here we show that variations in the diffraction patterns caused by positional changes of an object depend upon the spatial derivatives of the magnitude and phase of the incident field, with the latter strongly enhanced at phase singularities. Despite lower intensity near the singularity, an orders-of-magnitude increase in Fisher information contained in the diffraction patterns can be achieved when a nano-object is illuminated by light containing phase singularities, rather than a plane wave. Our work provides a fundamental explanation and motivation for singularity-based metrology with deeply subwavelength precision.

physics.optics

Breaking of Time Translation Symmetry and Ergodicity, and Entropy decrease in a Continuous Time Crystal Driven by Nonreciprocal Optical Forces

Nonreciprocal nonequilibrium process are attracting growing interest in sociology, animal behaviour, chemistry, and nanotechnology, and may have played a role in the origin of life. It is less widely recognized, however, that in open systems light can induce nonreciprocal predator-prey like forces between nanoparticles. Such forces provide access to the continuous time crystal state of matter, which has been demonstrated in a plasmonic metamaterial array of nanowires wherein light triggers a spontaneous mobilization transition to the robust oscillatory state, breaking time translation symmetry. Here, we report on the first experimental study of the transient dynamics of light-induced mobilization and demobilization in a time crystal. By analysing time resolved phase trajectories of the system of nanowires, we show that the mobilization transition is accompanied by breaking of continuous time translation symmetry and ergodicity, and a decrease in the entropy of motion. This insight into the transient dynamics of a nonreciprocity-driven time crystal is relevant to optical timetronics, an information and communications technology paradigm relying on the unique functionalities of time crystals, and applications of the interacting nanowire oscillator platform to modelling a wide range of nonreciprocal processes from many-body dynamics to the early stages of matter-to-life transitions.

physics.optics

Continuous Space-Time Crystal State Driven by Nonreciprocal Optical Forces

Continuous time crystals (CTCs) - media with broken continuous time translation symmetry - are an eagerly sought state of matter that spontaneously transition from a time-independent state to one of periodic motion in response to a small perturbation. The state has been realized recently in an array of nanowires decorated with plasmonic metamolecules illuminated with light. Here we show that this as-yet-unexplained CTC state can be understood as arising from a nonreciprocal phase transition induced by nonconservative radiation pressure forces among plasmonic metamolecules: above a certain intensity threshold, light drives the inhomogeneously broadened array of thermally-driven noisy nanowire oscillators to a synchronized coherent space-time crystal state and ergodicity of the system is broken. At the onset of synchronization, this mechanism does not require nonlinearity in the oscillators but depends instead on nonreciprocal forces. As such it is fundamentally different from the regimes of synchronization that depend on nonlinearity.

physics.optics

Picophotonics -- Subatomic Optical Localization Beyond Thermal Fluctuations

Despite recent tremendous progress in optical imaging and metrology, the resolution gap between atomic scale transmission electron microscopy and optical techniques has not been closed. Is optical imaging and metrology of nanostructures exhibiting Brownian motion possible with resolution beyond thermal fluctuations? Here we report on an experiment in which the average position of a nanowire with a thermal oscillation amplitude of ~150 pm is resolved in single-shot measurements with precision of 92 pm using light at a wavelength of λ = 488 nm, providing the first example of such sub-Brownian metrology with ~λ/5,300 precision. To localize the nanowire, we employ a deep learning analysis of the scattering of topologically structured light, which is highly sensitive to the nanowire's position. As a non-invasive optical metrology with sub-Brownian absolute errors, down to a fraction of the typical size of an atom (Si: 220 pm diameter), it opens the exciting field of picophotonics.

physics.optics

Photonic Metamaterial Analogue of a Continuous Time Crystal

Time crystals are an eagerly sought phase of matter with broken time-translation symmetry. Quantum time crystals with discretely broken time-translation symmetry have been demonstrated in trapped ions, atoms and spins while continuously broken time-translation symmetry has been observed in an atomic condensate inside an optical cavity. Here we report that a classical metamaterial nanostructure, a two-dimensional array of plasmonic metamolecules supported on flexible nanowires, can be driven to a state possessing all of the key features of a continuous time crystal: continuous coherent illumination by light resonant with the metamolecules' plasmonic mode triggers a spontaneous phase transition to a superradiant-like state of transmissivity oscillations, resulting from many-body interactions among the metamolecules, characterized by long-range order in space and time. The phenomenon is of interest to the study of dynamic classical many-body states in the strongly correlated regime and applications in all-optical modulation, frequency conversion and timing.

physics.optics

Optical Control of Nanomechanical Eigenfrequencies and Brownian Motion in Metamaterials

Nanomechanical photonic metamaterials provide a wealth of active switching, nonlinear and enhanced light-matter interaction functionalities by coupling optically and mechanically resonant subsystems. Thermal (Brownian) motion of the nanostructural components of such metamaterials leads to fluctuations in optical properties, which may manifest as noise, but which also present opportunity to characterize performance and thereby optimize design at the level of individual nanomechanical elements. We show that Brownian motion in an all-dielectric metamaterial ensemble of silicon-on-silicon-nitride nanowires can be controlled by light at sub-μW/μm2 intensities. Induced changes in nanowire temperature of just a few Kelvin, dependent upon nanowire dimensions, material composition, and the direction of light propagation, yield proportional changes of several percent in the few-MHz Eigenfrequencies and picometric displacement amplitudes of Brownian motion. The tuning mechanism can provide active control of frequency response in photonic metadevices and may serve as a basis for bolometric, mass and micro/nanostructural stress sensing.

physics.optics

Ballistic Dynamics of Flexural Thermal Movements in a Nano-membrane Revealed with Subatomic Resolution

Flexural oscillations of free-standing films, nano-membranes and nano-wires are attracting growing attention for their importance to the thermal, electrical and mechanical properties of 2D materials. Here we report on the observation of short-timescale ballistic motion in the flexural mode of a nano-membrane cantilever, driven by thermal fluctuation of flexural phonons, including measurements of ballistic velocities and displacements performed with sub-atomic resolution, using a new free electron edge-scattering technique. Within intervals <10 μs, the membrane moves ballistically at a constant velocity, typically ~300 μm/s, while Brownian-like dynamics emerge for longer observation periods. Access to the ballistic regime provides verification of the equipartition theorem and Maxwell-Boltzmann statistics for flexural modes, and can be used in fast thermometry and mass sensing during atomic absorption/desorption processes on the membrane. We argue that the ballistic regime should be accounted for in understanding the electrical, optical, thermal and mechanical properties of 2D materials.

cond-mat.stat-mech

Hyperspectral Nanomotion Microscopy

We have developed a technique that extends static scanning electron microscopic imaging to include hyperspectral mapping of fast thermal and externally-driven movements at up to Megahertz frequencies. It is based on spectral analysis of the secondary electron flux generated by a focused electron beam incident on the moving object. We demonstrate detection of nanowire Brownian motion and hyperspectral mapping of stimulated oscillations of flea setae with deep sub-nanometer displacement sensitivity.

physics.app-ph

All-dielectric free-electron-driven holographic light sources

It has recently been shown that holographically nanostructured surfaces can be employed to control the wavefront of (predominantly plasmonic) optical-frequency light emission generated by the injection of medium-energy electrons into a gold surface. Here we apply the concept to manipulation of the spatial distribution of transition radiation emission from high-refractive-index dielectric/semiconductor target materials, finding that concomitant incoherent luminescent emission at the same wavelength is unperturbed by holographic surface-relief structures, and thereby deriving a means of discriminating between the two emission components.

physics.optics

Smith-Purcell Radiation from Compound Blazed Gratings

Free electrons travelling in vacuum carry evanescent electric field, which can only be coupled to free space light via interaction with a surrounding or nearby medium: as Cherenkov radiation when travelling faster than the local velocity of light or as "Smith-Purcell" (SP) radiation when passing over the surface of a grating. The SP emission characteristics of simple gratings such as a regular array of wires or slits are a well-understood phenomenon. Here we show that for a compound grating made up of several closely-spaced slits repeated for each period, the characteristic angular dispersion of Smith-Purcell radiation can be selectively attenuated or enhanced. We analyze, in particular, the change in intensity as slit elements are added to the structure for two slit sizes and how this affects emission enhancement.

physics.optics

Fibre-optic metadevice for all-optical signal modulation based on coherent absorption

Recently, coherent control of the optical response of thin films of matter in standing waves has attracted considerable attention, ranging from applications in excitation-selective spectroscopy and nonlinear optics to demonstrations of all-optical image processing. Here we show that integration of metamaterial and optical fibre technologies allows the use of coherently controlled absorption in a fully fiberized and packaged switching metadevice. With this metadevice, that controls light with light in a nanoscale plasmonic metamaterial film on an optical fibre tip, we provide proof-of-principle demonstrations of logical functions XOR, NOT and AND that are performed within a coherent fully fiberized network at wavelengths between 1530 nm and 1565 nm. The metadevice performance has been tested with optical signals equivalent to a bitrate of up to 40 Gbit/s and sub-milliwatt power levels. Since coherent absorption can operate at the single photon level and also with 100 THz bandwidth, we argue that the demonstrated all-optical switch concept has potential applications in coherent and quantum information networks.

physics.optics

All-dielectric phase-change reconfigurable metasurface

We harness non-volatile, amorphous-crystalline transitions in the chalcogenide phase-change medium germanium antimony telluride (GST) to realize optically-switchable, all-dielectric metamaterials. Nanostructured, subwavelength-thickness films of GST present high-quality resonances that are spectrally shifted by laser-induced structural transitions, providing reflectivity and transmission switching contrast ratios of up to 5:1 (7 dB) at visible/near-infrared wavelengths selected by design.

cond-mat.mes-hall

Controlling light-with-light without nonlinearity

According to Huygens' superposition principle, light beams traveling in a linear medium will pass though one another without mutual disturbance. Indeed, it is widely held that controlling light signals with light requires intense laser fields to facilitate beam interactions in nonlinear media, where the superposition principle can be broken. We demonstrate here that two coherent beams of light of arbitrarily low intensity can interact on a metamaterial layer of nanoscale thickness in such a way that one beam modulates the intensity of the other. We show that the interference of beams can eliminate the plasmonic Joule losses of light energy in the metamaterial or, in contrast, can lead to almost total absorbtion of light. Applications of this phenomenon may lie in ultrafast all-optical pulse-recovery devices, coherence filters and THz-bandwidth light-by-light modulators.

physics.optics