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Kirk W. Baldwin

Publications and source records attributed to Kirk W. Baldwin.

At least 19 recordsLinked to original sources

Geometric control of hyperbolic exciton-polariton condensate dimers

Coupled many-body quantum systems exhibit rich emergent physics with diverse stationary and dynamical behaviors. By engineering platforms with tunable and distinct coupling mechanisms, new insights emerge into the collective behavior of coupled many body systems. Particles can be exchanged via evanescent or ballistic coupling: the former, based on proximity, yields large spectral splitting, while the latter requires strict phase-matching, analogous to phase-coupled harmonic oscillators, and has a smaller impact on the energy landscape. We demonstrate an all-optically tunable quantum fluid dimer based on exciton-polariton condensates in a photonic crystal waveguide with hyperbolic (saddle-like) dispersion. Varying the dimer's angle relative to the grating tunes the coupling from evanescent to ballistic. We directly observe spectral features and mass flow shaped by the saddle dispersion. This work highlights photonic crystals as powerful platforms to explore condensed matter phenomena lying at the interface between delay-coupled nonlinear oscillators and tight binding physics.

physics.optics↗

Electron Temperature and Electron-Electron Scattering Length in GaAs/AlGaAs Using Mesoscopic Multiparallel Aperture Geometries

Quantifying electron temperatures and electron-electron scattering lengths is essential for understanding electron transport regimes in two-dimensional systems. To that end, this work experimentally investigates low-temperature ballistic transport using semiclassical cyclotron orbits in a multiparallel aperture geometry. The mesoscopic geometry is fabricated on a GaAs/AlGaAs heterostructure of very high electron mobility. The amplitudes of maxima in magnetoresistance due to ballistic transport are observed to decay exponentially with temperature, allowing determination of the electron-electron scattering length from the data. A quantitative relation between electron temperature and an applied dc bias heating current is established by comparing magnetoresistance peak amplitudes measured as a function of temperature and dc bias, reflecting bias-induced Joule heating. In addition, the resistance measured near zero magnetic field decreases with increasing temperature, providing signatures of superballistic conductance.

cond-mat.mes-hall↗

Observation of even-denominator fractional quantum Hall states at $ν= 3/4$ and 5/4 in the lowest Landau level

Two-dimensional electron systems (2DESs) confined to wide GaAs quantum wells provide a unique platform to study exotic fractional quantum Hall states (FQHSs) because the 2DES has a bilayer charge distribution with significant interlayer tunneling. Precise control over the 2DES density allows the tuning of the interlayer tunneling over a wide range. Here, we present our discovery of new even-denominator FQHSs in the lowest Landau level (orbital index \textit{N} = 0) at filling factors $ν= 3/4$ and 5/4 in an ultrahigh-quality 2DES confined to a 72.5-nm-wide GaAs quantum well. The ground states at $ν= 3/4$ and 5/4 both evolve from composite fermion Fermi seas to FQHSs as the density is raised so that interlayer tunneling is sufficiently reduced and the 2DES becomes two-component, signaled by the behavior of the FQHSs flanking $ν= 3/4$ and 5/4. The two-component nature of the $ν=3/4$ and 5/4 FQHSs is also evident from their extreme sensitivity to the bilayer charge distribution symmetry: both states disappear quickly when the charge distribution is made asymmetric by only $\simeq 2\%$. We find a natural explanation for the 3/4 and 5/4 FQHSs in terms of two states linked by particle-hole symmetry, and using the Scarola-Jain bilayer composite fermion framework which is a generalization of the well-known, two-component, Halperin state ($Ψ_{331}$ state). Our observations elucidate the crucial role of competing energy and length scales in wide quantum wells in stabilizing new ground states.

cond-mat.mes-hall↗

Cascade of fractional quantum Hall states in 2D system

The observation of the fractional quantum Hall (FQH) effect in 2D electron gases ushered in investigations of topological phases driven by strong electron correlations. Their remarkable features include fractionalized elementary excitations, gapless boundary states, and non-trivial quantum entanglement patterns. Thanks to persistent efforts in the building of new platforms and making higher-quality samples, a diverse plethora of FQH states have been unveiled in experiments. We report a systematic study of ultrahigh-quality GaAs/AlGaAs quantum wells with mobility up to 3.7*10^7 cm^2/V/s using quantum transport measurements in nuclear adiabatic demagnetization and dilution refrigerators down to 1 mK. In addition to many FQH states that have already been identified in previous work, new longitudinal resistance dips are observed at filling factors 17/33 and 15/31. The application of an in-plane magnetic field causes disparate variations of the FQH states. The theoretical foundation of these states is discussed in the framework of composite fermion theory. While most fractions can be explained as non-interacting composite fermions forming integer quantum Hall states, a few states correspond to FQH states of composite fermions that arise from residual interaction between them. We summarize the observed fractions in the range of 0 < ν < 2 and propose a pattern to account for their experimental appearance that provides an intuitive picture about the relative strengths of different FQH states.

cond-mat.mes-hall↗

Observation of Superfluidity and Meissner Effect of Composite Bosons in GaAs Quantum Hall System

The quantum Hall effect (QHE) is theoretically understood as a superfluid condensate of composite bosons (CBs) -- bound states of electrons and magnetic flux quanta. While dissipationless transport is consistent with this picture, other signatures of superfluidity, such as the Meissner effect, remain elusive. Here, we present direct experimental evidence for CB superfluidity by probing the system's response to a controlled, time-varying magnetic field in Corbino disk geometries. We simultaneously observe the quantized Laughlin charge pumping and a new, quantized charge accumulation phenomenon, governed by the relation $ΔQ_{\rm a}/e = ν\,(ΔΦ/Φ_0)$. This relation signifies that the system actively maintains the fixed electron-to-flux ratio that defines the CBs, neutralizing excess flux by drawing in a precise number of electrons. Crucially, devices with multiple concentric top gates reveal that this charge accumulation is uniformly distributed across the bulk of the QHE fluid, demonstrating that it is a collective, bulk property rather than an edge effect -- a key signature of a superfluid condensate. Furthermore, the presence of a top gate determines the screening mechanism: in a "grand canonical" setting with a gate, low Coulomb energy favors a charge-mediated screening (generalized Meissner effect); without a gate, the system enters a "canonical" regime, exhibiting fixed electron density like type-II superconductors. These observations confirm the CB superfluid nature of the QHE ground state and establish a versatile platform for studying macroscopic quantum coherence and its screening transitions in two dimensions.

cond-mat.mes-hall↗

Observation of e/4 charge at $ν=1/2$ in GaAs

Even-denominator fractional quantum Hall states (FQHSs) fall outside the standard Laughlin's and Jain's odd-denominator hierarchy. In this work, we study the FQHS $ν=1/2$ in the lowest Landau level. The state is confined within a 70 nm-wide GaAs quantum well, where the electrons exhibit a bilayer-like charge distribution. Inter-layer interactions stabilize the $ν=1/2$ FQHS, which is predicted to host quasiparticles with charge e/4 - with either Abelian or non-Abelian topological order. Here, we report on shot-noise measurements of partitioned quasiparticles at $ν=1/2$, where charge partitioning is generated by a unique etch-defined quantum point contact. Our measurements were performed on two nominally identical devices, at two independent experimental setups. Analysis of shot noise in the weak-backscattering regime in each device reveals quasiparticles with charge e/4. These observations provide a clear benchmark for future studies aimed at probing the topological order of the $ν=1/2$ FQHS and its quasiparticles' exchange statistics.

cond-mat.mes-hall↗

Laughlin pumping assisted by surface acoustic waves

The quantum Hall effect is a fascinating electrical transport phenomenon signified by precise quantization of Hall conductivity $σ_\mathrm{xy}$ and vanishing longitudinal conductivity $σ_\mathrm{xx}$. Laughlin proposed an elegant explanation in which adiabatic insertion of a flux tube pumps charge through the system. This analysis unveils the fundamental role of gauge invariance and provides a compelling argument about the fractional charge of fractional quantum Hall states. While it has been used extensively as a theoretical tool, a quantitative experimental investigation is lacking despite multiple attempts. Here we report successful realizations of Laughlin pumping in several integer and fractional quantum Hall states. One essential technical innovation is using surface acoustic waves to periodically clear the charges accumulated during the pumping process. Magnetic fluxes are inserted at a constant rate so there is no need to perform complicated data fitting. Furthermore, our setting can reliably extract $σ_\mathrm{xx}$ that is several orders of magnitude lower than the limit of conventional techniques. Effective energy gaps can be deduced from the temperature dependence of $σ_\mathrm{xx}$, which are drastically different from those provided by conventional transport data. This work not only brings a famous gedanken experiment to reality but also serves as a portal for many future investigations.

cond-mat.mes-hall↗

Observation of a Stripe/nematic Phase of Composite Fermions

Electronic stripe/nematic phases are fascinating strongly-correlated states characterized by spontaneous rotational symmetry breaking. In the quantum Hall regime, such phases typically emerge at half-filled, high-orbital-index ($N\geq2$) Landau levels (LLs) where the short-range Coulomb interaction is softened by the nodes of electron wave functions. In the lowest ($N=0$) LLs, these phases are not expected. Instead, composite fermion (CF) liquids and fractional quantum Hall states, which are well explained in the picture of weakly interacting CF quasiparticles, are favored. Here we report the observation of an unexpected stripe/nematic phase in the \textit{lowest} LL at filling factor $ν=5/8$ in ultrahigh-quality GaAs two-dimensional \textit{hole} systems, evinced by a pronounced in-plane transport anisotropy. Remarkably, $ν=5/8$ can be mapped to a half-filled, high-index CF LL ($N_{\text{CF}}=2$), analogous to the $N=2$ hole LL. Our finding signals a novel stripe/nematic phase of CFs, driven by the residual long-range interaction among these emergent quasiparticles. This phase is surprisingly robust, surviving up to $\sim$100 mK. Its absence in electron-type systems suggests that severe LL mixing stemming from the large hole effective mass and non-linear LL fan diagram plays a crucial role in modifying the CF-CF interaction.

cond-mat.mes-hall↗

Fractional quantum Hall state at $ν= 1/2$ with energy gap up to 6 K, and possible transition from one- to two-component state

The fractional quantum Hall state (FQHS) observed in the lowest Landau level at filling factor $ν=1/2$ in wide quantum wells has been enigmatic for decades because the two-dimensional electron system (2DES) has a bilayer charge distribution but with significant interlayer tunneling. Of particular interest is whether the 1/2 FQHS in this system has a one-component (1C) or two-component (2C) origin; these are typically identified as the Pfaffian (non-Abelian) or the $Ψ_{331}$ (Abelian) FQHSs, respectively. We report here our experimental study of the evolution of the correlated states of an ultrahigh-quality 2DES confined to a 72.5-nm-wide GaAs quantum well. At the lowest densities, the 2DES displays only odd-denominator FQHSs, and the ground state at $ν= 1/2$ is a composite fermion Fermi sea. As the density is increased, a FQHS emerges at $ν= 1/2$, and becomes very strong. In a finite density range where the 1/2 FQHS is strongest, we also observe its daughter FQHSs at $ν= 8/17$ and 7/13, consistent with the theoretically expected daughter states of a Pfaffian 1/2 FQHS. At the highest densities, the 2DES becomes 2C, signaled by the emergence of a bilayer Wigner crystal state and the transitions of FQHSs flanking $ν=1/2$. The 1/2 FQHS remains robust near this transition and, notably, its charge transport energy gap exhibits an \textit{upward} cusp with a maximum value of about 6 K on the 1C side of the transition; this is the largest gap reported for any even-denominator FQHS. Our observation of the transition of the 2DES ground states near $ν=1/2$ to 2C states at high densities, and our measurements of the robustness of the 1/2 FQHS against charge distribution asymmetry, suggest that the 1/2 FQHS also makes a transition from 1C to 2C. Such a transition from a non-Abelian to Abelian state can open avenues for topological quantum information and quantum criticality.

cond-mat.mes-hall↗

Nonlinear transport of Wigner solid phase surrounding the two-flux composite fermion liquid

We have investigated the low temperature (T) transport properties of fractional quantum Hall (FQH) states in a high-mobility two-dimensional hole gas. According to the composite fermion (CF) model, FQH states stemming from a half-filled Landau level, specifically at filling factors $ν=p/(2p+1) (p=\pm 1,\pm 2,\pm 3,...)$, can be associated with two-flux-attached CFs at the corresponding Lambda filling factor p. The zero-resistance minima and Hall plateaus of these states exhibit unusual temperature dependencies, characterized by rapid increases in width below a threshold temperature around 100 mK. Differential conductivity measurements from Corbino samples reveal that the regimes surrounding the CF liquid display clear nonlinear transport characteristics. This nonlinearity implies that each CF liquid is surrounded by CF solid phase composed of dilute CF excitations. Quantitatively, the applied electric field E influences the motion of CF solid in a way analogous to T, which is dubbed the "E-T duality". Our analysis indicates that this E-T duality is consistent with the Berezinskii-Kosterlitz-Thouless theory in two-dimensional phase transitions.

cond-mat.mes-hall↗

Electrically tunable quantum correlations of dipolar polaritons with micrometer-scale blockade radii

An extreme yet reconfigurable nonlinear response to a single photon by a photonic system is crucial for realizing a universal two-photon gate, an elementary building block for photonic quantum computing. Yet such a response, characterized by the photon blockade effect, has only been achieved in atomic systems or solid states ones that are difficult to scale up. Here we demonstrate electrically tunable partial photon blockade in dipolar waveguide polaritons on a semiconductor chip, measured via photon-correlations. Remarkably, these "dipolar photons" display a two-orders-of-magnitude stronger nonlinearity compared to unpolarized polaritons, with an extracted dipolar blockade radius up to more than 4 $μ$m, significantly larger than the optical wavelength, and comparable to that of atomic Rydberg polaritons. Furthermore, we show that the dipolar interaction can be electrically switched and locally configured by simply tuning the gate voltage. Finally we show that with a simple modification of the design, a full photon blockade is expected, setting a new route towards scalable, reconfigurable, chip-integrated quantum photonic circuits with strong two-photon nonlinearities.

quant-ph↗

Design and Fabrication of Robust Hybrid Photonic Crystal Cavities

Heterogeneously integrated hybrid photonic crystal cavities enable strong light-matter interactions with solid-state, optically addressable quantum memories. A key challenge to realizing high quality factor (Q) hybrid photonic crystals is the reduced index contrast on the substrate compared to suspended devices in air. This challenge is particularly acute for color centers in diamond because of diamond's high refractive index, which leads to increased scattering loss into the substrate. Here we develop a design methodology for hybrid photonic crystals utilizing a detailed understanding of substrate-mediated loss, which incorporates sensitivity to fabrication errors as a critical parameter. Using this methodology we design robust, high-Q, GaAs-on-diamond photonic crystal cavities, and by optimizing our fabrication procedure we experimentally realize cavities with Q approaching 30,000 at a resonance wavelength of 955 nm.

physics.optics↗

Targeted Polariton Flow Through Tailored Photonic Defects

In non-Hermitian open quantum systems, such as polariton condensates, local tailoring of gains and losses opens up an interesting possibility to realize functional optical elements. Here, we demonstrate that deliberately introducing losses via a photonic defect, realized by reducing the quality factor of a DBR mirror locally within an ultrahigh-quality microcavity, may be utilized to create directed polariton currents towards the defect. We discuss the role of polariton-polariton interactions in the process and how to tailor the effective decay time of a polariton condensate via coupling to the defect. Our results highlight the far-reaching potential of non-Hermitian physics in polaritonics.

cond-mat.mes-hall↗

Reconfigurable quantum fluid molecules of bound states in the continuum

Topological bound states in the continuum are confined wave-mechanical objects that offer advantageous ways to enhance light-matter interactions in compact photonic devices. In particular, their large quality factor in the strong-coupling regime has recently enabled the demonstration of Bose-Einstein condensation of bound-state-in-the-continuum polaritons. Here, we show that condensation into a negative-mass bound state in the continuum exhibits interaction-induced state confinement, opening opportunities for optically reprogrammable molecular arrays of quantum fluids of light. We exploit this optical trapping mechanism to demonstrate that such molecular complexes show hybridization with macroscopic modes with unusual topological charge multiplicity. Additionally, we demonstrate the scalability of our technique by constructing extended mono- and diatomic chains of bound-state-in-the-continuum polariton fluids that display non-Hermitian band formation and the opening of a minigap. Our findings offer insights into large-scale, reprogrammable, driven, dissipative many-body systems in the strong-coupling regime.

physics.optics↗

Emerging supersolidity from a polariton condensate in a photonic crystal waveguide

A supersolid is a counter-intuitive phase of matter where its constituent particles are arranged into a crystalline structure, yet they are free to flow without friction. This requires the particles to share a global macroscopic phase while being able to reduce their total energy by spontaneous, spatial self-organisation. This exotic state of matter has been achieved in different systems using Bose-Einstein condensates coupled to cavities, possessing spin-orbit coupling, or dipolar interactions. Here we provide experimental evidence of a new implementation of the supersolid phase in a novel non-equilibrium context based on exciton-polaritons condensed in a topologically non-trivial, bound-in-the-continuum state with exceptionally low losses. We measure the density modulation of the polaritonic state indicating the breaking of translational symmetry with a remarkable precision of a few parts in a thousand. Direct access to the phase of the wavefunction allows us to additionally measure the local coherence of the superfluid component. We demonstrate the potential of our synthetic photonic material to host phonon dynamics and a multimode excitation spectrum.

cond-mat.mes-hall↗

Anomalous acousto-current within the quantum Hall plateaus

We systematically study the acousto-current of two-dimensional electron systems in the integer and fractional quantum Hall regimes using surface acoustic waves. We are able to separate the co-existing acoustic scattering and drag, when phonons induce drag current and tune the electron conductivity, respectively. At large acoustic power, the drag current is finite when the system is compressible and exhibits minima when incompressible quantum Hall effects appear. Surprisingly, it exhibits anomalously large bipolar spikes within the quantum Hall plateaus while it vanishes linearly with reduced acoustic power at compressible phases. The current peaks reverse their polarity at the two flanks of exact integer or fractional fillings, consistent with the opposite electric charge of the quasiparticle/quasihole.

cond-mat.mes-hall↗

Metastable Charge Distribution Between Degenerate Landau Levels

We study two dimensional electron systems confined in wide quantum wells whose subband separation is comparable with the Zeeman energy. Two N = 0 Landau levels from different subbands and with opposite spins are pinned in energy when they cross each other and electrons can freely transfer between them. When the disorder is strong, we observe clear hysteresis in our data corresponding to instability of the electron distribution in the two crossing levels. When the intra-layer interaction dominates, multiple minima appear when a Landau level is 1/3 or 2/3 filled and fractional quantum hall effect can be stabilized.

cond-mat.mes-hall↗

Probing quantum phases in ultra-high-mobility two-dimensional electron systems using surface acoustic waves

Transport measurement, which applies an electric field and studies the migration of charged particles, i.e. the current, is the most widely used technique in condensed matter studies. It is generally assumed that the quantum phase remains unchanged when it hosts a sufficiently small probing current, which is, surprisingly, rarely examined experimentally. In this work, we study the ultra-high mobility two-dimensional electron system using a propagating surface acoustic wave, whose traveling speed is affected by the electrons' compressibility. The acoustic power used in our study is several orders of magnitude lower than previous reports, and its induced perturbation to the system is smaller than the transport current. Therefore we are able to observe the quantum phases become more incompressible when hosting a perturbative current.

cond-mat.mes-hall↗