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L. E. Golub

Publications and source records attributed to L. E. Golub.

At least 19 recordsLinked to original sources

Electron spin resonance driven photogalvanic effect in graphene-based structures

We report an electron-spin-resonance-driven linear photogalvanic effect (LPGE) in unbiased monolayer graphene and WSe_2/graphene heterostructures. Under linearly polarized 45--75 GHz radiation, the photovoltage exhibits pronounced resonant features in both Faraday and Voigt geometries. Multiple resonances associated with the electron spin resonance in graphene are observed for both out-of-plane and in-plane magnetic-field orientations. Their magnetic-field positions vary linearly with frequency, their amplitudes reverse sign across the charge-neutrality point, and the resonant contribution has the opposite sign to the nonresonant Drude photogalvanic background. We develop a microscopic theory in which radiation-induced momentum alignment followed by skew scattering generates both contributions. Their opposite signs originate from the orthogonal momentum alignments produced by indirect Drude absorption and direct spin-resonant transitions. The theory describes well the main features of the observed resonant photocurrent and provides a microscopic description of ESR-induced LPGE in two-dimensional systems. These results establish the photogalvanic response as a probe of ESR in unbiased micron-scale graphene-based devices.

cond-mat.mtrl-sci↗

Terahertz field-driven nonlinear Hall effect and other second order transport phenomena in two-dimensional tellurene

We study terahertz field-driven second-order nonlinear electron transport phenomena, including the nonlinear Hall effect (NLHE), in two-dimensional tellurene flakes. The dc current excited by linearly polarized terahertz (THz) radiation in Hall bar samples is investigated in directions both along and perpendicular to the $c$-axis of tellurene. As expected for second-order transport phenomena, the current scales as the square of the in-plane electric field of the radiation $\bf E$, and depends on its orientation. The current results from a combination of three contributions, including the NLHE, the Nonlinear Longitudinal (NLL) and Nonlinear Diagonal (NLD) currents. We established the equivalence between NLH, NLL, and NLD transport currents and Linear photogalvanic effect (LPGE) contributions induced by the absorption of linearly polarized and unpolarized THz radiation. All contributions can be controlled by a gate voltage and have opposite signs for electron and hole conductivity. The magnitude of the current increases drastically when the samples are cooled from room temperature to 4.2 K. It also increases with decreasing radiation frequency. These results are well described by the developed phenomenological and microscopic theories. We show that the THz radiation-induced electric current originates from microscopic mechanisms such as skew scattering, side jump, and the Berry curvature dipole.

cond-mat.mes-hall↗

Coherent transport in non-Abelian quantum graphs

We study quantum charge transport in two-dimensional networks in the presence of a magnetic field and spin-orbit interaction. The interplay of the corresponding Abelian and non-Abelian gauge fields leads to an intricate behavior of the conductance, which has different periodicities in the diffusive and ballistic regimes. We classify all configurations of magnetic and spin-orbit fields where a logarithmically divergent weak-(anti)localization correction appears in the diffusive regime. The conductivity of topologically distinct configurations is the same in the diffusive regime but different in the ballistic regime. The proposed setup provides a feasible realization of quantum graphs with non-Abelian gauge fields.

cond-mat.mes-hall↗

Chirality Driven Ratchet Currents in Two-Dimensional Tellurene with an Asymmetric Grating

The emergence of the terahertz (THz) ratchet effect is a rapidly expanding field of research that utilizes broken spatial symmetry in low-dimensional materials to rectify alternating current (AC) induced by THz fields into direct current (DC). This mechanism is highly promising for next-generation, room-temperature terahertz applications, particularly in high-speed, sensitive detection and imaging. In this work, we explore a ratchet effect generated in two dimensional tellurene, a novel promising semiconductor material consisting of helical atomic chains, creating a structure with inherent chirality. As a key result, the DC circular ratchet current flowing in the chiral axis direction $c$ is determined by the helicity of the radiation and can be reversed by switching the helicity from right to left handed. The circular ratchet effect excited by THz laser radiation is demonstrated for room temperature. The effect is demonstrated at various gate voltages when the Fermi level lies in vicinity of the Weyl point in the conduction band, in the band gap, and in the valence band with almost parabolic energy dispersion. The results are described by the developed microscopic theory based on the Boltzmann kinetic equation approach.

cond-mat.mes-hall↗

Edge spin galvanic effect in altermagnets

The edge spin galvanic effect (ESGE) in $d$-wave altermagnets is proposed. ESGE is a creation of an electrical current flowing along the edge of the sample, which is driven by the spin orientation of charge carriers. The ESGE current is formed owing to the altermagnetic spin splitting and the scattering of carriers by the edge of the sample. The current is sensitive to the orientation of the edge in respect to the main axes of the altermagnet. The edge spin galvanic current reverses its direction upon a reversal of the non-equilibrium spin direction or the Néel vector. We also propose the pure spin edge photocurrent excited by polarized radiation and formed at the edges of a sample. Its dependence on the radiation polarization and frequency is analyzed. The application of an external magnetic field converts this pure spin photocurrent into an electric current along the edge.

cond-mat.mes-hall↗

Interplay of Rashba and valley-Zeeman splittings in weak localization of spin-orbit coupled graphene

Weak localization theory is developed for graphene heterostructures with transition metal dichalcogenides and topological insulators where the Rashba and valey-Zeeman spin-splittings of the energy spectrum are large enough. The anomalous magnetoresistance in low fields caused by weak localization is calculated. It is shown that the valley-Zeeman splitting has no effect on weak localization in the absence of Rashba splitting but it results in the change of the magnetoconductivity sign in the Rashba-coupled graphene. Inter-valley scattering also affects the quantum correction to the conductivity resulting in its sign reversal. Analytical expressions are obtained for the anomalous magnetoconductivity at arbitrary relations between the Rashba and valley-Zeeman splittings as well as the inter-valley scattering rates.

cond-mat.mes-hall↗

Intraband circular photogalvanic effect in Weyl semimetals

We apply the semiclassical theory including the Berry curvature dipole, side jumps and skew scattering for a quantitative description of the circular photogalvanic effect (CPGE) in Weyl semimetals at intraband absorption. In contrast to gapped systems where they completely exhaust all contributions to the CPGE current, all previously known semiclassical mechanisms give a result different from that obtained using a complete quantum-mechanical approach. We show that this difference in the existing quasiclassical and full quantum-mechanical approaches persists at all spatial ranges of the disorder potential. Apparently, the implementation of another microscopic mechanism into the quasiclassical description of the CPGE is required.

cond-mat.mes-hall↗

Bleaching of the Terahertz Magneto-Photogalvanic Effect in CdHgTe Crystals with Kane Fermions

We report the observation and comprehensive study of the complex nonlinear intensity dependence of the magneto-photogalvanic effect (MPGE) current induced by terahertz (THz) radiation in Cd$_{x}$Hg$_{1-x}$Te films with inverted ($x = 0.15$) and noninverted ($x = 0.22$) band structures. The nonlinearities are studied for the resonant MPGE caused by cyclotron resonance, interband transitions between Landau levels, and ionization impurities, as well as for nonresonant indirect Drude-like optical transitions. We show that all these processes lead to the saturation of the photocurrent caused by absorption bleaching. We develop a theoretical framework for each mechanism, which describes measured nonlinearities over an intensity range from 10$^{-3}$ to $4\times10^{4}$ W/cm$^2$. Furthermore, we demonstrate that the saturation processes for these absorption channels differ significantly, allowing us to analyze them independently by considering different intensity regimes. The observed nonlinearities enable us to determine the energy relaxation times of Kane fermions excited by CR and interband optical transitions.

cond-mat.mes-hall↗

Spin orientation by electric current in altermagnets

It is shown that the flow of electric current in an altermagnet results in the formation of a homogeneous electron spin orientation in the sample. The spin of the conduction electrons generated in altermagnets with $d$-wave spin-momentum couplings, is quadratic in the current magnitude, varies as the second angular harmonic under variation of the current direction and does not require broken inversion symmetry. The effect is thus distinct from conventional current induced spin polarization phenomena which are linear in the current, vary as a first angular harmonic under variation of current direction and require broken inversion symmetry. The current-induced spin orientation in altermagnets is obtained using the kinetic theory for distribution functions in the spin-splitted subbands. It is shown that an application of external magnetic field significantly enhances the electron spin.

cond-mat.mes-hall↗

Hanle effect in current induced spin orientation

Electrical spin orientation is the generation of electron spin proportional to the electric current. This phenomenon is allowed by symmetry in gyrotropic systems, e.g. in inversion-asymmetric structures with Rashba spin-orbit splitting. Here we develop a theory of electrical spin orientation for magnetic two-dimensional heterostructures. Spin-orbit coupled graphene and semiconductor heterostructures proximitized by ferromagnets are considered. The analytical theory is based on the Boltzmann kinetic equation for a spin-dependent distribution function and collision integral. We show that the induced spin demonstrates the Hanle effect: a direction of the spin depends on the out-of-plane magnetization. Importantly, the Hanle effect is extremely sensitive to the details of electron elastic scattering. In semiconductor heterostructures, the effect of magnetization is present for scattering by long-range disorder and absent for short-range scattering. In spin-orbit-coupled graphene, the Hanle effect occurs at any scattering potential, but the direction of the spin strongly changes with variation of the disorder type. The theory also describes the effect of valley-Zeeman splitting on the electrical spin orientation in graphene, where the spin experiences opposite Hanle effects in two valleys.

cond-mat.mes-hall↗

Magnetophotogalvanic Effects Driven by Terahertz Radiation in CdHgTe Crystals with Kane Fermions

We report on the observation and comprehensive study of the terahertz radiation induced magneto-photogalvanic effect (MPGE) in bulk CdHgTe crystals hosting Kane fermions. The MPGE has been detected in Cd$_{x}$Hg$_{1-x}$Te films with Cd contents $x = 0.15$ and $0.22$ subjected to an in-plane magnetic field. At liquid helium temperature we observed multiple resonances in MPGE current upon variation of magnetic field. In the $x = 0.22$ with noninverted band structure, the resonances are caused by cyclotron resonance (CR) and photoionization of an impurity level. In the $x = 0.15$ films with an inverted band structure, they originate from the CR and interband optical transitions. Band structure calculated by the Kane model perfectly describes positions of all resonances. In particularly, the resonant MPGE caused by interband transitions excited by THz radiation is caused by the gapless energy spectrum of Kane fermions realized in materials with certain Cd contents and temperature range. In addition to the resonant MPGE current we detected a nonresonant one due to indirect optical transitions (Drude-like). This contribution has a nonmonotonic magnetic field dependence increasing linearly at low magnetic field $B$, approaching a maximum at moderate field and decreasing at high $B$. While the nonresonant MPGE decreases drastically with increasing temperature, it is well measurable up to room temperature. The developed theory demonstrates that the MPGE current arises due to cubic in momentum spin-dependent terms in the scattering probability. The asymmetry caused by these effects results in a pure spin current which is converted into an electric current due to the Zeeman effect.

cond-mat.mes-hall↗

Thermoelectric and viscous contributions to the hydrodynamic ratchet effect

We study thermoelectric and viscous contributions to the ratchet effect, i.e. radiation-induced generation of the direct electric current, $J_{\rm rat},$ in asymmetric dual-grating gate structure without inversion center. Previously [E.Mönch et al, Phys. Rev. B {\bf 105}, 045404 (2022)], it was demonstrated that frequency dependence of the $J_{\rm rat}$ is essentially different within hydrodynamic (HD) and drift-diffusion (DD) regimes of the electron transport: $ J_{\rm rat}^{\rm HD} \propto 1/ω^6 $ and $ J_{\rm rat}^{\rm DD} \propto 1/ω^2 $ for $ω\to \infty.$ Here we analyze previously neglected thermoelectric contribution and find that it yields high-frequency asymptotic $1/ω^2$ even in the HD regime and can change sign of the response. Account of the finite viscosity of the electron liquid yields contribution which scales at high frequency as $1/ω^4.$ We also find plasmonic resonances in the $J_{\rm rat},$ and demonstrate that asymmetry of the structure allows for excitation of the so-called directional travelling plasmons.

cond-mat.mes-hall↗

Circular THz ratchets in a 2D-modulated Dirac system

We report on the observation of the circular ratchet effect excited by terahertz laser radiation in a specially designed two-dimensional metamaterial consisting of a graphene monolayer deposited on a graphite gate patterned with an array of triangular antidots. We show that a periodically driven Dirac fermion system with spatial asymmetry converts the a.c. power into a d.c. current, whose direction reverses when the radiation helicity is switched. The circular ratchet effect is demonstrated for room temperature and a radiation frequency of 2.54 THz. It is shown that the ratchet current magnitude can be controllably tuned by the patterned and uniform back gate voltages. The results are analyzed in the light of the developed microscopic theory considering electronic and plasmonic mechanisms of the ratchet current formation.

cond-mat.mes-hall↗

Terahertz ratchet in graphene 2D metamaterial formed by a patterned gate with an antidot arrayd

We report the observation of the terahertz-induced ratchet effect in graphene-based two-dimensional (2D) metamaterials. The metamaterial consists of a graphite gate patterned with an array of triangular antidots placed under a graphene monolayer. We show that the ratchet current appears due to the noncentrosymmetry of the periodic structure unit cell. The ratchet current is generated owing to the combined action of a spatially periodic in-plane electrostatic potential and a periodically modulated radiation electric field caused by near-field diffraction. The magnitude and direction of the ratchet current are shown to be controlled by voltages applied to both back and patterned gates, which change the lateral asymmetry, carrier type and density. The phenomenological and microscopic theories of ratchet effects in graphene-based 2D metamaterials are developed. The experimental data are discussed in the light of the theory based on the solution of the Boltzmann kinetic equation and the calculated electrostatic potential profile. The theory describes well all the experimental results and shows that the observed ratchet current consists of the Seebeck thermoratchet contribution as well as the linear contribution, which is sensitive to the orientation of the radiation electric field vector with respect to the triangles.

cond-mat.mes-hall↗

Photocurrents in bulk tellurium

We report a comprehensive study of polarized infrared/terahertz photocurrents in bulk tellurium crystals. We observe different photocurrent contributions and show that, depending on the experimental conditions, they are caused by the trigonal photogalvanic effect, the transverse linear photon drag effect, and the magnetic field induced linear and circular photogalvanic effects. All observed photocurrents have not been reported before and are well explained by the developed phenomenological and microscopic theory. We show that the effects can be unambiguously distinguished by studying the polarization, magnetic field, and radiation frequency dependence of the photocurrent. At frequencies around 30 THz, the photocurrents are shown to be caused by the direct optical transitions between subbands in the valence band. At lower frequencies of 1 to 3 THz, used in our experiment, these transitions become impossible and the detected photocurrents are caused by the indirect optical transitions (Drude-like radiation absorption).

cond-mat.mes-hall↗

Theory of weak localization in graphene with spin-orbit interaction

Theory of weak localization in graphene with Rashba splitting of energy spectrum is developed. Anomalous magnetoresistance caused by weak localization is calculated with account for inter- and intravalley, spin-orbit and spin-valley scattering processes. It is shown that the anomalous magnetoresistance is described by the expression different from the traditional Hikami-Larkin-Nagaoka formula. The reason is that the effect of Rashba splitting gives rise to the spin-orbit vector potential which is not reduced to a spin dephasing only. The developed theory can be applied to heterostructures of graphene with transition metal dichalcogenides.

cond-mat.mes-hall↗

Electrical Magnetochiral current in Tellurium

We have studied theoretically the effect of Electrical Magneto-Chiral Anisotropy (eMChA) in $p$-type tellurium crystals. It is shown that the terms $k_i B_j$ in the hole Hamiltonian, linear both in the wave vector ${\mathbf k}$ and the magnetic field ${\mathbf B}$, do not lead to the eMChA and one needs to include the higher-order terms like $k_i^3 B_j$. Two microscopic mechanisms of the effect are considered. In the first one only elastic scattering of holes by impurities or imperfections are taken into consideration only. In the second mechanism, besides the elastic scattering processes the hole gas heating and its energy relaxation are taken into account. It is demonstrated that he both contributions to the magneto-induced rectification are comparable in magnitude. The calculation is performed by using two independent approaches, namely, in the time relaxation approximation and in the limit of of small chiral band parameter $β$. A bridge is thrown between the eMChA and magneto-induced photogalvanic effects.

cond-mat.mes-hall↗

Terahertz spin ratchet effect in magnetic metamaterials

We report on spin ratchet currents driven by terahertz radiation electric fields in a Co/Pt magnetic metamaterial formed by triangle-shaped holes forming an antidots lattice and subjected to an external magnetic field applied perpendicularly to the metal film plane. We show that for a radiation wavelength substantially larger than the period of the antidots array the radiation causes a polarization-independent spin-polarized ratchet current. The current is generated by the periodic asymmetric radiation intensity distribution caused by the near-field diffraction at the edges of the antidots, which induces spatially inhomogeneous periodic electron gas heating, and a phase-shifted periodic asymmetric electrostatic force. The developed microscopic theory shows that the magnetization of the Co/Pt film results in a spin ratchet current caused by both the anomalous Hall and the anomalous Nernst effects. Additionally, we observed a polarization-dependent trigonal spin photocurrent, which is caused by the scattering of electrons at the antidot boundaries resulting in a spin-polarized current due to the magnetization. Microscopic theory of these effects reveals that the trigonal photocurrent is generated at the boundaries of the triangle antidots, whereas the spin ratchet is generated due to the spatially periodic temperature gradient over the whole film. This difference causes substantially different hysteresis widths of these two currents.

cond-mat.mes-hall↗