arXiv subjects

L. N. Pfeiffer

Publications and source records attributed to L. N. Pfeiffer.

At least 55 records · Page 3Linked to original sources

arXiv2023

Bose-Einstein Condensation in Gap-Confined Exciton-Polariton States

The development of patterned multi-quantum well heterostructures in GaAs/AlGaAs waveguides has recently allowed to achieve exciton-polariton condensation in a topologically protected bound state in the continuum (BIC). Remarkably, condensation occurred above a saddle point of the polariton dispersion. A rigorous analysis of the condensation phenomenon in these systems, as well as the role of the BIC, is still missing. In the present Letter we theoretically and experimentally fill this gap, by showing that polariton confinement resulting from the negative effective mass and the photonic energy gap in the dispersion play a key role in enhancing the relaxation towards the condensed state. In fact, our results show that low-threshold polariton condensation is achieved within the effective trap created by the exciting laser spot regardless of whether the resulting confined mode is long-lived (polariton BIC) or short-lived (lossy mode). In both cases, the spatial quantization of the polariton condensate and the threshold differences associated to the corresponding state lifetime are measured and characterized. For a given negative mass, a slightly lower condensation threshold from the polariton BIC mode is found and associated to its suppressed radiative losses as compared to the lossy one.

cond-mat.mes-hall↗

arXiv2023

Anomalous quantized plateaus in two-dimensional electron gas with gate confinement

Quantum information can be coded by the topologically protected edges of fractional quantum Hall (FQH) states. Investigation on FQH edges in the hope of searching and utilizing non-Abelian statistics has been a focused challenge for years. Manipulating the edges, e.g. to bring edges close to each other or to separate edges spatially, is a common and essential step for such studies. The FQH edge structures in a confined region are typically presupposed to be the same as that in the open region in analysis of experimental results, but whether they remain unchanged with extra confinement is obscure. In this work, we present a series of unexpected plateaus in a confined single-layer two-dimensional electron gas (2DEG), which are quantized at anomalous fractions such as 9/4, 17/11, 16/13 and the reported 3/2. We explain all the plateaus by assuming surprisingly larger filling factors in the confined region. Our findings enrich the understanding of edge states in the confined region and in the applications of gate manipulation, which is crucial for the experiments with quantum point contact and interferometer.

cond-mat.mes-hall↗

arXiv2023

Valley-tunable, even-denominator fractional quantum Hall state in the lowest Landau level of an anisotropic system

Fractional quantum Hall states (FQHSs) at even-denominator Landau level filling factors ($ν$) are of prime interest as they are predicted to host exotic, topological states of matter. We report here the observation of a FQHS at $ν=1/2$ in a two-dimensional electron system of exceptionally high quality, confined to a wide AlAs quantum well, where the electrons can occupy multiple conduction-band valleys with an anisotropic effective mass. The anisotropy and multi-valley degree of freedom offer an unprecedented tunability of the $ν=1/2$ FQHS as we can control both the valley occupancy via the application of in-plane strain, and the ratio between the strengths of the short- and long-range Coulomb interaction by tilting the sample in the magnetic field to change the electron charge distribution. Thanks to this tunability, we observe phase transitions from a compressible Fermi liquid to an incompressible FQHS and then to an insulating phase as a function of tilt angle. We find that this evolution and the energy gap of the $ν=1/2$ FQHS depend strongly on valley occupancy.

cond-mat.mes-hall↗

arXiv2023

Interference measurements of non-Abelian e/4 & Abelian e/2 quasiparticle braiding

The quantum Hall states at filling factors $ν=5/2$ and $7/2$ are expected to have Abelian charge $e/2$ quasiparticles and non-Abelian charge $e/4$ quasiparticles. The non-Abelian statistics of the latter has been predicted to display a striking interferometric signature, the even-odd effect. By measuring resistance oscillations as a function of magnetic field in Fabry-Pérot interferometers using new high purity heterostructures, we for the first time report experimental evidence for the non-Abelian nature of excitations at $ν=7/2$. At both $ν=5/2$ and $7/2$ we also examine, for the first time, the fermion parity, a topological quantum number of an even number of non-Abelian quasiparticles. The phase of observed $e/4$ oscillations is reproducible and stable over long times (hours) near both filling factors, indicating stability of the fermion parity. At both fractions, when phase fluctuations are observed, they are predominantly $π$ phase flips, consistent with either fermion parity change or change in the number of the enclosed $e/4$ quasiparticles. We also examine lower-frequency oscillations attributable to Abelian interference processes in both states. Taken together, these results constitute new evidence for the non-Abelian nature of $e/4$ quasiparticles; the observed life-time of their combined fermion parity further strengthens the case for their utility for topological quantum computation.

cond-mat.mes-hall↗

arXiv2023

Coexistence of two hole phases in high-quality $p$-GaAs/AlGaAs in the vicinity of Landau level filling factors $ν$=1 and $ν$=(1/3)

We focused on the transverse AC magneto-conductance of a high mobility $p$-GaAs/AlGaAs quantum well ($p=1.2\times 10^{11}$~cm$^{-2}$) in the vicinity of two values of the Landau level filling factor $ν$: $ν=1$ (integer quantum Hall effect) and $ν=1/3$ (fractional quantum Hall effect). The complex transverse AC conductance, $σ_{xx}^{AC} (ω)$, was found from simultaneous measurements of attenuation and velocity of surface acoustic waves (SAWs) propagating along the interface between a piezoelectric crystal and the two-dimensional hole system under investigation. We analyzed both the real and imaginary parts of the hole conductance and compared the similarities and differences between the results for filling factor 1 and filling factor 1/3. Both to the left and to the right of these values maxima of a specific shape, "wings", arose in the $σ(ν)$ dependences at those two $ν$. Analysis of the results of our acoustic measurements at different temperatures and surface acoustic wave frequencies allowed us to attribute these wings to the formation of collective localized states, namely the domains of a pinned Wigner crystal, i.e., a Wigner solid. While the Wigner solid has been observed in 2D hole systems previously, we were able to detect 20 it at the highest hole density and, therefore, the lowest hole-hole interaction reported.

cond-mat.mes-hall↗

arXiv2023

A Highly Correlated Topological Bubble Phase of Composite Fermions

Strong interactions and topology drive a wide variety of correlated ground states. Some of the most interesting of these ground states, such as fractional quantum Hall states and fractional Chern insulators, have fractionally charged quasiparticles. Correlations in these phases are captured by the binding of electrons and vortices into emergent particles called composite fermions. Composite fermion quasiparticles are randomly localized at high levels of disorder and may exhibit charge order when there is not too much disorder in the system. However, more complex correlations were predicted when composite fermion quasiparticles cluster into a bubble, then these bubbles order on a lattice. Such a highly correlated ground state was termed the bubble phase of composite fermions. Here we report the observation of this bubble phase of composite fermions, evidenced by the reentrance of the fractional quantum Hall effect. We associate this reentrance with a bubble phase with two composite fermion quasiparticles per bubble. Our results demonstrate the existence of a new class of strongly correlated topological phases driven by clustering and charge ordering of emergent quasiparticles.

cond-mat.str-el↗

arXiv2022

Reanalysis of experimental determinations of polariton-polariton interactions in microcavities

The polariton-polariton interaction strength is an important parameter for all kinds of applications using the nonlinear properties of polaritons, such as optical switching and single-photon blockade devices. In this paper, we review and compare the results of a series of experiments on polariton-polariton interactions in GaAs/Al$_x$Ga$_{-1x}$As microcavity polariton structures, and present new theoretical analysis of these experiments. We show that not just the energy shift of the spectral lines, but also the results of measurements sensitive to the polariton scattering rate are important for the calibration of the interaction parameter at low excitation density. We find that when adjustments are made to correct for new understanding of the experiments, the value of the interaction parameter at low density is lower than previous reported, but still significantly higher than theoretically predicted.

cond-mat.quant-gas↗

arXiv2022

Fractional quantum Hall valley ferromagnetism in the extreme quantum limit

Electrons' multiple quantum degrees of freedom can lead to rich physics, including a competition between various exotic ground states, as well as novel applications such as spintronics and valleytronics. Here we report magneto-transport experiments demonstrating how the valley degree of freedom impacts the fractional quantum states (FQHSs), and the related magnetic-flux-electron composite fermions (CFs), at very high magnetic fields in the extreme quantum limit when only the lowest Landau level is occupied. Unlike in other multivalley two-dimensional electron systems such as Si or monolayer graphene and transition-metal dichalcogenides, in our AlAs sample we can continuously tune the valley polarization via the application of in-situ strain. We find that the FQHSs remain exceptionally strong even as they make valley polarization transitions, revealing a surprisingly robust ferromagnetism of the FQHSs and the underlying CFs. Our observation implies that the CFs are strongly interacting in our system. We are also able to obtain a phase diagram for the FQHS and CF valley polarization in the extreme quantum limit as we monitor transitions of the FHQSs with different valley polarizations.

cond-mat.mes-hall↗

arXiv2022

Robust Quantum Hall Ferromagnetism near a Gate-Tuned ν = 1 Landau Level Crossing

In a low-disorder two-dimensional electron system, when two Landau levels of opposite spin or pseudospin cross at the Fermi level, the dominance of the exchange energy can lead to a ferromagnetic, quantum Hall ground state whose gap is determined by the exchange energy and has skyrmions as its excitations. This is normally achieved via applying either hydrostatic pressure or uniaxial strain. We study here a very high-quality, low-density, two-dimensional hole system, confined to a 30-nm-wide (001) GaAs quantum well, in which the two lowest-energy Landau levels can be gate tuned to cross at and near filling factor $ν=1$. As we tune the field position of the crossing from one side of $ν=1$ to the other by changing the hole density, the energy gap for the quantum Hall state at $ν=1$ remains exceptionally large, and only shows a small dip near the crossing. The gap overall follows a $\sqrt{B}$ dependence, expected for the exchange energy. Our data are consistent with a robust quantum Hall ferromagnet as the ground state.

cond-mat.mes-hall↗

arXiv2022

Even-Denominator Fractional Quantum Hall State at Filling Factor ν = 3/4

Fractional quantum Hall states (FQHSs) exemplify exotic phases of low-disorder two-dimensional (2D) electron systems when electron-electron interaction dominates over the thermal and kinetic energies. Particularly intriguing among the FQHSs are those observed at even-denominator Landau level filling factors, as their quasi-particles are generally believed to obey non-Abelian statistics and be of potential use in topological quantum computing. Such states, however, are very rare and fragile, and are typically observed in the excited Landau level of 2D electron systems with the lowest amount of disorder. Here we report the observation of a new and unexpected even-denominator FQHS at filling factor ν = 3/4 in a GaAs 2D hole system with an exceptionally high quality (mobility). Our magneto-transport measurements reveal a strong minimum in the longitudinal resistance at ν = 3/4, accompanied by a developing Hall plateau centered at (h/e2)/(3/4). This even-denominator FQHS is very unusual as it is observed in the lowest Landau level and in a 2D hole system. While its origin is unclear, it is likely a non-Abelian state, emerging from the residual interaction between composite fermions.

cond-mat.mes-hall↗

arXiv2022

Fermi edge singularity in neutral electron-hole system

In neutral dense electron-hole (e-h) systems at low temperatures, theory predicts Cooper-pair-like excitons at the Fermi energy and a BCS-like exciton condensation. Optical excitation allows creating e-h systems with the densities controlled by the excitation power. However, the intense optical excitations required to achieve high densities cause substantial heating of the e-h system that prevents the realization of dense and cold e-h systems in conventional semiconductors. In this work, we study e-h systems created by optical excitation in separated electron and hole layers. The layer separation increases the e-h recombination time and, in turn, the density for a given optical excitation by orders of magnitude and, as a result, enables the realization of the dense and cold e-h system. We found a strong enhancement of photoluminescence intensity at the Fermi energy of the neutral dense ultracold e-h system that evidences the emergence of excitonic Fermi edge singularity due to the Cooper-pair-like excitons at the Fermi energy.

cond-mat.quant-gas↗

arXiv2022

Composite Fermion Mass

Composite fermions (CFs), exotic quasi-particles formed by pairing an electron and an even number of magnetic flux quanta emerge at high magnetic fields in an interacting electron system, and can explain phenomena such as the fractional quantum Hall state (FQHS) and other many-body phases. CFs possess an effective mass ($m_{CF}$) whose magnitude is inversely related to the most fundamental property of a FQHS, namely its energy gap. We present here experimental measurements of $m_{CF}$ in ultra-high quality two-dimensional electron systems confined to GaAs quantum wells of varying thickness. An advantage of measuring $m_{CF}$ over gap measurements is that mass values are insensitive to disorder and are therefore ideal for comparison with theoretical calculations, especially for high-order FQHS. Our data reveal that $m_{CF}$ increases with increasing well width, reflecting a decrease in the energy gap as the electron layer becomes thicker and the in-plane Coulomb energy softens. Comparing our measured masses with available theoretical results, we find significant quantitative discrepancies, highlighting that more rigorous and accurate calculations are needed to explain the experimental data.

cond-mat.mes-hall↗

arXiv2022

Anisotropic, two-dimensional, disordered Wigner solid

The interplay between the Fermi sea anisotropy, electron-electron interaction, and localization phenomena can give rise to exotic many-body phases. An exciting example is an anisotropic two-dimensional (2D) Wigner solid (WS), where electrons form an ordered array with an anisotropic lattice structure. Such a state has eluded experiments up to now as its realization is extremely demanding: First, a WS entails very low densities where the Coulomb interaction dominates over the kinetic (Fermi) energy. Attaining such low densities while keeping the disorder low is very challenging. Second, the low-density requirement has to be fulfilled in a material that hosts an anisotropic Fermi sea. Here, we report transport measurements in a clean (low-disorder) 2D electron system with anisotropic effective mass and Fermi sea. The data reveal that at extremely low electron densities, when the r_s parameter, the ratio of the Coulomb to the Fermi energy, exceeds 38, the current-voltage characteristics become strongly nonlinear at small dc biases. Several key features of the nonlinear characteristics, including their anisotropic voltage thresholds, are consistent with the formation of a disordered, anisotropic WS pinned by the ubiquitous disorder potential.

cond-mat.str-el↗

arXiv2022

Understanding limits to mobility in ultra-high-mobility GaAs two-dimensional electron systems: The quest for 100 million cm$^2$/Vs and beyond

For several decades now, ultra-high-mobility GaAs two-dimensional electron systems (2DESs) have served as the hallmark platform for various branches of research in condensed matter physics. Fundamental to this long-standing history of success for GaAs 2DESs was continuous sample quality improvement, which enabled scattering-free transport over macroscopic length scales as well as the emergence of a diverse range of exotic many-body phenomena. While the recent breakthrough in the quality of GaAs 2DESs grown by molecular beam epitaxy is highly commendable in this context, it is also important and timely to establish an up-to-date understanding of what obstructs us from pushing the mobility limit even further. Here, we present mobility data taken at a temperature of 0.3 K for a wide variety of state-of-the-art GaAs 2DESs, exhibiting a maximum, world-record mobility of $μ\simeq57\times10^6$ cm$^2$/Vs at a 2DES density of $n=1.55\times10^{11}$ /cm$^2$. We also provide comprehensive analyses of the collective scattering mechanisms that can explain the results. Furthermore, based on our study, we discuss potential scenarios where GaAs 2DES mobility values exceeding $100\times10^6$ cm$^2$/Vs could be achieved.

cond-mat.mes-hall↗

arXiv2022

Hydrodynamic charge transport in GaAs/AlGaAs ultrahigh-mobility two-dimensional electron gas

Viscous fluid in an ultrahigh-mobility two-dimensional electron gas (2DEG) in GaAs/AlGaAs quantum wells is systematically studied through measurements of negative magnetoresistance (NMR) and photoresistance under microwave radiation, and the data are analyzed according to recent theoretical work by e.g., Alekseev, Physical Review Letters 117,166601 (2016). Size-dependent and temperature dependent NMR are found to conform to the theoretical predictions. In particular, transport of 2DEG with relatively weak Coulomb interaction (interparticle interaction parameter r_s<1) manifests a crossover between viscous liquid and viscous gas. The size dependence of microwave induced resistance oscillations and that of the '2nd harmonic' peak indicate that 2DEG in a moderate magnetic field should be regarded as viscous fluid as well. Our results suggest that the hydrodynamic effects must be considered in order to understand semiclassical electronic transport in a clean 2DEG.

cond-mat.mes-hall↗

arXiv2022

Fabrication of Nanostructured GaAs/AlGaAs Waveguide for Low-Density Polariton Condensation from a Bound State in the Continuum

Exciton-polaritons are hybrid light-matter states that arise from strong coupling between an exciton resonance and a photonic cavity mode. As bosonic excitations, they can undergo a phase transition to a condensed state that can emit coherent light without a population inversion. This aspect makes them good candidates for thresholdless lasers, yet short exciton-polariton lifetime has made it difficult to achieve condensation at very low power densities. In this sense, long-lived symmetry-protected states are excellent candidates to overcome the limitations that arise from the finite mirror reflectivity of monolithic microcavities. In this work we use a photonic symmetry protected bound state in the continuum coupled to an excitonic resonance to achieve state-of-the-art polariton condensation threshold in GaAs/AlGaAs waveguide. Most important, we show the influence of fabrication control and how surface passivation via atomic layer deposition provides a way to reduce exciton quenching at the grating sidewalls.

physics.optics↗

arXiv2022

Correlated states of 2D electrons near the Landau level filling $ν=1/7$

The ground state of two-dimensional electron systems (2DESs) at low Landau level filling factors ($ν\lesssim1/6$) has long been a topic of interest and controversy in condensed matter. Following the recent breakthrough in the quality of ultra-high-mobility GaAs 2DESs, we revisit this problem experimentally and investigate the impact of reduced disorder. In a GaAs 2DES sample with density $n=6.1\times10^{10}$ /cm$^2$ and mobility $μ=25\times10^6$ cm$^2$/Vs, we find a deep minimum in the longitudinal magnetoresistance ($R_{xx}$) at $ν=1/7$ when $T\simeq104$ mK. There is also a clear sign of a developing minimum in the $R_{xx}$ at $ν=2/13$. While insulating phases are still predominant when $ν\lesssim1/6$, these minima strongly suggest the existence of fractional quantum Hall states at filling factors that comply with the Jain sequence $ν=p/(2mp\pm1)$ even in the very low Landau level filling limit. The magnetic field dependent activation energies deduced from the relation $R_{xx}\propto e^{E_A/2kT}$ corroborate this view, and imply the presence of pinned Wigner solid states when $ν\neq p/(2mp\pm1)$. Similar results are seen in another sample with a lower density, further generalizing our observations.

cond-mat.mes-hall↗

arXiv2022

Record-quality GaAs two-dimensional hole systems

The complex band structure, large spin-orbit induced band splitting, and heavy effective mass of two-dimensional (2D) hole systems hosted in GaAs quantum wells render them rich platforms to study many-body physics and ballistic transport phenomena. Here we report ultra-high-quality (001) GaAs 2D hole systems, fabricated using molecular beam epitaxy and modulation doping, with mobility values as high as $5.8\times10^6$ cm$^2$/Vs at a hole density of $p=1.3\times10^{11}$ /cm$^2$, implying a mean-free path of $\simeq27$ $μ$m. In the low-temperature magnetoresistance trace of this sample, we observe high-order fractional quantum Hall states up to the Landau level filling $ν=12/25$ near $ν=1/2$. Furthermore, we see a deep minimum develop at $ν=1/5$ in the magnetoresistance of a sample with a much lower hole density of $p=4.0\times10^{10}$ /cm$^2$ where we measure a mobility of $3.6\times10^6$ cm$^2$/Vs. These improvements in sample quality were achieved by reduction of residual impurities both in the GaAs channel and the AlGaAs barrier material, as well as optimization in design of the sample structure.

cond-mat.mes-hall↗