arXiv subjects

L. N. Pfeiffer

Publications and source records attributed to L. N. Pfeiffer.

At least 73 records · Page 4Linked to original sources

arXiv2022

Capacitive Response of Wigner Crystals at the Quantum Hall Plateau

In this report, we study ultra-high-mobility two-dimensional (2D) electron/hole systems with high precision capacitance measurement. We find that the capacitance charge appears only at the fringe of the gate at high magnetic field when the 2D conductivity decreases significantly. At integer quantum Hall effects, the capacitance vanishes and forms a plateau at high temperatures $T\gtrsim 300$ mK, which surprisingly, disappears at $T\lesssim 100$ mK. This anomalous behavior is likely a manifestation that the dilute particles/vacancies in the top-most Landau level form Wigner crystal, which has finite compressibility and can host polarization current.

cond-mat.mes-hall↗

arXiv2021

Reconstruction of Bloch wavefunctions of holes in a semiconductor

A central goal of condensed-matter physics is to understand how the diverse electronic and optical properties of crystalline materials emerge from the wavelike motion of electrons through periodically arranged atoms. However, more than 90 years after Bloch derived the functional forms of electronic waves in crystals [1] (now known as Bloch wavefunctions), rapid scattering processes have so far prevented their direct experimental reconstruction. In high-order sideband generation [2-9], electrons and holes generated in semiconductors by a near-infrared laser are accelerated to a high kinetic energy by a strong terahertz field, and recollide to emit near-infrared sidebands before they are scattered. Here we reconstruct the Bloch wavefunctions of two types of hole in gallium arsenide at wavelengths much longer than the spacing between atoms by experimentally measuring sideband polarizations and introducing an elegant theory that ties those polarizations to quantum interference between different recollision pathways. These Bloch wavefunctions are compactly visualized on the surface of a sphere. High-order sideband generation can, in principle, be observed from any direct-gap semiconductor or insulator. We thus expect that the method introduced here can be used to reconstruct low-energy Bloch wavefunctions in many of these materials, enabling important insights into the origin and engineering of the electronic and optical properties of condensed matter.

cond-mat.mtrl-sci↗

arXiv2021

Dresselhaus spin-orbit interaction in the p-AlGaAs/GaAs/AlGaAs structure with a square quantum well: Surface Acoustic Waves Study

The effect of spin-orbit interaction was studied in a high-quality $p$-AlGaAs/GaAs/AlGaAs structure with a square quantum well using acoustic methods. The structure grown on a GaAs (100) substrate was symmetrically doped with carbon on both sides of the quantum well. Shubnikov-de Haas-type oscillations of the ac conductance of two-dimensional holes were measured. At a low magnetic field $B <$2 T conductance oscillations undergo beating induced by a spin-orbit interaction. Analysis of the beating character made it possible to separate the conductance contributions from the two heavy holes subbands split by the spin-orbit interaction. For each of the subbands the values of the effective masses and quantum relaxation times have been determined, and then the energy of the spin-orbit interaction was obtained. The quantum well profile, as well as the small magnitude of the spin-orbit interaction, allowed us to conclude that the spin-orbit splitting is governed by the Dresselhaus mechanism.

cond-mat.mes-hall↗

arXiv2021

Magnetotransport patterns of collective localization near $ν=1$ in a high-mobility two-dimensional electron gas

We report complex magnetotransport patterns of the $ν=1$ integer quantum Hall state in a GaAs/AlGaAs sample from the newest generation with a record high electron mobility. The reentrant integer quantum Hall effect in the flanks of the $ν=1$ plateau indicates the formation of the integer quantum Hall Wigner solid, a collective insulator. Moreover, at a fixed filling factor, the longitudinal resistance versus temperature in the region of the integer quantum Hall Wigner solid exhibits a sharp peak. Such sharp peaks in the longitudinal resistance versus temperature so far were only detected for bubble phases forming in high Landau levels but were absent in the region of the Anderson insulator. We suggest that in samples of sufficiently low disorder sharp peaks in the longitudinal resistance versus temperature traces are universal transport signatures of all isotropic electron solids that form in the flanks of integer quantum Hall plateaus. We discuss possible origins of these sharp resistance peaks and we draw a stability diagram for the insulating phases in the $ν$-$T$ phase space.

cond-mat.str-el↗

arXiv2021

Particle-Hole Symmetry and the Reentrant Integer Quantum Hall Wigner Solid

The interplay of strong Coulomb interactions and of topology is currently under intense scrutiny in various condensed matter and atomic systems. One example of this interplay is the phase competition of fractional quantum Hall states and the Wigner solid in the two-dimensional electron gas. Here we report a Wigner solid at $ν=1.79$ and its melting due to fractional correlations occurring at $ν=9/5$. This Wigner solid, that we call the reentrant integer quantum Hall Wigner solid, develops in a range of Landau level filling factors that is related by particle-hole symmetry to the so called reentrant Wigner solid. We thus find that the Wigner solid in the GaAs/AlGaAs system straddles the partial filling factor $1/5$ not only at the lowest filling factors, but also near $ν=9/5$. Our results highlight the particle-hole symmetry as a fundamental symmetry of the extended family of Wigner solids and paint a complex picture of the competition of the Wigner solid with fractional quantum Hall states.

cond-mat.str-el↗

arXiv2021

Melting phase diagram of bubble phases in high Landau levels

A low-disorder, two-dimensional electron system (2DES) subjected to a large perpendicular magnetic field and cooled to very low temperatures provides a rich platform for studies of many-body quantum phases. The magnetic field quenches the electrons' kinetic energy and quantizes the energy into a set of Landau levels, allowing the Coulomb interaction to dominate. In excited Landau levels, the fine interplay between short- and long-range interactions stabilizes bubble phases, Wigner crystals with more than one electron per unit cell. Here we present the screening properties of bubble phases, probed via a simple capacitance technique where the 2DES is placed between a top and a bottom gate and the electric field penetrating through the 2DES is measured. The bubbles formed at very low temperatures screen the electric field poorly as they are pinned by the residual disorder potential, allowing a large electric field to reach the top gate. As the temperature is increased, the penetrating electric field decreases and, surprisingly, exhibits a pronounced minimum at a temperature that appears to coincide with the melting temperature of the bubble phase. We deduce a quantitative phase diagram for the transition from bubble to liquid phases for Landau level filling factors $4\leqν\leq5$.

cond-mat.mes-hall↗

arXiv2021

Dynamic ordering transitions in charged solid

The phenomenon of group motion is common in nature, ranging from the schools of fish, birds and insects, to avalanches, landslides and sand drift. If we treat objects as collectively moving particles, such phenomena can be studied from a physical point of view, and the research on many-body systems has proved that marvelous effects can arise from the simplest individuals. The motion of numerous individuals presents different dynamic phases related to the ordering of the system. However, it is usually difficult to study the dynamic ordering and their transitions through experiments. Electron bubble states formed in a two-dimensional electron gas, as a type of electron solids, can be driven by an external electric field and provide a platform to study the dynamic collective behaviors. Here, we demonstrate that noise spectrum is a powerful method to investigate the dynamics of bubble states. We observed not only the phenomena from dynamically ordered and disordered structures, but also unexpected alternations between them. Our results show that a dissipative system can convert between chaotic structures and ordered structures when tuning global parameters, which is concealed in conventional transport measurements of resistance or conductance. Moreover, charging the objects to study electrical noise spectrum in collective motions can be an additional approach to revealing dynamic ordering transitions.

cond-mat.mes-hall↗

arXiv2021

Anomalous nematic-to-stripe phase transition driven by in-plane magnetic fields

Anomalous nematic states, recently discovered in ultraclean two-dimensional electron gas, emerge from quantum Hall stripe phases upon further cooling. These states are hallmarked by a local minimum (maximum) in the hard (easy) longitudinal resistance and by an incipient plateau in the Hall resistance in nearly half-filled Landau levels. Here, we demonstrate that a modest in-plane magnetic field, applied either along $\left < 110 \right >$ or $\left < 1\bar10 \right >$ crystal axis of GaAs, destroys anomalous nematic states and restores quantum Hall stripe phases aligned along their native $\left < 110 \right >$ direction. These findings confirm that anomalous nematic states are distinct from other ground states and will assist future theories to identify their origin.

cond-mat.mes-hall↗

arXiv2021

Design rules for modulation-doped AlAs quantum wells

Thanks to their multi-valley, anisotropic, energy band structure, two-dimensional electron systems (2DESs) in modulation-doped AlAs quantum wells (QWs) provide a unique platform to investigate electron interaction physics and ballistic transport. Indeed, a plethora of phenomena unseen in other 2DESs have been observed over the past decade. However, a foundation for sample design is still lacking for AlAs 2DESs, limiting the means to achieve optimal quality samples. Here we present a systematic study on the fabrication of modulation-doped AlAs and GaAs QWs over a wide range of AlxGa1-xAs barrier alloy compositions. Our data indicate clear similarities in modulation doping mechanisms for AlAs and GaAs, and provide guidelines for the fabrication of very high quality AlAs 2DESs. We highlight the unprecedented quality of the fabricated AlAs samples by presenting the magnetotransport data for low density (~1X1011 cm2) AlAs 2DESs that exhibit high-order fractional quantum Hall signatures.

cond-mat.mes-hall↗

arXiv2021

Ultra-high quality two-dimensional electron systems

Two-dimensional electrons confined to GaAs quantum wells are hallmark platforms for probing electron-electron interaction. Many key observations have been made in these systems as sample quality improved over the years. Here, we present a breakthrough in sample quality via source-material purification and innovation in GaAs molecular beam epitaxy vacuum chamber design. Our samples display an ultra-high mobility of $44\times10^6$ cm$^2$/Vs at an electron density of $2.0\times10^{11}$ /cm$^2$. These results imply only 1 residual impurity for every $10^{10}$ Ga/As atoms. The impact of such low impurity concentration is manifold. Robust stripe/bubble phases are observed, and several new fractional quantum Hall states emerge. Furthermore, the activation gap of the $ν=5/2$ state, which is widely believed to be non-Abelian and of potential use for topological quantum computing, reaches $Δ\simeq820$ mK. We expect that our results will stimulate further research on interaction-driven physics in a two-dimensional setting and significantly advance the field.

cond-mat.mes-hall↗

arXiv2021

Heterostructure design to achieve high quality, high density GaAs 2D electron system with $g$-factor tending to zero

Hydrostatic pressure is a useful tool that can tune several key parameters in solid state materials. For example, the Landé $g$-factor in GaAs two-dimensional electron systems (2DESs) is expected to change from its bulk value $g\simeq-0.44$ to zero and even to positive values under a sufficiently large hydrostatic pressure. Although this presents an intriguing platform to investigate electron-electron interaction in a system with $g=0$, studies are quite limited because the GaAs 2DES density decreases significantly with increasing hydrostatic pressure. Here we show that a simple model, based on pressure-dependent changes in the conduction band alignment, quantitatively explains this commonly observed trend. Furthermore, we demonstrate that the decrease in the 2DES density can be suppressed by more than a factor of 3 through an innovative heterostructure design.

cond-mat.mes-hall↗

arXiv2021

Fractional quantum Hall effect energy gap: role of electron layer thickness

The fractional quantum Hall effect (FQHE) stands as a quintessential manifestation of an interacting two-dimensional electron system. One of FQHE's most fundamental characteristics is the energy gap separating the incompressible ground state from its excitations. Yet, despite nearly four decades of investigations, a quantitative agreement between the theoretically calculated and experimentally measured energy gaps is lacking. Here we report a quantitative comparison between the measured energy gaps and the available theoretical calculations that take into account the role of finite layer thickness and Landau level mixing. Our systematic experimental study of the FQHE energy gaps uses very high-quality two-dimensional electron systems confined to GaAs quantum wells with varying well widths. All the measured energy gaps fall bellow the calculations, but as the electron layer thickness increases, the results of experiments and calculations come closer. Accounting for the role of disorder in a phenomenological manner, we find the measured energy gaps to be in reasonable quantitative agreement with calculations, although some discrepancies remain.

cond-mat.mes-hall↗

arXiv2021

Topological phase transition in an all-optical exciton-polariton lattice

Topological insulators are a class of electronic materials exhibiting robust edge states immune to perturbations and disorder. This concept has been successfully adapted in photonics, where topologically nontrivial waveguides and topological lasers were developed. However, the exploration of topological properties in a given photonic system is limited to a fabricated sample, without the flexibility to reconfigure the structure in-situ. Here, we demonstrate an all-optical realization of the orbital Su-Schrieffer-Heeger (SSH) model in a microcavity exciton-polariton system, whereby a cavity photon is hybridized with an exciton in a GaAs quantum well. We induce a zigzag potential for exciton polaritons all-optically, by shaping the nonresonant laser excitation, and measure directly the eigenspectrum and topological edge states of a polariton lattice in a nonlinear regime of bosonic condensation. Furthermore, taking advantage of the tunability of the optically induced lattice we modify the intersite tunneling to realize a topological phase transition to a trivial state. Our results open the way to study topological phase transitions on-demand in fully reconfigurable hybrid photonic systems that do not require sophisticated sample engineering.

physics.optics↗

arXiv2021

Low-energy collective oscillations and Bogoliubov sound in an exciton-polariton condensate

We report the observation of low-energy, low-momenta collective oscillations of an excitonpolariton condensate in a round "box" trap. The oscillations are dominated by the dipole and breathing modes, and the ratio of the frequencies of the two modes is consistent with that of a weakly interacting two-dimensional trapped Bose gas. The speed of sound extracted from the dipole oscillation frequency is smaller than the Bogoliubov sound, which can be partly explained by the influence of the incoherent reservoir. These results pave the way for understanding the effects of reservoir, dissipation, energy relaxation, and finite temperature on the superfluid properties of exciton-polariton condensates and other two-dimensional open-dissipative quantum fluids.

cond-mat.quant-gas↗

arXiv2020

Collective excitations of exciton-polariton condensates in a synthetic gauge field

Collective (elementary) excitations of quantum bosonic condensates, including condensates of exciton polaritons in semiconductor microcavities, are a sensitive probe of interparticle interactions. In anisotropic microcavities with momentum-dependent TE-TM splitting of the optical modes, the excitations dispersions are predicted to be strongly anisotropic, which is a consequence of the synthetic magnetic gauge field of the cavity, as well as the interplay between different interaction strengths for polaritons in the singlet and triplet spin configurations. Here, by directly measuring the dispersion of the collective excitations in a high-density optically trapped exciton-polariton condensate, we observe excellent agreement with the theoretical predictions for spinor polariton excitations. We extract the inter- and intra-spin polariton interaction constants and map out the characteristic spin textures in an interacting spinor condensate of exciton polaritons.

cond-mat.quant-gas↗

arXiv2020

Observation of spontaneous valley polarization of itinerant electrons

Memory or transistor devices based on electron's spin rather than its charge degree of freedom offer certain distinct advantages and comprise a cornerstone of spintronics. Recent years have witnessed the emergence of a new field, valleytronics, which seeks to exploit electron's valley index rather than its spin. An important component in this quest would be the ability to control the valley index in a convenient fashion. Here we show that the valley polarization can be switched from zero to one by a small reduction in density, simply tuned by a gate bias, in a two-dimensional electron system. This phenomenon arises fundamentally as a result of electron-electron interaction in an itinerant, dilute electron system. Essentially, the kinetic energy favors an equal distribution of electrons over the available valleys, whereas the interaction between electrons prefers single-valley occupancy below a critical density. The gate-bias-tuned transition we observe is accompanied by a sudden, two-fold change in sample resistance, making the phenomenon of interest for potential valleytronic transistor device applications. Our observation constitutes a quintessential demonstration of valleytronics in a very simple experiment.

cond-mat.mes-hall↗

arXiv2020

Dynamics of spin polarization in tilted polariton rings

We have observed the effect of pseudo magnetic field originating from the polaritonic analog of spin-orbit coupling (TE$-$TM splitting) on a polariton condensate in a ring-shaped microcavity. The effect gives rise to a stable four-leaf pattern around the ring as seen from the linear polarization measurements of the condensate photoluminescence. This pattern is found to originate from the interplay of the cavity potential, energy relaxation, and TE-TM splitting in the ring. Our observations are compared to the dissipative one-dimensional spinor Gross-Pitaevskii equation with the TE-TM splitting energy which shows good qualitative agreement.

cond-mat.quant-gas↗

arXiv2020

Observation of Spontaneous Ferromagnetism in a Two-Dimensional Electron System

What are the ground states of an interacting, low-density electron system? In the absence of disorder, it has long been expected that as the electron density is lowered, the exchange energy gained by aligning the electron spins should exceed the enhancement in the kinetic (Fermi) energy, leading to a (Bloch) ferromagnetic transition. At even lower densities, another transition to a (Wigner) solid, an ordered array of electrons, should occur. Experimental access to these regimes, however, has been limited because of the absence of a material platform that supports an electron system with very high-quality (low disorder) and low density simultaneously. Here we explore the ground states of interacting electrons in an exceptionally-clean, two-dimensional electron system confined to a modulation-doped AlAs quantum well. The large electron effective mass in this system allows us to reach very large values of the interaction parameter $r_s$, defined as the ratio of the Coulomb to Fermi energies. As we lower the electron density via gate bias, we find a sequence of phases, qualitatively consistent with the above scenario: a paramagnetic phase at large densities, a spontaneous transition to a ferromagnetic state when $r_s$ surpasses 35, and then a phase with strongly non-linear current-voltage characteristics, suggestive of a pinned Wigner solid, when $r_s$ exceeds $\simeq 38$. However, our sample makes a transition to an insulating state at $r_s\simeq 27$, preceding the onset of the spontaneous ferromagnetism, implying that, besides interaction, the role of disorder must also be taken into account in understanding the different phases of a realistic dilute electron system.

cond-mat.str-el↗