arXiv subjects

L. Schultz

Publications and source records attributed to L. Schultz.

50 records · Page 3Linked to original sources

arXiv2005

Weak inter-band coupling in Mg$^{10}$B$_{2}$: a specific heat analysis

The superconducting state of Mg$^{10}$B$_{2}$ is investigated by specific heat measurements in detail. The specific heat in the normal state is analyzed using a recently developed computer code. This allows for an extraction of the electronic specific heat in the superconducting state with high accuracy and a fair determination of the main lattice features. One of the two investigated samples shows a hump in the specific heat at low temperatures within the superconducting state, accompanied by an unusual low value of the small gap, $Δ_π(0)=1.32 meV$, pointing to a very weak inter-band coupling. This sample allows for a detailed analysis of the contribution from the $π$-band to the electronic specific heat in the superconducting state. Therefore the usual analysis method is modified, to include the individual conservation of entropy of both bands. From analyzing the deviation function $D(t)$ of MgB$_{2}$, the theoretically predicted weak inter-band coupling scenario is confirmed.

cond-mat.supr-con↗

arXiv2005

The role of carbon for superconductivity in MgC$_{x}$Ni$_{3}$ from specific heat

The influence of carbon deficiency on superconductivity of MgCNi$_{3}$ is investigated by specific heat measurements in the normal and superconducting state. In order to perform a detailed analysis of the normal state specific heat, a computer code is developed which allows for an instantaneous estimate of the main features of the lattice dynamics. By analyzing the evolution of the lattice vibrations within the series and simultaneously considering the visible mass enhancement, the loss in the electron-phonon coupling can be attributed to significant changes of the prominent Ni vibrations. The present data well supports the recently established picture of strong electron-phonon coupling and ferromagnetic spin fluctuations in this compound.

cond-mat.supr-con↗

arXiv2005

Magnetic-field induced band-structure change in CeBiPt

We report on a field-induced change of the electronic band structure of CeBiPt as evidenced by electrical-transport measurements in pulsed magnetic fields. Above ~25 T, the charge-carrier concentration increases nearly 30% with a concomitant disappearance of the Shubnikov-de Haas signal. These features are intimately related to the Ce 4f electrons since for the non-4f compound LaBiPt the Fermi surface remains unaffected. Electronic band-structure calculations point to a 4f-polarization-induced change of the Fermi-surface topology.

cond-mat.str-el↗

arXiv2004

Evidence for strong electron-phonon coupling in MgCNi_3

The title compound is investigated by specific heat measurements in the normal and superconducting state supplemented by upper critical field transport, susceptibility and magnetization measurements. From a detailed analysis including also full potential electronic structure calculations for the Fermi surface sheets, Fermi velocities and partial densities of states the presence of both strong electron-phonon interactions and considerable pair-breaking has been revealed. The specific heat and the upper critical field data can be described to first approximation by an effective single band model close to the clean limit derived from a strongly coupled predominant hole subsystem with small Fermi velocities. However, in order to account also for Hall-conductivity and thermopower data in the literature, an effective general two-band model is proposed. This two-band model provides a flexible enough frame to describe consistently all available data within a scenario of phonon mediated s-wave superconductivity somewhat suppressed by sizeable electron-paramagnon or electron-electron Coulomb interaction. For quantitative details the relevance of soft phonons and of a van Hove type singularity in the electronic density of states near the Fermi energy is suggested.

cond-mat.supr-con↗

arXiv2002

Observation of minority spin character of the new electron doped manganite La_0.7Ce_0.3MnO_3 from tunneling magnetoresistance

We report the magnetotransport characteristics of a trilayer ferromagnetic tunnel junction build of an electron doped manganite (La_0.7Ce_0.3MnO_3) and a hole doped manganite (La_0.7Ca_0.3MnO_3). At low temperatures the junction exhibits a large positive tunneling magnetoresistance (TMR), irrespective of the bias voltage. At intermediate temperatures below T_C the sign of the TMR is dependent on the bias voltage across the junction. The magnetoresistive characteristics of the junction strongly suggest that La_0.7Ce_0.3MnO_3 is a minority spin carrier ferromagnet with a high degree of spin polarization, i.e. a transport half metal.

cond-mat.str-el↗

arXiv2002

MgCNi3 : Complex behavior in a strongly coupled superconductor

Polycrystalline samples of the recently discovered MgCNi3 superconductor were investigated by transport, ac susceptibility, dc magnetization and specific heat measurements in magnetic fields up to 16 T. Consistent results were obtained for the temperature dependence of the upper critical field H_c2(T) from resistance, ac susceptibility and specific heat measurements. A WHH like temperature dependence of H_c2(T) and the quadratic relationship H_c2(0) ~ T_c^2 point to an effective predominant single band behavior near the quasi clean limit. Evidence for strong electron-phonon and electron-paramagnon coupling was found analyzing the specific heat data. The corresponding s- and p-wave scenarios are briefly discussed using calculated densities of states of different Fermi surface sheets.

cond-mat.supr-con↗

arXiv2002

Comparative Study of Dense Bulk MgB$_2$ Materials Prepared by Different Methods

We report on the results of a comparative investigation of highly dense bulk MgB$_2$ samples prepared by three methods: (i) hot deformation; (ii) high pressure sintering; and (iii) mechanical alloying of Mg and B powders with subsequent hot compaction. All types of samples were studied by ac-susceptibility, dc-magnetization and resistivity measurements in magnetic fields up to $μ_0H=160$ kOe. A small but distinct anisotropy of the upper critical field $H_{c2}^{a,b}/H_{c2}^{c}\sim1.2$ connected with some texture of MgB$_2$ grains was found for the hot deformed samples. The samples prepared by high pressure sintering as well as by mechanical alloying show improved superconducting properties, including high upper critical fields $H_{c2}$ ($μ_0H_{c2}(0)\sim23$ T), irreversibility fields $H_{irr}$ which are strongly shifted towards higher values $H_{irr}(T)\sim0.8H_{c2}(T)$ and high critical current $J_c$ ($J_c=10^5$ A/cm$^2$ at 20 K and 1 T).

cond-mat.supr-con↗

arXiv2001

Improved superconducting properties in nanocrystalline bulk MgB_2

Highly dense nanocrystalline MgB_2 bulk superconductors with distinctly improved pinning were prepared by mechanical alloying of Mg and B powders and hot compaction at ambient temperatures. The nanocrystalline samples reveal high critical current densities of 105 A/cm2 at 20 K and 1 T together with a strongly shifted irreversibility line towards higher fields resulting in H_irr(T) ~ 0.8 H_c2(T), whereas typically H_irr(T) ~ 0.5 H_c2(T) is observed for bulk untextured samples. These values exceed that of all other so far reported bulk samples and are in the range of the values of thin films. The improved pinning of this material which mainly consists of spherical grains of about 40-100 nm in size is attributed to the large number of grain boundaries.

cond-mat.supr-con↗

arXiv2001

A 'p-n' diode with hole and electron-doped lanthanum manganite

The hole-doped manganite La0.7Ca0.3MnO3 and the electron-doped manganite La0.7Ce0.3MnO3 undergo an insulator to metal transition at around 250 K, above which both behave as a polaronic semiconductor. We have successfully fabricated an epitaxial trilayer (La0.7Ca0.3MnO3/SrTiO3/La0.7Ce0.3MnO3), where SrTiO3 is an insulator. At room temperature, i.e. in the semiconducting regime, it exhibits asymmetric current-voltage (I-V) characteristics akin to a p-n diode. The observed asymmetry in the I-V characteristics disappears at low temperatures where both the manganite layers are metallic. To the best of our knowledge, this is the first report of such a p-n diode, using the polaronic semiconducting regime of doped manganites.

cond-mat.str-el↗

arXiv2001

Fully dense MgB_2 superconductor textured by hot deformation

Bulk textured MgB_2 material of nearly full density showing a weak c-axis alignment of the hexagonal MgB_2 grains parallel to the pressure direction was obtained by hot deformation of a stoichiometric MgB_2 pellet prepared by a gas-solid reaction. The texture of the material was verified by comparing the x-ray diffraction patterns of the hot deformed material with isotropic MgB_2 powder. A small, but distinct anisotropy of the upper critical field up to Hc2^{a,b}/Hc2^{c}~1.2 depending on degree of texture was found by resistance and susceptibility measurements. No anisotropy of the critical current density determined from magnetization measurements was found for the textured material.

cond-mat.supr-con↗

arXiv2001

Superconducting Bulk Magnets: Very High Trapped Fields and Cracking

Improved trapped fields are reported for bulk melt-textured YBa2Cu3O7-x (YBCO) material in the temperature range between 20 K and 50 K. Trapped fields up to 12.2 T were obtained at 22 K on the surface of single YBCO disks (with Ag and Zn additions). In YBCO mini-magnets, maximum trapped fields of 16 T (at 24 K) and of 11.2 T (at 47 K) were achieved using (Zn + Ag) and Zn additions, respectively. In all cases, the YBCO disks were encapsulated in steel tubes in order to reinforce the material against the large tensile stress acting during the magnetizing process and to avoid cracking. We observed cracking not only during the magnetizing process, but also as a consequence of flux jumps due to thermomagnetic instabilities in the temperature range betweeen 20 K and 30 K.

cond-mat.supr-con↗

arXiv2001

Upper critical field and irreversibility line in superconducting MgB_2

The upper critical field Hc2(T) of sintered pellets of the recently discovered MgB_2 superconductor was investigated by transport, ac susceptibility and dc magnetization measurements in magnetic fields up to 16 T covering a temperature range between Tc ~ 39 K and T = 3 K ~ 0.1Tc. The temperature dependence of the upper critical field, Hc2(T), shows a positive curvature near Tc similar to that found for the borocarbides YNi_2B_2C and LuNi_2B_2C indicating that MgB_2 is in the clean limit. The irreversibility line was consistently determined from dc magnetization measurements and from the imaginary component of ac susceptibility. The irreversibility field was found to increase up to 8.5 T at 10 K.

cond-mat.supr-con↗

arXiv2000

Current-induced conductance switching in epitaxial La0.7Sr0.3MnO3/SrTiO3 multilayers

We report on the non-linear in-plane electrical transport in coherently grown [La0.7Sr0.3MnO3/SrTiO3] multilayers with ultrathin (< 3 nm) single layers. Current-induced switching of the conductance, with low conductance at larger currents, is demonstrated. The conductance switching is modified under a magnetic field, resulting in an extremely large magnetoresistance of negative, or in a special case even positive, sign. Our results suggest a percolative nature of transport where a large local current density gives rise to a spin-polarizing and a thermal effect of current.

cond-mat.str-el↗

arXiv1997

Evidence for Kondo Effect in Au80Co20 Ribbons

A minimum in resistivity as a function of temperature for an as-quenched Au80Co20 ribbon prepared by melt-spinning using a wheel surface speed of 20 m s^{-1} is found at 25 K. No resistivity minimum is found for an as-quenched ribbon using a wheel surface speed of 60 m s^{-1}, however, upon heat treatment of this ribbon a resistivity minimum is recovered. The temperature of the minimum decreases with increasing total time of heat treatment. These observations are interpretted as evidence for the microstructural control of the Kondo effect typically found in dilute magnetic alloys in a giant magnetoresistance granular material.

cond-mat.mtrl-sci↗