arXiv subjects

Laurens W. Molenkamp

Publications and source records attributed to Laurens W. Molenkamp.

At least 19 recordsLinked to original sources

arXiv2026

Imaging short- and long-range magnetic order in a quantum anomalous Hall insulator

The quantum anomalous Hall effect has been observed in several magnetically doped topological insulators, where its robustness and macroscopic magnetization properties have been taken to suggest the presence of long-range ferromagnetic order. However, experiments in such systems have found evidence for both long- and short-range order, leaving the precise nature of the magnetism in these systems unclear. Here, we use scanning superconducting quantum interference device microscopy to study magnetic domains in V-doped (Bi,Sb)$_2$Te$_3$ exhibiting a quantum anomalous Hall effect with precise quantization. By imaging stray magnetic fields as a function of applied field, we map the formation and evolution of domains through magnetic reversal. We reconstruct the magnetization configuration underlying the measured stray field and find that magnetic domains and crystallographic grains are of similar size. Moreover, magnetic reversal is found to occur through domain expansion, typical of ferromagnets, rather than through nucleation at random sites. Our measurements thus reveal a coexistence of both local magnetic interactions within crystallographic grains and long-range ferromagnetic coupling between grains. This behavior in V-doped (Bi,Sb)$_2$Te$_3$ is markedly distinct from that previously reported for Cr-doped (Bi,Sb)$_2$Te$_3$.

cond-mat.mtrl-sci↗

arXiv2026

Interfering trajectories in a ballistic Andreev cavity

The conventional description of transport through the interface between a normal conductor and a superconductor reduces the system to a one-dimensional problem treating Andreev reflection based on a zero-dimensional Sharvin type point-contact model, and effectively neglects all considerations of device geometry. While this has been successful in systems where conductance in the normal material is in the diffusive transport regime, such an over-simplification of the problem fails in other transport regimes. In particular, when transport is ballistic as in a typical semiconductor-superconductor hybrid structure, geometrical effects are inherently important, and a proper description must consider a one-dimension contact injecting into a two-dimensional ballistic cavity. We present the first study of this regime and explore the bias-voltage dependence of Andreev transport in a cavity-type device comprised of a high mobility HgTe quantum well side-contacted by one superconducting and one normal contact, each creating a one-dimensional interface. The enhanced conductance from Andreev transport features two finite bias conductance peaks, observed at energies within the energy gap of the superconductor. Interestingly, these two peaks respond differently to the application of a perpendicular-to-plane magnetic field. Using a semi-classical model for the quantum transport within the cavity, we are able to attribute each peak to a different class of ballistic trajectories. One class is dominated by normal reflection, and its interference condition is independent of magnetic field, whereas the other one contains retro-reflected Andreev processes at the superconductor interface. These create closed trajectories that are strongly suppressed by magnetic field due to Aharonov-Bohm and Doppler shift effects.

cond-mat.mes-hall↗

arXiv2026

Limits of Thermal Conductance Quantization in Chiral Topological Josephson Junctions

We investigate thermal and non-local electrical transport in four-terminal Josephson junctions formed by a normal region coupled to two transverse chiral superconducting leads, supporting phases characterized by Chern numbers ${\cal C}=0,\,1$\,and\,2. We identify the conditions under which a single chiral Majorana mode (${\cal C}=1$) produces a robust half-quantized thermal conductance, while non-local electrical conductance remains strongly suppressed by particle-hole symmetry. Thermal conductance quantization occurs near a superconducting phase difference $π$, but only in the low-doping regime of the central region and in the intermediate- to long-junction limits. At finite Zeeman fields, the thermal response broadly follows the topology of the isolated superconducting leads for the $C=1$ phase while, in the ${\cal C}=2$ phase, the thermal conductance generally deviates from quantization, depending on the momentum-space location of the Majorana modes. Our results establish clear criteria for probing chiral Majorana modes in Josephson junctions and highlight the essential role of momentum-space structure, finite-size geometry, and sample parameters in thermal transport.

cond-mat.supr-con↗

arXiv2025

Self-Consistent Model for Gate Control of Narrow-, Broken-, and Inverted-Gap (Topological) Heterostructures

Even small electrostatic potentials can dramatically influence the band structure of narrow-, broken-, and inverted-gap materials. A quantitative understanding often necessitates a self-consistent Hartree approach. The valence and conduction band states strongly hybridize and/or cross in these systems. This makes distinguishing between electrons and holes impossible and the assumption of a flat charge carrier distribution at the charge neutrality point hard to justify. Consequently the wide-gap approach often fails in these systems. An alternative is the full-band envelope-function approach by Andlauer and Vogl, which has been implemented into the open-source software package kdotpy (arXiv:2407.12651). We show that this approach and implementation gives numerically stable and quantitatively accurate results where the conventional method fails by modeling the experimental subband density evolution with top-gate voltage in thick (26 nm - 110 nm), topologically inverted HgTe quantum wells. We expect our openly-available implementation to greatly benefit the investigation of narrow-, broken-, and inverted-gap materials.

cond-mat.mes-hall↗

arXiv2025

Wiedemann-Franz behavior at the Weyl points in compressively strained HgTe

Weyl semimetals, with their unique electronic band structure, have drawn significant interest for their potential to explore quantum anomalies in condensed matter systems. In this study, we investigate the large positive magneto-thermal conductance associated with the gravitational anomaly -- one of the predicted anomalies -- for a Weyl semimetal based on a compressively strained HgTe layer. We clearly identify the Weyl regime in our device and accurately extract the thermal conductance by performing thermometry measurements at liquid helium temperatures using fully electronic methods. We observe the anticipated increase in thermal conductance, and it perfectly matches the electrical conductance according to the Wiedemann-Franz law. This finding indicates that, despite the unique electronic spectrum of Weyl semimetals, the mechanism governing heat transport in this system is the same as that for electrical transport, with no additional violations of conservation laws.

cond-mat.mes-hall↗

arXiv2025

Femtosecond photocurrents by the Dresselhaus bulk spin-galvanic effect in an inversion-asymmetric ferromagnet

We study ultrafast photocurrents in thin films of a model ferromagnetic metal with broken bulk inversion symmetry, the half-metallic Heusler compound NiMnSb, following excitation with an optical pump pulse with photon energy 1.55 eV. Remarkably, in terms of the direction of the sample magnetization M, all photocurrents are found to be a superposition of a component with Rashba- and Dresselhaus-type symmetry. We explain the Dresselhaus bulk photocurrent as follows: Pump-induced electron heating induces an excess of spin μ_s||M, which transfers spin angular momentum into states with Dresselhaus-type spin-momentum locking. The resulting charge current relaxes on a time scale of 10 fs by momentum relaxation and, thus, follows μ_s quasi-instantaneously. The relaxation of μ_s is governed by the cooling of the electrons and not by the significantly slower spin-lattice relaxation of half-metals. Our findings add the Dresselhaus spin-galvanic effect (SGE) to the set of ultrafast spin-charge-conversion phenomena. They indicate a route to more efficient spintronic terahertz emitters and detectors based on the volume scaling of the bulk SGE.

cond-mat.mtrl-sci↗

arXiv2024

Phase-dependent supercurrent and microwave dissipation of HgTe quantum well Josephson junctions

We measured the microwave response of a HgTe quantum well Josephson junction embedded into an RF SQUID loop which is inductively coupled to a superconducting resonator. The side-contacted devices studied here operate in bulk transport mode, with a separation between the superconducting contacts smaller than both the estimated carrier mean free path and superconducting coherence length. We extract the current-phase relation and the phase-dependent microwave dissipation, that, at low temperature, primarily is related to photon-induced transitions between the Andreev bound states. We study the effects of gate voltage and temperature on our devices and compare the measurements with a tight-binding model based on the Bogoliubov-de Gennes equations. A combined analysis of both microwave admittance components allows us to confirm the presence of a small gap in the Andreev bound state spectrum at phase $π$, indicating high interface transparency, matching our observations in DC measurements of a similar device. Our work demonstrates the versatility of microwave measurements as a tool for Josephson junction characterization and highlights the importance of the interface properties for side-contacted Josephson devices.

cond-mat.supr-con↗

arXiv2024

Highly efficient broadband THz upconversion with Dirac materials

The use of the THz frequency domain in future network generations offers an unparalleled level of capacity, which can enhance innovative applications in wireless communication, analytics, and imaging. Communication technologies rely on frequency mixing, enabling signals to be converted from one frequency to another and transmitted from a sender to a receiver. Technically, this process is implemented using nonlinear components such as diodes or transistors. However, the highest operation frequency of this approach is limited to sub-THz bands. Here, we demonstrate the upconversion of a weak sub-THz signal from a photoconductive antenna to multiple THz bands. The key element is a high-mobility HgTe-based heterostructure with electronic band inversion, leading to one of the strongest third-order nonlinearities among all materials in the THz range. Due to the Dirac character of electron dispersion, the highly intense sub-THz radiation is efficiently mixed with the antenna signal, resulting in a THz response at linear combinations of their frequencies. The field conversion efficiency above 2$\%$ is provided by a bare tensile-strained HgTe layer with a thickness below 100 nm at room temperature under ambient conditions. Devices based on Dirac materials allow for high degree of integration, with field-enhancing metamaterial structures, making them very promising for THz communication with unprecedented data transfer rate.

physics.optics↗

arXiv2024

Majorana-mediated thermoelectric transport in multiterminal junctions

The unambiguous identification of Majorana zero modes (MZMs) is one of the most outstanding problems of condensed matter physics. Thermal transport provides a detection tool that is sensitive to these chargeless quasiparticles. We study thermoelectric transport between metallic leads transverse to a Josephson junction. The central double quantum dot hosts conventional or topological Andreev states that depend on the phase difference $ϕ$. We show that the presence of MZMs can be identified by a significant amplification of both the electrical and thermal conductance at $ϕ\approx π$ as well as the Seebeck coefficient at $ϕ\approx 0$. In addition, we show that the Wiedemann-Franz law is strongly violated in the presence of MZMs around $ϕ\approx π$ when compared to the conventional case. We further investigate the robustness of our results against Cooper pair splitting processes.

cond-mat.mes-hall↗

arXiv2024

Period-doubling in the phase dynamics of a shunted HgTe quantum well Josephson junction

The fractional AC Josephson effect is a discerning property of topological superconductivity in hybrid Josephson junctions. Recent experimental observations of missing odd Shapiro steps and half Josephson frequency emission in various materials have sparked significant debate regarding their potential origin in the effect. In this study, we present microwave emission measurements on a resistively shunted Josephson junction based on a HgTe quantum well. We demonstrate that, with significant spurious inductance in the shunt wiring, the experiment operates in a nonlinear dynamic regime characterized by period-doubling. This leads to additional microwave emission peaks at half of the Josephson frequency, $f_J/2$, which can mimic the $4π$-periodicity of topological Andreev states. The observed current-voltage characteristics and emission spectra are well-described by a simple RCLSJ model. Furthermore, we show that the nonlinear dynamics of the junction can be controlled using gate voltage, magnetic field, and temperature, with our model accurately reproducing these effects without incorporating any topological attributes. Our observations urge caution in interpreting emission at $f_J/2$ as evidence for gapless Andreev bound states in topological junctions and suggest the appropriate parameter range for future experiments.

cond-mat.mes-hall↗

arXiv2024

kdotpy: $\mathbf{k}\cdot\mathbf{p}$ theory on a lattice for simulating semiconductor band structures

The software project kdotpy provides a Python application for simulating electronic band structures of semiconductor devices with $\mathbf{k}\cdot\mathbf{p}$ theory on a lattice. The application implements the widely used Kane model, capable of reliable predictions of transport and optical properties for a large variety of topological and non-topological materials with a zincblende crystal structure. The application automates the tedious steps of simulating band structures. The user inputs the relevant physical parameters on the command line, for example materials and dimensions of the device, magnetic field, and temperature. The program constructs the appropriate matrix Hamiltonian on a discretized lattice of spatial coordinates and diagonalizes it. The physical observables are extracted from the eigenvalues and eigenvectors and saved as output. The program is highly customizable with a large set of configuration options and material parameters.

cond-mat.mes-hall↗

arXiv2024

Overlapping Top Gate Electrodes based on Low Temperature Atomic Layer Deposition for Nanoscale Ambipolar Lateral Junctions

We present overlapping top gate electrodes for the formation of gate defined lateral junctions in semiconducting layers as an alternative to the back gate/top gate combination and to the split gate configuration. The optical lithography microfabrication of the overlapping top gates is based on multiple layers of low-temperature atomic layer deposited hafnium oxide, which acts as a gate dielectric and as a robust insulating layer between two overlapping gate electrodes exhibiting a large dielectric breakdown field of > 1E9 V/m. The advantage of overlapping gates over the split gate approach is confirmed in model calculations of the electrostatics of the gate stack. The overlapping gate process is applied to Hall bar devices of mercury telluride in order to study the interaction of different quantum Hall states in the nn', np, pn and pp' regime.

cond-mat.mes-hall↗

arXiv2024

Spectral asymmetry induces a re-entrant quantum Hall effect in a topological insulator

The band inversion of topological materials in three spatial dimensions is intimately connected to the parity anomaly of two-dimensional massless Dirac fermions. At finite magnetic fields, the parity anomaly reveals itself as a non-zero spectral asymmetry, i.e., a non-zero difference between the number of conduction and valence band Landau levels, due to the unpaired zero Landau level. Here, we realize this two-dimensional Dirac physics at a single surface of the three-dimensional topological insulator (Hg,Mn)Te. We observe an unconventional re-entrant quantum Hall effect that can be directly related to the occurrence of spectral asymmetry in a single topological surface state. The effect should be observable in any topological insulator where the transport is dominated by a single Dirac surface state.

cond-mat.mes-hall↗

arXiv2024

Balanced Quantum Hall Resistor

The quantum anomalous Hall effect in magnetic topological insulators has been recognized as a promising platform for applications in quantum metrology. The primary reason for this is the electronic conductance quantization at zero external magnetic field, which allows to combine it with the quantum standard of voltage. Here we demonstrate a measurement scheme that increases the robustness of the zero magnetic field quantum anomalous Hall resistor, allowing for higher operational currents. This is achieved by simultaneous current injection into the two disconnected perimeters of a multi-terminal Corbino device to balance the electrochemical potential between the edges, screening the electric field that drives back-scattering through the bulk, and thus improving the stability of the quantization at increased currents. This approach is not only applicable to devices based on the quantum anomalous Hall effect, but more generally can also be applied to existing quantum resistance standards that rely on the integer quantum Hall effect.

cond-mat.mes-hall↗

arXiv2023

Nonlinear planar magnetotransport due to tilted Dirac cones in topological materials

Nonlinear planar magnetotransport is ubiquitous in topological HgTe structures, both in tensile (topological insulator) or compressively strained layers (Weyl semimetal phase). We show that the common reason for the nonlinear planar magnetotransport is the presence of tilted Dirac cones combined with the formation of charge puddles. The origin of the tilted Dirac cones is the mix of the Zeeman term due to the in-plane magnetic field and quadratic contributions to the dispersion relation. We develop a network model that mimics transport of tilted Dirac fermions in the landscape of charge puddles. The model captures the essential features of the experimental data. It should be relevant for nonlinear planar magnetotransport in a variety of topological and small band gap materials.

cond-mat.mes-hall↗

arXiv2023

Velocity and confinement of edge plasmons in HgTe-based 2D topological insulators

High-frequency transport in the edge states of the quantum spin Hall (QSH) effect has to date rarely been explored, though it could cast light on the scattering mechanisms taking place therein. We here report on the measurement of the plasmon velocity in topological HgTe quantum wells both in the QSH and quantum Hall (QH) regimes, using harmonic GHz excitations and phase-resolved detection. We observe low plasmon velocities corresponding to large transverse widths, which we ascribe to the prominent influence of charge puddles forming in the vicinity of edge channels. Together with other recent works, it suggests that puddles play an essential role in the edge state physics and probably constitute a main hurdle on the way to clean and robust edge transport.

cond-mat.mes-hall↗

arXiv2022

Topological band inversion in HgTe(001): surface and bulk signatures from photoemission

HgTe is a versatile topological material and has enabled the realization of a variety of topological states, including two- and three-dimensional (3D) topological insulators and topological semimetals. Nevertheless, a quantitative understanding of its electronic structure remains challenging, in particular due to coupling of the Te 5p-derived valence electrons to Hg 5d core states at shallow binding energy. We present a joint experimental and theoretical study of the electronic structure in strained HgTe(001) films in the 3D topological-insulator regime, based on angle-resolved photoelectron spectroscopy and density functional theory. The results establish detailed agreement in terms of (i) electronic band dispersions and orbital symmetries, (ii) surface and bulk contributions to the electronic structure, and (iii) the importance of Hg 5d states in the valence-band formation. Supported by theory, our experiments directly image the paradigmatic band inversion in HgTe, underlying its non-trivial band topology.

cond-mat.mtrl-sci↗

arXiv2022

The topological Faraday effect cannot be observed in a realistic sample

A striking feature of 3 dimensional (3D) topological insulators (TIs) is the theoretically expected topological magneto-electric (TME) effect, which gives rise to additional terms in Maxwell's laws of electromagnetism with an universal quantized coefficient proportional to half-integer multiples of the fine structure constant $α$. In an ideal scenario one therefore expects also quantized contributions in the magneto-optical response of TIs. We review this premise by taking into account the trivial dielectric background of the TI bulk and potential host substrates, and the often present contribution of itinerant bulk carriers. We show that (i) one obtains a non-universal magneto-optical response whenever there is impedance mismatch between different layers and (ii) that the detectable signals due to the TME rapidly approach vanishingly small values as the impedance mismatch is detuned from zero. We demonstrate that it is methodologically impossible to deduce the existence of a TME exclusively from an optical experiment in the thin film limit of 3D TIs at high magnetic fields.

cond-mat.mes-hall↗