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Liantuan Xiao

Publications and source records attributed to Liantuan Xiao.

At least 73 records · Page 4Linked to original sources

Observation of interaction-induced mobility edge in a disordered atomic wire

Mobility edge, a critical energy separating localized and extended excitations, is a key concept for understanding quantum localization. Aubry-André (AA) model, a paradigm for exploring quantum localization, does not naturally allow mobility edges due to self-duality. Using the momentum-state lattice of quantum gas of Cs atoms to synthesize a nonlinear AA model, we provide experimental evidence for mobility edge induced by interactions. By identifying the extended-to-localized transition of different energy eigenstates, we construct a mobility-edge phase diagram. The location of mobility edge in the low- or high-energy region is tunable via repulsive or attractive interactions. Our observation is in good agreement with the theory, and supports an interpretation of such interaction-induced mobility edge via a generalized AA model. Our work also offers new possibilities to engineer quantum transport and phase transitions in disordered systems.

quant-ph↗

Anti-chiral edge states and hinge states based on the Haldane model

Different from the chiral edge states, antichiral edge states propagating in the same direction on the opposite edges are theoretically proposed based on the modified Haldane model, which is recently experimentally realized in photonic crystal and electric lattice systems. Here, we instead present that the antichiral edge states in the two-dimensional system can also be achieved based on the original Haldane model by combining two subsystems with the opposite chirality. Most importantly, by stacking these two-dimensional systems into three-dimension, it is found that the copropagating antichiral hinge states localized on the two opposite diagonal hinge cases of the system can be implemented. Interestingly, the location of antichiral hinge states can be tuned via hopping parameters along the third dimension. By investigating the local Chern number/layer Chern number and transmission against random disorders, we confirm that the proposed antichiral edge states and hinge states are topologically protected and robust against disorders. Our proposed model systems are expected to be realized in photonic crystal and electric lattice systems.

cond-mat.mes-hall↗

Quantum compressed sensing of ultra-wideband radio-frequency signal

Real-time sensing of ultra-wideband radio-frequency signal with high frequency resolution is challenging, which is confined by the sampling rate of electronic analog-to-digital converter and the capability of digital signal processing. By combining quantum mechanics with compressed sensing, quantum compressed sensing is proposed for wideband radio-frequency signal frequency measurement. By using an electro-optical crystal as a sensor which modulates the wave function of the coherent photons with the signal to be measured. The frequency spectrum could be recovered by detecting the modulated sparse photons with a low time-jitter single-photon detector and a time-to-digital converter. More than 50 GHz real-time analysis bandwidth is demonstrated with the Fourier transform limit resolution. The further simulation shows it can be extended to more than 300 GHz with the present technologies.

quant-ph↗

High bandwidth laser-frequency-locking for wideband noise suppression

Ultra-low frequency noise lasers have been widely used in laser-based experiments. Most narrow-linewidth lasers are implemented by actively suppressing their frequency noise through a frequency noise servo loop (FNSL). The loop bandwidths (LBW) of FNSLs are currently below megahertz, which is gradually tricky to meet application requirements, especially for wideband quantum sensing experiments. This article has experimentally implemented an FNSL with loop-delay-limited 3.5 MHz LBW, which is an order higher than the usual FNSLs. Using this FNSL, we achieved 70 dB laser frequency noise suppression over 100 kHz Fourier frequency range. This technology has broad applications in vast fields where wideband laser frequency noise suppression is inevitable.

physics.optics↗

Super interference fringes of two-photon photoluminescence in individual Au nanoparticles: the critical role of the intermediate state

The interaction between light and metal nanoparticles enables investigations of microscopic phenomena on nanometer length and ultrashort time scales, benefiting from strong confinement and enhancement of the optical field. However, the ultrafast dynamics of these nanoparticles are primarily investigated by multiphoton photoluminescence on picoseconds or photoemission on femtoseconds independently. Here, we presented two-photon photoluminescence (TPPL) measurements on individual Au nanobipyramids (AuNP) to reveal their ultrafast dynamics by two-pulse excitation on a global time scale ranging from sub-femtosecond to tens of picoseconds. Two-orders-of-magnitude photoluminescence enhancement, namely super interference fringes, has been demonstrated on tens of femtoseconds. Power-dependent measurements uncovered the transform of the nonlinearity from 1 to 2 when the interpulse delay varied from tens of femtoseconds to tens of picoseconds. We proved that the real intermediate state plays a critical role in the observed phenomena, supported by numerical simulations with a three eigenstates model and further experiments on Au nanospheres with different diameters. The crucial parameters, including the dephasing time, the radiative rate, and the coupling between different states, have been estimated using numerical simulations. Our results provide insight into the role of intermediate states in the ultrafast dynamics of noble metal nanoparticles. The giant photoluminescence in super interference fringes enables potential practical applications in imaging, sensing, and nanophotonics.

physics.optics↗

Microwave-assisted coherent control of ultracold polar molecules with a ladder-type rotational states

We have demonstrated microwave-assisted coherent control of ultracold $^{85}$Rb$^{133}$Cs molecules with a ladder-type configuration of rotational states. A probe microwave (MW) field is used to couple a lower state $X^1Σ^+(v=0, J=1)$ and a middle state $X^1Σ^+(v=0, J=2)$, while a control MW field couples the middle state and a upper state $X^1Σ^+(v=0, J=3)$. In the presence of the control field, the population of middle rotational states, $X^1Σ^+(v=0, J=2)$, can be reduced by a control MW field. Broadening of spectral splitting and shift of central frequency in this coherent spectrum are observed to be dependent on Rabi frequency of the control MW field. Applying Akaike's information criterion, we conclude that our observed coherent spectra happen through the crossover range of electromagnetically induced transparency and Aulter-Townes splitting as Rabi frequency of control field increases. Our work is a significant development in microwave-assisted quantum control of ultracold polar molecules with multilevel configuration, and also offers a great potential in quantum information based on ultracold molecules.

physics.atom-ph↗

Digital Simulation of Topological Matter on Programmable Quantum Processors

Simulating the topological phases of matter in synthetic quantum simulators is a topic of considerable interest. Given the universality of digital quantum simulators, the prospect of digitally simulating exotic topological phases is greatly enhanced. However, it is still an open question how to realize digital quantum simulation of topological phases of matter. Here, using common single- and two-qubit elementary quantum gates, we propose and demonstrate an approach to design topologically protected quantum circuits on the current generation of noisy quantum processors where spin-orbital coupling and related topological matter can be digitally simulated. In particular, a low-depth topological quantum circuit is performed on both IBM and Rigetti quantum processors. In the experiments, we not only observe but also distinguish the 0 and $π$ energy topological edge states by measuring qubit excitation distribution at the output of the circuits.

quant-ph↗

Investigation on the Cs 6S1=2 to 7D electric quadrupole transition via monochromatic two-photon process at 767 nm

We experimentally demonstrate the cesium electric quadrupole transition from the 6S1/2 ground state to the 7D3/2,5/2 excited state through a virtual level by using a single laser at 767 nm. The excited state energy level population is characterized by varying the laser power, the temperature of the vapor, and the polarization combinations of the laser beams. The optimized experimental parameters are obtained for a high resolution transition interval identification. The magnetic dipole coupling constant A and electric quadrupole coupling constant B for the 7D3/2,5/2 states are precisely determined by using the hyper ne levels intervals. The results, A = 7.39 (0.06) MHz, B = -0.19 (0.18) MHz for the 7D3/2 state, and A = -1.79 (0.05) MHz, B =1.05 (0.29) MHz for the 7D5/2 state, are in good agreement with the previous reported results. This work is beneficial for the determination of atomic structure information and parity non-conservation, which paves the way for the field of precision measurements and atomic physics.

physics.atom-ph↗

Microwave coherent control of ultracold ground-state molecules formed by short-range photoassociation

We report the observation of microwave coherent control of rotational states of ultracold $^{85}$Rb$^{133}$Cs molecules formed in their vibronic ground state by short-range photoassociation. Molecules are formed in the single rotational state $X(v=0,J=1)$ by exciting pairs of atoms to the short-range state $(2)^{3}Π_{0^{-}} (v=11, J=0)$, followed by spontaneous decay. We use depletion spectroscopy to record the dynamic evolution of the population distribution and observe clear Rabi oscillations while irradiating on a microwave transition between coupled neighbouring rotational levels. A density-matrix formalism that accounts for longitudinal and transverse decay times reproduces both the dynamic evolution during the coherent process and the equilibrium population. The coherent control reported here is valuable both for investigating coherent quantum effects and for applications of cold polar molecules produced by continuous short-range photoassociation.

physics.atom-ph↗

All-optical reversible manipulation of exciton and trion emissions in monolayer WS2

Monolayer transition metal dichalcogenides (TMDs) are direct gap semiconductors emerging promising applications in diverse optoelectronic devices. To improve performance, recent investigations have been systematically focused on the tuning of their optical properties. However, an all-optical approach with the reversible feature is still a challenge. Here we demonstrate the tunability of the photoluminescence (PL) properties of monolayer WS2 via laser irradiation. The modulation of PL intensity, as well as the conversion between neutral exciton and charged trion have been readily and reversibly achieved by using different laser power densities. We attribute the reversible manipulation to the laser-assisted adsorption and desorption of gas molecules, which will deplete or release free electrons from the surface of WS2 and thus modify its PL properties. This all-optical manipulation, with advantages of reversibility, quantitative control, and high spatial resolution, suggests promising applications of TMDs monolayers in optoelectronic and nanophotonic applications, such as optical data storage, micropatterning, and display.

cond-mat.mtrl-sci↗

Excitonic Transport and Intervalley Scattering in Exfoliated MoSe2 Monolayer Revealed by Four-Wave-Mixing Transient Grating Spectroscopy

Exciton intervalley scattering, annihilation and relaxation dynamics, and diffusive transport in a monolayer transition metal dichalcogenides are central to the functionality of devices based on them. This motivated us to investigate these properties in exfoliated high-quality monolayer MoSe2 using heterodyned nonlinear four-wave-mixing transient grating spectroscopy. While free exciton excitations are found to be long-lived (~230 ps), an extremely fast intervalley scattering ( less than 120 fs) is observed leading to a negligible valley polarization, consistent with steady state photoluminescence measurements. The exciton population decay shows an appreciable contribution from exciton-exciton annihilation reactions with an annihilation constant of ~ 0.01 cm2s-1, which in addition leads to an extra contribution to the transient grating response. The underlying excitonic dynamics were numerically modeled by including exciton-exciton annihilation, also in the diffusion equation, which allows extraction of the diffusion constant, D ~1.4 cm2s-1. Our results provide a method that allows for the disentanglement of the intricate dynamics involving many-body annihilation processes and a detailed characterization of the excitonic properties of monolayer MoSe2

cond-mat.mes-hall↗

Incoherent phonon population and exciton-exciton annihilation in monolayer WS2 revealed by time-resolved spontaneous Raman scattering

Atomically thin layer transition metal dichalcogenides have been intensively investigated for their rich optical properties and potential applications in nano-electronics. In this work, we study the incoherent optical phonon and exciton population dynamics in monolayer WS2 by time-resolved spontaneous Raman scattering spectroscopy. Upon excitation of the exciton transition, both the Stokes and anti-Stokes optical phonon scattering strength exhibit a large reduction. Based on the detailed balance, the optical phonon population is retrieved, which shows an instant build-up and a relaxation lifetime of around 4 ps at an exciton density E12 cm-2. The corresponding optical phonon temperature rises by 25 K, eventually, after some 10s of picoseconds, leading to a lattice heating by only around 3 K. The exciton relaxation dynamics extracted from the transient vibrational Raman response shows a strong excitation density dependence, signaling an important bi-molecular contribution to the decay. The exciton relaxation rate is found to be (70 ps)-1 and exciton-exciton annihilation rate 0.1 cm2s-1. These results provide valuable insight into the thermal dynamics after optical excitation and enhance the understanding of the fundamental exciton dynamics in two-dimensional transition metal materials.

cond-mat.mtrl-sci↗

Topological magnon insulator and quantized pumps from strongly-interacting bosons in optical superlattices

We propose a scheme realizing topological insulators and quantized pumps for magnon excitations, based on strongly-interacting two-component ultracold atoms trapped in optical superlattices. Specifically, we show how to engineer the Su-Schrieffer-Heeger model for magnons using state-independent superlattices, and the Rice-Mele model using state-dependent superlattices. We describe realistic experimental protocols to detect the topological signatures of magnon excitations in these two models. In particular, we show that the non-equilibrium dynamics of a single magnon can be exploited to directly detect topological winding numbers and phase transitions. We also describe how topological (quantized) pumps can be realized with magnons, and study how this phenomenon depends on the initial magnon state preparation. Our study opens a new avenue for exploring magnonic topological phases of matter and their potential applications in the context of topological magnon transport.

cond-mat.quant-gas↗

Quantum superhet based on microwave-dressed Rydberg atoms

The highly sensitive, phase- and frequency-resolved detection of microwave electric fields is of central importance for diverse fields ranging from astronomy, remote sensing, communication and microwave quantum technology. However, present quantum sensing of microwave electric fields primarily relies on atom-based electrometers only enabling amplitude measurement. Moreover, the best sensitivity of atom-based electrometers is limited by photon shot noise to few $μ$Vcm$^{-1}$Hz$^{-1/2}$: While going beyond is in principle possible by using squeezed light or Schrödinger-cat state, the former is very challenging for atomic experiments while the latter is feasible in all but very small atomic systems. Here we report a novel microwave electric field quantum sensor termed as quantum superhet, which, for the first time, enables experimental measurement of phase and frequency, and makes a sensitivity few tens of nVcm$^{-1}$Hz$^{-1/2}$ readily accessible for current experiments. This sensor is based on microwave-dressed Rydberg atoms and tailored optical spectrum, with very favorable scalings on sensitivity gains. We can experimentally achieve a sensitivity of $55$ nVcm$^{-1}$Hz$^{-1/2}$, with the minimum detectable field being three orders of magnitude smaller than existing quantum electrometers. We also measure phase and frequency, being able to reach a frequency accuracy of few tens of $μ$Hz for microwave field of just few tens of nVcm$^{-1}$. Our technique can be also applied to sense electric fields at terahertz or radio frequency. This work is a first step towards realizing the long sought-after electromagnetic-wave quantum sensors with quantum projection noise limited sensitivity, promising broad applications such as in radio telescope, terahertz communication and quantum control.

physics.atom-ph↗

Topological pumping of a single magnon in a one-dimensional spin-dependent optical superlattice

Topological pumping of ultracold atomic gases has recently been demonstrated in two experiments (Nat. Phys. 12, 296; 12, 350 (2016)). Here we study the topological pumping of a single magnon in a dynamically controlled spin-dependent optical superlattice. When the interaction between atoms is strong, this system supports a dynamical version of topological magnon insulator phase. By initially putting a single magnon in the superlattice and slowly varying the dynamical controlled parameter over one period, the shift of the magnon density center is quantized and equal to the topological Chern number. Moreover, we also find that the direction of this quantized shift is entanglement-dependent. Our result provides a route for realizing topological pumping of quasiparticles in strongly correlated ultracold atomic system and for studying the interplay between topological pumping and quantum entanglement.

cond-mat.quant-gas↗

Gate tunable giant anisotropic resistance in ultra-thin GaTe

In crystals, the duplication of atoms often follows different periodicity along different directions. It thus gives rise to the so called anisotropy, which is usually even more pronounced in two dimensional (2D) materials due to the absence of $\textbf{z}$ dimension. Indeed, in the emerging 2D materials, electrical anisotropy has been one of the focuses in recent experimental efforts. However, key understandings of the in-plane anisotropic resistance in low-symmetry 2D materials, as well as demonstrations of model devices taking advantage of it, have proven difficult. Here, we show that, in few-layered semiconducting GaTe, electrical conductivity along $\textbf{x}$ and $\textbf{y}$ directions of the 2D crystal can be gate tuned from a ratio of less than one order to as large as 10$^{3}$. This effect is further demonstrated to yield an anisotropic memory resistor behaviour in ultra-thin GaTe, when equipped with an architecture of van der Waals floating gate. Our findings of gate tunable giant anisotropic resistance (GAR) effect pave the way for potential applications in nano-electronics such as multifunctional directional memories in the 2D limit.

cond-mat.mes-hall↗

Dynamical process of optically trapped singlet ground state $^{85}$Rb$^{133}$Cs molecules produced via short-range photoassociation

We investigate the dynamical process of optically trapped X$^{1}$$Σ$$^{+}$ (v" = 0) state $^{85}$Rb$^{133}$Cs molecules distributing in J" = 1 and J" = 3 rotational states. The considered molecules, formed from short-range photoassociation of mixed cold atoms, are subsequently confined in a crossed optical dipole trap. Based on a phenomenological rate equation, we provide a detailed study of the dynamics of $^{85}$Rb$^{133}$Cs molecules during the loading and holding processes. The inelastic collisions of $^{85}$Rb$^{133}$Cs molecules in the X$^{1}$$Σ$$^{+}$ (v" = 0, J" = 1 and J" = 3) states with ultracold $^{85}$Rb (or $^{133}$Cs) atoms are measured to be 1.0 (2)$\times$10$^{-10}$ cm$^{3}$s$^{-1}$ (1.2 (3)$ \times$ 10$^{-10}$ cm$^{3}$s$^{-1}$). Our work provides a simple and generic procedure for studying the dynamical process of trapped cold molecules in the singlet ground states.

physics.atom-ph↗

Security proof of the two-way quantum secure direct communication with channel loss and noise

Quantum secure direct communication is one of the important mode of quantum communication, which sends secret information through a quantum channel directly without setting up a prior key. Over the past decade, numerous protocols have been proposed, and part of them have been experimentally demonstrated. However, the strict security proof is still in suspense. Two-way protocol is seen as one of the most practical protocol, in this paper, the security of the two-way quantum secure direct communication protocol will be proved against general attacks when the noisy and lossy channel is taken into account. There are two steps included in the proof, firstly, we need to prove that the mutual information between Alice and Bob is larger than the mutual information shared between Alice and the eavesdropper when the error rate in control mode is less than the predetermined threshold. Secondly, once the error rate is lower than the threshold, one can always find out a forward error correction code to guarantee the security of information transmission.

quant-ph↗