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Lingyao Kong

Publications and source records attributed to Lingyao Kong.

At least 19 recordsLinked to original sources

Ferrimagnetic Skyrmions in a Tetragonal Mn1.9Co0.1Sb Single Crystal at Room Temperature

The development of room temperature small-sized ferrimagnetic skyrmion materials is significant for topological spintronic device applications. As a room temperature ferrimagnetic material, the tetragonal Mn1.9Co0.1Sb crystal exhibits multiple phase transitions, including spin reorientation transitions. However, the magnetic spin textures and their evolution mechanisms during magnetic phase transitions in Mn1.9Co0.1Sb crystals remain unexplored. Using Lorentz transmission electron microscopy, we discovered and verified dipolar skyrmion behavior and its magnetic evolution at room temperature. We established a stable phase diagram of magnetic textures as functions of temperature and magnetic field, while also investigating the evolution mechanisms of spin textures across multiple temperature-induced magnetic phase transitions. Through micromagnetic simulations, a ferrimagnetic configuration with in-plane ferromagnetic coupling and interlayer antiferromagnetic arrangement was established, which stands in contrast to synthetic ferrimagnetic/antiferromagnetic systems that exhibit interlayer antiferromagnetic coupling via the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction. We determined that the intrinsic frequency of ferrimagnetic skyrmions can reach the THz regime due to strong interlayer antiparallel exchange interactions. These findings highlight the diversity of room temperature ferrimagnetic skyrmion regulation behaviors in Mn1.9Co0.1Sb and their dynamic evolution characteristics, opening new avenues for developing novel spintronic devices with enhanced functionalities capable of operating under ambient conditions.

cond-mat.mtrl-sci

Current-induced creation and dynamics of embedded magnetic skyrmion bags

Magnetic skyrmion bags-vortex-like structures hosting multiple skyrmions with tunable topological charge (Q)-hold significant promise for next-generation spintronic computing. However, while their creation using magnetic fields has been demonstrated, their direct electrical generation remains an outstanding challenge. Here, we report the direct current-induced formation and manipulation of embedded skyrmion bags in a FeGe nanoplate under zero magnetic field. Using in-situ Lorentz transmission electron microscopy, we capture the transformation of a distorted helical ground state into embedded skyrmion bags with diverse configurations, driven by nanosecond current pulses. Theoretical analysis indicates that this process is driven by the spin-transfer-torque-induced fracture of the helical state. Furthermore, we demonstrate electrically-induced transitions between skyrmion bags of different Q, leading to the stabilization of complex three-dimensional topological structures, including experimental signatures of magnetic monopoles and bobbers. Our work establishes a foundation for all-electrical control of high-Q topological spin textures and topological defects, paving the way for their application in functional spintronic devices.

cond-mat.mes-hall

Deterministic Electrical Control of Single Magnetic Bubbles in Nanostructured Cells

Localized particle-like spin textures have been found to exhibit emergent electromagnetic properties, which hold promise for the development of intriguing spintronic devices. Among these textures, magnetic bubbles represent localized spin configurations that could serve as data bits. However, the precise methods for their electrical manipulation remain uncertain. Here, we demonstrate the deterministic electrical manipulations and detections of single magnetic bubbles in kagome-latticed Fe3Sn2 magnetic nanostructured cells. The current-induced dynamics of magnetic bubbles were explored using nanosecond pulsed currents. We show single pulsed currents with low and high densities can be applied for the creation and deletion of a single bubble, respectively. The mutual writing-deleting operations on single bubbles are attributed to the thermal heating and non-thermal spin-transfer torque effects in combination with micromagnetic simulations. We also realized the in-situ detection of a single bubble using the anisotropic magnetoresistance effect through a standard four-probe method. Our results could propel the development of bubble-based spintronic devices.

cond-mat.mes-hall

Creating and Deleting a Single Dipolar Skyrmion by Surface Spin Twists

We report deterministic operations on single dipolar skyrmions confined in nanostructured cuboids using in-plane currents. We achieve highly reversible writing and deleting of skyrmions in the simple cuboid without any artificial defects or pinning sites. The current-induced creation of skyrmions is well-understood through the spin-transfer torque acting on surface spin twists of the spontaneous 3D ferromagnetic state, caused by the magnetic dipole-dipole interaction of the uniaxial Fe3Sn2 magnet with a low-quality factor. Current-induced deletions of skyrmions result from the combined effects of magnetic hysteresis and Joule thermal heating. Our results are replicated consistently through 3D micromagnetic simulations. Our approach offers a viable method for achieving reliable single-bit operations in skyrmionic devices for applications such as random-access memories.

cond-mat.mes-hall

Skyrmion Sliding Switch in a 90-nm-Wide Nanostructured Chiral Magnet

Magnetic skyrmions, renowned for their fascinating electromagnetic properties, hold potential for next-generation topological spintronic devices. Recent advancements have unveiled a rich tapestry of 3D topological magnetism. Nevertheless, the practical application of 3D topological magnetism in the development of topological spintronic devices remains a challenge. Here, we showcase the experimental utilization of 3D topological magnetism through the exploitation of skyrmion-edge attractive interactions in 90-nm-wide confined chiral FeGe and CoZnMn magnetic nanostructures. These attractive interactions result in two degenerate equilibrium positions, which can be naturally interpreted as binary bits for a skyrmion sliding switch. Our theory and simulation reveal current-driven spiral motions of skyrmions, governed by the anisotropic gradient of the potential landscape. Our experiments validate the theory that predicts a tunable threshold current density via magnetic field and temperature modulation of the energy barrier. Our results offer an approach for implementing universal on-off switch functions in 3D topological spintronic devices.

cond-mat.mes-hall

Current-controlled creations, deletions, and topological transformations of a single magnetic antiskyrmion in nanostructured cells

Topological magnetic solitons have emerged as promising candidates for information carriers in spintronic devices, thanks to their fascinating electromagnetic properties. For fundamental device applications, the ability to electrically manipulate individual solitons is crucial. However, electrical manipulation of single antiskyrmions has been rarely demonstrated. In this work, we present current-controlled manipulations, encompassing the creation, deletion, and topological transformation of a single antiskyrmion within FeNiPdP nanostructured cells at room temperature. This nanostructure is uniquely designed with dimensions of about 400 nm in width and length, enabling the stabilization of a single antiskyrmion. By simply adjusting the density of nanosecond single-pulsed currents, we achieve the reversible creation and deletion of single antiskyrmions. Moreover, we uncover a rich variety of current-controlled topological transformations among individual antiskyrmions, skyrmions, bubbles, and ferromagnetic states. Our experimental findings are corroborated by micromagnetic simulations, highlighting the pivotal role of current-induced combined effects, such as spin transfer torque and Joule heating. Our results hold potential for advancing antiskyrmion-based device applications.

cond-mat.mes-hall

Orientational phase transitions induced by two-patch interactions

For two-patch particles in two dimensions, we find that the coupling of anisotropic patchy interactions and the triangular lattice leads to novel phase behaviors. For asymmetric patch-patch (PP) and nonpatch-nonpatch (NN) interactions, the system has dual orientationally ordered phases of the same symmetry, intermediated by a nematic phase. Both phase transitions from the nematic phase to dual ordered phases are continuous and belong to the same universality class, and they lead to highly nonmonotonic variations of the nematic order parameter. The system becomes disordered at high temperature through another continuous transition. When the PP and NN interactions become symmetric, the system has subextensive ground-state entropy, and with increasing temperature it undergoes two Berezinskii-Kosterlitz-Thouless phase transitions, with a critical phase connecting a nematic phase and a disordered phase. These results open up new opportunities for designing patchy interactions to study orientational phase transitions and critical phenomena.

cond-mat.soft

Stable Neel-Twisted Skyrmion Bags in a van der Waals Magnet Fe3-xGaTe2 at Room Temperature

Magnetic skyrmion bags with diverse topological charges Q, offer prospects for future spintronic devices based on freedom of Q. While their emergence in van der Waals magnets holds the potential in developing Q-based 2D topological spintronics. However, previous room-temperature skyrmion bags necessitate special anisotropy engineering through disorder Fe intercalation, and the stable phase diagram for skyrmion bags across room temperature regions is lacking. Here, we demonstrate the observation and electrical manipulation of room temperature skyrmion bags in Fe3-xGaTe2 without specially designed Fe intercalation. Combining the pulsed currents with the assistance of magnetic fields, skyrmion bags with various topological charges are generated and annihilated. Especially double nested skyrmion bags are also discovered at room temperature. The stable temperature-field diagram of skyrmion bags has been established. We also demonstrate the electrical-controlled topological phase transformations of skyrmion bags. Our results will provide novel insights for the design of 2D skyrmion-based high-performance devices.

cond-mat.mtrl-sci

MicroMagnetic.jl: A Julia package for micromagnetic and atomistic simulations with GPU support

MicroMagnetic.jl is an open-source Julia package for micromagnetic and atomistic simulations. Using the features of the Julia programming language, MicroMagnetic.jl supports CPU and various GPU platforms, including NVIDIA, AMD, Intel, and Apple GPUs. Moreover, MicroMagnetic.jl supports Monte Carlo simulations for atomistic models and implements the Nudged-Elastic-Band method for energy barrier computations. With built-in support for double and single precision modes and a design allowing easy extensibility to add new features, MicroMagnetic.jl provides a versatile toolset for researchers in micromagnetics and atomistic simulations.

cond-mat.mes-hall

Sewing skyrmion and antiskyrmion by quadrupole of Bloch points

We report three-dimensional topological spin configurations including a novel form of skyrmion-antiskyrmion coupling in D2d chiral magnets. The skyrmion-antiskyrmion coupled string, consisting of skyrmions located in the near-surface layers and antiskyrmions in the interior of the nanostructured sample that are sewn together by emergent Bloch points, is a hybrid three-dimensional soliton solution resulting from the application of micromagnetic equations. We further provide experimental evidence of these 3D topological skyrmionic strings in a FeNiPdP chiral magnet with S4 symmetry. Our results demonstrate reversible topological magnetic transformations between skyrmion-antiskyrmion and skyrmion-bubble strings, which are mediated by the creation and annihilation of Bloch points.

cond-mat.mtrl-sci

Current-Controlled Skyrmion Number in Confined Ferromagnetic Nanostripes

Skyrmions are vortex-like localized magnetic structures that possess an integer-valued topological index known as the skyrmion number or topological charge. Skyrmion number determines the topology-related emergent magnetism, which is highly desirable for advanced storage and computing devices. In order to achieve device functions, it is necessary to manipulate the skyrmion number in confined nanostructured geometries using electrical methods. Here, we report the reliable current-controlled operations for manipulating the skyrmion number through reversible topological transformations between skyrmion chains and stripe domains in confined Fe3Sn2 nanostripes. The results of micromagnetic simulations are successful in numerically reproducing our experiments and explaining them through the combined effect of current-induced Joule heating and magnetic hysteresis. These findings hold the potential to advance the development of topological spintronic devices.

cond-mat.mtrl-sci

Skyrmion-Bubble Bundles in an X-type Sr2Co2Fe28O46 Hexaferrite above Room Temperature

Magnetic skyrmions are spin swirls that possess topological nontriviality and are considered particle-like entities. They are distinguished by an integer topological charge Q. The presence of skyrmion bundles provides an opportunity to explore the range of values for Q, which is crucial for the advancement of topological spintronic devices with multi-Q properties. In this study, we present a new material candidate, Sr2Co2Fe28O46 hexaferrite of the X-type, which hosts small dipolar skyrmions at room temperature and above. By exploiting reversed magnetic fields from metastable skyrmion bubbles at zero fields, we can incorporate skyrmion-bubble bundles with different interior skyrmion/bubble numbers, topological charges, and morphologies at room temperature. Our experimental findings are consistently supported by micromagnetic simulations. Our results highlight the versatility of topological spin textures in centrosymmetric uniaxial magnets, thereby paving the way for the development of room-temperature topological spintronic devices with multi-Q characteristics.

cond-mat.mtrl-sci

Observation of Hybrid Magnetic Skyrmion Bubbles in Fe3Sn2 Nanodisks

It is well known that there are two types of magnetic bubbles in uniaxial magnets. Here, using Lorentz-transimission electronic microscopy magnetic imaging, we report the direct experimental observation of 3D type-III hybrid bubbles, which comprise Néel-twisted skyrmion bubbles with topological charge Q = -1 in near-surface layers and type-II bubbles with Q = 0 in interior layers, in Fe3Sn2 nanodisks. Using the tilted magnetic field, we further show the controlled topological magnetic transformations of three types of bubbles in a confined ferromagnetic nanodisk. Our observations are well reproduced using micromagnetic simulations based on measured magnetic parameters. Our results advance fundamental classification and understanding of magnetic bubbles, which could propel the applications of three-dimensional magnetism.

cond-mat.mtrl-sci

Combined Magnetic Imaging and Anisotropic Magnetoresistance Detection of Dipolar Skyrmions

Magnetic skyrmions are localized particle-like nontrivial swirls that are promising in building high-performance topological spintronic devices. The read-out functions in skyrmionic devices require the translation of magnetic skyrmions to electrical signals. Here, we report combined real-space magnetic imaging and anisotropic magnetoresistance studies on dipolar skyrmions. A single skyrmion chain and single skyrmion are observed using Lorentz transmission electron microscopy imaging. Meanwhile, the field, helicity, and skyrmion count dependence of anisotropic magnetoresistance of the Fe3Sn2 nanostructures are obtained simultaneously. Our results demonstrate that the anisotropic magnetoresistance of skyrmions is independent of the helicity and proportional to the skyrmion count. Our work could promote read-out operations in skyrmion-based spintronic devices.

cond-mat.mes-hall

Imaging the ultrafast coherent control of a skyrmion crystal

Exotic magnetic textures emerging from the subtle interplay between thermodynamic and topological fluctuation have attracted intense interest due to their potential applications in spintronic devices. Recent advances in electron microscopy have enabled the imaging of random photo-generated individual skyrmions. However, their deterministic and dynamical manipulation is hampered by the chaotic nature of such fluctuations and the intrinsically irreversible switching between different minima in the magnetic energy landscape. Here, we demonstrate a method to coherently control the rotation of a skyrmion crystal by discrete amounts at speeds which are much faster than previously observed. By employing circularly polarized femtosecond laser pulses with an energy below the bandgap of the Mott insulator Cu2OSeO3, we excite a collective magnon mode via the inverse Faraday effect. This triggers coherent magnetic oscillations that directly control the rotation of a skyrmion crystal imaged by cryo-Lorentz Transmission Electron Microscopy. The manipulation of topological order via ultrafast laser pulses shown here can be used to engineer fast spin-based logical devices.

cond-mat.str-el

Two-dimensional characterization of three-dimensional magnetic bubbles in Fe$_3$Sn$_2$ nanostructures

We report differential phase contrast scanning transmission electron microscopy (TEM) of nanoscale magnetic objects in Kagome ferromagnet Fe$_3$Sn$_2$ nanostructures. This technique can directly detect the deflection angle of a focused electron beam, thus allowing clear identification of the real magnetic structures of two magnetic objects including three-ring and complex arch-shaped vortices in Fe$_3$Sn$_2$ by Lorentz transmission electron microscopy imaging. Numerical calculations based on real material-specific parameters well reproduced the experimental results, showing that the magnetic objects can be attributed to integral magnetizations of two types of complex three-dimensional (3D) magnetic skyrmion bubbles with depth-modulated spin twisting. Magnetic configurations obtained using the high-resolution TEM are generally considered as two-dimensional (2D) magnetic objects previously. Our results imply the importance of the integral magnetizations of underestimated 3D magnetic structures in 2D TEM magnetic characterizations.

cond-mat.mtrl-sci

Magnetic Skyrmion Bundles and Their Current-Driven Dynamics

Quantization of topological charges determines the various topological spin textures that are expected to play a key role in future spintronic devices. While the magnetic skyrmion with a unit topological charge Q has been extensively studied, spin textures with other integer valued have not been verified well so far. Here, we report the real-space image, creation, and manipulation of a type of multi Q three-dimensional skyrmionic texture, where a circular spin spiral ties a bunch of skyrmion tubes. We define these objects as skyrmion bundles, and show they have arbitrarily integer values Q from negative up to at least 55 in our experiment. These textures behave as quasiparticles in dynamics for the collective motions driven by electric pulses. Similar to the skyrmion, skyrmion bundles with non zero Q exhibit the skyrmion Hall effects with a Hall angle of 62 degree. Of particular interest, the skyrmion bundle with Q = 0 propagates collinearly with respect to the current flow without the skyrmion Hall effect. Our results open a new perspective for possible applications of multi Q magnetic objects in future spintronic devices.

cond-mat.mtrl-sci

Giant nonlinear anomalous Hall effect induced by spin-dependent band structure evolution

Anomalous Hall effect (AHE) is the key transport signature unlocking topological properties of magnetic materials. While AHE is usually proportional to the magnetization, the nonlinearity suggests the existence of complex magnetic and electron orders. Nonlinear AHE includes the topological Hall effect (THE) that has been widely used to identify the presence of spin chirality in real space. But it can in principle be induced by band structure evolution via Berry curvatures in the reciprocal space. This effect has been largely overlooked due to the intertwined mechanisms in both real and reciprocal spaces. Here, we observed a giant nonlinear AHE with the resistivity up to 383.5 uohm cm, contributing unprecedentedly 97% of the total Hall response in EuCd2As2. Moreover, it can be further enhanced by tilting the magnetic field 30° away from [001] direction, reaching a large anomalous Hall angle up to 21%. Although it shows exactly the same double-peak feature as THE, our scaling analysis and first-principles calculations reveal that the Berry phase is extremely sensitive to the spin canting, and nonlinear AHE is a consequence of band structure evolution under the external magnetic fields. When the spins gradually tilt from the in-plane antiferromagnetic ground state to out-of-plane direction, band crossing and band inversion occur, introducing a bandgap at Γ point at a canting angle of 45°. That contributes to the enhancement of Berry curvature and consequently a large intrinsic Hall conductivity. Our results unequivocally reveal the sensitive dependence of band structures on spin tilting process under external magnetic fields and its pronounced influence on the transport properties, which also need to be taken into consideration in other magnetic materials.

cond-mat.mtrl-sci