arXiv subjects

Lukas Novotny

Publications and source records attributed to Lukas Novotny.

At least 37 records · Page 2Linked to original sources

arXiv2023

Cavity-mediated long-range interactions in levitated optomechanics

The ability to engineer cavity-mediated interactions has emerged as a powerful tool for the generation of non-local correlations and the investigation of non-equilibrium phenomena in many-body systems. Levitated optomechanical systems have recently entered the multi-particle regime, with promise for using arrays of massive strongly coupled oscillators for exploring complex interacting systems and sensing. Here, by combining advances in multi-particle optical levitation and cavity-based quantum control, we demonstrate, for the first time, programmable cavity-mediated interactions between nanoparticles in vacuum. The interaction is mediated by photons scattered by spatially separated particles in a cavity, resulting in strong coupling ($G_\text{zz}/Ω_\text{z} = 0.238\pm0.005$) that does not decay with distance within the cavity mode volume. We investigate the scaling of the interaction strength with cavity detuning and inter-particle separation, and demonstrate the tunability of interactions between different mechanical modes. Our work paves the way towards exploring many-body effects in nanoparticle arrays with programmable cavity-mediated interactions, generating entanglement of motion, and using interacting particle arrays for optomechanical sensing.

quant-ph↗

arXiv2023

Exciton-assisted electron tunneling in van der Waals heterostructures

The control of elastic and inelastic electron tunneling relies on materials with well defined interfaces. Van der Waals materials made of two-dimensional constituents form an ideal platform for such studies. Signatures of acoustic phonons and defect states have been observed in current-to-voltage ($I-V$) measurements. These features can be explained by direct electron-phonon or electron-defect interactions. Here, we use a novel tunneling process that involves excitons in transition metal dichalcogenides (TMDs). We study tunnel junctions consisting of graphene and gold electrodes separated by hexagonal boron nitride (hBN) with an adjacent TMD monolayer and observe prominent resonant features in $I-V$ measurements. These resonances appear at bias voltages that correspond to TMD exciton energies. By placing the TMD outside of the tunneling pathway, we demonstrate that this phonon-exciton mediated tunneling process does not require any charge injection into the TMD. This work demonstrates the appearance of optical modes in electrical transport measurements and introduces a new functionality for optoelectronic devices based on van der Waals materials.

cond-mat.mes-hall↗

arXiv2023

Overbias photon emission from light-emitting devices based on monolayer transition metal dichalcogenides

Tunneling light-emitting devices (LEDs) based on transition metal dichalcogenides (TMDs) and other 2D materials are a new platform for on-chip optoelectronic integration. Some of the physical processes underlying this LED architecture are not fully understood, especially the emission at photon energies higher than the applied electrostatic potential, so-called overbias emission. Here we report overbias emission for potentials that are near half of the optical bandgap energy in TMD-based tunneling LEDs. We show that this emission is not thermal in nature, but consistent with exciton generation via a two-electron coherent tunneling process.

cond-mat.mes-hall↗

arXiv2023

Full control of the libration potential in rotational levitodynamics

Control of the potential energy and free evolution lie at the heart of levitodynamics as key requirements for sensing, wave function expansion, and mechanical squeezing protocols. Here, we experimentally demonstrate full control over the optical potential governing the librational degrees of freedom of a levitated anisotropic nanoparticle. This control is achieved by introducing the degree of polarization as a new tool for rotational levitodynamics. We demonstrate the free rotation of a levitated anisotropic scatterer around its short axis and and we use the rotational degrees of freedom to probe the local spin of a strongly focused laser beam.

physics.optics↗

arXiv2023

Surface-Sensitive Raman Scattering by Transferable Nanoporous Plasmonic Membranes

Raman spectroscopy is a powerful technique to characterize materials. It probes non-destructively chemical composition, crystallinity, defects, strain and coupling phenomena. However, the Raman response of surfaces or thin films is often weak and obscured by dominant bulk signals. Here we overcome this limitation by placing a transferable porous gold membrane (PAuM) on top of the surface of interest. Slot-like nanopores in the membrane act as plasmonic slot antennas and enhance the Raman response of the surface or thin film underneath. Simultaneously, the PAuM suppresses the penetration of the excitation laser into the bulk, efficiently blocking the bulk Raman signal. Using graphene as a model surface, we show that these two simultaneous effects lead to an increase in the surface-to-bulk Raman signal ratio by three orders of magnitude. We find that 90% of the Raman enhancement occurs within the top 2.5 of the material, demonstrating truly surface-sensitive Raman scattering. To validate our approach, we analyze the surface of a LaNiO3 thin film. We observe a Raman mode splitting for the LaNiO3 surface-layer, which is spectroscopic evidence that the surface structure differs from the bulk. This result underpins that PAuM give direct access to Raman signatures of surfaces and their structural properties.

cond-mat.mtrl-sci↗

arXiv2022

Waveguide-coupled light emitting devices made of 2D materials

Optical information processing using photonic integrated circuits is a key goal in the field of nanophotonics. Extensive research efforts have led to remarkable progress in integrating active and passive device functionalities within one single photonic circuit. Still, to date, one of the central components - i.e. light sources - remain a challenge to be integrated. Here, we demonstrate waveguide-coupled electrically driven light emitters in an on-chip photonics platform based on 2D materials. We combine light-emitting devices (LEDs), based on exciton recombination in transition metal dichalcogenides (TMDs), with hexagonal boron nitride (h-BN) photonic waveguides in a single van der Waals (vdW) heterostructure. Waveguide-coupled light emission is achieved by sandwiching the LED between two h-BN slabs and patterning the complete vdW stack into a photonic structure. Our demonstration of on-chip light generation and waveguiding is a key component for future integrated vdW optoelectronics.

physics.optics↗

arXiv2022

Simultaneous ground-state cooling of two mechanical modes of a levitated nanoparticle

The quantum ground state of a massive mechanical system is a steppingstone for investigating macroscopic quantum states and building high fidelity sensors. With the recent achievement of ground-state cooling of a single motional mode, levitated nanoparticles have entered the quantum domain. To overcome detrimental cross-coupling and decoherence effects, quantum control needs to be expanded to more system dimensions, but the effect of a decoupled dark mode has thus far hindered cavity-based ground state cooling of multiple mechanical modes. Here, we demonstrate two-dimensional (2D) ground-state cooling of an optically levitated nanoparticle. Utilising coherent scattering into an optical cavity mode, we reduce the occupation numbers of two separate centre-of-mass modes to 0.83 and 0.81, respectively. By controlling the frequency separation and the cavity coupling strengths of the nanoparticle's mechanical modes, we show the transition from 1D to 2D ground-state cooling while avoiding the effect of dark modes. Our results lay the foundations for generating quantum-limited high orbital angular momentum states with applications in rotation sensing. The demonstrated 2D control, combined with already shown capabilities of ground-state cooling along the third motional axis, opens the door for full 3D ground-state cooling of a massive object.

quant-ph↗

arXiv2022

Optomechanical sideband asymmetry explained by stochastic electrodynamics

Within the framework of stochastic electrodynamics we derive the noise spectrum of a laser beam reflected from a suspended mirror. The electromagnetic field follows Maxwell's equations and is described by a deterministic part that accounts for the laser field and a stochastic part that accounts for thermal and zero-point background fluctuations.Likewise, the mirror motion satisfies Newton's equation of motion and is composed of deterministic and stochastic parts, similar to a Langevin equation. We consider a photodetector that records the power of the field reflected from the mirror interfering with a frequency-shifted reference beam (heterodyne interferometry). We theoretically show that the power spectral density of the photodetector signal is composed of four parts: (i) a deterministic term with beat notes, (ii) shot noise, (iii) the actual heterodyne signal of the mirror motion and (iv) a cross term resulting from the correlation between measurement noise (shot noise) and backaction noise (radiation pressure shot noise). The latter gives rise to the Raman sideband asymmetry observed with ultracold atoms, cavity optomechanics and with levitated nanoparticles. Our classical theory fully reproduces experimental observations and agrees with the results obtained by a quantum theoretical treatment.

quant-ph↗

arXiv2022

Energy transfer from tunneling electrons to excitons

Excitons in optoelectronic devices have been generated through optical excitation, external carrier injection, or employing pre-existing charges. Here, we reveal a new way to electrically generate excitons in transition metal dichalcogenides (TMDs). The TMD is placed on top of a gold-hBN-graphene tunnel junction, outside of the tunneling pathway. This electrically driven device features a photoemission spectrum with a distinct peak at the exciton energy of the TMD. We interpret this observation as exciton generation by energy transfer from tunneling electrons, which is further supported by a theoretical model based on inelastic electron tunneling. Our findings introduce a new paradigm for exciton creation in van der Waals heterostructures and provide inspiration for a new class of optoelectronic devices in which the optically active material is separated from the electrical pathway.

cond-mat.mes-hall↗

arXiv2022

Molecular encapsulation from the liquid phase and graphene nanoribbon growth in carbon nanotubes

Growing graphene nanoribbons from small organic molecules encapsulated in carbon nanotubes can result in products with uniform width and chirality. We propose a method based on encapsulation of 1,2,4-trichlorobenzene from the liquid phase and subsequent annealing. This procedure results in graphene nanoribbons several tens of nanometers long. The presence of nanoribbons was proven by Raman spectra both on macroscopic samples and on the nanoscale by tip-enhanced Raman scattering and high-resolution transmission electron microscopic images.

cond-mat.mtrl-sci↗

arXiv2022

White-noise fluctuation theorem for Langevin dynamics

Fluctuation theorems based on time-reversal have provided remarkable insight into the non-equilibrium statistics of thermodynamic quantities like heat, work, and entropy production. These types of laws impose constraints on the distributions of certain trajectory functionals that reflect underlying dynamical symmetries. In this work, we introduce a detailed fluctuation theorem for Langevin dynamics that follows from the statistics of Gaussian white noise rather than from time-reversal. The theorem, which originates from a point-wise symmetry in phase space, holds individually for each degree of freedom coupled to additive or multiplicative noise. The relation is independent of the phase space distribution generated by the dynamics and can be used to derive a versatile parameter inference algorithm applicable to the a wide range of systems, including non-conservative and non-Markovian ones.

cond-mat.stat-mech↗

arXiv2022

Encoding information in the mutual coherence of spatially separated light beams

Coherence has been used as a resource for optical communications since its earliest days. It is widely used for multiplexing of data, but not for encoding of data. Here we introduce a coding scheme, which we call \textit{mutual coherence coding}, to encode information in the mutual coherence of spatially separated light beams. We describe its implementation and analyze its performance by deriving the relevant figures of merit (signal-to-noise ratio, maximum bit-rate, and spectral efficiency) with respect to the number of transmitted beams. Mutual coherence coding yields a quadratic scaling of the number of transmitted signals with the number of employed light beams, which might have benefits for cryptography and data security.

physics.optics↗

arXiv2022

Scalable all-optical cold damping of levitated nanoparticles

The field of levitodynamics has made significant progress towards controlling and studying the motion of a levitated nanoparticle. Motional control relies on either autonomous feedback via a cavity or measurement-based feedback via external forces. Recent demonstrations of measurement-based ground-state cooling of a single nanoparticle employ linear velocity feedback, also called cold damping, and require the use of electrostatic forces on charged particles via external electrodes. Here we introduce a novel all-optical cold damping scheme based on spatial modulation of the trap position that is scalable to multiple particles. The scheme relies on using programmable optical tweezers to provide full independent control over trap frequency and position of each tweezer. We show that the technique cools the center-of-mass motion of particles down to $17\,$mK at a pressure of $2 \times 10^{-6}\,$mbar and demonstrate its scalability by simultaneously cooling the motion of two particles. Our work paves the way towards studying quantum interactions between particles, achieving 3D quantum control of particle motion without cavity-based cooling, electrodes or charged particles, and probing multipartite entanglement in levitated optomechanical systems.

physics.optics↗

arXiv2022

Optimal orientation detection of an anisotropic dipolar scatterer

The angular orientation of an anisotropic scatterer with cylindrical symmetry in a linearly polarized light field represents an optomechanical librator. Here, we propose and theoretically analyze an optimal measurement scheme for the two angular degrees of freedom of such a librator. The imprecision-backaction product of this scheme reaches the Heisenberg uncertainty limit. Furthermore, we propose and analyze a realistic measurement scheme and show that, in the absence of spinning motion around the symmetry axis, measurement-based ground-state cooling of the rotational degrees of freedom of an anisotropic point scatterer levitated in an optical trap is feasible.

physics.optics↗

arXiv2022

Ponderomotive squeezing of light by a levitated nanoparticle in free space

A mechanically compliant element can be set into motion by the interaction with light. In turn, this light-driven motion can give rise to ponderomotive correlations in the electromagnetic field. In optomechanical systems, cavities are often employed to enhance these correlations up to the point where they generate quantum squeezing of light. In free-space scenarios, where no cavity is used, observation of squeezing remains possible but challenging due to the weakness of the interaction, and has not been reported so far. Here, we measure the ponderomotively squeezed state of light scattered by a nanoparticle levitated in a free-space optical tweezer. We observe a reduction of the optical fluctuations by up to $25$~\% below the vacuum level, in a bandwidth of about $15$~kHz. Our results are well explained by a linearized dipole interaction between the nanoparticle and the electromagnetic continuum. These ponderomotive correlations open the door to quantum-enhanced sensing and metrology with levitated systems, such as force measurements below the standard quantum limit.

quant-ph↗

arXiv2022

MAQRO -- BPS 2023 Research Campaign Whitepaper

The objective of the proposed MAQRO mission is to harness space for achieving long free-fall times, extreme vacuum, nano-gravity, and cryogenic temperatures to test the foundations of physics in macroscopic quantum experiments. This will result in the development of novel quantum sensors and a means to probe the foundations of quantum physics at the interface with gravity. Earlier studies showed that the proposal is feasible but that several critical challenges remain, and key technologies need to be developed. These new technologies will open up the potential for achieving additional science objectives. The proposed research campaign aims to advance the state of the art and to perform the first macroscopic quantum experiments in space. Experiments on the ground, in micro-gravity, and in space will drive the proposed research campaign during the current decade to enable the implementation of MAQRO within the subsequent decade.

quant-ph↗

arXiv2021

Freestanding and permeable nanoporous gold membranes for surface-enhanced Raman scattering

Surface-enhanced Raman spectroscopy (SERS) demands reliable, high enhancement substrates in order to be used in different fields of application. Here, we introduce freestanding porous gold membranes (PAuM) as easy to produce, scalable, mechanically stable, and effective SERS substrates. We fabricate large-scale sub-30 thick PAuM, that form freestanding membranes with varying morphologies depending on the nominal gold thickness. These PAuM are mechanically stable for pressures up to $>3$ bar, and exhibit surface-enhanced Raman scattering with local enhancement factors of $10^4$ to $10^5$, which we demonstrate by wavelength-dependent and spatially resolved Raman measurements using graphene as a local Raman probe. Numerical simulations reveal that the enhancement arises from individual, nanoscale pores in the membrane acting as optical slot antennas. Our PAuM are mechanically stable, provide robust SERS enhancement for excitation power densities up to $10^6$W$\,$cm$^{-2}$, and may find use as a building block in flow-through sensor applications based on SERS.

physics.optics↗

arXiv2021

Controlling spatial coherence with an optical complex medium

Control over optical spatial coherence is a key requirement in diverse applications including imaging, optical trapping, and communications. Current approaches to controlling spatial coherence are constrained by speed or limited to a single pair of optical fields. Here, we propose a method to achieve single-shot control of the spatial coherence between an arbitrary number of fields. Our method employs a multi-port linear optical device, which we realize by shaping the wavefront of the input light fields and transmitting them through a complex medium. To demonstrate the capabilities of our method, we experimentally realize a 3x3-port system and use it to generate three output beams with desired mutual correlations.

physics.optics↗