arXiv subjects

M. Ansmann

Publications and source records attributed to M. Ansmann.

16 recordsLinked to original sources

arXiv2025

Quantum computation of molecular geometry via many-body nuclear spin echoes

Quantum-information-inspired experiments in nuclear magnetic resonance spectroscopy may yield a pathway towards determining molecular structure and properties that are otherwise challenging to learn. We measure out-of-time-ordered correlators (OTOCs) [1-4] on two organic molecules suspended in a nematic liquid crystal, and investigate the utility of this data in performing structural learning tasks. We use OTOC measurements to augment molecular dynamics models, and to correct for known approximations in the underlying force fields. We demonstrate the utility of OTOCs in these models by estimating the mean ortho-meta H-H distance of toluene and the mean dihedral angle of 3',5'-dimethylbiphenyl, achieving similar accuracy and precision to independent spectroscopic measurements of both quantities. To ameliorate the apparent exponential classical cost of interpreting the above OTOC data, we simulate the molecular OTOCs on a Willow superconducting quantum processor, using AlphaEvolve-optimized [5] quantum circuits and arbitrary-angle fermionic simulation gates. We implement novel zero-noise extrapolation techniques based on the Pauli pathing model of operator dynamics [6], to repeat the learning experiments with root-mean-square error $0.05$ over all circuits used. Our work highlights a computational protocol to interpret many-body echoes from nuclear magnetic systems using low resource quantum computation.

quant-ph↗

arXiv2023

Stable Quantum-Correlated Many Body States through Engineered Dissipation

Engineered dissipative reservoirs have the potential to steer many-body quantum systems toward correlated steady states useful for quantum simulation of high-temperature superconductivity or quantum magnetism. Using up to 49 superconducting qubits, we prepared low-energy states of the transverse-field Ising model through coupling to dissipative auxiliary qubits. In one dimension, we observed long-range quantum correlations and a ground-state fidelity of 0.86 for 18 qubits at the critical point. In two dimensions, we found mutual information that extends beyond nearest neighbors. Lastly, by coupling the system to auxiliaries emulating reservoirs with different chemical potentials, we explored transport in the quantum Heisenberg model. Our results establish engineered dissipation as a scalable alternative to unitary evolution for preparing entangled many-body states on noisy quantum processors.

quant-ph↗

arXiv2023

Phase transition in Random Circuit Sampling

Undesired coupling to the surrounding environment destroys long-range correlations on quantum processors and hinders the coherent evolution in the nominally available computational space. This incoherent noise is an outstanding challenge to fully leverage the computation power of near-term quantum processors. It has been shown that benchmarking Random Circuit Sampling (RCS) with Cross-Entropy Benchmarking (XEB) can provide a reliable estimate of the effective size of the Hilbert space coherently available. The extent to which the presence of noise can trivialize the outputs of a given quantum algorithm, i.e. making it spoofable by a classical computation, is an unanswered question. Here, by implementing an RCS algorithm we demonstrate experimentally that there are two phase transitions observable with XEB, which we explain theoretically with a statistical model. The first is a dynamical transition as a function of the number of cycles and is the continuation of the anti-concentration point in the noiseless case. The second is a quantum phase transition controlled by the error per cycle; to identify it analytically and experimentally, we create a weak link model which allows varying the strength of noise versus coherent evolution. Furthermore, by presenting an RCS experiment with 67 qubits at 32 cycles, we demonstrate that the computational cost of our experiment is beyond the capabilities of existing classical supercomputers, even when accounting for the inevitable presence of noise. Our experimental and theoretical work establishes the existence of transitions to a stable computationally complex phase that is reachable with current quantum processors.

quant-ph↗

arXiv2022

Purification-based quantum error mitigation of pair-correlated electron simulations

An important measure of the development of quantum computing platforms has been the simulation of increasingly complex physical systems. Prior to fault-tolerant quantum computing, robust error mitigation strategies are necessary to continue this growth. Here, we study physical simulation within the seniority-zero electron pairing subspace, which affords both a computational stepping stone to a fully correlated model, and an opportunity to validate recently introduced ``purification-based'' error-mitigation strategies. We compare the performance of error mitigation based on doubling quantum resources in time (echo verification) or in space (virtual distillation), on up to $20$ qubits of a superconducting qubit quantum processor. We observe a reduction of error by one to two orders of magnitude below less sophisticated techniques (e.g. post-selection); the gain from error mitigation is seen to increase with the system size. Employing these error mitigation strategies enables the implementation of the largest variational algorithm for a correlated chemistry system to-date. Extrapolating performance from these results allows us to estimate minimum requirements for a beyond-classical simulation of electronic structure. We find that, despite the impressive gains from purification-based error mitigation, significant hardware improvements will be required for classically intractable variational chemistry simulations.

quant-ph↗

arXiv2010

Demonstration of a Tuneable Coupler for Superconducting Qubits Using Coherent, Time Domain, Two-Qubit Operations

A major challenge in the field of quantum computing is the construction of scalable qubit coupling architectures. Here, we demonstrate a novel tuneable coupling circuit that allows superconducting qubits to be coupled over long distances. We show that the inter-qubit coupling strength can be arbitrarily tuned over nanosecond timescales within a sequence that mimics actual use in an algorithm. The coupler has a measured on/off ratio of 1000. The design is self-contained and physically separate from the qubits, allowing the coupler to be used as a module to connect a variety of elements such as qubits, resonators, amplifiers, and readout circuitry over long distances. Such design flexibility is likely to be essential for a scalable quantum computer.

quant-ph↗

arXiv2009

Decoherence Dynamics of Complex Photon States in a Superconducting Circuit

Quantum states inevitably decay with time into a probabilistic mixture of classical states, due to their interaction with the environment and measurement instrumentation. We present the first measurement of the decoherence dynamics of complex photon states in a condensed-matter system. By controllably preparing a number of distinct, quantum-superposed photon states in a superconducting microwave resonator, we show that the subsequent decay dynamics can be quantitatively described by taking into account only two distinct decay channels, energy relaxation and dephasing. Our ability to prepare specific initial quantum states allows us to measure the evolution of specific elements in the quantum density matrix, in a very detailed manner that can be compared with theory.

cond-mat.mes-hall↗

arXiv2009

Improving the Coherence Time of Superconducting Coplanar Resonators

The quality factor and energy decay time of superconducting resonators have been measured as a function of material, geometry, and magnetic field. Once the dissipation of trapped magnetic vortices is minimized, we identify surface two-level states (TLS) as an important decay mechanism. A wide gap between the center conductor and the ground plane, as well as use of the superconductor Re instead of Al, are shown to decrease loss. We also demonstrate that classical measurements of resonator quality factor at low excitation power are consistent with single-photon decay time measured using qubit-resonator swap experiments.

cond-mat.mes-hall↗

arXiv2009

Energy Decay in Josephson Qubits from Non-equilibrium Quasiparticles

We calculate the energy decay rate of Josephson qubits and superconducting resonators from non-equilibrium quasiparticles. The decay rates from experiments are shown to be consistent with predictions based on a prior measurement of the quasiparticle density n_qp = 10/um^3, which suggests that non-equilibrium quasiparticles are an important decoherence source for Josephson qubits. Calculations of the energy-decay and diffusion of quasiparticles also indicate that prior engineered gap and trap structures, which reduce the density of quasiparticles, should be redesigned to improve their efficacy. This model also explains a striking feature in Josephson qubits and resonators - a small reduction in decay rate with increasing temperature.

cond-mat.mes-hall↗

arXiv2008

Measurement of the decay of Fock states in a superconducting quantum circuit

We demonstrate the controlled generation of Fock states with up to 15 photons in a microwave coplanar waveguide resonator coupled to a superconducting phase qubit. The subsequent decay of the Fock states, due to dissipation, is then monitored by varying the time delay between preparing the state and performing a number-state analysis. We find that the decay dynamics can be described by a master equation where the lifetime of the n-photon Fock state scales as 1/n, in agreement with theory. We have also generated a coherent state in the microwave resonator, and monitored its decay process. We demonstrate that the coherent state maintains a Poisson distribution as it decays, with an average photon number that decreases with the same characteristic decay time as the one-photon Fock state.

cond-mat.mes-hall↗

arXiv2008

Uncollapsing of a quantum state in a superconducting phase qubit

We demonstrate in a superconducting qubit the conditional recovery ("uncollapsing") of a quantum state after a partial-collapse measurement. A weak measurement extracts information and results in a non-unitary transformation of the qubit state. However, by adding a rotation and a second partial measurement with the same strength, we erase the extracted information, effectively canceling the effect of both measurements. The fidelity of the state recovery is measured using quantum process tomography and found to be above 70% for partial-collapse strength less than 0.6.

quant-ph↗

arXiv2008

Transformed Dissipation in Superconducting Quantum Circuits

Superconducting quantum circuits must be designed carefully to avoid dissipation from coupling to external control circuitry. Here we introduce the concept of current transformation to quantify coupling to the environment. We test this theory with an experimentally-determined impedance transformation of $\sim 10^5$ and find quantitative agreement better than a factor of 2 between this transformation and the reduced lifetime of a phase qubit coupled to a tunable transformer. Higher-order corrections from quantum fluctuations are also calculated with this theory, but found not to limit the qubit lifetime. We also illustrate how this simple connection between current and impedance transformation can be used to rule out dissipation sources in experimental qubit systems.

cond-mat.supr-con↗

arXiv2008

Microwave Dielectric Loss at Single Photon Energies and milliKelvin Temperatures

The microwave performance of amorphous dielectric materials at very low temperatures and very low excitation strengths displays significant excess loss. Here, we present the loss tangents of some common amorphous and crystalline dielectrics, measured at low temperatures (T < 100 mK) with near single-photon excitation energies, using both coplanar waveguide (CPW) and lumped LC resonators. The loss can be understood using a two-level state (TLS) defect model. A circuit analysis of the half-wavelength resonators we used is outlined, and the energy dissipation of such a resonator on a multilayered dielectric substrate is considered theoretically.

cond-mat.supr-con↗

arXiv2008

High-fidelity gates in a Josephson qubit

We demonstrate new experimental procedures for measuring small errors in a superconducting quantum bit (qubit). By carefully separating out gate and measurement errors, we construct a complete error budget and demonstrate single qubit gate fidelities of 0.98, limited by energy relaxation. We also introduce a new metrology tool -- a Ramsey interference error filter -- that can measure the occupation probability of the state $\ket{2}$ down to $10^{-4}$, a magnitude near the fault tolerant threshold.

quant-ph↗

arXiv2007

1/f Flux Noise in Josephson Phase Qubits

We present a new method to measure 1/f noise in Josephson quantum bits (qubits) that yields low-frequency spectra below 1Hz. Comparison of noise taken at positive and negative bias of a phase qubit shows the dominant noise source to be flux noise and not junction critical-current noise, with a magnitude similar to that measured previously in other systems. Theoretical calculations show that the level of flux noise is not compatible with the standard model of noise from two-level state defects in the surface oxides of the films.

cond-mat.supr-con↗

arXiv2007

Temperature dependence of coherent oscillations in Josephson phase qubits

We experimentally investigate the temperature dependence of Rabi oscillations and Ramsey fringes in superconducting phase qubits driven by microwave pulses. In a wide range of temperatures, we find that both the decay time and the amplitude of these coherent oscillations remain nearly unaffected by thermal fluctuations. The oscillations are observed well above the crossover temperature from thermally activated escape to quantum tunneling for undriven qubits. In the two-level limit, coherent qubit response rapidly vanishes as soon as the energy of thermal fluctuations kT becomes larger than the energy level spacing of the qubit. Our observations shed new light on the origin of decoherence in superconducting qubits. The experimental data suggest that, without degrading already achieved coherence times, phase qubits can be operated at temperatures much higher than those reported till now.

cond-mat.supr-con↗

arXiv2006

State tomography of capacitively shunted phase qubits with high fidelity

We introduce a new design concept for superconducting quantum bits (qubits) in which we explicitly separate the capacitive element from the Josephson tunnel junction for improved qubit performance. The number of two-level systems (TLS) that couple to the qubit is thereby reduced by an order of magnitude and the measurement fidelity improves to 90%. This improved design enables the first demonstration of quantum state tomography with superconducting qubits using single shot measurements.

cond-mat.supr-con↗