arXiv subjects

M. Dumm

Publications and source records attributed to M. Dumm.

8 recordsLinked to original sources

arXiv2013

Charge Order Breaks Magnetic Symmetry in Molecular Quantum Spin Chains

Charge order affects most of the electronic properties but is believed not to alter the spin arrangement since the magnetic susceptibility remains unchanged. We present electron-spin-resonance experiments on quasi-one-dimensional (TMTTF)2X salts (X= PF6, AsF6 and SbF6), which reveal that the magnetic properties are modified below TCO when electronic ferroelectricity sets in. The coupling of anions and organic molecules rotates the g-tensor out of the molecular plane creating magnetically non-equivalent sites on neighboring chains at domain walls. Due to anisotropic Zeeman interaction a novel magnetic interaction mechanism in the charge-ordered state is observed as a doubling of the rotational periodicity of Delta H.

cond-mat.str-el↗

arXiv2010

Comprehensive transport studies of anisotropy and ordering phenomena in quasi-one-dimensional (TMTTF)2X salts (X = PF6, AsF6, SbF6; BF4, ClO4, ReO4)

The temperature dependent dc resistivity of the quasi-one-dimensional organic salts (TMTTF)2X ( X = PF6, AsF6, SbF6; BF4, ClO4, ReO4) has been measured in all three crystal directions in order to investigate anisotropy, localization effects, charge and anion ordering phenomena at low temperatures. For all compounds and directions we extract the transport mechanisms in different regimes. The data are thoroughly analyzed, related to structural properties, and extensively discussed in view of previous studies and latest theories. It becomes apparent that the anions have a severe influence on the physical properties of the TMTTF salts.

cond-mat.str-el↗

arXiv2007

Quasiparticles at the verge of localization near the Mott metal-insulator transition in a two-dimensional material

The dynamics of charge carriers close to the Mott transition is explored theoretically and experimentally in the quasi two-dimensional organic charge-transfer salt $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br$_x$Cl$_{1-x}$, with varying Br content. The frequency dependence of the conductivity deviates significantly from simple Drude model behavior: there is a strong redistribution of spectral weight as the Mott transition is approached and with temperature. The effective mass of the quasiparticles increases considerably when coming close to the insulating phase. A dynamical mean-field-theory treatment of the relevant Hubbard model gives a good quantitative description of the experimental data.

cond-mat.str-el↗

arXiv2006

Charge Localization due to RKKY Interaction in the Spin Glass AuFe

Measurements of electrodynamic response of of spin glass AuFe films in comparison with pure gold films are performed at frequencies from 0.3 THz (10 cm-1) up to 1000 THz (33000 cm-1) using different spectroscopic methods. At room temperatures the spectra of pure gold and of AuFe are typically metallic with the scattering rate of carriers in AuFe being significantly enlarged due to scattering on localized magnetic moments of Fe ions. In the spin-glass phase of AuFe at T = 5 K a pseudogap in the conductivity spectrum is detected with the magnitude close to the Ruderman-Kittel-Kasuya-Yosida (RKKY) energy for AuFe: Delta(RKKY) = 2.2 meV. The origin of the pseudogap is associated with partial localization of electrons which mediate the RKKY interaction between localized magnetic Fe centers.

cond-mat.str-el↗

arXiv2005

Mobility gap in intermediate valent TmSe

The infrared optical conductivity of intermediate valence compound TmSe reveals clear signatures for hybridization of light $d$- and heavy f-electronic states with m* ~ 1.6 m_0 and m* ~ 16 m_0, respectively. At moderate and high temperatures, the metal-like character of the heavy carriers dominate the low-frequency response while at low temperatures (T_N < T < 100 K) a gap-like feature is observed in the conductivity spectra below 10 meV which is assigned to be a mobility gap due to localization of electrons on local Kondo singlets, rather than a hybridization gap in the density of states.

cond-mat.str-el↗

arXiv2005

Constant effective mass across the phase diagram of high-T$_{c}$ cuprates

We investigate the hole dynamics in two prototypical high temperature superconducting systems: La$_{2-x}$Sr$_{x}$CuO$_{4}$ and YBa$_{2}$Cu$_{3}% $O$_{y}$ using a combination of DC transport and infrared spectroscopy. By exploring the effective spectral weight obtained with optics in conjunction with DC Hall results we find that the transition to the Mott insulating state in these systems is of the "vanishing carrier number" type since we observe no substantial enhancement of the mass as one proceeds to undoped phases. Further, the effective mass remains constant across the entire underdoped regime of the phase diagram. We discuss the implications of these results for the understanding of both transport phenomena and pairing mechanism in high-T$_{c}$ systems.

cond-mat.str-el↗

arXiv2005

Electrodynamics of the Nodal Metal in Weakly Doped High-$T_{c}$ Cuprates

We report on the detailed analysis of the infrared (IR) conductivity of two prototypical high-$T_{c}$ systems YBa$_{2}$Cu$_{3}$O$_{y}$ and La$_{2-x}$Sr$%_{x}$CuO$_{4}$ throughout the complex phase diagram of these compounds. Our focus in this work is to thoroughly document the electromagnetic response of the nodal metal state which is initiated with only few holes doped in parent antiferromagnetic systems and extends up to the pseudogap boundary in the phase diagram. The key signature of the nodal metal is the two-component conductivity: the Drude mode at low energies followed by a resonance in mid-IR. The Drude component can be attributed to the response of coherent quasiparticles residing on the Fermi arcs detected in photoemission experiments. The microscopic origin of the mid-IR band is yet to be understood. A combination of transport and IR data uncovers fingerprints of the Fermi liquid behavior in the response of the nodal metal. The comprehensive nature of the data sets presented in this work allows us to critically re-evaluate common approaches to the interpretation of the optical data. Specifically we re-examine the role of magnetic excitations in generating electronic self energy effects through the analysis of the IR data in high magnetic field.

cond-mat.supr-con↗

arXiv2005

Infrared signatures of hole and spin stripes in La{2-x}Sr{x}CuO{4}

We investigate the hole and lattice dynamics in a prototypical high temperature superconducting system La{2-x}Sr{x}CuO{4} using infrared spectroscopy. By exploring the anisotropy in the electronic response of CuO2 planes we show that our results support the notion of stripes. Nevertheless, charge ordering effects are not apparent in the phonon spectra. All crystals show only the expected infrared active modes for orthorhombic phases without evidence for additional peaks that may be indicative of static charge ordering. Strong electron-phonon interaction manifests itself through the Fano lineshape of several phonon modes. This analysis reveals anisotropic electron-phonon coupling across the phase diagram, including superconducting crystals. Due to the ubiquity of the CuO2 plane, these results may have implications for other high Tc superconductors.

cond-mat.supr-con↗