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M. Fujita

Publications and source records attributed to M. Fujita.

At least 91 records · Page 5Linked to original sources

Field-Induced Uniform Antiferromagnetic Order Associated with Superconductivity in Pr$_{1-x}$LaCe$_{x}$CuO$_{4-δ}$

Strong correlation between field-induced antiferromagnetic (AF) order and superconductivity is demonstrated for an electron-doped cuprate superconductor, Pr$_{1-x}$LaCe$_{x}$CuO$_{4-δ}$ (PLCCO). In addition to the specimen with $x=0.11$ (which is close to the AF phase boundary, $x\simeq0.10$), we show that the one with $x=0.15$ ($T_c\simeq16$ K at zero field) also exhibits the field-induced AF order with a reduced magnitude of the induced moment. The uniform muon Knight shift at a low magnetic field ($\sim10^2$ Oe) indicates that the AF order is not localized within the cores of flux lines, which is in a marked contrast with theoretical prediction for hole-doped cuprates. The presence of anomalous non-diagonal hyperfine coupling between muons and Pr ions is also demonstrated in detail.

cond-mat.supr-con↗

Direct Observation of Non-Monotonic dx2-y2-Wave Superconducting Gap in Electron-Doped High-Tc Superconductor Pr0.89LaCe0.11CuO4

We performed high-resolution angle-resolved photoemission spectroscopy on electron-doped high-Tc superconductor Pr0.89LaCe0.11CuO4 to study the anisotropy of the superconducting gap. The observed momentum dependence is basically consistent with the dx2-y2-wave symmetry, but obviously deviates from the monotonic dx2-y2 gap function. The maximum gap is observed not at the zone boundary, but at the hot spot where the antiferromagnetic spin fluctuation strongly couples to the electrons on the Fermi surface. The present experimental results unambiguously indicate the spin-mediated pairing mechanism in electron-doped high-Tc superconductors.

cond-mat.supr-con↗

Universal magnetic excitation spectrum in cuprates

We have recently used inelastic neutron scattering to measure the magnetic excitation spectrum of La(1.875)Ba(0.125)CuO(4) up to 200 meV. This particular cuprate is of interest because it exhibits static charge and spin stripe order. The observed spectrum is remarkably similar to that found in superconducting YBa(2)Cu(3)O(6+x) and La(2-x)Sr(x)CuO(4); the main differences are associated with the spin gap. We suggest that essentially all observed features of the magnetic scattering from cuprate superconductors can be described by a universal magnetic excitation spectrum multiplied by a spin gap function with a material-dependent spin-gap energy.

cond-mat.supr-con↗

Soft phonons and structural phase transitions in La$_{1.875}$Ba$_{0.125}$CuO$_{4}$

Soft phonon behavior associated with a structural phase transition from the low-temperature-orthorhombic (LTO) phase ($Bmab$ symmetry) to the low-temperature-tetragonal (LTT) phase ($P4_{2}/ncm$ symmetry) was investigated in La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ using neutron scattering. As temperature decreases, the TO-mode at $Z$-point softens and approaches to zero energy around $T_{\rm d2}=62$ K, where the LTO -- LTT transition occurs. Below $T_{\rm d2}$, the phonon hardens quite rapidly and it's energy almost saturates below 50 K. At $T_{\rm d2}$, the energy dispersion of the soft phonon along in-plane direction significantly changes while the dispersion along out-of-plane direction is almost temperature independent. Coexistence between the LTO phase and the LTT phase, seen in both the soft phonon spectra and the peak profiles of Bragg reflection, is discussed in context of the order of structural phase transitions.

cond-mat.supr-con↗

Relationship between charge stripe order and structural phase transitions in La$_{1.875}$Ba$_{0.125-x}$Sr$_{x}$CuO$_{4}$

The nature of charge stripe order and its relationship with structural phase transitions were studied using synchrotron X-ray diffraction in La$_{1.875}$Ba$_{0.125-x}$Sr$_{x}$CuO$_{4}$ ($0.05\leq x\leq 0.10$). For $x=0.05$, as temperature increased, incommensurate superlattice peaks associated with the charge order disappeared just at the structural phase transition temperature, $T_{\rm d2}$. However, for $x=0.075$ and 0.09, the superlattice peaks still existed as a short range correlation even above $T_{\rm d2}$, indicating a precursor of charge ordering. Furthermore, temperature dependences of the superlattice peak intensity, correlation length, and incommensurability for $x=0.05$ are different from those for $x=0.075$ and 0.09. These results suggest that the transition process into the charge stripe order strongly correlates with the order of the structural phase transitions. A quantitative comparison of the structure factor associated with the charge order have been also made for all the samples.

cond-mat.supr-con↗

Reflectivity measurements in uniaxial superconductors: a methodological discussion applied to the case of La(2-x)Sr(x)CuO(4)

Most of the novel superconductors are uniaxial crystals, with metallic planes ($ab$) orthogonal to an insulating axis ($c$). Far-infrared measurements of the reflectivity $R_{ab} (ω)$ provide valuable information on their low-energy electrodynamics, but involve delicate experimental issues. Two of them are a possible contamination of $R_{ab} (ω)$ from the c axis and the extrapolation of the $R_{ab}$ data to $ω$ =0, both above and below $T_c$. Here we discuss quantitatively these issues with particular regard to La$_{2-x}$Sr$_x$CuO$_{4+y}$, one of the most studied high-$T_c$ materials.

cond-mat.supr-con↗

Strong correlation between field-induced magnetism and superconductivity in Pr$_{0.89}$LaCe$_{0.11}$CuO$_{4}$

We report the local magnetic response of an electron-doped cuprate superconductor, Pr$_{0.89}$LaCe$_{0.11}$CuO$_{4}$ ($T_c\simeq26$ K), studied by muon spin rotation (\msr) over a field range from 200 Oe to 50 kOe. In the paramagnetic state, the muon Knight shift along the crystal c-axis ($K_μ^z$) is proportional to the in-plane susceptibility $χ_{ab}$. More surprisingly, $K_μ^z$ is strongly enhanced by the occurrence of superconductivity (below $\sim$40 kOe), changing its sign from positive to negative around $\sim1$ kOe with increasing field. This finding can be understood by considering the weak polarization of Pr ions due to superexchange interaction with the antiferromagnetic Cu sublattice, which coexists with superconductivity.

cond-mat.supr-con↗

Quantum Magnetic Excitations from Stripes in Copper-Oxide Superconductors

In the copper-oxide parent compounds of the high-transition-temperature superconductors, the valence electrons are localized, one per copper site, due to strong intraatomic Coulomb repulsion. A symptom of the localization is antiferromagnetism, where the spins of localized electrons alternate between up and down. The superconductivity appears when mobile 'holes' are doped into this insulating state, and it coexists with antiferromagnetic fluctuations. In one approach to the coexistence, the holes are believed to self-organize into 'stripes' that alternate with antiferromagnetic (insulating) regions within copper-oxide planes. Such an unusual electronic state would necessitate an unconventional mechanism of superconductivity. There is an apparent problem with this picture, however: measurements of magnetic excitations in superconducting YBa(2)Cu(3)O(6+x) near optimum doping are incompatible with the naive expectations for a material with stripes. Here we report neutron scattering measurements on stripe-ordered La(1.875)Ba(0.125)CuO(4). We show that the measured excitations are, surprisingly, quite similar to those in YBa(2)Cu(3)O(6+x) (i.e., the predicted spectrum of magnetic excitations is wrong). We find instead that the observed spectrum can be understood within a stripe model by taking account of quantum excitations. Our results support the concept that stripe correlations are essential to high-transition-temperature superconductivity.

cond-mat.supr-con↗

Stripe order, depinning, and fluctuations in La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ and La$_{1.875}$Ba$_{0.075}$Sr$_{0.050}$CuO$_{4}$

We present a neutron scattering study of stripe correlations measured on a single crystal of La$_{1.875}$Ba$_{0.125}$CuO$_{4}$. Within the low-temperature-tetragonal (LTT) phase, superlattice peaks indicative of spin and charge stripe order are observed below 50 K. For excitation energies $\hbarω\le12$ meV, we have characterized the magnetic excitations that emerge from the incommensurate magnetic superlattice peaks. In the ordered state, these excitations are similar to spin waves. Following these excitations as a function of temperature, we find that there is relatively little change in the {\bf Q}-integrated dynamical spin susceptibility for $\hbarω\sim10$ meV as stripe order disappears and then as the structure transforms from LTT to the low-temperature-orthorhombic (LTO) phase. The {\bf Q}-integrated signal at lower energies changes more dramatically through these transitions, as it must in a transformation from an ordered to a disordered state. We argue that the continuous evolution through the transitions provides direct evidence that the incommensurate spin excitations in the disordered state are an indicator of dynamical charge stripes. An interesting feature of the thermal evolution is a variation in the incommensurability of the magnetic scattering. Similar behavior is observed in measurements on a single crystal of La$_{1.875}$Ba$_{0.075}$Sr$_{0.050}$CuO$_{4}$; maps of the scattered intensity in a region centered on the antiferromagnetic wave vector and measured at $\hbarω=4$ meV are well reproduced by a model of disordered stripes with a temperature-dependent mixture of stripe spacings. We discuss the relevance of our results to understanding the magnetic excitations in cuprate superconductors.

cond-mat.str-el↗

Precision spectroscopy of pionic 1s states of Sn nuclei and evidence for partial restoration of chiral symmetry in the nuclear medium

Deeply bound 1s states of $π^-$ in $^{115,119,123}$Sn were preferentially observed using the Sn($d$,$^3$He) pion-transfer reaction under the recoil-free condition. The 1s binding energies and widths were precisely determined, and were used to deduce the isovector parameter of the s-wave pion-nucleus potential to be $b_1 =-0.115\pm 0.007 ~m_π^{-1}$. The observed enhancement of $|b_1|$ over the free $πN$ value ($b_1^{\rm free}/b_1 = 0.78 \pm 0.05$) indicates a reduction of the chiral order parameter, $f^{*}_π (ρ)^2/f_π^2 \approx 0.64$, at the normal nuclear density, $ρ= ρ_0$.

nucl-ex↗

Magnetic Field Effect on Static Antiferromagnetism in Electron-Doped Superconductor Pr$_{1-x}$LaCe$_x$CuO$_4$ ($x$=0.11 and 0.15)

Effects of magnetic fields (applied along the c-axis) on static spin correlation were studied for the electron-doped superconductors Pr$_{1-x}$LaCe$_{x}$CuO$_4$ with $x$=0.11 ($T_c$=26 K) and $x$=0.15 ($T_c$=16 K) by neutron scattering measurements. In the $x$=0.11 sample located near the antiferromagnetic(AF) and superconducting phase boundary, the field dependence of both the magnetic intensity at T=3 K and the onset temperature of the magnetic order exhibits a peak at $\sim$5 T. In contrast, in the overdoped $x$=0.15 sample a static AF order is neither observed at zero-field nor induced by the field up to 8.5 T. Difference and similarity of the field effect between the hole- and electron-doped high-$T_c$ cuprates are discussed.

cond-mat.supr-con↗

Fermi-liquid ground state in n-type copper-oxide superconductor Pr0.91Ce0.09LaCuO4-y

We report nuclear magnetic resonance studies on the low-doped n-type copper-oxide Pr_{0.91}LaCe_{0.09}CuO_{4-y} (T_c=24 K) in the superconducting state and in the normal state uncovered by the application of a strong magnetic field. We find that when the superconductivity is removed, the underlying ground state is the Fermi liquid state. This result is at variance with that inferred from previous thermal conductivity measurement and contrast with that in p-type copper-oxides with a similar doping level where high-T_c superconductivity sets in within the pseudogap phase. The data in the superconducting state are consistent with the line-nodes gap model.

cond-mat.supr-con↗

Synchrotron X-ray diffraction study of a charge stripe order in 1/8-doped La$_{1.875}$Ba$_{0.125-x}$Sr$_{x}$CuO$_{4}$

Lattice distortions associated with charge stripe order in 1/8 hole-doped La$_{1.875}$Ba$_{0.125-x}$Sr$_{x}$CuO$_{4}$ are studied using synchrotron X-ray diffraction for $x=0.05$ and $x=0.075$. The propagation wave vector and charge order correlation lengths are determined with a high accuracy, revealing that the oblique charge stripes in orthorhombic $x=0.075$ crystal are more disordered than the aligned stripes in tetragonal $x=0.05$ crystal. The twofold periodicity of lattice modulations along the c-axis is explained by long-range Coulomb interactions between holes on neighboring CuO$_{2}$ planes.

cond-mat.supr-con↗

Pionic Atom Formation in Halo Nuclei by (d,3He) Reactions

We investigate the formation cross sections of the deeply bound pionic atoms on halo nuclei theoretically. We consider one-neutron pick-up (d,3He) reaction for the pionic atom formation and find that the formation rate is significantly increased by the existence of the halo neutron with long tail of the wave function. This enhancement is expected to increase the experimental feasibility for the formation of the deeply bound pionic states on beta-unstable nuclei.

nucl-th↗

Structural effect on the static spin and charge correlations in La$_{1.875}$Ba$_{0.125-x}$Sr$_{x}$CuO$_{4}$

We report the results of elastic neutron scattering measurements performed on 1/8-hole doped La$_{1.875}$Ba$_{0.125-x}$Sr$_{x}$CuO$_{4}$ single crystals with {\it x}=0.05, 0.06, 0.075 and 0.085. In the low-temperature less-orthorhombic (LTLO, {\it Pccn} symmetry) phase, the charge-density-wave (CDW) and spin-density-wave (SDW) wavevectors were found to tilt in a low-symmetric direction with one-dimensional anisotropy in the CuO$_{2}$ plane, while they were aligned along the high-symmetry axis in the low-temperature tetragonal (LTT, {\it P}4$_2$/{\it ncm} symmetry) phase. The coincident direction of two wavevectors suggests a close relation between CDW and SDW orders. The SDW wavevector systematically deviates from the Cu-O bond direction in the LTLO phase upon Sr substitution and the tilt angle in the LTLO phase is smaller than that in the low-temperature orthorhombic phase (LTO, {\it B}{\it mab} symmetry) with comparable in-plane orthorhombic distortion. These results demonstrate a correlation between the corrugated pattern of CuO$_{2}$ plane and the deviations.

cond-mat.supr-con↗

Magnetic and superconducting phase diagram of electron-doped Pr$_{1-x}$LaCe$_{x}$CuO$_{4}$

We have investigated the magnetism and the superconductivity of an electron-doped Pr$_{1-x}$LaCe$_{x}$CuO$_{4}$ (PLCCO) using single crystal and powder samples by means of zero-field muon spin rotation/relaxation (ZF-$μ$SR) and magnetic susceptibility measurements. Muon spin rotation corresponding to antiferromagnetic (AF) order was observed in the sample with 0.04$\leq${\it x}$\leq$0.11. Changes in magnetic properties of Cu spins upon Ce doping were revealed because the effect of the rare earth moment was negligible. Bulk superconductivity was identified in a wide Ce concentration range of 0.09$\leq${\it x}$\leq$0.20 with a maximum transition temperature of 26 K. At low temperatures, the superconducting (SC) phase abruptly appears by doping with linking quick destroy of the AF ordered phase at {\it x}$\sim$0.09, indicating the competitive relation between two phases.

cond-mat.supr-con↗

Commensurate spin dynamics in the superconducting state of an electron-doped cuprate superconductor

We report neutron scattering studies on single crystals of the electron-doped (n-type) superconducting cuprate Nd2-xCexCuO4 (x=0.15) with Tc = 18 K and 25 K. Unlike the hole-doped (p-type) superconducting cuprates where incommensurate magnetic fluctuations commonly exist, the n-type cuprate shows commensurate magnetic fluctuations at the tetragonal (1/2 1/2 0) reciprocal points both in the superconducting and in the normal state. A spin gap opens up when the n-type cuprate becomes superconducting, as in the optimally doped p-type La2-xSrxCuO4. The gap energy, however, increases gradually up to about 4 meV as T decreases from Tc to 2 K, which contrasts with the spin pseudogap behavior with a T-independent gap energy in the superconducting state of p-type cuprates.

cond-mat.str-el↗