SearcharxivSearch

arXiv subjects

M. Grifoni

Publications and source records attributed to M. Grifoni.

At least 19 recordsLinked to original sources

Heat transport in the quantum Rabi model: Universality and ultrastrong coupling effects

Heat transport in the quantum Rabi model at weak interaction with the heat baths is controlled by the qubit-oscillator coupling. Universality of the linear conductance versus the temperature is found for $T\lesssim T_K$, with $T_K$ a coupling-dependent Kondo-like temperature. At low temperature, coherent heat transfer via virtual processes yields a $\sim T^3$ behavior with destructive interference in the presence of quasi-degeneracies in the spectrum. As the temperature increases, incoherent emission and absorption dominate and a maximum is reached at $T\sim T_K/2$. In the presence of a bias on the qubit, the conductance makes a transition from a resonant to a broad, zero-bias peak regime. Parallels and differences are found compared to the spin-boson model in [K. Saito and T. Kato, Phys. Rev. Lett. \textbf{111}, 214301 (2013)], where the qubit-bath coupling instead of the internal qubit-oscillator coupling rules thermal transport.

cond-mat.mes-hall

A unified diagrammatic approach to quantum transport in few-level junctions for bosonic and fermionic reservoirs: Application to the quantum Rabi model

We apply the Nakajima-Zwanzig approach to open quantum systems to study steady-state transport across generic multi-level junctions coupled to bosonic or fermionic reservoirs. The method allows for a unified diagrammatic formulation in Liouville space, with diagrams being classified according to an expansion in the coupling strength between the reservoirs and the junction. Analytical, approximate expressions are provided up to fourth order for the steady-state boson transport that generalize to multi-level systems the known results for the low-temperature thermal conductance in the spin-boson model. The formalism is applied to the problem of heat transport in a qubit-resonator junction modeled by the quantum Rabi model. Nontrivial transport features emerge as a result of the interplay between the qubit-oscillator detuning and coupling strength. For quasi-degenerate spectra, nonvanishing steady-state coherences cause a suppression of the thermal conductance.

quant-ph

Transmission spectra of the driven, dissipative Rabi model in the USC regime

We present theoretical transmission spectra of a strongly driven, damped, flux qubit coupled to a dissipative resonator in the ultrastrong coupling regime. Such a qubit-oscillator system, described within a dissipative Rabi model, constitutes the building block of superconducting circuit QED platforms. The addition of a strong drive allows one to characterize the system properties and study novel phenomena, leading to a better understanding and control of the qubit-oscillator system. In this work, the calculated transmission of a weak probe field quantifies the response of the qubit, in frequency domain, under the influence of the quantized resonator and of the strong microwave drive. We find distinctive features of the entangled driven qubit-resonator spectrum, namely resonant features and avoided crossings, modified by the presence of the dissipative environment. The magnitude, positions, and broadening of these features are determined by the interplay among qubit-oscillator detuning, the strength of their coupling, the driving amplitude, and the interaction with the heat bath. This work establishes the theoretical basis for future experiments in the driven ultrastrong coupling regime and their impact to develop novel quantum technologies with superconducting circuits.

quant-ph

Feynman-Vernon influence functional approach to quantum transport in interacting nanojunctions: An analytical hierarchical study

We present a nonperturbative and formally exact approach for the charge transport in interacting nanojunctions based on a real time path integral formulation of the reduced system dynamics. An expansion of the influence functional in terms of the number of tunneling transitions, and integration of the Grassmann variables between the tunneling times, allows us to obtain a still exact generalized master equation (GME) for the populations of the reduced density matrix (RDM) in the occupation number representation, as well as a formally exact expression for the current. By borrowing the nomenclature of the famous spin-boson problem, we characterize the two-state dynamics of such degrees of freedom on the forward and backward branches in terms of single four-state paths with alternating blips and sojourns. This allows a diagrammatic representation of the GME kernel and its parametrization in terms of sequences of blips and sojourns. We apply our formalism to the exactly solvable resonant level model (RLM) and to the the single impurity Anderson model (SIAM). We demonstrate a hierarchical diagrammatic structure of the exact GME kernel. While the hierarchy closes at the second-tier level for the RLM, this is not the case for the interacting SIAM. Upon inspection of the GME, known results from various perturbative and nonperturbative approximation schemes to quantum transport in the SIAM are recovered. Finally, a noncrossing approximation for the hierarchical kernel is developed, which enables us to systematically decrease temperature at each next level of the approximation. Analytical results are presented, both in equilibrium and nonequilibrium, including the case of an applied magnetic field.

cond-mat.mes-hall

Fabry-Pérot oscillations in correlated carbon nanotubes

We report the observation of an intriguing behaviour in the transport properties of nanodevices operating in a regime between the Fabry-Pérot and the Kondo limits. Using ultra-high quality nanotube devices, we study how the conductance oscillates when sweeping the gate voltage. Surprisingly, we observe a four-fold enhancement of the oscillation period upon decreasing temperature, signaling a crossover from single-electron tunneling to Fabry-Pérot interference. These results suggest that the Fabry-Pérot interference occurs in a regime where electrons are correlated. The link between the measured correlated Fabry-Pérot oscillations and the SU(4) Kondo effect is discussed.

cond-mat.mes-hall

Shaping electron wave functions in a carbon nanotube with a parallel magnetic field

A magnetic field, through its vector potential, usually causes measurable changes in the electron wave function only in the direction transverse to the field. Here we demonstrate experimentally and theoretically that in carbon nanotube quantum dots, combining cylindrical topology and bipartite hexagonal lattice, a magnetic field along the nanotube axis impacts also the longitudinal profile of the electronic states. With the high (up to 17T) magnetic fields in our experiment the wave functions can be tuned all the way from "half-wave resonator" shape, with nodes at both ends, to "quarter-wave resonator" shape, with an antinode at one end. This in turn causes a distinct dependence of the conductance on the magnetic field. Our results demonstrate a new strategy for the control of wave functions using magnetic fields in quantum systems with nontrivial lattice and topology.

cond-mat.mes-hall

Probing the strongly driven spin-boson model in a superconducting quantum circuit

Quantum two-level systems interacting with the surroundings are ubiquitous in nature. The interaction suppresses quantum coherence and forces the system towards a steady state. Such dissipative processes are captured by the paradigmatic spin-boson model, describing a two-state particle, the "spin", interacting with an environment formed by harmonic oscillators. A fundamental question to date is to what extent intense coherent driving impacts a strongly dissipative system. Here we investigate experimentally and theoretically a superconducting qubit strongly coupled to an electromagnetic environment and subjected to a coherent drive. This setup realizes the driven Ohmic spin-boson model. We show that the drive reinforces environmental suppression of quantum coherence, and that a coherent-to-incoherent transition can be achieved by tuning the drive amplitude. An out-of-equilibrium detailed balance relation is demonstrated. These results advance fundamental understanding of open quantum systems and bear potential for the design of entangled light-matter states.

quant-ph

Topology and zero energy edge states in carbon nanotubes with superconducting pairing

We investigate the spectrum of finite-length carbon nanotubes in the presence of onsite and nearest-neighbor superconducting pairing terms. A one-dimensional ladder-type lattice model is developed to explore the low-energy spectrum and the nature of the electronic states. We find that zero energy edge states can emerge in zigzag class carbon nanotubes as a combined effect of curvature-induced Dirac point shift and strong superconducting coupling between nearest-neighbor sites. The chiral symmetry of the system is exploited to define a winding number topological invariant. The associated topological phase diagram shows regions with nontrivial winding number in the plane of chemical potential and superconducting nearest-neighbor pair potential (relative to the onsite pair potential). A one-dimensional continuum model reveals the topological origin of the zero energy edge states: A bulk-edge correspondence is proven, which shows that the condition for nontrivial winding number and that for the emergence of edge states are identical. For armchair class nanotubes, the presence of edge states in the superconducting gap depends on the nanotube's boundary shape. For the minimal boundary condition, the emergence of the subgap states can also be deduced from the winding number.

cond-mat.mes-hall

Blocking transport resonances via Kondo entanglement in quantum dots

Many-body entanglement is at the heart of the Kondo effect, which has its hallmark in quantum dots as a zero-bias conductance peak at low temperatures. It signals the emergence of a conducting singlet state formed by a localized dot degree of freedom and conduction electrons. Carbon nanotubes offer the possibility to study the emergence of the Kondo entanglement by tuning many-body correlations with a gate voltage. Here we quantitatively show an undiscovered side of Kondo correlations, which counterintuitively tend to block conduction channels: inelastic cotunneling lines in the magnetospectrum of a carbon nanotube strikingly disappear when tuning the gate voltage. Considering the global \SUT\ $\otimes $ \SUT\ symmetry of a carbon nanotube coupled to leads, we find that only resonances involving flips of the Kramers pseudospins, associated to this symmetry, are observed at temperatures and voltages below the corresponding Kondo scale. Our results demonstrate the robust formation of entangled many-body states with no net pseudospin.

cond-mat.mes-hall

Secondary electron interference from trigonal warping in clean carbon nanotubes

We investigate Fabry-Perot interference in an ultraclean carbon nanotube resonator. The conductance shows a clear superstructure superimposed onto conventional Fabry-Perot oscillations. A sliding average over the fast oscillations reveals a characteristic slow modulation of the conductance as a function of the gate voltage. We identify the origin of this secondary interference in intervalley and intravalley backscattering processes which involve wave vectors of different magnitude, reflecting the trigonal warping of the Dirac cones. As a consequence, the analysis of the secondary interference pattern allows us to estimate the chiral angle of the carbon nanotube.

cond-mat.mes-hall

Broken SU(4) symmetry in a Kondo-correlated carbon nanotube

Understanding the interplay between many-body phenomena and non-equilibrium in systems with entangled spin and orbital degrees of freedom is a central objective in nano-electronics. We demonstrate that the combination of Coulomb interaction, spin-orbit coupling and valley mixing results in a particular selection of the inelastic virtual processes contributing to the Kondo resonance in carbon nanotubes at low temperatures. This effect is dictated by conjugation properties of the underlying carbon nanotube spectrum at zero and finite magnetic field. Our measurements on a clean carbon nanotube are complemented by calculations based on a new approach to the non-equilibrium Kondo problem which well reproduces the rich experimental observations in Kondo transport.

cond-mat.mes-hall

Double island Coulomb blockade in (Ga,Mn)As-nanoconstrictions

We report on a systematic study of the Coulomb blockade effects in nanofabricated narrow constrictions in thin (Ga,Mn)As films. Different low-temperature transport regimes have been observed for decreasing constriction sizes: the ohmic, the single electron tunnelling (SET) and a completely insulating regime. In the SET, complex stability diagrams with nested Coulomb diamonds and anomalous conductance suppression in the vicinity of charge degeneracy points have been observed. We rationalize these observations in the SET with a double ferromagnetic island model coupled to ferromagnetic leads. Its transport characteristics are analyzed in terms of a modified orthodox theory of Coulomb blockade which takes into account the energy dependence of the density of states in the metallic islands.

cond-mat.mes-hall

Thermally induced subgap features in the cotunneling spectroscopy of a carbon nanotube

We report on nonlinear cotunneling spectroscopy of a carbon nanotube quantum dot coupled to Nb superconducting contacts. Our measurements show rich subgap features in the stability diagram which become more pronounced as the temperature is increased. Applying a transport theory based on the Liouville-von Neumann equation for the density matrix, we show that the transport properties can be attributed to processes involving sequential as well as elastic and inelastic cotunneling of quasiparticles thermally excited across the gap. In particular, we predict thermal replicas of the elastic and inelastic cotunneling peaks, in agreement with our experimental results.

cond-mat.mes-hall

Sub-gap spectroscopy of thermally excited quasiparticles in a Nb contacted carbon nanotube quantum dot

We present electronic transport measurements of a single wall carbon nanotube quantum dot coupled to Nb superconducting contacts. For temperatures comparable to the superconducting gap peculiar transport features are observed inside the Coulomb blockade and superconducting energy gap regions. The observed temperature dependence can be explained in terms of sequential tunneling processes involving thermally excited quasiparticles. In particular, these new channels give rise to two unusual conductance peaks at zero bias in the vicinity of the charge degeneracy point and allow to determine the degeneracy of the ground states involved in transport. The measurements are in good agreement with model calculations.

cond-mat.mes-hall

Sources of negative tunneling magneto-resistance in multilevel quantum dots with ferromagnetic contacts

We analyze distinct sources of spin-dependent energy level shifts and their impact on the tunneling magnetoresistance (TMR) of interacting quantum dots coupled to collinearly polarized ferromagnetic leads. Level shifts due to virtual charge fluctuations can be quantitatively evaluated within a diagrammatic representation of our transport theory. The theory is valid for multilevel quantum dot systems and we exemplarily apply it to carbon nanotube quantum dots, where we show that the presence of many levels can qualitatively influence the TMR effect.

cond-mat.mes-hall

Direct observation of band-gap closure for a semiconducting carbon nanotube in a large parallel magnetic field

We have investigated the magnetoconductance of semiconducting carbon nanotubes (CNTs) in pulsed, parallel magnetic fields up to 60 T, and report the direct observation of the predicted band-gap closure and the reopening of the gap under variation of the applied magnetic field. We also highlight the important influence of mechanical strain on the magnetoconductance of the CNTs.

cond-mat.mes-hall

Spin-orbit interaction in chiral carbon nanotubes probed in pulsed magnetic fields

The magneto-conductance of an open carbon nanotube (CNT)-quantum wire was measured in pulsed magnetic fields. At low temperatures we find a peculiar split magneto-conductance peak close to the charge neutrality point. Our analysis of the data reveals that this splitting is intimately connected to the spin-orbit interaction and the tube chirality. Band structure calculations suggest that the current in the peak regions is highly spin-polarized, which calls for application in future CNT-based spintronic devices.

cond-mat.mes-hall

A benzene interference single-electron transistor

Interference effects strongly affect the transport characteristics of a benzene single-electron transistor (SET) and for this reason we call it interference SET (I-SET). We focus on the effects of degeneracies between many-body states of the isolated benzene. We show that the particular current blocking and selective conductance suppression occurring in the benzene I-SET are due to interference effects between the orbitally degenerate states. Further we study the impact of reduced symmetry due to anchor groups or potential drop over the molecule. We identify in the quasi-degeneracy of the involved molecular states the necessary condition for the robustness of the results.

cond-mat.str-el