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M. Grilli

Publications and source records attributed to M. Grilli.

At least 73 records · Page 4Linked to original sources
arXiv2008

On the contribution of nearly-critical spin and charge collective modes to the Raman spectra of high-Tc cuprates

We discuss how Raman spectra are affected by nearly-critical spin and charge collective modes, which are coupled to charge carriers near a stripe quantum critical point. We show that specific fingerprints of nearly-critical collective modes can indeed be observed in Raman spectra and that the selectivity of Raman spectroscopy in momentum space may also be exploited to distinguish the spin and charge contribution. We apply our results to discuss the spectra of high-Tc superconducting cuprates finding that the collective modes should have masses with substantial temperature dependence in agreement with their nearly critical character. Moreover spin modes should be more diffusive than charge modes indicating that in stripes the charge is nearly ordered, while spin modes are strongly overdamped and fluctuate with high frequency.

cond-mat.supr-con↗
arXiv2008

Low-energy signatures of charge and spin fluctuations in Raman and optical spectra of the cuprates

We calculate the optical and Raman response within a phenomenological model of fermion quasiparticles coupled to nearly critical collective modes. We find that, whereas critical scaling properties might be masked in optical spectra due to charge conservation, distinct critical signatures of charge and spin fluctuations can be detected in Raman spectra exploiting specific symmetry properties. We compare our results with recent experiments on the cuprates.

cond-mat.supr-con↗
arXiv2007

Optical conductivity near finite-wavelength quantum criticality

We study the optical conductivity sigma(Omega) of an electron system near a quantum-critical point with finite-wavelength ordering. sigma(Omega) vanishes in clean Galilean-invariant systems, unless electrons are coupled to dynamical collective modes, which dissipate the current. This coupling introduces a nonuniversal energy scale. Depending on the parameters of each specific system, a variety of responses arise near criticality: scaling peaks at a temperature- and doping-dependent frequency, peaks at a fixed frequency, or no peaks to be associated with criticality. Therefore the lack of scaling in the far-infrared conductivity in cuprates does not necessarily call for new concepts of quantum criticality.

cond-mat.supr-con↗
arXiv2007

Disorder effects in the quantum Heisenberg model: An Extended Dynamical mean-field theory analysis

We investigate a quantum Heisenberg model with both antiferromagnetic and disordered nearest-neighbor couplings. We use an extended dynamical mean-field approach, which reduces the lattice problem to a self-consistent local impurity problem that we solve by using a quantum Monte Carlo algorithm. We consider both two- and three-dimensional antiferromagnetic spin fluctuations and systematically analyze the effect of disorder. We find that in three dimensions for any small amount of disorder a spin-glass phase is realized. In two dimensions, while clean systems display the properties of a highly correlated spin-liquid (where the local spin susceptibility has a non-integer power-low frequency and/or temperature dependence), in the present case this behavior is more elusive unless disorder is very small. This is because the spin-glass transition temperature leaves only an intermediate temperature regime where the system can display the spin-liquid behavior, which turns out to be more apparent in the static than in the dynamical susceptibility.

cond-mat.dis-nn↗
arXiv2006

Spectroscopic evidences of quantum critical charge fluctuations in cuprates

We calculate the optical conductivity in a clean system of quasiparticles coupled to charge-ordering collective modes. The absorption induced by these modes may produce an anomalous frequency and temperature dependence of low-energy optical absorption in some cuprates. However, the coupling with lattice degrees of freedom introduces a non-universal energy scale leading to scaling violation in low-temperature optical conductivity.

cond-mat.str-el↗
arXiv2006

Checkerboard and stripe inhomogeneities in cuprates

We systematically investigate charge-ordering phases by means of a restricted and unrestricted Gutzwiller approximation to the single-band Hubbard model with nearest ($t$) and next-nearest neighbor hopping ($t'$). When $|t'/t|$ is small, as appropriate for ${\rm La_{2-x}Sr_xCuO_4}$, stripes are found, whereas in compounds with larger $|t'/t|$ (such as ${\rm Ca_{2-x}Na_x CuO_2Cl_2}$ and ${\rm Bi_2Sr_2CaCu_2O_{8+δ}}$) checkerboard structures are favored. In contrast to the linear doping dependence found for stripes the charge periodicity of checkerboard textures is locked to 4 unit cells over a wide doping range. In addition we find that checkerboard structures are favored at surfaces.

cond-mat.str-el↗
arXiv2006

Effective electron-electron and electron-phonon interactions in the Hubbard-Holstein model

We investigate the interplay between the electron-electron and the electron-phonon interaction in the Hubbard-Holstein model. We implement the flow-equation method to investigate within this model the effect of correlation on the electron-phonon effective coupling and, conversely, the effect of phonons in the effective electron-electron interaction. Using this technique we obtain analytical momentum-dependent expressions for the effective couplings and we study their behavior for different physical regimes. In agreement with other works on this subject, we find that the electron-electron attraction mediated by phonons in the presence of Hubbard repulsion is peaked at low transferred momenta. The role of the characteristic energies involved is also analyzed.

cond-mat.str-el↗
arXiv2005

Extended paraconductivity regime in underdoped cuprates

We reconsider transport experiments in strongly anisotropic superconducting cuprates and we find that universal Aslamazov-Larkin (AL) paraconductivity in two dimensions is surprisingly robust even in the underdoped regime below the pseudogap crossover temperature T^*. We also establish that the underlying normal state resistivity in the pseudogap phase is (almost) linear in temperature, with all the deviations being quantitatively accounted by AL paraconductivity. The disappearence of paraconductivity is governed by the disappearence of gaussian pair fluctuations at an energy scale related to T^*.

cond-mat.supr-con↗
arXiv2005

Charge-fluctuation contribution to the Raman response in superconducting cuprates

We calculate the Raman response contribution due to collective modes, finding a strong dependence on the photon polarizations and on the characteristic wavevectors of the modes. We compare our results with recent Raman spectroscopy experiments in underdoped cuprates, $La_{2-x}Sr_xCuO_4$ and $(Y_{1.97}Ca_{0.3})Ba_2CuO_{6.05}$, where anomalous low-energy peaks are observed, which soften upon lowering the temperature. We show that the specific dependence on doping and on photon polarizations of these peaks is only compatible with charge collective excitations at finite wavelength.

cond-mat.supr-con↗
arXiv2005

Electron-phonon Interaction close to a Mott transition

The effect of Holstein electron-phonon interaction on a Hubbard model close to a Mott-Hubbard transition at half-filling is investigated by means of Dynamical Mean-Field Theory. We observe a reduction of the effective mass that we interpret in terms of a reduced effective repulsion. When the repulsion is rescaled to take into account this effect, the quasiparticle low-energy features are unaffected by the electron-phonon interaction. Phonon features are only observed within the high-energy Hubbard bands. The lack of electron-phonon fingerprints in the quasiparticle physics can be explained interpreting the quasiparticle motion in terms of rare fast processes.

cond-mat.str-el↗
arXiv2004

Theory of isotope effect in photoemission spectra of high-T_c superconducting cuprates

We investigate the effect of isotope substitution on the electronic spectral functions within a model where the charge carriers are coupled to bosonic charge-order (CO) fluctuations centered around some mean frequency ω_0 and with enhanced scattering at wave-vector q_c. It is shown that a mass dependence of ω_0 is not sufficient in order to account, especially at high energies, for the dispersion shifts experimentally observed in an optimally doped superconducting cuprate. We argue that isotope substitution induces a change of the spatial CO correlations which gives good account of the experimental data.

cond-mat.supr-con↗
arXiv2004

Charge critical fluctuations in cuprates: Isotope effect, pseudogap, conductivity, and Raman spectroscopy

Within the stripe quantum critical point theory for high T_c superconductors, we point out that there is a direct contribution of charge collective fluctuations to the optical absorption and to the Raman spectra. In this latter case, we find that the critical charge collective modes can or can not be excited depending on the direction of their wavevector and on the polarization of the incoming and outgoing photons. This indicates a marked distinction between quasiparticles which are strongly and weakly coupled to critical collective modes and provides a direct confirmation that the order associated to the quantum critical point near optimal doping of cuprates occurs at finite wavevectors.

cond-mat.supr-con↗
arXiv2004

Effect of mesoscopic inhomogeneities on local tunnelling density of states

We carry out a theoretical analysis of the momentum dependence of the Fourier-transformed local density of states (LDOS) in the superconducting cuprates within a model considering the interference of quasiparticles scattering on quenched impurities. The impurities introduce an external scattering potential, which is either nearly local in space or it can acquire a substantial momentum dependence due to a possible strong momentum dependence of the electronic screening near a charge modulation instability. The key new effect that we introduce is an additional mesoscopic disorder aiming to reproduce the inhomogeneities experimentally observed in scanning tunnelling microscopy. The crucial effect of this mesoscopic disorder is to give rise to point-like spectroscopic features, to be contrasted with the curve-like shape of the spectra previously calculated within the interfering-quasiparticle schemes. It is also found that stripe-like charge modulations play a relevant role to correctly reproduce all the spectral features of the experiments.

cond-mat.supr-con↗
arXiv2004

Phase Separation close to the density-driven Mott transition in the Hubbard-Holstein model

The density driven Mott transition is studied by means of Dynamical Mean-Field Theory in the Hubbard-Holstein model, where the Hubbard term leading to the Mott transition is supplemented by an electron-phonon (e-ph) term. We show that an intermediate e-ph coupling leads to a first-order transition at T=0, which is accompanied by phase separation between a metal and an insulator. The compressibility in the metallic phase is substantially enhanced. At quite larger values of the coupling a polaronic phase emerges coexisting with a non-polaronic metal.

cond-mat.str-el↗
arXiv2004

Doping-driven transition to a time-reversal breaking state in the phase diagram of the cuprates

Motivated by recent tunnelling and Andreev-reflection experiments, we study the conditions for a quantum transition within the superconducting phase of the cuprates,in which a bulk imaginary (time-reversal breaking) $id_{xy}$component appears in addition to the $d_{x^2 - y^2}$ order parameter. We examine in detail the role of some important physical features of the cuprates.In particular we show that a closed Fermi surface,a bilayer splitting, an orthorhombic distortion,and the proximity to a quantum critical point around optimal doping favor the appearance of the imaginary component. These findings could explain why the mixed $d_{x^2 - y^2}+ id_{xy}$ order parameter is observed in YBCO and LSCO, and suggest that it could appear also in Bi2212. We also predict that, in all cuprates, the mixed state should be stable only in a limited doping region all contained beneath the $d_{x^2 - y^2}$ dome. The behavior of the specific heat at the secondary transition is discussed.

cond-mat.supr-con↗
arXiv2003

A large-N analysis of the local quantum critical point and the spin-liquid phase

We study analytically the Kondo lattice model with an additional nearest-neighbor antiferromagnetic interaction in the framework of large-N theory. We find that there is a local quantum critical point between two phases, a normal Fermi-liquid and a spin-liquid in which the spins are decoupled from the conduction electrons. The local spin susceptibility displays a power-law divergence throughout the spin liquid phase. We check the reliability of the large-N results by solving by quantum Monte Carlo simulation the N=2 spin-liquid problem with no conduction electrons and find qualitative agreement. We show that the spin-liquid phase is unstable at low temperatures, suggestive of a first-order transition to an ordered phase.

cond-mat.str-el↗