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M. Hukkanen

Publications and source records attributed to M. Hukkanen.

At least 19 recordsLinked to original sources
arXiv2026

Island of Inversion in neutron-rich cobalt isotopes revealed from mass measurements

Mass measurements of the ground and isomeric states of $^{68-70}$Co have been performed using the JYFLTRAP Penning-trap mass spectrometer at the IGISOL facility. The masses were measured, either for the first time for the isomeric states of $^{68}$Co and $^{70}$Co, or with greatly improved precision for the others, removing ambiguities in the mass surface beyond $N=40$. The ordering of the low and high-spin states in $^{68}$Co and $^{70}$Co has also been established. The results, supported by Large-Scale Shell Model and Discrete Non-Orthogonal Shell-Model calculations, show a gradual lowering of intruder states with increasing neutron number, eventually leading to an inversion in $^{70}$Co. These findings clarify previously proposed contradictory interpretations. Finally, we demonstrate the importance of including induced effective 3N forces for a consistent description of binding energies in the island of inversion near $N=40$.

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arXiv2026

Study of $\boldsymbol{\beta}$ Decay Shape Factors in First-Forbidden Transitions with $\boldsymbol{\Delta I^\pi = 0^-}$ for Reactor Antineutrino Spectra Predictions

The electron spectra of the $\beta$ decays of $^{92}$Rb and $^{142}$Cs, key contributors to the reactor antineutrino spectrum, were measured at the IGISOL facility using radioactive beams of high isotopic purity. The shapes of the measured $\beta$ spectra were compared with various $\beta$ shape models, including first-forbidden correction factors for $\Delta I^\pi = 0^-$ ground-state to ground-state transitions. Comparisons with previous experimental results are also provided. The shapes of the newly measured $\beta$ spectra are well reproduced employing feedings extracted from total absorption gamma spectroscopy measurements.

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arXiv2025

Study of beta spectrum shapes relevant to the prediction of reactor antineutrino spectra

The shapes of the beta spectra of 92Rb and 142Cs, two of the beta decays most relevant for the prediction of the antineutrino spectrum in reactors, have been measured. A new setup composed of two dE-E telescopes has been used. High purity radioactive beams of the isotopes of interest were provided by the IGISOL facility using the JYFLTRAP double Penning trap. The resulting beta spectra have been compared with model predictions using beta decay feedings from total absorption gamma spectroscopy measurements and shape corrections employed in the calculation of the antineutrino spectrum, validating both further. The procedure can be extended to other relevant nuclei in the future, providing solid ground for the prediction of the antineutrino spectrum in reactors.

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arXiv2025

Two-proton correlations in the decay of 48Ni and 45Fe

The main observables of the rare two-proton emission process - half-life, total energy of the decay as well as energy and angular correlations between the emitted protons - have been measured for 48Ni and 45Fe in a recent experiment performed at the GANIL/LISE3 facility. The results, together with previous experimental work, are compared for the first time with calculations performed in the recently developed Gamow Coupled-Channel (GCC) framework and to 3-body predictions from literature. The comparison of the 48Ni and the 45Fe two-proton angular distributions with the GCC calculations confirms the adopted strength of the proton-proton interaction for both nuclei and the predominant small-angle emission. A comparison with 3-body model angular distributions indicates the shell closure of the f_7/2 orbital for 48Ni and a substantial occupancy of the p-orbital for 45Fe. Discrepancies between experimental data and theoretical predictions are found when studying the other observables: half-lives, total energy of the decay and energy correlations, showing the complexity of the description of the two-proton emission process.

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arXiv2025

$β$-delayed neutron spectroscopy of $^{85, 86}$As with MONSTER at IGISOL

The $β$-delayed neutron emission in the $^{85, 86}$As $β$-decays has been measured at the Ion Guide Isotope Separator On Line facility of the Accelerator Laboratory of the University of Jyväskylä. The complete $β$-decays have been studied with a complex setup that consists of a plastic scintillator for $β$-particles, MONSTER -- the MOdular Neutron time-of-flight SpectromeTER -- for neutrons, and a high-purity germanium and four LaBr$_3$ crystals for $γ$-rays. The $β$-delayed neutron energy distributions have been determined by unfolding the time-of-flight spectra with an innovative methodology based on the iterative Bayesian unfolding method and accurate Monte Carlo simulations. The results obtained for $^{85}$As are in excellent agreement with the existing evaluated data, validating the proposed methodology. In the case of $^{86}$As, a stronger neutron intensity at higher energies than previously predicted is discovered.

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arXiv2025

High-precision mass measurements of the ground and isomeric states in $^{124,125}$Ag

The masses of the ground and isomeric states in $^{124,125}$Ag have been measured using the phase-imaging ion-cyclotron-resonance technique at the JYFLTRAP double Penning trap mass spectrometer. The ground states of $^{124}$Ag and $^{125}$Ag were found to be 30(250) keV and 250(430) keV less bound but 36 and 110 times more precise than in the Atomic Mass Evaluation 2020, respectively. The excitation energy of $^{124}$Ag$^{m}$, ${E_x = 188.2(25)}$ keV, was determined for the first time. The new precise mass values have been utilised to study the evolution of nuclear structure via two-neutron separation energies. The impact on the astrophysical rapid neutron capture process has been investigated via neutron-capture reaction rate calculations. The precision measurements indicate a more linear trend in two-neutron separation energies and reduce the mass-related uncertainties for the neutron-capture rate of $^{124}$Ag$(n,γ)^{125}$Ag by a factor of around 100. The new mass values also improve the mass of $^{123}$Pd, previously measured using $^{124}$Ag as a reference.

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arXiv2025

Isomeric states of fission fragments explored via Penning trap mass spectrometry at IGISOL

The masses of $^{84}$Br, $^{105}$Mo, $^{115,119,121}$Pd, $^{122}$Ag, $^{127,129}$In, $^{132}$Sb and their respective isomeric states have been measured with the JYFLTRAP Penning trap mass spectrometer using the phase-imaging ion-cyclotron-resonance technique. The excitation energies of the isomeric states in $^{132}$Sb and $^{119}$Pd were experimentally determined for the first time, while for $^{84}$Br, $^{115}$Pd and $^{127,129}$In, the precision of the mass values was substantially improved. In $^{105}$Mo and $^{121}$Pd there were no signs of a long-lived isomeric state. The ground-state measurements of $^{119}$Pd and $^{122}$Ag indicated that both are significantly more bound than the literature values. For $^{122}$Ag, there was no indication of a proposed third long-lived state. The results for the $N=49$ nucleus $^{84}$Br and isomers close to doubly magic $^{132}$Sn have been compared to the shell-model and the microscopic quasiparticle-phonon model calculations.

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arXiv2024

Prominent bump in the two-neutron separation energies of neutron-rich lanthanum isotopes revealed by high-precision mass spectrometry

We report on high-precision atomic mass measurements of $^{148\text{-}153}$La and $^{151}$Ce performed with the JYFLTRAP double Penning trap using the Phase-Imaging Ion-Cyclotron-Resonance technique. The masses of $^{152,153}$La were experimentally determined for the first time. We confirm the sharp kink in the two-neutron separation energies at the neutron number ${N=93}$ in the cerium (${Z=58}$) isotopic chain. Our precision mass measurements of the most exotic neutron-rich lanthanum (${Z=57}$) isotopes reveal a sudden increase in two-neutron separation energies from ${N=92}$ to ${N=93}$. Unlike in the cerium isotopic chain, the kink is not sharp but extends to ${N=94}$ forming a prominent bump. The gain in energy is about 0.4 MeV, making it one of the strongest changes in two-neutron separation energies over the whole chart of nuclides, away from nuclear shell closures. The results call for further studies to elucidate the structure of neutron-rich lanthanum isotopes.

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arXiv2024

Binding energies, charge radii, spins and moments: odd-odd Ag isotopes and discovery of a new isomer

We report on the masses and hyperfine structure of ground and isomeric states in $^{114,116,118,120}$Ag isotopes, measured with the phase-imaging ion-cyclotron-resonance technique (PI-ICR) with the JYFLTRAP mass spectrometer and the collinear laser spectroscopy beamline at the Ion Guide Isotope Separator On-Line (IGISOL) facility, Jyväskylä, Finland. We measured the masses and excitation energies, electromagnetic moments, and charge radii, and firmly established the nuclear spins of the long-lived states. A new isomer was discovered in $^{118}$Ag and the half-lives of $^{118}$Ag long-lived states were reevaluated. We unambiguously pinned down the level ordering of all long-lived states, placing the inversion of the $I = 0^-$ and $I = 4^+$ states at $A = 118$ $(N = 71)$. Lastly, we compared the electromagnetic moments of each state to empirical single-particle moments to identify the dominant configuration where possible.

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arXiv2024

Probing the N=104 midshell region for the r process via precision mass spectrometry of neutron-rich rare-earth isotopes with the JYFLTRAP double Penning trap

We have performed high-precision mass measurements of neutron-rich rare-earth Tb, Dy and Ho isotopes using the Phase-Imaging Ion-Cyclotron-Resonance technique at the JYFLTRAP double Penning trap. We report on the first experimentally determined mass values for $^{169}$Tb, $^{170}$Dy and $^{171}$Dy, as well as the first high-precision mass measurements of $^{169}$Dy and $^{169\text{-}171}$Ho. For $^{170}$Ho, the two long-lived ground and isomeric states were resolved and their mass measured, yielding an isomer excitation energy of $E_\text{exc}=150.8(54)$~keV. In addition, we have performed independent crosschecks of previous Penning-trap values obtained for $^{167\text{,} 168}$Tb and $^{167\text{,} 168}$Dy. We have extended the systematics of two-neutron separation energies to the neutron midshell at $N=104$ in all of the studied isotopic chains. Our updated and new mass measurements provide better mass-related constraints for the neutron-capture reaction rates relevant to the astrophysical rapid neutron capture (r) process. The r-process abundances calculated with the new mass values seem to produce a steeper minimum at A=170 and differ by around 15-30\% from the abundances computed with the Atomic Mass Evaluation 2020 values.

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arXiv2024

High-precision Penning-trap mass measurements of Cd and In isotopes at JYFLTRAP remove the fluctuations in the two-neutron separation energies

We report on the first direct mass measurements of the $^{118,119}$Cd and $^{117-119}$In isotopes performed at the Ion Guide Isotope Separator On-Line facility using the JYFLTRAP double Penning trap mass spectrometer. The masses of $^{117}$In and $^{118}$Cd isotopes are in agreement with the literature, while $^{118,119}$In and $^{119}$Cd differ from literature by 49, 13 and 85 keV (6.1, 1.9 and 2.1 standard deviations), respectively. The excitation energy of the $^{118}$In first isomeric state, $E_x = 40.3(25)$ keV, was determined for the first time. The updated mass values removed the fluctuations observed in the two-neutron separation energies and lead to a smoother linear decrease of both isotopic chains. The $\log(ft)$ value for the $^{118}$Cd decay is also found to increase from 3.93(6) to 4.089(8). The reported results indicate an absence of significant structural changes around $N=70$.

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arXiv2024

Precision mass measurements in the zirconium region pin down the mass surface across the neutron midshell at $N=66$

Precision mass measurements of $^{104}$Y, $^{106}$Zr, $^{104,104m,109}$Nb, and $^{111,112}$Mo have been performed with the JYFLTRAP double Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line facility. The order of the long-lived states in $^{104}$Nb was unambiguously established. The trend in two-neutron separation energies around the $N=66$ neutron midshell appeared to be steeper with respect to the Atomic Mass Evaluation 2020 extrapolations for the $_{39}$Y and $_{40}$Zr isotopic chains and less steep for the $_{41}$Nb chain, indicating a possible gap opening around $Z=40$. The experimental results were compared to the BSkG2 model calculations performed with and without vibrational and rotational corrections. All of them predict two low-lying minima for $^{106}$Zr. While the unaltered BSkG2 model fails to predict the trend in two-neutron separation energies, selecting the more deformed minima in calculations and removing the vibrational correction, the calculations are more in line with experimental data. The same is also true for the $2^+_1$ excitation energies and differences in charge radii in the Zr isotopes. The results stress the importance of improved treatment of collective corrections in large-scale models and further development of beyond-mean-field techniques.

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arXiv2024

Mass measurements in the $^{132}$Sn region with the JYFLTRAP double Penning trap mass spectrometer

We report on new precision mass measurements of neutron-rich $^{137}$Sb and $^{136-142}$I isotopes from the JYFLTRAP double Penning trap mass spectrometer. We confirm the value from the previous Penning-trap measurement of $^{137}$Sb at the Canadian Penning Trap and therefore rule out the conflicting result from the Experimental Storage Ring. The ground state and isomer in $^{136}$I were resolved and measured directly for the first time. The isomer excitation energy, $E_x = 215.1(43)$ keV, agrees with the literature but is three times more precise. The measurements have improved the precision of the mass values and confirmed previous results in the majority of cases. However, for $^{138,140}$I the results differ by 17(6) keV and 23(12) keV, respectively. This could be explained by an unresolved contamination or different ratio of unresolved isomeric states in the case of $^{140}$I.

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arXiv2024

Direct high-precision measurement of the mass difference of $^{77}$As-$^{77}$Se related to neutrino mass determination

The first direct determination of the ground-state-to-ground-state ${β^{-}}$-decay $Q$-value of $^{77}$As to $^{77}$Se was performed by measuring their atomic mass difference utilizing the double Penning trap mass spectrometer, JYFLTRAP. The resulting $Q$-value is 684.463(70) keV, representing a remarkable 24-fold improvement in precision compared to the value reported in the most recent Atomic Mass Evaluation (AME2020). With the significant reduction of the uncertainty of the ground-state-to-ground-state $Q$-value and knowledge of the excitation energies in $^{77}$Se from $γ$-ray spectroscopy, the ground-state-to-excited-state $Q$-value of the transition $^{77}$As (3/2$^{-}$, ground state) $\rightarrow$ $^{77}$Se$^{*}$ (5/2$^{+}$, 680.1035(17) keV) was refined to be 4.360(70) keV. We confirm that this potential low $Q$-value ${β^{-}}$-decay transition for neutrino mass determination is energetically allowed at a confidence level of about 60$σ$. Nuclear shell-model calculations with two well-established effective Hamiltonians were used to estimate the partial half-life for the low $Q$-value transition. The half-life was found to be of the order of 10$^{9}$ years for this first-forbidden non-unique transition, which rules out this candidate a potential source for rare-event experiments searching for the electron antineutrino mass.

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arXiv2023

Precision mass measurement of $^{173}$Hf for nuclear structure of $^{173}$Lu and the $γ$ process

We report on the precise mass measurement of the $^{173}$Hf isotope performed at the Ion Guide Isotope Separator On-Line facility using the JYFLTRAP double Penning trap mass spectrometer. The new mass-excess value, ${\mathrm{ME} = -55390.8(30)}$ keV, is in agreement with the literature while being nine times more precise. The newly determined $^{173}$Hf electron-capture $Q$ value, $Q_{EC} = 1490.2(34)$ keV, allows us to firmly reject the population of an excited state at 1578 keV in $^{173}$Lu and 11 transitions tentatively assigned to the decay of $^{173}$Hf. Our refined mass value of $^{173}$Hf reduces mass-related uncertainties in the reaction rate of $^{174}$Hf$(γ,n)^{173}$Hf. Thus, the rate for the main photodisintegration destruction channel of the $p$ nuclide $^{174}$Hf in the relevant temperature region for the $γ$ process is better constrained.

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arXiv2023

Nuclear charge radius of $^{26m}$Al and its implication for V$_{ud}$ in the quark-mixing matrix

Collinear laser spectroscopy was performed on the isomer of the aluminium isotope $^{26m}$Al. The measured isotope shift to $^{27}$Al in the $3s^{2}3p\;^{2}\!P^\circ_{3/2} \rightarrow 3s^{2}4s\;^{2}\!S_{1/2}$ atomic transition enabled the first experimental determination of the nuclear charge radius of $^{26m}$Al, resulting in $R_c$=\qty{3.130\pm.015}{\femto\meter}. This differs by 4.5 standard deviations from the extrapolated value used to calculate the isospin-symmetry breaking corrections in the superallowed $β$ decay of $^{26m}$Al. Its corrected $\mathcal{F}t$ value, important for the estimation of $V_{ud}$ in the CKM matrix, is thus shifted by one standard deviation to \qty{3071.4\pm1.0}{\second}.

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arXiv2023

Binding energies of ground and isomeric states in neutron-rich ruthenium isotopes: measurements at JYFLTRAP and comparison to theory

We report on precision mass measurements of $^{113,115,117}$Ru performed with the JYFLTRAP double Penning trap mass spectrometer at the Accelerator Laboratory of University of Jyväskylä. The phase-imaging ion-cyclotron-resonance technique was used to resolve the ground and isomeric states in $^{113,115}$Ru and enabled for the first time a measurement of the isomer excitation energies, $E_x(^{113}$Ru$^{m})=100.5(8)$ keV and $E_x(^{115}$Ru$^{m})=129(5)$ keV. The ground state of $^{117}$Ru was measured using the time-of-flight ion-cyclotron-resonance technique. The new mass-excess value for $^{117}$Ru is around 36 keV lower and 7 times more precise than the previous literature value. With the more precise ground-state mass values, the evolution of the two-neutron separation energies is further constrained and a similar trend as predicted by the BSkG1 model is obtained up to the neutron number $N=71$.

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arXiv2023

High-precision measurements of low-lying isomeric states in $^{120-124}$In with JYFLTRAP double Penning trap

Neutron-rich $^{120-124}$In isotopes have been studied utilizing the double Penning trap mass spectrometer JYFLTRAP at the IGISOL facility. Using the phase-imaging ion-cyclotron-resonance technique, the isomeric states were resolved from ground states and their excitation energies measured with high precision in $^{121,123,124}$In. In $^{120,122}$In, the $1^+$ states were separated and their masses were measured while the energy difference between the unresolved $5^+$ and $8^-$ states, whose presence was confirmed by post-trap decay spectroscopy was determined to be $\leq15$ keV. In addition, the half-life of $^{122}$Cd, $T_{1/2} = 5.98(10)$ s, was extracted. Experimental results were compared with energy density functionals, density functional theory and shell-model calculations.

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