arXiv subjects

M. J. Biercuk

Publications and source records attributed to M. J. Biercuk.

At least 19 recordsLinked to original sources

arXiv2025

Experimental Quantum Simulation of Chemical Dynamics

Accurate simulation of dynamical processes in molecules and reactions is among the most challenging problems in quantum chemistry. Quantum computers promise efficient chemical simulation, but the existing quantum algorithms require many logical qubits and gates, placing practical applications beyond existing technology. Here, we carry out the first quantum simulations of chemical dynamics by employing a more hardware-efficient encoding scheme that uses both qubits and bosonic degrees of freedom. Our trapped-ion device accurately simulates the dynamics of non-adiabatic chemical processes, which are among the most difficult problems in computational chemistry because they involve strong coupling between electronic and nuclear motions. We demonstrate the programmability and versatility of our approach by simulating the dynamics of three different molecules as well as open-system dynamics in the condensed phase, all with the same quantum resources. Our approach requires orders of magnitude fewer resources than equivalent qubit-only quantum simulations, demonstrating the potential of using hybrid encoding schemes to accelerate quantum simulations of complex chemical processes, which could have applications in fields ranging from energy conversion and storage to biology and drug design.

quant-ph↗

arXiv2024

Universal Quantum Gate Set for Gottesman-Kitaev-Preskill Logical Qubits

The realisation of a universal quantum computer at scale promises to deliver a paradigm shift in information processing, providing the capability to solve problems that are intractable with conventional computers. A key limiting factor of realising fault-tolerant quantum information processing (QIP) is the large ratio of physical-to-logical qubits that outstrip device sizes available in the near future. An alternative approach proposed by Gottesman, Kitaev, and Preskill (GKP) encodes a single logical qubit into a single harmonic oscillator, alleviating this hardware overhead in exchange for a more complex encoding. Owing to this complexity, current experiments with GKP codes have been limited to single-qubit encodings and operations. Here, we report on the experimental demonstration of a universal gate set for the GKP code, which includes single-qubit gates and -- for the first time -- a two-qubit entangling gate between logical code words. Our scheme deterministically implements energy-preserving quantum gates on finite-energy GKP states encoded in the mechanical motion of a trapped ion. This is achieved by a novel optimal control strategy that dynamically modulates an interaction between the ion's spin and motion. We demonstrate single-qubit gates with a logical process fidelity as high as 0.960 and a two-qubit entangling gate with a logical process fidelity of 0.680. We also directly create a GKP Bell state from the oscillators' ground states in a single step with a logical state fidelity of 0.842. The overall scheme is compatible with existing hardware architectures, highlighting the opportunity to leverage optimal control strategies as a key accelerant towards fault tolerance.

quant-ph↗

arXiv2024

Robust and Deterministic Preparation of Bosonic Logical States in a Trapped Ion

Encoding logical qubits in bosonic modes provides a potentially hardware-efficient implementation of fault-tolerant quantum information processing. Here, we demonstrate high-fidelity and deterministic preparation of highly non-classical bosonic states in the mechanical motion of a trapped ion. Our approach implements error-suppressing pulses through optimized dynamical modulation of laser-driven spin-motion interactions to generate the target state in a single step. We demonstrate logical fidelities for the Gottesman-Kitaev-Preskill (GKP) state as high as $\bar{\mathcal{F}}=0.940(8)$, a distance-3 binomial state with an average fidelity of $\mathcal{F}=0.807(7)$, and a 12.91(5) dB squeezed vacuum state.

quant-ph↗

arXiv2023

Enhancing the sensitivity of atom-interferometric inertial sensors using robust control

Atom-interferometric quantum sensors could revolutionize navigation, civil engineering, and Earth observation. However, operation in real-world environments is challenging due to external interference, platform noise, and constraints on size, weight, and power. Here we experimentally demonstrate that tailored light pulses designed using robust control techniques mitigate significant error sources in an atom-interferometric accelerometer. To mimic the effect of unpredictable lateral platform motion, we apply laser-intensity noise that varies up to 20$\%$ from pulse-to-pulse. Our robust control solution maintains performant sensing, while the utility of conventional pulses collapses. By measuring local gravity, we show that our robust pulses preserve interferometer scale factor and improve measurement precision by 10$\times$ in the presence of this noise. We further validate these enhancements by measuring applied accelerations over a 200 $μg$ range up to 21$\times$ more precisely at the highest applied noise level. Our demonstration provides a pathway to improved atom-interferometric inertial sensing in real-world settings.

quant-ph↗

arXiv2021

Precision Characterization of the $^2$D$_{5/2}$ State and Quadratic Zeeman Coefficient in $^{171}$Yb$^+$

We report measurements of the branching fraction, hyperfine constant, and second-order Zeeman coefficient of the D$_{5/2}$ level in $^{171}$Yb$^+$ with up to two orders-of-magnitude improvement in precision compared to previously reported values. We estimate the electric quadrupole reduced matrix element of the S$_{1/2}$ $\leftrightarrow$ D$_{5/2}$ transition to be 12.5(4) $e a_0^2$. Furthermore, we determine the transition frequency of the F$_{7/2}$ $\leftrightarrow$ $^{1}$D$[3/2]_{3/2}$ at 760 nm with a $\sim$25-fold improvement in precision. These measurements provide benchmarks for quantum-many-body atomic-physics calculations and provide valuable data for efforts to improve quantum information processors based on Yb$^+$.

physics.atom-ph↗

arXiv2020

Scalable hyperfine qubit state detection via electron shelving in the ${}^2$D$_{5/2}$ and ${}^2$F$_{7/2}$ manifolds in ${}^{171}$Yb$^{+}$

Qubits encoded in hyperfine states of trapped ions are ideal for quantum computation given their long lifetimes and low sensitivity to magnetic fields, yet they suffer from off-resonant scattering during detection often limiting their measurement fidelity. In ${}^{171}$Yb$^{+}$ this is exacerbated by a low fluorescence yield, which leads to a need for complex and expensive hardware - a problematic bottleneck especially when scaling up the number of qubits. We demonstrate a detection routine based on electron shelving to address this issue in ${}^{171}$Yb$^{+}$ and achieve a 5.6$\times$ reduction in single-ion detection error on an avalanche photodiode to $1.8(2)\times10^{-3}$ in a 100 $μ$s detection period, and a 4.3$\times$ error reduction on an electron multiplying CCD camera, with $7.7(2)\times10^{-3}$ error in 400 $μ$s. We further improve the characterization of a repump transition at 760 nm to enable a more rapid reset of the auxiliary $^2$F$_{7/2}$ states populated after shelving. Finally, we examine the detection fidelity limit using the long-lived $^2$F$_{7/2}$ state, achieving a further 300$\times$ and 12$\times$ reduction in error to $6(7)\times10^{-6}$ and $6.3(3)\times10^{-4}$ in 1 ms on the respective detectors. While shelving-rate limited in our setup, we suggest various techniques to realize this detection method at speeds compatible with quantum information processing, providing a pathway to ultra-high fidelity detection in ${}^{171}$Yb$^{+}$.

quant-ph↗

arXiv2019

Dynamically corrected gates suppress spatio-temporal error correlations as measured by randomized benchmarking

Quantum error correction provides a path to large-scale quantum computers, but is built on challenging assumptions about the characteristics of the underlying errors. In particular, the mathematical assumption of statistically independent errors in quantum logic operations is at odds with realistic environments where error sources may exhibit strong temporal and spatial correlations. We present experiments using trapped ions to demonstrate that the use of dynamically corrected gates (DCGs), generally considered for the reduction of error magnitudes, can also suppress error correlations in space and time throughout quantum circuits. We present a first-principles analysis of the manifestation of error correlations in randomized benchmarking, and validate this model through experiments performed using engineered errors. We find that standard DCGs can reduce error correlations by $\sim50\times$, while increasing the magnitude of uncorrelated errors by a factor scaling linearly with the extended DCG duration compared to a primitive gate. We then demonstrate that the correlation characteristics of intrinsic errors in our system are modified by use of DCGs, consistent with a picture in which DCGs whiten the effective error spectrum induced by external noise.

quant-ph↗

arXiv2017

Measuring and Suppressing Error Correlations in Quantum Circuits

Quantum error correction provides a path to large-scale quantum computers, but is built on challenging assumptions about the characteristics of the underlying errors. In particular, the mathematical assumption of independent errors in quantum logic operations is at odds with realistic environments where error-sources may exhibit strong temporal correlations. We present experiments enabling the identification of error correlations between operations in quantum circuits, using only projective measurements at the end of the circuit. Using a single trapped ion qubit and engineered noise with tunable temporal correlations, we identify a clear signature of error correlations between sequential gates in randomly composed quantum circuits, and extract quantitative measures linked to the underlying noise correlation length. By replacing all gates in these circuits with "virtual" dynamically corrected gates (DCGs), we demonstrate that even in the presence of strongly correlated noise the signatures of error correlations between sequential gates appear similar to standard gates exposed to uncorrelated noise. A theoretical model applied to our experiments reveals that common DCGs suppress the correlated error component by over $270\times$ with $95\%$ confidence. Using block-correlated noise, we explore the scaling of the effective error correlation length at the virtual level, and show that DCGs exhibit error correlations indistinguishable from those arising from uncorrelated noise.

quant-ph↗

arXiv2017

Experimental quantum verification in the presence of temporally correlated noise

Growth in the complexity and capabilities of quantum information hardware mandates access to practical techniques for performance verification that function under realistic laboratory conditions. Here we experimentally characterise the impact of common temporally correlated noise processes on both randomised benchmarking (RB) and gate-set tomography (GST). We study these using an analytic toolkit based on a formalism mapping noise to errors for arbitrary sequences of unitary operations. This analysis highlights the role of sequence structure in enhancing or suppressing the sensitivity of quantum verification protocols to either slowly or rapidly varying noise, which we treat in the limiting cases of quasi-DC miscalibration and white noise power spectra. We perform experiments with a single trapped $^{171}$Yb$^{+}$ ion as a qubit and inject engineered noise ($\propto σ^z$) to probe protocol performance. Experiments on RB validate predictions that the distribution of measured fidelities over sequences is described by a gamma distribution varying between approximately Gaussian for rapidly varying noise, and a broad, highly skewed distribution for the slowly varying case. Similarly we find a strong gate set dependence of GST in the presence of correlated errors, leading to significant deviations between estimated and calculated diamond distances in the presence of correlated $σ^z$ errors. Numerical simulations demonstrate that expansion of the gate set to include negative rotations can suppress these discrepancies and increase reported diamond distances by orders of magnitude for the same error processes. Similar effects do not occur for correlated $σ^x$ or $σ^y$ errors or rapidly varying noise processes, highlighting the critical interplay of selected gate set and the gauge optimisation process on the meaning of the reported diamond norm in correlated noise environments.

quant-ph↗

arXiv2017

Application of optimal band-limited control protocols to quantum noise sensing

Industrial, metrological, and medical applications provide a strong technological pull for advanced nanoscale sensors exploiting the unique sensitivity of quantum coherent systems to their environments. Essential to the functionality of these devices is the availability of control protocols which shape the sensor's response to the environment in frequency space. However, a key challenge in these applications is that common control routines result in out-of-band spectral leakage which complicates interpretation of the sensor's signal. In this work we demonstrate provably optimal narrowband control protocols ideally suited to quantum sensing. Our results, based on experiments with trapped ions using modulation in the form of discrete prolate spheroidal sequences (aka Slepian functions), demonstrate reduction of spectral leakage by orders of magnitude over conventional controls. We tune the narrowband sensitivity using concepts from RF engineering and experimentally reconstruct complex noise spectra using engineered noise for quantitative performance evaluation. We then deploy these techniques to identify previously immeasurable frequency-resolved amplitude noise in our qubit synthesis chain with calibrated sensitivity better than 0.001 dB.

quant-ph↗

arXiv2016

A functional basis for efficient physical-layer classical control in quantum processors

The rapid progress seen in the development of quantum coherent devices for information processing has motivated serious consideration of quantum computer architecture and organization. One topic which remains open for investigation and optimization relates to the design of the classical-quantum interface, where control operations on individual qubits are applied according to higher-level algorithms; accommodating competing demands on performance and scalability remains a major outstanding challenge. In this work we present a resource-efficient, scalable framework for the implementation of embedded physical-layer classical controllers for quantum information systems. Design drivers and key functionalities are introduced, leading to the selection of Walsh functions as an effective functional basis for both programming and controller hardware implementation. This approach leverages the simplicity of real-time Walsh-function generation in classical digital hardware, and the fact that a wide variety of physical-layer controls such as dynamic error suppression are known to fall within the Walsh family. We experimentally implement a real-time FPGA-based Walsh controller producing Walsh timing signals and Walsh-synthesized analog waveforms appropriate for critical tasks in error-resistant quantum control and noise characterization. These demonstrations represent the first step towards a unified framework for the realization of physical-layer controls compatible with large-scale quantum information processing.

quant-ph↗

arXiv2016

The role of master clock stability in scalable quantum information processing

Experimentalists seeking to improve the coherent lifetimes of quantum bits have generally focused on mitigating decoherence mechanisms through, for example, improvements to qubit designs and materials, and system isolation from environmental perturbations. In the case of the phase degree of freedom in a quantum superposition, however, the coherence that must be preserved is not solely internal to the qubit, but rather necessarily includes that of the qubit relative to the "master clock" (e.g. a local oscillator) that governs its control system. In this manuscript we articulate the impact of instabilities in the master clock on qubit phase coherence, and provide tools to calculate the contributions to qubit error arising from these processes. We first connect standard oscillator phase-noise metrics to their corresponding qubit dephasing spectral densities. We then use representative lab-grade and performance-grade oscillator specifications to calculate operational fidelity bounds on trapped-ion and superconducting qubits with relatively slow and fast operation times. We discuss the relevance of these bounds for quantum error correction in contemporary experiments and future large-scale quantum information systems, and discuss potential means to improve master clock stability.

quant-ph↗

arXiv2016

Vibration-induced field fluctuations in a superconducting magnet

Superconducting magnets enable precise control of nuclear and electron spins, and are used in experiments that explore biological and condensed matter systems, and fundamental atomic particles. In high-precision applications, a common view is that that slow (<1 Hz) drift of the homogeneous magnetic field limits control and measurement precision. We report on previously undocumented higher-frequency field noise (10 Hz to 200 Hz) that limits the coherence time of 9Be+ electron-spin qubits in the 4.46 T field of a superconducting magnet. We measure a spin-echo T2 coherence time of ~6 ms for the 9Be+ electron-spin resonance at 124 GHz, limited by part-per-billion fractional fluctuations in the magnet's homogeneous field. Vibration isolation of the magnet improved T2 to ~50 ms.

quant-ph↗

arXiv2016

Analytically exploiting noise correlations inside the feedback loop to improve locked-oscillator performance

We introduce concepts from optimal estimation to the stabilization of precision frequency standards limited by noisy local oscillators. We develop a theoretical framework casting various measures for frequency standard variance in terms of frequency-domain transfer functions, capturing the effects of feedback stabilization via a time-series of Ramsey measurements. Using this framework we introduce a novel optimized hybrid predictive feedforward measurement protocol which employs results from multiple past measurements and transfer-function-based calculations of measurement covariance to improve the accuracy of corrections within the feedback loop. In the presence of common non-Markovian noise processes these measurements will be correlated in a calculable manner, providing a means to capture the stochastic evolution of the LO frequency during the measurement cycle. We present analytic calculations and numerical simulations of oscillator performance under competing feedback schemes and demonstrate benefits in both correction accuracy and long-term oscillator stability using hybrid feedforward. Simulations verify that in the presence of uncompensated dead time and noise with significant spectral weight near the inverse cycle time predictive feedforward outperforms traditional feedback, providing a path towards developing a new class of stabilization "software" routines for frequency standards limited by noisy local oscillators.

quant-ph↗

arXiv2014

Walsh-synthesized noise-filtering quantum logic

We study a novel class of open-loop control protocols constructed to perform arbitrary nontrivial single-qubit logic operations robust against time-dependent non-Markovian noise. Amplitude and phase modulation protocols are crafted leveraging insights from functional synthesis and the basis set of Walsh functions. We employ the experimentally validated generalized filter-transfer function formalism in order to find optimized control protocols for target operations in SU(2) by defining a cost function for the filter-transfer function to be minimized through the applied modulation. Our work details the various techniques by which we define and then optimize the filter-synthesis process in the Walsh basis, including the definition of specific analytic design rules which serve to efficiently constrain the available synthesis space. This approach yields modulated-gate constructions consisting of chains of discrete pulse-segments of arbitrary form, whose modulation envelopes possess intrinsic compatibility with digital logic and clocking. We derive novel families of Walsh-modulated noise filters designed to suppress dephasing and coherent amplitude-damping noise, and describe how well-known sequences derived in NMR also fall within the Walsh-synthesis framework. Finally, our work considers the effects of realistic experimental constraints such as limited modulation bandwidth on achievable filter performance.

quant-ph↗

arXiv2014

Phase-modulated decoupling and error suppression in qubit-oscillator systems

We present a scheme designed to suppress the dominant source of infidelity in entangling gates between quantum systems coupled through intermediate bosonic oscillator modes. Such systems are particularly susceptible to residual qubit-oscillator entanglement at the conclusion of a gate period which reduces the fidelity of the target entangling operation. We demonstrate how the exclusive use of discrete phase shifts in the field moderating the qubit-oscillator interaction - easily implemented with modern synthesizers - is sufficient to both ensure multiple oscillator modes are decoupled and to suppress the effects of fluctuations in the driving field. This approach is amenable to a wide variety of technical implementations including geometric phase gates in superconducting qubits and the Molmer-Sorensen gate for trapped ions. We present detailed example protocols tailored to trapped-ion experiments and demonstrate that our approach allows multiqubit gate implementation with a significant reduction in technical complexity relative to previously demonstrated protocols.

quant-ph↗

arXiv2014

Experimental noise filtering by quantum control

Instabilities due to extrinsic interference are routinely faced in systems engineering, and a common solution is to rely on a broad class of $\textit{filtering}$ techniques in order to afford stability to intrinsically unstable systems. For instance, electronic systems are frequently designed to incorporate electrical filters composed of, $\textit{e.g.}$ RLC components, in order to suppress the effects of out-of-band fluctuations that interfere with desired performance. Quantum coherent systems are now moving to a level of complexity where challenges associated with realistic time-dependent noise are coming to the fore. Unfortunately, standard control solutions involving feedback are generally impossible due to the strictures of quantum mechanics, and existing error-suppressing gate constructions generally rely on unphysical bang-bang controls or quasi-static error models that do not reflect realistic laboratory environments. In this work we use the theory of quantum control engineering and experiments with trapped $^{171}$Yb$^{+}$ ions to demonstrate the construction of novel $\textit{noise filters}$ which are specifically designed to mitigate the effect of realistic time-dependent fluctuations on qubits \emph{during useful operations}. Starting with desired filter characteristics and the Walsh basis functions, we use a combination of analytic design rules and numeric search to construct time-domain noise filters tailored to a desired state transformation. Our results validate the generalized filter-transfer function framework for arbitrary quantum control operations, and demonstrate that it can be leveraged as an effective and efficient tool for developing novel robust control protocols.

quant-ph↗

arXiv2014

Experimental bath engineering for quantitative studies of quantum control

We develop and demonstrate a technique to engineer universal unitary baths in quantum systems. Using the correspondence between unitary decoherence due to ambient environmental noise and errors in a control system for quantum bits, we show how a wide variety of relevant classical error models may be realized through In-Phase/Quadrature modulation on a vector signal generator producing a resonant carrier signal. We demonstrate our approach through high-bandwidth modulation of the 12.6 GHz carrier appropriate for trapped $^{171}$Yb$^{+}$ ions. Experiments demonstrate the reduction of coherent lifetime in the system in the presence of an engineered bath, with the observed $T_{2}$ scaling as predicted by a quantitative model described herein. These techniques form the basis of a toolkit for quantitative tests of quantum control protocols, helping experimentalists characterize the performance of their quantum coherent systems.

quant-ph↗