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M. J. Dolinski

Publications and source records attributed to M. J. Dolinski.

At least 19 recordsLinked to original sources

Characterization of CRYO ASIC for charge readout in the nEXO experiment

nEXO is a proposed next-generation experiment searching for the neutrinoless double beta decay of $^{136}$Xe using a tonne-scale liquid xenon (LXe) time projection chamber (TPC). To image the ionization signals from events in the liquid xenon, the detector will employ metallized fused-silica charge collection tiles instrumented with cryogenic application-specific integrated circuits (ASICs), referred to as CRYO ASIC, which are designed to operate directly in LXe to minimize input capacitance and pick-up noise. Here we present the performance of the CRYO ASIC mounted on an auxiliary printed circuit board and evaluated both in a cryogenic environmental chamber and in a dedicated LXe test stand. We demonstrate that the ASICs achieve the desired performance at liquid xenon temperatures, showing a gain stability better than 0.2% over 24-hour operation and reliable in-situ calibration using an on-chip pulser. In the LXe test stand, we show that boiling caused by the chip heat dissipation can be mitigated by operating the system above ~0.1 MPa. The in-LXe noise measured agrees with simulation, which indicates it the $150~e^-$ design requirement can be satisfied. These results establish CRYO ASIC as a viable low-noise in-LXe charge readout solution for nEXO.

physics.ins-det

Gamma Backgrounds for Experiments at the High Flux Isotope Reactor

This article describes the deployment of a germanium detector at Oak Ridge National Lab's High Flux Isotope Reactor (HFIR) for the purpose of understanding the energy and spatial distribution of the gamma field in the experiment hall where the Precision Reactor Oscillation and Spectrum Experiment (PROSPECT) took data and future neutrino experiments could be located. The sources from both the reactor and the neutron beamlines are described in detail, along with their temporal variations due to reactor power and their spatial variations due to the geometry of the beamlines and building materials in the vicinity. Additionally, a shielding study was performed to assess the amount that backgrounds in tens of keV range can be mitigated. This work helps inform backgrounds for future experiments at reactors such as IBD-based neutrino measurements and CEvNS measurements.

hep-ex

The nEXO Radioassay Program

Material radioactivity compilations, such as the one presented here, are important enablers of science. They are useful for the selection of radiopure materials used in the design and construction of low-energy rare-event search experiments. They allow researchers developing such experiments to save time on material studies and avoid costly duplication of effort. The data presented here were generated in support of the planned nEXO double-beta decay search. This work contains among the most restrictive constraints on the natural radioactivity content of materials of general interest to the low-radioactivity community, found in any tabulation of this kind. In this study, various techniques were employed; they are described here.

physics.ins-det

New Deep Learning Data Analysis Method for PROSPECT using GAPE: Genetic Algorithm Powered Evolution

We propose a genetic algorithm powered evolution (GAPE) method to create deep learning solutions for energy and position estimation for reactor antineutrino interactions in the Precision Reactor Oscillation and Spectrum Experiment (PROSPECT) at the highly enriched High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory. We also apply GAPE to create classification models to distinguish signatures of inverse beta decay (IBD) interactions of reactor antineutrinos from common background types. The GAPE method can also be adopted for optimization of other types of problems that utilize machine learning (ML) models for particle physics applications. When applied in the PROSPECT context, we find that the models selected by GAPE can, in some cases, outperform the traditional models previously used for PROSPECT data analysis. In particular, when benchmarked against conventional PROSPECT neutrino identification pathways using the same underlying information, the classifier offers the promise of improving the signal-to-background ratio by nearly 2.8 times. Performance biases uncovered during initial IBD classifier validation were primarily caused by differences in time-dependent response between background and signal training datasets. Biases were effectively mitigated through a data-period-specific training regimen, offering a pathway towards realizing an unbiased IBD signal classifier for future reactor neutrino datasets.

physics.data-an

Design of a high voltage delivery system for noble liquid time projection chambers

Noble liquid time projection chambers (TPCs) are a leading technology in the detection of ionizing radiation, particularly in applications such as accelerator neutrino physics, dark matter detection, and neutrinoless double beta decay. This paper addresses the design considerations for implementing stable high voltage (HV) systems within large noble liquid TPCs, with a focus on the nEXO experiment. Utilizing insights from prior HV research and experimental investigations, we outline factors influencing HV stability and discuss design choices to improve stability and prevent electrical discharges. A novel HV delivery system concept is presented, tailored for the nEXO TPC, which incorporates these design considerations while also meeting the stringent radiopurity requirements of the nEXO neutrinoless double beta decay search. These design considerations and their specific implementation towards a HV delivery system offer guidance to future experiments applying high voltage in noble liquid environments.

physics.ins-det

Search for Double Beta Decays of $^{134}$Xe with EXO-200 Phase II

EXO-200 was a leading double beta decay experiment consisting of a single-phase, enriched liquid xenon time projection chamber filled with an admixture of 80.672% $^{136}$Xe and 19.098% $^{134}$Xe. The detector operated at WIPP between 2010 and 2018 and was designed to search for double beta decay of $^{136}$Xe. Data was acquired in two phases separated by a period of detector upgrades. We report on the search for $0νββ$ and $2νββ$ decay of $^{134}$Xe with Phase II EXO-200 data, with median 90% C.L. exclusion sensitivity $T_{1/2}^{0ν} \geq 3.7\times 10^{23}$ yr and $T_{1/2}^{2ν} \geq 2.6 \times 10^{21}$ yr, respectively. No statistically significant signal is observed for either decay mode. We set a world-leading lower limit on the half-life of the neutrinoless decay mode of $^{134}$Xe of $T_{1/2}^{0ν} \geq 8.7\times10^{23}$ (90% C.L.) and the second strongest constraint on the two-neutrino decay of $T_{1/2}^{2ν} \geq 2.9\times10^{21}$ (90% C.L.), a 3-fold improvement over the EXO-200 Phase I measurement. New constraints are also set for the $2νββ$ and $0νββ$ decays of $^{134}$Xe to the lowest excited state of $^{134}$Ba.

nucl-ex

Final Search for Short-Baseline Neutrino Oscillations with the PROSPECT-I Detector at HFIR

The PROSPECT experiment is designed to perform precise searches for antineutrino disappearance at short distances (7 - 9~m) from compact nuclear reactor cores. This Letter reports results from a new neutrino oscillation analysis performed using the complete data sample from the PROSPECT-I detector operated at the High Flux Isotope Reactor in 2018. The analysis uses a multi-period selection of inverse beta decay neutrino interactions with reduced backgrounds and enhanced statistical power to set limits on electron-flavor disappearance caused by mixing with sterile neutrinos with 0.2 - 20 eV$^2$ mass splittings. Inverse beta decay positron energy spectra from six different reactor-detector distance ranges are found to be statistically consistent with one another, as would be expected in the absence of sterile neutrino oscillations. The data excludes at 95% confidence level the existence of sterile neutrinos in regions above 3~eV$^2$ previously unexplored by terrestrial experiments, including all space below 10~eV$^2$ suggested by the recently strengthened Gallium Anomaly. The best-fit point of the Neutrino-4 reactor experiment's claimed observation of short-baseline oscillation is ruled out at more than five standard deviations.

hep-ex

Ultra-pure Nickel for Structural Components of Low-Radioactivity Instruments

The next generation of rare-event search experiments in nuclear and particle physics demand structural materials combining exceptional mechanical strength with ultra-low levels of radioactive contamination. This study evaluates chemical vapor deposition (CVD) nickel as a candidate structural material for such applications. Manufacturer-supplied CVD Ni grown on aluminum substrates underwent tensile testing before and after welding alongside standard Ni samples. CVD Ni exhibited a planar tensile strength of ~600 MPa, significantly surpassing standard nickel. However, welding and heat treatment were found to reduce the tensile strength to levels comparable to standard Ni, with observed porosity in the welds likely contributing to this reduction. Material assay via inductively coupled plasma mass spectrometry (ICP-MS) employing isotope-dilution produced measured bulk concentration of 232-Th, 238-U, and nat-K at the levels of ~70 ppq, <100 ppq, and ~900 ppt, respectively, which is the lowest reported in nickel. Surface-etch profiling uncovered higher concentrations of these contaminants extending ~10 micrometer beneath the surface, likely associated with the aluminum growth substrate. The results reported are compared to the one other well documented usage of CVD Ni in a low radioactive background physics research experiment and a discussion is provided on how the currently reported results may arise from changes in CVD fabrication or testing process. These results establish CVD Ni as a promising low-radioactivity structural material, while outlining the need for further development in welding and surface cleaning techniques to fully realize its potential in large-scale, low radioactive background rare-event search experiments.

nucl-ex

Ultra-sensitive radon assay using an electrostatic chamber in a recirculating system

Rare event searches such as neutrinoless double beta decay and Weakly Interacting Massive Particle detection require ultra-low background detectors. Radon contamination is a significant challenge for these experiments, which employ highly sensitive radon assay techniques to identify and select low-emission materials. This work presents the development of ultra-sensitive electrostatic chamber (ESC) instruments designed to measure radon emanation in a recirculating gas loop, for future lower background experiments. Unlike traditional methods that separate emanation and detection steps, this system allows continuous radon transport and detection. This is made possible with a custom-built recirculation pump. A Python-based analysis framework, PyDAn, was developed to process and fit time-dependent radon decay data. Radon emanation rates are given for various materials measured with this instrument. A radon source of known activity provides an absolute calibration, enabling statistically-limited minimal detectable activities of 20 $μ$Bq. These devices are powerful tools for screening materials in the development of low-background particle physics experiments.

physics.ins-det

Machine Learning for Single-Ended Event Reconstruction in PROSPECT Experiment

The Precision Reactor Oscillation and Spectrum Experiment, PROSPECT, was a segmented antineutrino detector that successfully operated at the High Flux Isotope Reactor in Oak Ridge, TN, during its 2018 run. Despite challenges with photomultiplier tube base failures affecting some segments, innovative machine learning approaches were employed to perform position and energy reconstruction, and particle classification. This work highlights the effectiveness of convolutional neural networks and graph convolutional networks in enhancing data analysis. By leveraging these techniques, a 3.3\% increase in effective statistics was achieved compared to traditional methods, showcasing their potential to improve analysis performance. Furthermore, these machine learning methodologies offer promising applications for other segmented particle detectors, underscoring their versatility and impact.

physics.data-an

Sensitivity of nEXO to $^{136}$Xe Charged-Current Interactions: Background-free Searches for Solar Neutrinos and Fermionic Dark Matter

We study the sensitivity of nEXO to solar neutrino charged-current interactions, $ν_e + ^{136}$Xe$\rightarrow ^{136}$Cs$^* + e^-$, as well as analogous interactions predicted by models of fermionic dark matter. Due to the recently observed low-lying isomeric states of $^{136}$Cs, these interactions will create a time-delayed coincident signal observable in the scintillation channel. Here we develop a detailed Monte Carlo of scintillation emission, propagation, and detection in the nEXO detector to model these signals under different assumptions about the timing resolution of the photosensor readout. We show this correlated signal can be used to achieve background discrimination on the order of $10^{-9}$, enabling nEXO to make background-free measurements of solar neutrinos above the reaction threshold of 0.668 MeV. We project that nEXO could measure the flux of CNO solar neutrinos with a statistical uncertainty of 25%, thus contributing a novel and competitive measurement towards addressing the solar metallicity problem. Additionally, nEXO could measure the mean energy of the $^7$Be neutrinos with a precision of $σ\leq 1.5$ keV and could determine the survival probability of $^{7}$Be and $pep$ solar $ν_e$ with precision comparable to state-of-the-art. These quantities are sensitive to the Sun's core temperature and to non-standard neutrino interactions, respectively. Furthermore, the strong background suppression would allow nEXO to search for for charged-current interactions of fermionic dark matter in the mass range $m_χ$ = $0.668$-$7$ MeV with a sensitivity up to three orders of magnitude better than current limits.

nucl-ex

Supernova electron-neutrino interactions with xenon in the nEXO detector

Electron-neutrino charged-current interactions with xenon nuclei were modeled in the nEXO neutrinoless double-$β$ decay detector (~5 metric ton, 90% ${}^{136}$Xe, 10% ${}^{134}$Xe) to evaluate its sensitivity to supernova neutrinos. Predictions for event rates and detectable signatures were modeled using the Model of Argon Reaction Low Energy Yields (MARLEY) event generator. We find good agreement between MARLEY's predictions and existing theoretical calculations of the inclusive cross sections at supernova neutrino energies. The interactions modeled by MARLEY were simulated within the nEXO simulation framework and were run through an example reconstruction algorithm to determine the detector's efficiency for reconstructing these events. The simulated data, incorporating the detector response, were used to study the ability of nEXO to reconstruct the incident electron-neutrino spectrum and these results were extended to a larger xenon detector of the same isotope enrichment. We estimate that nEXO will be able to observe electron-neutrino interactions with xenon from supernovae as far as 5-8 kpc from Earth, while the ability to reconstruct incident electron-neutrino spectrum parameters from observed interactions in nEXO is limited to closer supernovae.

hep-ph

Reactor Antineutrino Directionality Measurement with the PROSPECT-I Detector

The PROSPECT-I detector has several features that enable measurement of the direction of a compact neutrino source. In this paper, a detailed report on the directional measurements made on electron antineutrinos emitted from the High Flux Isotope Reactor is presented. With an estimated true neutrino (reactor to detector) direction of $ϕ= 40.8\unicode{xB0} \pm 0.7\unicode{xB0}$ and $θ= 98.6\unicode{xB0} \pm 0.4\unicode{xB0}$, the PROSPECT-I detector is able to reconstruct an average neutrino direction of $ϕ= 39.4\unicode{xB0} \pm 2.9\unicode{xB0}$ and $θ= 97.6\unicode{xB0} \pm 1.6\unicode{xB0}$. This measurement is made with approximately 48000 Inverse Beta Decay signal events and is the most precise directional reconstruction of reactor antineutrinos to date.

nucl-ex

Imaging of single barium atoms in a second matrix site in solid xenon for barium tagging in a $^{136}$Xe double beta decay experiment

Neutrinoless double beta decay is one of the most sensitive probes for new physics beyond the Standard Model of particle physics. One of the isotopes under investigation is $^{136}$Xe, which would double beta decay into $^{136}$Ba. Detecting the single $^{136}$Ba daughter provides a sort of ultimate tool in the discrimination against backgrounds. Previous work demonstrated the ability to perform single atom imaging of Ba atoms in a single-vacancy site of a solid xenon matrix. In this paper, the effort to identify signal from individual barium atoms is extended to Ba atoms in a hexa-vacancy site in the matrix and is achieved despite increased photobleaching in this site. Abrupt fluorescence turn-off of a single Ba atom is also observed. Significant recovery of fluorescence signal lost through photobleaching is demonstrated upon annealing of Ba deposits in the Xe ice. Following annealing, it is observed that Ba atoms in the hexa-vacancy site exhibit antibleaching while Ba atoms in the tetra-vacancy site exhibit bleaching. This may be evidence for a matrix site transfer upon laser excitation. Our findings offer a path of continued research toward tagging of Ba daughters in all significant sites in solid xenon.

physics.atom-ph

Search for Two-neutrino Double-Beta Decay of $^{136}\rm Xe$ to the $0^+_1$ excited state of $^{136}\rm Ba$ with the Complete EXO-200 Dataset

A new search for two-neutrino double-beta ($2νββ$) decay of $^{136}\rm Xe$ to the $0^+_1$ excited state of $^{136}\rm Ba$ is performed with the full EXO-200 dataset. A deep learning-based convolutional neural network is used to discriminate signal from background events. Signal detection efficiency is increased relative to previous searches by EXO-200 by more than a factor of two. With the addition of the Phase II dataset taken with an upgraded detector, the median 90$\%$ confidence level half-life sensitivity of $2νββ$ decay to the $0^+_1$ state of $^{136}\rm Ba$ is $2.9 \times 10^{24}~\rm yr$ using a total $^{136}\rm Xe$ exposure of $234.1~\rm kg~yr$. No statistically significant evidence for $2νββ$ decay to the $0^+_1$ state is observed, leading to a lower limit of $T^{2ν}_{1/2}(0^+ \rightarrow 0^+_1) > 1.4\times10^{24}~\rm yr$ at 90$\%$ confidence level, improved by 70$\%$ relative to the current world's best constraint.

hep-ex

Final Measurement of the U235 Antineutrino Energy Spectrum with the PROSPECT-I Detector at HFIR

This Letter reports one of the most precise measurements to date of the antineutrino spectrum from a purely U235-fueled reactor, made with the final dataset from the PROSPECT-I detector at the High Flux Isotope Reactor. By extracting information from previously unused detector segments, this analysis effectively doubles the statistics of the previous PROSPECT measurement. The reconstructed energy spectrum is unfolded into antineutrino energy and compared with both the Huber-Mueller model and a spectrum from a commercial reactor burning multiple fuel isotopes. A local excess over the model is observed in the 5MeV to 7MeV energy region. Comparison of the PROSPECT results with those from commercial reactors provides new constraints on the origin of this excess, disfavoring at 2.2 and 3.2 standard deviations the hypotheses that antineutrinos from U235 are solely responsible and non-contributors to the excess observed at commercial reactors respectively.

nucl-ex

An integrated online radioassay data storage and analytics tool for nEXO

Large-scale low-background detectors are increasingly used in rare-event searches as experimental collaborations push for enhanced sensitivity. However, building such detectors, in practice, creates an abundance of radioassay data especially during the conceptual phase of an experiment when hundreds of materials are screened for radiopurity. A tool is needed to manage and make use of the radioassay screening data to quantitatively assess detector design options. We have developed a Materials Database Application for the nEXO experiment to serve this purpose. This paper describes this database, explains how it functions, and discusses how it streamlines the design of the experiment.

physics.ins-det

Generative Adversarial Networks for Scintillation Signal Simulation in EXO-200

Generative Adversarial Networks trained on samples of simulated or actual events have been proposed as a way of generating large simulated datasets at a reduced computational cost. In this work, a novel approach to perform the simulation of photodetector signals from the time projection chamber of the EXO-200 experiment is demonstrated. The method is based on a Wasserstein Generative Adversarial Network - a deep learning technique allowing for implicit non-parametric estimation of the population distribution for a given set of objects. Our network is trained on real calibration data using raw scintillation waveforms as input. We find that it is able to produce high-quality simulated waveforms an order of magnitude faster than the traditional simulation approach and, importantly, generalize from the training sample and discern salient high-level features of the data. In particular, the network correctly deduces position dependency of scintillation light response in the detector and correctly recognizes dead photodetector channels. The network output is then integrated into the EXO-200 analysis framework to show that the standard EXO-200 reconstruction routine processes the simulated waveforms to produce energy distributions comparable to that of real waveforms. Finally, the remaining discrepancies and potential ways to improve the approach further are highlighted.

hep-ex