arXiv subjects

M. J. Graf

Publications and source records attributed to M. J. Graf.

At least 37 records · Page 2Linked to original sources

arXiv2011

Competing Interactions and Magnetic Frustration in Yb4LiGe4

We have studied polycrystalline Yb4LiGe4, a ternary variant of the R5T4 family of layered compounds characterized by a very strong coupling between the magnetic and crystallographic degrees of freedom. The system is mixed valent, with non-magnetic Yb2+ and magnetic Yb3+ present, and is characterized by coexisting ferromagnetic and antiferromagnetic correlations. We present measurements of resistivity, AC-susceptibility, specific heat, and muon spin relaxation (muSR), below 1 K. The low temperature measurements suggest a transition to a mesoscopically inhomogeneous magnetically ordered state below 2 K characterized by fluctuations well below the ordering temperature. This unusual state is believed to result from the enhanced two-dimensionality produced by Li substitution and frustration effects inherent in the Yb sub-lattice geometry.

cond-mat.str-el↗

arXiv2011

Superconductivity of Bi Confined in an Opal Host

Superconductivity is observed in a composite of rhombohedral crystalline bismuth nanoparticles imbedded in an insulating porous opal host via electrical transport and AC magnetic susceptibility. The onset of superconductivity in this system occurs in two steps, with upper critical temperature Tc,U = 4.1 K and lower transition temperature of Tc,L = 0.7 K, which we attribute to the granular nature of the composite. The transition at Tc,U is observed to split into two transitions with the application of a magnetic field, and has upper critical field extrapolated to T = 0 K of Hc2,1(0) = 0.7 T and Hc2,2(0) = 1.0 T, corresponding to coherence lengths of xi1(0) = 21 nm and xi2(0) = 18 nm, respectively. We suggest that because of the lack of bulk-like states in the Bi nanoparticles due to confinement effects, superconductivity originates from surface states arising from Rashba spin-orbit scattering at the interface. This prospect suggests that nanostructured Bi may be an interesting system to search for Majorana fermions.

cond-mat.supr-con↗

arXiv2011

Thermoelectric prospects of nanomaterials with spin-orbit surface bands

Nanostructured composites and nanowire arrays of traditional thermoelectrics like Bi, Bi(1-x)Sb(x) and Bi(2)Te(3) have metallic Rashba surface spin-orbit bands featuring high mobilities rivaling that of the bulk for which topological insulator behavior has been proposed. Nearly pure surface electronic transport has been observed at low temperatures in Bi nanowires with diameter around the critical diameter, 50 nm, for the semimetal-to semiconductor transition. The surface contributes strongly to the thermopower, actually dominating for temperatures T < 100 K in these nanowires. The surface thermopower was found to be -1 T microvolt/(K^2), a value that is consistent with theory. We show that surface electronic transport together with boundary phonon scattering leads to enhanced thermoelectric performance at low temperatures of Bi nanowire arrays. We compare with bulk n-BiSb alloys, optimized CsBi(4)Te(6) and optimized Bi(2)Te(3). Surface dominated electronic transport can be expected in nanomaterials of the other traditional thermoelectrics.

cond-mat.mtrl-sci↗

arXiv2011

Interplay of Rotational, Relaxational, and Shear Dynamics in Solid 4He

Using a high-sensitivity torsional oscillator technique, we mapped the rotational and relaxational dynamics of solid helium-4 throughout the parameter range of the proposed supersolidity. We found evidence that the same microscopic excitations controlling the torsional oscillator motions are generated independently by thermal and mechanical stimulation. Moreover, a measure for the relaxation times of these excitations diverges smoothly without any indication for a critical temperature or critical velocity of a supersolid transition. Finally, we demonstrated that the combined temperature-velocity dependence of the TO response is indistinguishable from the combined temperature-strain dependence of the solid's shear modulus. This implies that the rotational responses of solid helium-4 attributed to supersolidity are associated with generation of the same microscopic excitations as those produced by direct shear strain.

cond-mat.other↗

arXiv2011

Electronic inhomogeneity in a Kondo lattice

Inhomogeneous electronic states resulting from entangled spin, charge, and lattice degrees of freedom are hallmarks of strongly correlated electron materials; such behavior has been observed in many classes of d-electron materials, including the high-Tc copper-oxide superconductors, manganites, and most recently the iron-pnictide superconductors. The complexity generated by competing phases in these materials constitutes a considerable theoretical challenge-one that still defies a complete description. Here, we report a new manifestation of electronic inhomogeneity in a strongly correlated f-electron system, using CeCoIn5 as an example. A thermodynamic analysis of its superconductivity, combined with nuclear quadrupole resonance measurements, shows that nonmagnetic impurities (Y, La, Yb, Th, Hg and Sn) locally suppress unconventional superconductivity, generating an inhomogeneous electronic "Swiss cheese" due to disrupted periodicity of the Kondo lattice. Our analysis may be generalized to include related systems, suggesting that electronic inhomogeneity should be considered broadly in Kondo lattice materials.

cond-mat.str-el↗

arXiv2011

Surface state band mobility and thermopower in semiconducting bismuth nanowires

Many thermoelectrics like Bi exhibit Rashba spin-orbit surface bands for which topological insulator behavior consisting of ultrahigh mobilities and enhanced thermopower has been predicted. Bi nanowires realize surface-only electronic transport since they become bulk insulators when they undergo the bulk semimetal-semiconductor transition as a result of quantum confinement for diameters close to 50 nm. We studied 20-, 30-, 50- and 200-nm trigonal Bi wires. Shubnikov-de Haas magnetoresistance oscillations caused by surface electrons and bulklike holes enable the determination of their densities and mobilities. Surface electrons have high mobilities exceeding 2(m^2)/(Vsec) and contribute strongly to the thermopower, dominating for temperatures T< 100 K. The surface thermopower is - 1.2 T microvolt/(K^2), a value that is consistent with theory, raising the prospect of developing nanoscale thermoelectrics based on surface bands.

cond-mat.mes-hall↗

arXiv2011

μSR Study of Spin Dynamics in LiY$_{1-x}$Ho$_{x}$F$_{4}$

We present zero-field μSR measurements for LiY$_{1-x}$Ho$_{x}$F$_{4}$ samples with x = 0.0017, 0.0085, 0.0406, and 0.0855. We characterize the dynamics associated with the formation of the (F-μ-F)$^{-1}$ complex by comparing our data to Monte Carlo simulations to determine the concentration range over which the spin dynamics are determined primarily by the Ho$^{3+}$-μ interaction rather than the F-μ interaction. Simulations show that F-μ-F oscillations should evolve into a Lorentzian Kubo-Toyabe decay for an increasing static magnetic field distribution Γ (i.e., increasing x), but the data do not show this behavior, consistent with the recently reported existence of strong magnetic fluctuations in this system at low temperatures. Anisotropy in the field distribution is shown to cause small errors of order 10% from behavior predicted for an isotropic distribution. Finally, numerical calculations show that values of Γ calculated in the single ion limit greatly exceed the values extracted from curve fits, suggesting that strong correlations play an important role in this system.

cond-mat.str-el↗

arXiv2011

Vortex-induced dissipation in narrow current-biased thin-film superconducting strips

A vortex crossing a thin-film superconducting strip from one edge to the other, perpendicular to the bias current, is the dominant mechanism of dissipation for films of thickness d on the order of the coherence length XI; and of width w much narrower than the Pearl length LAMBDA >> w >> XI. At high bias currents, I* < I < Ic, the heat released by the crossing of a single vortex suffices to create a belt-like normal-state region across the strip, resulting in a detectable voltage pulse. Here Ic is the critical current at which the energy barrier vanishes for a single vortex crossing. The belt forms along the vortex path and causes a transition of the entire strip into the normal state. We estimate I* to be roughly Ic/3. Further, we argue that such "hot" vortex crossings are the origin of dark counts in photon detectors, which operate in the regime of metastable superconductivity at currents between I* and Ic. We estimate the rate of vortex crossings and compare it with recent experimental data for dark counts. For currents below I*, i.e., in the stable superconducting but resistive regime, we estimate the amplitude and duration of voltage pulses induced by a single vortex crossing.

cond-mat.supr-con↗

arXiv2010

Spin and charge dynamics in [TbPc$_2$]$^0$ and [DyPc$_2$]$^0$ single molecule magnets

Magnetization, AC susceptibility and $μ$SR measurements have been performed in neutral phthalocyaninato lanthanide ([LnPc$_2]^0$) single molecule magnets in order to determine the low-energy levels structure and to compare the low-frequency spin excitations probed by means of macroscopic techniques, such as AC susceptibility, with the ones explored by means of techniques of microscopic character, such as $μ$SR. Both techniques show a high temperature thermally activated regime for the spin dynamics and a low temperature tunneling one. While in the activated regime the correlation times for the spin fluctuations estimated by AC susceptibility and $μ$SR basically agree, clear discrepancies are found in the tunneling regime. In particular, $μ$SR probes a faster dynamics with respect to AC susceptibility. It is argued that the tunneling dynamics probed by $μ$SR involves fluctuations which do not yield a net change in the macroscopic magnetization probed by AC susceptibiliy. Finally resistivity measurements in [TbPc$_2]^0$ crystals show a high temperature nearly metallic behaviour and a low temperature activated behaviour.

cond-mat.mes-hall↗

arXiv2009

NMR Studies of Field Induced Magnetism in CeCoIn$_5$

Recent Nuclear Magnetic Resonance and elastic neutron scattering experiments have revealed conclusively the presence of static incommensurate magnetism in the field-induced B phase of CeCoIn5. We analyze the NMR data assuming the hyperfine coupling to the In(2) nuclei is anisotropic and simulate the spectra for several different magnetic structures. The NMR data are consistent with ordered Ce moments along the [001] direction, but are relatively insensitive to the direction of the incommensurate wavevector.

cond-mat.str-el↗

arXiv2009

The glassy response of solid He-4 to torsional oscillations

We calculated the glassy response of solid He-4 to torsional oscillations assuming a phenomenological glass model. Making only a few assumptions about the distribution of glassy relaxation times in a small subsystem of otherwise rigid solid He-4, we can account for the magnitude of the observed period shift and concomitant dissipation peak in several torsion oscillator experiments. The implications of the glass model for solid He-4 are threefold: (1) The dynamics of solid He-4 is governed by glassy relaxation processes. (2) The distribution of relaxation times varies significantly between different torsion oscillator experiments. (3) The mechanical response of a torsion oscillator does not require a supersolid component to account for the observed anomaly at low temperatures, though we cannot rule out its existence.

cond-mat.mtrl-sci↗

arXiv2009

Uncovering the Hidden Order in URu2Si2 by Impurity Doping

We report the use of impurities to probe the hidden order parameter of the strongly correlated metal URu_2Si_2 below the transition temperature T_0 ~ 17.5 K. The nature of this order parameter has eluded researchers for more than two decades, but is accompanied by the development of a partial gap in the single particle density of states that can be detected through measurements of the electronic specific heat and nuclear spin-lattice relaxation rate. We find that impurities in the hidden order phase give rise to local patches of antiferromagnetism. An analysis of the coupling between the antiferromagnetism and the hidden order reveals that the former is not a competing order parameter but rather a parasitic effect of the latter.

cond-mat.str-el↗

arXiv2008

Torsional oscillators and the entropy dilemma of putative supersolid He-4

Solid He-4 is viewed as a nearly perfect Debye solid. Yet, recent calorimetry measurements by the PSU group (J. Low Temp. Phys. 138, 853 (2005) and Nature 449, 1025 (2007)) indicate that at low temperatures the specific heat has both cubic and linear contributions. These features appear in the same temperature range where measurements of the torsional oscillator period suggest a supersolid transition. We analyze the specific heat and compare the measured with the estimated entropy for a proposed supersolid transition with 1% superfluid fraction and find that the observed entropy is too small. We suggest that the low-temperature linear term in the specific heat is due to a glassy state that develops at low temperatures and is caused by a distribution of tunneling systems in the crystal. We propose that dislocation related defects produce those tunneling systems. Further, we argue that the reported putative mass decoupling, that means an increase in the oscillator frequency, is consistent with a glass-like transition. The glass scenario offers an alternative interpretation of the torsional oscillator experiments in contrast to the supersolid scenario of nonclassical rotational inertia.

cond-mat.mtrl-sci↗

arXiv2008

Observation of three-dimensional behavior in surface states of bismuth nanowires and the evidence for bulk Bi charge fractionalization

Whereas bulk bismuth supports very-high mobility, light, Dirac electrons and holes in its interior, its boundaries support a layer of heavy electrons in surface states formed by spin orbit interaction in the presence of the surface electric field. Small diameter d trigonal Bi nanowires (30 nm < d < 200 nm) were studied via magnetotransport at low temperatures and for fields up to 14 T in order to investigate the role of surfaces in electronic transport. A two-dimensional behavior was expected for surface charges; however we found instead a three-dimensional behavior, with a rich spectrum of Landau levels in a nearly spherical Fermi surface. This is associated with the long penetration length of surface states of trigonal wires. The prospect of the participation of surface transport and surface-induced relaxation of bulk carriers in the electronic properties of macroscopic samples is evaluated. We show that recent observations of magnetoquantum peaks in the Nernst thermopower coefficient, attributed to two-dimensional electron gas charge fractionalization, can be more plausibly interpreted in terms of these surface states.

cond-mat.str-el↗

arXiv2008

19F nuclear spin relaxation and spin diffusion effects in the single ion magnet LiYF4:Ho3+

Temperature and magnetic field dependences of the 19F nuclear spin-lattice relaxation in a single crystal of LiYF4 doped with holmium are described by an approach based on a detailed consideration of the magnetic dipole-dipole interactions between nuclei and impurity paramagnetic ions and nuclear spin diffusion processes. The observed non-exponential long time recovery of the nuclear magnetization after saturation at intermediate temperatures is in agreement with predictions of the spin-diffusion theory in a case of the diffusion limited relaxation. At avoided level crossings in the spectrum of electron-nuclear states of the Ho3+ ion, rates of nuclear spin-lattice relaxation increase due to quasi-resonant energy exchange between nuclei and paramagnetic ions, in contrast to the predominant role played by electronic cross-relaxation processes in the low-frequency ac-susceptibility.

cond-mat.other↗

arXiv2008

Pauli-limited upper critical field in dirty d-wave superconductors

We calculate the Pauli-limited upper critical field and the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) instability for {\it dirty} d-wave superconductors within the quasiclassical theory using the self-consistent $\hat{t}$-matrix approximation for impurities. We find that the phase diagram depends sensitively on the scattering rate and phase shift of nonmagnetic impurities. The transition into the superconducting state is always second order for weak (Born) scattering, while in the unitarity (strong) scattering limit a first-order transition into both uniform and spatially modulated superconducting states is stabilized. Contrary to general belief, we find that the FFLO phase is robust against disorder and survives impurity scattering equivalent to a $T_c$ suppression of roughly 40%. Our results bear on the search of FFLO states in heavy-fermion and layered organic superconductors.

cond-mat.supr-con↗

arXiv2008

Electronic Duality in Strongly Correlated Matter

Superconductivity develops from an attractive interaction between itinerant electrons that creates electron pairs which condense into a macroscopic quantum state--the superconducting state. On the other hand, magnetic order in a metal arises from electrons localized close to the ionic core and whose interaction is mediated by itinerant electrons. The dichotomy between local moment magnetic order and superconductivity raises the question of whether these two states can coexist and involve the same electrons. Here we show that the single 4f-electron of cerium in CeRhIn5 simultaneously produces magnetism, characteristic of localization, and superconductivity that requires itinerancy. The dual nature of the 4f-electron allows microscopic coexistence of antiferromagnetic order and superconductivity whose competition is tuned by small changes in pressure and magnetic field. Electronic duality contrasts with conventional interpretations of coexisting spin-density magnetism and superconductivity and offers a new avenue for understanding complex states in classes of materials.

cond-mat.str-el↗

arXiv2007

Muon spin rotation studies of spin dynamics at avoided level crossings in LiY0.998Ho0.002F4

We have studied the Ho3+ spin dynamics for LiY0.998Ho0.002F4 through the positive muon (mu+) transverse field depolarization rate lambda_TF as a function of temperature and magnetic field. We find sharp reductions in lambda_TF(H) at fields of 23, 46 and 69 mT, for which the Ho3+ ion system has field-induced (avoided) level crossings. The reduction scales with calculated level repulsions, suggesting that mu+ depolarization by slow fluctuations of non-resonant Ho3+ spin states is partially suppressed when resonant tunneling opens new fluctuation channels at frequencies much greater than the muon precession frequency.

cond-mat.mes-hall↗