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arXiv · 1110.0118

Competing Interactions and Magnetic Frustration in Yb4LiGe4

S. M. Disseler·J. N. Svensson·S. C. Peter·C. P. Byers·C. Baines·A. Amato·S. R. Giblin·P. Carretta·M. J. Graf
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Abstract

We have studied polycrystalline Yb4LiGe4, a ternary variant of the R5T4 family of layered compounds characterized by a very strong coupling between the magnetic and crystallographic degrees of freedom. The system is mixed valent, with non-magnetic Yb2+ and magnetic Yb3+ present, and is characterized by coexisting ferromagnetic and antiferromagnetic correlations. We present measurements of resistivity, AC-susceptibility, specific heat, and muon spin relaxation (muSR), below 1 K. The low temperature measurements suggest a transition to a mesoscopically inhomogeneous magnetically ordered state below 2 K characterized by fluctuations well below the ordering temperature. This unusual state is believed to result from the enhanced two-dimensionality produced by Li substitution and frustration effects inherent in the Yb sub-lattice geometry.

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S. M. Disseler, J. N. Svensson, S. C. Peter, C. P. Byers, C. Baines, A. Amato, S. R. Giblin, P. Carretta, M. J. Graf. 2011-10-01. Competing Interactions and Magnetic Frustration in Yb4LiGe4. https://doi.org/10.1103/physrevb.84.174429

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