arXiv subjects

M. Lang

Publications and source records attributed to M. Lang.

At least 19 recordsLinked to original sources

arXiv2026

The High-Energy Light Isotope eXperiment (HELIX) Instrument

The HELIX detector is a balloon-borne instrument designed to measure the flux of light (Z < 11) cosmic-ray isotopes. In this paper we describe the initial configuration of HELIX, optimized for measurements in the energy range from approximately 0.2 GeV per nucleon to beyond 3 GeV per nucleon. In addition to a spectrometer, which is based on a one-tesla superconducting magnet and a drift-chamber tracker, HELIX employs scintillator-based time-of-flight counters and a ring-imaging Cherenkov detector, allowing event-by-event reconstruction of primary particle mass, charge, and magnetic rigidity.

astro-ph.IM↗

arXiv2024

Persistence of small polarons into the superconducting phase of Ba$_{1-x}$K$_x$BiO$_3$

Bipolaronic superconductivity is an exotic pairing mechanism proposed for materials like Ba$_{1-x}$K$_x$BiO$_3$ (BKBO); however, conclusive experimental evidence for a (bi)polaron metallic state in this material remains elusive. Here, we combine resonant inelastic x-ray and neutron total scattering techniques with advanced modelling to study the local lattice distortions, electronic structure, and electron-phonon coupling ($e$-ph) in BKBO as a function of doping. Data for the parent compound ($x = 0$) indicates that the electronic gap opens in predominantly oxygen-derived states strongly coupled to a long-range ordered breathing distortion of the oxygen sublattice. Upon doping, short-range breathing distortions and sizable ($e$-ph) coupling persist into the superconducting regime ($x = 0.4$). Comparisons with exact diagonalization and determinant quantum Monte Carlo calculations further support this conclusion. Our results provide compelling evidence that BKBO's metallic phase hosts a liquid of small (bi)polarons derived from local breathing distortions of the lattice, with implications for understanding the low-temperature superconducting instability

cond-mat.supr-con↗

arXiv2024

Two-step growth of high-quality single crystals of the Kitaev magnet $\alpha$-RuCl$_{3}$

The layered honeycomb magnet $\alpha$-RuCl$_3$ is the most promising candidate for a Kitaev quantum spin liquid (KQSL) that can host charge-neutral Majorana fermions. Recent studies have shown significant sample dependence of thermal transport properties, which are a key probe of Majorana quasiparticles in the KQSL state, highlighting the importance of preparing high-quality single crystals of $\alpha$-RuCl$_3$. Here, we present a relatively simple and reliable method to grow high-quality single crystals of $\alpha$-RuCl$_3$. We use a two-step crystal growth method consisting of a purification process by chemical vapor transport (CVT) and a main crystal growth process by sublimation. The obtained crystals exhibit a distinct first-order structural phase transition from the monoclinic ($C2/m$) to the rhombohedral ($R\bar{3}$) structure at $\sim150$ K, which is confirmed by the nuclear quadrupole resonance spectra with much sharper widths than previously reported. The Raman spectra show the absence of defect-induced modes, supporting the good crystallinity of our samples. The jumps in the thermal expansion coefficient and specific heat at the antiferromagnetic (AFM) transition at 7.6-7.7 K are larger and sharper than those of previous samples grown by the CVT and Bridgman methods and do not show any additional AFM transitions at 10-14 K due to stacking faults. The longitudinal thermal conductivity in the AFM phase is significantly larger than previously reported, indicating a very long mean free path of heat carriers. All the results indicate that our single crystals are of superior quality with good crystallinity and few stacking faults, which provides a suitable platform for studying the Kitaev physics.

cond-mat.str-el↗

arXiv2023

The High Energy Light Isotope eXperiment program of direct cosmic-ray studies

HELIX is a new NASA-sponsored instrument aimed at measuring the spectra and composition of light cosmic-ray isotopes from hydrogen to neon nuclei, in particular the clock isotopes 10Be (radioactive, with 1.4 Myr lifetime) and 9Be (stable). The latter are unique markers of the production and Galactic propagation of secondary cosmic-ray nuclei, and are needed to resolve such important mysteries as the proportion of secondary positrons in the excess of antimatter observed by the AMS-02 experiment. By using a combination of a 1 T superconducting magnet spectrometer (with drift-chamber tracker) with a high-resolution time-of-flight detector system and ring-imaging Cherenkov detector, mass-resolved isotope measurements of light cosmic-ray nuclei will be possible up to 3 GeV/n in a first stratospheric balloon flight from Kiruna, Sweden to northern Canada, anticipated to take place in early summer 2024. An eventual longer Antarctic balloon flight of HELIX will yield measurements up to 10 GeV/n, sampling production from a larger volume of the Galaxy extending into the halo. We review the instrument design, testing, status and scientific prospects.

astro-ph.IM↗

arXiv2022

The new APD-Based Readout of the Crystal Barrel Calorimeter -- An Overview

The Crystal Barrel is an electromagnetic calorimeter consisting of 1380 CsI(Tl) scintillators, and is currently installed at the CBELSA/TAPS experiment where it is used to detect decay products from photoproduction of mesons. The readout of the Crystal Barrel has been upgraded in order to integrate the detector into the first level of the trigger and to increase its sensitivity for neutral final states. The new readout uses avalanche photodiodes in the front-end and a dual back-end with branches optimized for energy and time measurement, respectively. An FPGA-based cluster finder processes the whole hit pattern within less than 100 ns. The important downside of APDs -- the temperature dependence of their gain -- is handled with a temperature stabilization and a compensating bias voltage supply. Additionally, a light pulser system allows the APDs' gains to be measured during beamtimes.

physics.ins-det↗

arXiv2022

Characterization of electroless nickel-phosphorus plating for ultracold-neutron storage

Electroless nickel plating is an established industrial process that provides a robust and relatively low-cost coating suitable for transporting and storing ultracold neutrons (UCN). Using roughness measurements and UCN-storage experiments we characterized UCN guides made from polished aluminum or stainless-steel tubes plated by several vendors. All electroless nickel platings were similarly suited for UCN storage with an average loss probability per wall bounce of $2.8\cdot10^{-4}$ to $4.1\cdot10^{-4}$ for energies between 90 neV and 190 neV, or a ratio of imaginary to real Fermi potential $\eta$ of $1.7\cdot10^{-4}$ to $3.3\cdot10^{-4}$. Measurements at different elevations indicate that the energy dependence of UCN losses is well described by the imaginary Fermi potential. Some special considerations are required to avoid an increase in surface roughness during the plating process and hence a reduction in UCN transmission. Increased roughness had only a minor impact on storage properties. Based on these findings we chose a vendor to plate the UCN-production vessel that will contain the superfluid-helium converter for the new TRIUMF UltraCold Advanced Neutron (TUCAN) source, achieving acceptable UCN-storage properties with ${\eta=3.5(5)\cdot10^{-4}}$.

nucl-ex↗

arXiv2022

Polarization observables in double neutral pion photoproduction

Measurements of target asymmetries and double-polarization observables for the reaction $\gamma p\to p\pi^0\pi^0$ are reported. The data were taken with the CBELSA/TAPS experiment at the ELSA facility (Bonn University) using the Bonn frozen-spin butanol (C$_4$H$_9$OH) target, which provided transversely polarized protons. Linearly polarized photons were produced via bremsstrahlung off a diamond crystal. The data cover the photon energy range from $E_{\gamma}$=650 MeV to $E_{\gamma}$=2600 MeV and nearly the complete angular range. The results have been included in the BnGa partial wave analysis. Experimental results and the fit agree very well. Observed systematic differences in the branching ratios for decays of $N^*$ and $\Delta^*$ resonances are attributed to the internal structure of these excited nucleon states. Resonances which can be assigned to SU(6)$\times$O(3) two-oscillator configurations show larger branching ratios to intermediate states with non-zero intrinsic orbital angular momenta than resonances assigned to one-oscillator configurations.

nucl-ex↗

arXiv2022

Combined experimental and theoretical study of hydrostatic (He-gas) pressure effects in $\alpha$-RuCl$_3$

We report a detailed experimental and theoretical study on the effect of hydrostatic pressure on the structural and magnetic aspects of the layered honeycomb antiferromagent $\alpha$-RuCl$_{3}$. Magnetic susceptibility measurements performed under almost ideal hydrostatic-pressure conditions yield that the phase transition to zigzag-type antiferromagnetic order at $T_N$ = 7.3 K can be rapidly suppressed to about 6.1 K. A further suppression with increasing pressure is impeded due to the occurrence of a pressure-induced structural transition at $p \geq$ 104 MPa, accompanied by a strong dimerization of Ru-Ru bonds, which gives rise to a collapse of the magnetic susceptibility. Whereas the dimerization transition is strongly first order, as reflected by large discontinuous changes in $\chi$ and pronounced hysteresis effects, the magnetic transition under varying pressure and magnetic field also reveals indications for a weakly first-order transition. We assign this observation to a strong magnetoelastic coupling in this system. Measurements of $\chi$ under varying pressure in the paramagnetic regime ($T > T_N$) and before dimerization ($p <$ 100 MPa) reveal a considerable increase of $\chi$ with pressure. These experimental observations are consistent with the results of ab-initio Density Functional Theory (DFT) calculations on the pressure-dependent structure and the corresponding pressure-dependent magnetic model. Comparative susceptibility measurements on a second crystal showing two consecutive magnetic transitions instead of one, indicating the influence of stacking faults. Using different temperature-pressure protocols the effect of these stacking faults can be temporarily overcome, transforming the magnetic state from a multiple-$T_N$ into a single-$T_N$ state.

cond-mat.str-el↗

arXiv2022

A new benchmark of soft X-ray transition energies of Ne, CO$_2$, and SF$_6$: paving a pathway towards ppm accuracy

A key requirement for the correct interpretation of high-resolution X-ray spectra is that transition energies are known with high accuracy and precision. We investigate the K-shell features of Ne, CO$_2$, and SF$_6$ gases, by measuring their photo ion-yield spectra at the BESSY II synchrotron facility simultaneously with the 1s-np fluorescence emission of He-like ions produced in the Polar-X EBIT. Accurate ab initio calculations of transitions in these ions provide the basis of the calibration. While the CO$_2$ result agrees well with previous measurements, the SF$_6$ spectrum appears shifted by ~0.5 eV, about twice the uncertainty of the earlier results. Our result for Ne shows a large departure from earlier results, but may suffer from larger systematic effects than our other measurements. The molecular spectra agree well with our results of time-dependent density functional theory. We find that the statistical uncertainty allows calibrations in the desired range of 1-10 meV, however, systematic contributions still limit the uncertainty to ~40-100 meV, mainly due to the temporal stability of the monochromator energy scale. Combining our absolute calibration technique with a relative energy calibration technique such as photoelectron energy spectroscopy will be necessary to realize its full potential of achieving uncertainties as low as 1-10 meV.

astro-ph.IM↗

arXiv2021

Observation of a structure in the M$_{p\eta}$ invariant mass distribution near 1700 MeV/$c^2$ in the $\mathbf{\gamma p \rightarrow p \pi^0 \eta} $ reaction

The reaction $\gamma p \rightarrow p \pi^0 \eta$ has been studied with the CBELSA/TAPS detector at the electron stretcher accelerator ELSA in Bonn for incident photon energies from threshold up to 3.1 GeV. This paper has been motivated by the recently claimed observation of a narrow structure in the M$_{N\eta}$ invariant mass distribution at a mass of 1678 MeV/$c^2$. The existence of this structure cannot be confirmed in the present work. Instead, for E$_{\gamma}$ = 1400 - 1500 MeV and the cut M$_{p\pi^0} \le 1190 $ MeV/$c^2$ a statistically significant structure in the M$_{p\eta}$ invariant mass distribution near 1700 MeV/$c^2$ is observed with a width of $\Gamma\approx 35$ MeV/$c^2$ while the mass resolution is $\sigma_{res}$ = 5 MeV/$c^2$. Increasing the incident photon energy from 1420 to 1540 MeV this structure shifts in mass from $\approx$ 1700MeV/c$^2$ to $\approx$ 1725 MeV/$c^2$; the width increases to about 50 MeV/$c^2$ and decreases thereafter. The cross section associated with this structure reaches a maximum of $\approx$ 100 nb around E$_{\gamma} \approx$ 1490 MeV (W $\approx $ 1920 MeV), which coincides with the $p a_0$ threshold. Three scenarios are discussed which might be the origin of this structure in the M$_{p\eta}$ invariant mass distribution. The most likely interpretation is that it is due to a triangular singularity in the $\gamma p \rightarrow p a_0 \rightarrow p \pi^0 \eta$ reaction

nucl-ex↗

arXiv2021

Fluctuation driven height reduction of crosslinked polymer brushes

We study the changes in the conformations of brushes upon the addition of crosslinks between the chains using the bond fluctuation model. The Flory-Rehner model applied to uni-axially swollen networks predicts a collapse for large degrees of crosslinking $q$ proportional to $q^{-1/3}$ in disagreement with our simulation data. We show that the height reduction of the brushes is driven by monomer fluctuations in direction perpendicular to the grafting plane and not due to network elasticity. We observe that the impact of crosslinking is different for reactions between monomers of the same or on different chains. If the length reduction of the effective chain length due to both types of reactions is accounted for in a function $\beta(q)$, the height of the brush can be derived from a Flory approach for the equilibrium brush height leading to $H(q)\approx H_{b}\beta(q)^{1/3}$, whereby $H_{b}$ denotes the height of the non-crosslinked brush.

cond-mat.soft↗

arXiv2020

High-Precision Determination of Oxygen-K$\alpha$ Transition Energy Excludes Incongruent Motion of Interstellar Oxygen

We demonstrate a widely applicable technique to absolutely calibrate the energy scale of x-ray spectra with experimentally well-known and accurately calculable transitions of highly charged ions, allowing us to measure the K-shell Rydberg spectrum of molecular O$_2$ with 8 meV uncertainty. We reveal a systematic $\sim$450 meV shift from previous literature values, and settle an extraordinary discrepancy between astrophysical and laboratory measurements of neutral atomic oxygen, the latter being calibrated against the aforementioned O$_2$ literature values. Because of the widespread use of such, now deprecated, references, our method impacts on many branches of x-ray absorption spectroscopy. Moreover, it potentially reduces absolute uncertainties there to below the meV level.

physics.atom-ph↗

arXiv2019

Gamma-ray Emission of 60Fe and 26Al Radioactivities in our Galaxy

The isotopes $^{60}$Fe and $^{26}$Al originate from massive stars and their supernovae, reflecting ongoing nucleosynthesis in the Galaxy. We studied the gamma-ray emission from these isotopes at characteristic energies 1173, 1332, and 1809 keV with over 15 years of SPI data, finding a line flux in $^{60}$Fe combined lines of $(0.31\pm 0.06) \times 10^{-3}$ ph cm$^{-2}$ s$^{-1}$ and the $^{26}$Al line flux of $(16.8\pm 0.7) \times 10^{-4}$ ph cm$^{-2}$ s$^{-1}$ above the background and continuum emission for the whole sky. Based on the exponential-disk grid maps, we characterise the emission extent of $^{26}$Al to find scale parameters $R_0 =7.0^{+1.5}_{-1.0}$ kpc and $z_0=0.8^{+0.3}_{-0.2}$ kpc, however the $^{60}$Fe lines are too weak to spatially constrain the emission. Based on a point source model test across the Galactic plane, the $^{60}$Fe emission would not be consistent with a single strong point source in the Galactic center or somewhere else, providing a hint for a diffuse nature. We carried out comparisons of emission morphology maps using different candidate-source tracers for both $^{26}$Al and $^{60}$Fe emissions, and suggests that the $^{60}$Fe emission is more likely to be concentrated towards the Galactic plane. We determine the $^{60}$Fe/$^{26}$Al $γ$-ray flux ratio at $(18.4\pm4.2)\,\%$ , when using a parameterized spatial morphology model. Across the range of plausible morphologies, it appears possible that $^{26}$Al and $^{60}$Fe are distributed differently in the Galaxy. Using the best fitting maps for each of the elements, we constrain flux ratios in the range 0.2--0.4. We discuss its implications for massive star models and their nucleosynthesis.

astro-ph.HE↗

arXiv2019

Impurity Moments Conceal Low-Energy Relaxation of Quantum Spin Liquids

We scrutinize the magnetic properties of $\kappa$-(BEDT-TTF)$_2$Hg(SCN)$_2$Cl through its first-order metal-insulator transition at $T_{\rm CO}=30$ K by means of $^1$H nuclear magnetic resonance (NMR). While in the metal we find Fermi-liquid behavior with temperature-independent $(T_1T)^{-1}$, the relaxation rate exhibits a pronounced enhancement when charge order sets in. The NMR spectra remain unchanged through the transition and no magnetic order stabilizes down to 25 mK. Similar to the isostructural spin-liquid candidates $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ and $\kappa$-(BEDT-TTF)$_2$Ag$_2$(CN)$_3$, $T_1^{-1}$ acquires a dominant maximum (here around 5 K). Field-dependent experiments identify the low-temperature feature as a dynamic inhomogeneity contribution that is typically dominant over the intrinsic relaxation but gets suppressed with magnetic field.

cond-mat.str-el↗

arXiv2019

New data on $\vec{\gamma} \vec{p}\rightarrow \eta p$ with polarized photons and protons and their implications for $N^* \to N\eta$ decays

The polarization observables $T, E, P, H$, and $G$ in photoproduction of $\eta$ mesons off protons are measured for photon energies from threshold to $W=2400\,$MeV ($T$), 2280 MeV ($E$), 1620 MeV ($P, H$), or 1820 MeV ($G$), covering nearly the full solid angle. The data are compared to predictions from the SAID, MAID, J\"uBo, and BnGa partial-wave analyses. A refit within the BnGa approach including further data yields precise branching ratios for the $N\eta$ decay of nucleon resonances. A $N\eta$-branching ratio of $0.33\pm 0.04$ for $N(1650)1/2^-$ is found, which reduces the large and controversially discussed $N\eta$-branching ratio difference of the two lowest mass $J^P=1/2^-$-resonances significantly.

nucl-ex↗

arXiv2019

A fast-switching magnet serving a spallation-driven ultracold neutron source

A fast-switching, high-repetition-rate magnet and power supply have been developed for and operated at TRIUMF, to deliver a proton beam to the new ultracold neutron (UCN) facility. The facility possesses unique operational requirements: a time-averaged beam current of 40~$μ$A with the ability to switch the beam on or off for several minutes. These requirements are in conflict with the typical operation mode of the TRIUMF cyclotron which delivers nearly continuous beam to multiple users. To enable the creation of the UCN facility, a beam-sharing arrangement with another facility was made. The beam sharing is accomplished by the fast-switching (kicker) magnet which is ramped in 50~$μ$s to a current of 193~A, held there for approximately 1~ms, then ramped down in the same short period of time. This achieves a 12~mrad deflection which is sufficient to switch the proton beam between the two facilities. The kicker magnet relies on a high-current, low-inductance coil connected to a fast-switching power supply that is based on insulated-gate bipolar transistors (IGBTs). The design and performance of the kicker magnet system and initial beam delivery results are reported.

physics.acc-ph↗

arXiv2019

Measurement of the Helicity Asymmetry $E$ for the reaction $ γp\to π^0 p$

A measurement of the double-polarization observable $E$ for the reaction $γp\to π^0 p$ is reported. The data were taken with the CBELSA/TAPS experiment at the ELSA facility in Bonn using the Bonn frozen-spin butanol (C$_4$H$_9$OH) target, which provided longitudinally-polarized protons. Circularly-polarized photons were produced via bremsstrahlung of longitudinally-polarized electrons. The data cover the photon energy range from $E_γ=600$~MeV to $E_γ=2310$~MeV and nearly the complete angular range. The results are compared to and have been included in recent partial wave analyses.

nucl-ex↗

arXiv2019

Magneto-structural properties of the layered quasi-2D triangular-lattice antiferromagnets Cs$_2$CuCl$_{4-x}$Br$_x$ for ${x}$ = 0,1,2 and 4

We present a study of the magnetic susceptibility $χ_{mol}$ under variable hydrostatic pressure on single crystals of Cs$_2$CuCl$_{4-x}$Br$_x$. This includes the border compounds \textit{x} = 0 and 4, known as good realizations of the distorted triangular-lattice spin-1/2 Heisenberg antiferromagnet, as well as the isostructural stoichiometric systems Cs$_2$CuCl$_{3}$Br$_1$ and Cs$_2$CuCl$_{2}$Br$_2$. For the determination of the exchange coupling constants $J$ and $J^{\prime}$, $χ_{mol}$ data were fitted by a $J-J^{\prime}$ model \cite{Schmidt2015}. Its application, validated for the border compounds, yields a degree of frustration $J^{\prime}$/$J$ = 0.47 for Cs$_2$CuCl$_3$Br$_1$ and $J^{\prime}$/$J$ $\simeq$ 0.63 - 0.78 for Cs$_2$CuCl$_2$Br$_2$, making these systems particular interesting representatives of this family. From the evolution of the magnetic susceptibility under pressure up to about 0.4\,GPa, the maximum pressure applied, two observations were made for all the compounds investigated here. First, we find that the overall energy scale, given by $J_c = (J^2$ + $J^{\prime 2}$)$^{1/2}$, increases under pressure, whereas the ratio $J^{\prime}$/$J$ remains unchanged in this pressure range. These experimental observations are in accordance with the results of DFT calculations performed for these materials. Secondly, for the magnetoelastic coupling constants, extraordinarily small values are obtained. We assign these observations to a structural peculiarity of this class of materials.

cond-mat.str-el↗