arXiv subjects

M. Lang

Publications and source records attributed to M. Lang.

At least 37 records · Page 2Linked to original sources

arXiv2019

Specific Heat Study of 1D and 2D Excitations in the Layered Frustrated Quantum Antiferromagnets Cs$_2$CuCl$_{4-x}$Br$_x$

We report an experimental and theoretical study of the low-temperature specific heat $C$ and magnetic susceptibility $χ$ of the layered anisotropic triangular-lattice spin-1/2 Heisenberg antiferromagnets Cs$_2$CuCl$_{4-x}$Br$_x$ with $x$ = 0, 1, 2, and 4. We find that the ratio $J'/J$ of the exchange couplings ranges from 0.32 to $\approx 0.78$, implying a change (crossover or quantum phase transition) in the materials' magnetic properties from one-dimensional (1D) behavior for $J'/J < 0.6$ to two-dimensional (2D) behavior for $J'/J \approx 0.78$ behavior. For $J'/J < 0.6$, realized for $x$ = 0, 1, and 4, we find a magnetic contribution to the low-temperature specific heat, $C_{\rm m} \propto T$, consistent with spinon excitations in 1D spin-1/2 Heisenberg antiferromagnets. Remarkably, for $x$ = 2, where $J'/J \approx 0.78$ implies a 2D magnatic character, we also observe $C_{\rm m} \propto T$. This finding, which contrasts the prediction of $C_{\rm m} \propto T^2$ made by standard spin-wave theories, shows that Fermi-like statistics also plays a significant role for the magnetic excitations in frustrated spin-1/2 2D antiferromagnets.

cond-mat.str-el↗

arXiv2018

A beamline for fundamental neutron physics at TRIUMF

This article describes the new primary proton beamline 1U at TRIUMF. The purpose of this beamline is to produce ultracold neutrons (UCN) for fundamental-physics experiments. It delivers up to 40 microA of 480 MeV protons from the TRIUMF cyclotron to a tungsten spallation target and uses a fast kicker to share the beam between the Center for Molecular and Materials Science and UCN. The beamline has been successfully commissioned and operated with a beam current up to 10 microA, facilitating first large-scale UCN production in Canada.

physics.ins-det↗

arXiv2018

First ultracold neutrons produced at TRIUMF

We installed a source for ultracold neutrons at a new, dedicated spallation target at TRIUMF. The source was originally developed in Japan and uses a superfluid-helium converter cooled to 0.9$\,$K. During an extensive test campaign in November 2017, we extracted up to 325000 ultracold neutrons after a one-minute irradiation of the target, over three times more than previously achieved with this source. The corresponding ultracold-neutron density in the whole production and guide volume is 5.3$\,$cm$^{-3}$. The storage lifetime of ultracold neutrons in the source was initially 37$\,$s and dropped to 24$\,$s during the eighteen days of operation. During continuous irradiation of the spallation target, we were able to detect a sustained ultracold-neutron rate of up to 1500$\,$s$^{-1}$. Simulations of UCN production, UCN transport, temperature-dependent UCN yield, and temperature-dependent storage lifetime show excellent agreement with the experimental data and confirm that the ultracold-neutron-upscattering rate in superfluid helium is proportional to $T^7$.

physics.ins-det↗

arXiv2018

The η'-carbon potential at low meson momenta

The production of $η^\prime$ mesons in coincidence with forward-going protons has been studied in photon-induced reactions on $^{12}$C and on a liquid hydrogen (LH$_2$) target for incoming photon energies of 1.3-2.6 GeV at the electron accelerator ELSA. The $η^\prime$ mesons have been identified via the $η^\prime\rightarrow π^0 π^0η\rightarrow 6 γ$ decay registered with the CBELSA/TAPS detector system. Coincident protons have been identified in the MiniTAPS BaF$_2$ array at polar angles of $2^{\circ} \le θ_{p} \le 11^{\circ}$. Under these kinematic constraints the $η^\prime$ mesons are produced with relatively low kinetic energy ($\approx$ 150 MeV) since the coincident protons take over most of the momentum of the incident-photon beam. For the C-target this allows the determination of the real part of the $η^\prime$-carbon potential at low meson momenta by comparing with collision model calculations of the $η^\prime$ kinetic energy distribution and excitation function. Fitting the latter data for $η^\prime$ mesons going backwards in the center-of-mass system yields a potential depth of V = $-$(44 $\pm$ 16(stat)$\pm$15(syst)) MeV, consistent with earlier determinations of the potential depth in inclusive measurements for average $η^\prime$ momenta of $\approx$ 1.1 GeV/$c$. Within the experimental uncertainties, there is no indication of a momentum dependence of the $η^\prime$-carbon potential. The LH$_2$ data, taken as a reference to check the data analysis and the model calculations, provide differential and integral cross sections in good agreement with previous results for $η^\prime$ photoproduction off the free proton.

nucl-ex↗

arXiv2018

Relaxation dynamics in the one-dimensional organic charge-transfer salt δ-(EDT-TTF-CONMe$_2$)$_2$Br

A detailed investigation of the charge-ordered charge-transfer salt δ-(EDT-TTF-CONMe$_{2}$)$_{2}$Br by thermal-expansion measurements and dielectric spectroscopy reveals three dynamic processes of relaxational character. The slowest one exhibits the characteristics of glassy freezing and is ascribed to the conformational dynamics of terminal ethylene groups of the organic molecules. Such a process was previously found for related charge-transfer salts where, however, the anions form polymerlike chains, in contrast to the spherical anions of the present material. Dielectric spectroscopy reveals two additional relaxational processes. The characteristics of the faster one are consistent with excitations of a one-dimensional Wigner lattice as recently observed in this material by infrared spectroscopy, which are also accompanied by conformational changes of the molecules. However, at low temperature the ethylene-group relaxation exhibits the cooperativity-induced dramatic slowing down that is typical for glassy freezing, while the defect-related Wigner-lattice excitation follows thermally activated behavior as expected for single-dipole relaxations.

cond-mat.str-el↗

arXiv2017

Kondo-like phonon scattering in thermoelectric clathrates

Crystalline solids are generally known as excellent heat conductors, amorphous materials or glasses as thermal insulators. It has thus come as a surprise that certain crystal structures defy this paradigm. A prominent example are type-I clathrates and other materials with guest-host structures. They sustain low-energy Einstein-like modes in their phonon spectra, but are also prone to various types of disorder and phonon-electron scattering and thus the mechanism responsible for their ultralow thermal conductivities has remained elusive. While recent ab initio lattice dynamics simulations show that the Einstein-like modes enhance phonon-phonon Umklapp scattering, they reproduce experimental data only at low temperatures. Here we show that a new effect, an "all phononic Kondo effect", can resolve this discrepancy. This is evidenced by our thermodynamic and transport measurements on various clathrate single crystal series and their comparison with ab initio simulations. Our new understanding devises design strategies to further suppress the thermal conductivity of clathrates and other related materials classes, with relevance for the field of thermoelectric waste heat recovery but also more generally for phononic applications. More fundamentally, it may trigger theoretical work on strong correlation effects in phonon systems.

cond-mat.str-el↗

arXiv2017

Sensitivity of Fields Generated within Magnetically Shielded Volumes to Changes in Magnetic Permeability

Future experiments seeking to measure the neutron electric dipole moment (nEDM) require stable and homogeneous magnetic fields. Normally these experiments use a coil internal to a passively magnetically shielded volume to generate the magnetic field. The stability of the magnetic field generated by the coil within the magnetically shielded volume may be influenced by a number of factors. The factor studied here is the dependence of the internally generated field on the magnetic permeability $μ$ of the shield material. We provide measurements of the temperature-dependence of the permeability of the material used in a set of prototype magnetic shields, using experimental parameters nearer to those of nEDM experiments than previously reported in the literature. Our measurements imply a range of $\frac{1}μ\frac{dμ}{dT}$ from 0-2.7\%/K. Assuming typical nEDM experiment coil and shield parameters gives $\fracμ{B_0}\frac{dB_0}{dμ}=0.01$, resulting in a temperature dependence of the magnetic field in a typical nEDM experiment of $\frac{dB_0}{dT}=0-270$~pT/K for $B_0=1~μ$T. The results are useful for estimating the necessary level of temperature control in nEDM experiments.

physics.ins-det↗

arXiv2017

Photoproduction of eta mesons from the neutron: cross sections and double polarization observable E

Photoproduction of $η$ mesons from neutrons} \abstract{Results from measurements of the photoproduction of $η$ mesons from quasifree protons and neutrons are summarized. The experiments were performed with the CBELSA/TAPS detector at the electron accelerator ELSA in Bonn using the $η\to3π^{0}\to6γ$ decay. A liquid deuterium target was used for the measurement of total cross sections and angular distributions. The results confirm earlier measurements from Bonn and the MAMI facility in Mainz about the existence of a narrow structure in the excitation function of $γn\rightarrow nη$. The current angular distributions show a forward-backward asymmetry, which was previously not seen, but was predicted by model calculations including an additional narrow $P_{11}$ state. Furthermore, data obtained with a longitudinally polarized, deuterated butanol target and a circularly polarized photon beam were analyzed to determine the double polarization observable $E$. Both data sets together were also used to extract the helicity dependent cross sections $σ_{1/2}$ and $σ_{3/2}$. The narrow structure in the excitation function of $γn\rightarrow nη$ appears associated with the helicity-1/2 component of the reaction.

nucl-ex↗

arXiv2017

Many-body theory of magneto-elasticity in one dimension

We construct a many-body theory of magneto-elasticity in one dimension and show that the dynamical correlation functions of the quantum magnet, connecting the spins with phonons, involve all energy scales. Accounting for all magnetic states non-perturbatively via the exact diagonalisation techniques of Bethe ansatz, we find that the renormalisation of the phonon velocity is a non-monotonous function of the external magnetic field and identify a new mechanism for attenuation of phonons - via hybridisation with the continuum of excitations at high energy. We conduct ultrasonic measurements on a high-quality single crystal of the frustrated spin-1/2 Heisenberg antiferromagnet $\textrm{Cs}_{2}\textrm{CuCl}_{4}$ in its one-dimensional regime and confirm the theoretical predictions, demonstrating that ultrasound can be used as a powerful probe of strong correlations in one dimension.

cond-mat.mes-hall↗

arXiv2016

Momentum dependence of the imaginary part of the $ω$- and $η^\prime$-nucleus optical potential

The photoproduction of $ω$ and $η^\prime$ mesons off carbon and niobium nuclei has been measured as a function of the meson momentum for incident photon energies of 1.2-2.9 GeV at the electron accelerator ELSA. The mesons have been identified via the $ω\rightarrow π^0 γ\rightarrow 3 γ$ and $η^\prime\rightarrow π^0 π^0η\rightarrow 6 γ$ decays, respectively, registered with the CBELSA/TAPS detector system. From the measured meson momentum distributions the momentum dependence of the transparency ratio has been determined for both mesons. Within a Glauber analysis the in-medium $ω$ and $η^\prime$ widths and the corresponding absorption cross sections have been deduced as a function of the meson momentum. The results are compared to recent theoretical predictions for the in-medium $ω$ width and $η^\prime$-N absorption cross sections. The energy dependence of the imaginary part of the $ω$- and $η^\prime$-nucleus optical potential has been extracted. The finer binning of the present data compared to the existing data allows a more reliable extrapolation towards the production threshold. The modulus of the imaginary part of the $η^\prime$ nucleus potential is found to be about three times smaller than recently determined values of the real part of the $η^\prime$-nucleus potential, which makes the $η^\prime$ meson a suitable candidate for the search for meson-nucleus bound states. For the $ω$ meson, the modulus of the imaginary part near threshold is comparable to the modulus of the real part of the potential. As a consequence, only broad structures can be expected which makes the observation of $ω$ mesic states very difficult experimentally.

nucl-ex↗

arXiv2016

Determination of the real part of the η'-Nb optical potential

The excitation function and momentum distribution of η' mesons have been measured in photoproduction off 93^Nb in the energy range of 1.2-2.9 GeV. The experiment has been performed with the combined Crystal Barrel and MiniTAPS detector system, using tagged photon beams from the ELSA electron accelerator. Information on the sign and magnitude of the real part of the η'-Nb potential has been extracted from a comparison of the data with model calculations. An attractive potential of -(41 \pm 10(stat) \pm 15(syst)) MeV depth at normal nuclear matter density is deduced within model uncertainties. This value is consistent with the potential depth of -(37 \pm 10(stat) \pm 10(syst)) MeV obtained in an earlier measurement for a light nucleus (carbon). This relatively shallow η'-nucleus potential will make the search for η'-nucleus bound states more difficult.

nucl-ex↗

arXiv2016

Magneto-acoustic study near the quantum critical point of the frustrated quantum antiferromagnet Cs2CuCl4

Magneto-acoustic investigations of the frustrated triangular-lattice antiferromagnet Cs2CuCl4 were performed for the longitudinal modes c11 and c33 in magnetic fields along the a-axis. The temperature dependence of the sound velocity at zero field shows a mild softening at low temperature and displays a small kink-like anomaly at TN. Isothermal measurements at T < TN of the sound attenuation reveal two closely-spaced features of different character on approaching the materials quantum-critical point (QCP) around Bs = 8.5 T for B // a. The peak at slightly lower fields remains sharp down to the lowest temperature and can be attributed to the ordering temperature TN(B). The second anomaly which is rounded and which becomes reduced in size upon cooling is assigned to the materials spin-liquid properties preceding the long-range antiferromagnetic ordering. These two features merge upon cooling suggesting a coincidence at the QCP. The elastic constant at lowest temperatures of our experiment at 32 mK can be well described by a Landau free energy model with a very small magnetoelastic coupling constant G/kB = 2.8 K. The applicability of this classical model indicates the existence of a small gap in the magnetic excitation spectrum which drives the system away from quantum criticality.

cond-mat.str-el↗

arXiv2016

Combined effects of Sr substitution and pressure on the ground states in CaFe$_2$As$_2$

We present a detailed study of the combined effects of Sr substitution and hydrostatic pressure on the ground-state properties of CaFe$_2$As$_2$. Measurements of the electrical resistance and magnetic susceptibility, both at ambient and finite pressure $P$ $\leq$ 2$\,$GPa, were performed on Ca$_{1-x}$Sr$_x$Fe$_2$As$_2$ single crystals grown out of Sn flux. We find that upon Sr substitution the ranges of stability of both the structural-magnetic transition and the transition into the non-magnetic collapsed tetragonal phase are shifted to higher pressure levels with the latter moving at a higher rate. This suggests the possibility of separating the two phase lines, which intersect already at elevated temperatures for $x$ = 0 and low Sr concentration levels. For $x$ = 0.177 we find strong evidence that both phases remain separated down to lowest temperature and that a zero-resistance state emerges in this intermediate pressure window. This observation indicates that Sr-substitution combined with hydrostatic pressure provides another route for stabilizing superconductivity in CaFe$_2$As$_2$. Our results are consistent with the notion that (i) preserving the fluctuations associated with the structural-magnetic transition to low temperatures is vital for superconductivity to form in this material and that (ii) the non-magnetic collapsed tetragonal phase is detrimental for superconductivity.

cond-mat.supr-con↗

arXiv2016

Double-polarization observable G in neutral-pion photoproduction off the proton

This paper reports on a measurement of the double-polarization observable G in $π^0$ photoproduction off the proton using the CBELSA/TAPS experiment at the ELSA accelerator in Bonn. The observable G is determined from reactions of linearly-polarized photons with longitudinally-polarized protons. The polarized photons are produced by bremsstrahlung off a properly oriented diamond radiator. A frozen spin butanol target provides the polarized protons. The data cover the photon energy range from 617 to 1325 MeV and a wide angular range. The experimental results for G are compared to predictions by the Bonn-Gatchina (BnGa), Jülich-Bonn (JüBo), MAID and SAID partial wave analyses. Implications of the new data for the pion photoproduction multipoles are discussed.

nucl-ex↗

arXiv2015

High statistics study of the reaction $γp\to p\;2π^0$

The photoproduction of 2$π^0$ mesons off protons was studied with the Crystal Barrel/TAPS experiment at the electron accelerator ELSA in Bonn. The energy of photons produced in a radiator was tagged in the energy range from 600\,MeV to 2.5\,GeV. Differential and total cross sections and $pπ^0π^0$ Dalitz plots are presented. Part of the data was taken with a diamond radiator producing linearly polarized photons, and beam asymmetries were derived. Properties of nucleon and $Δ$ resonances contributing to the $pπ^0π^0$ final state were determined within the BnGa partial wave analysis. The data presented here allow us to determine branching ratios of nucleon and $Δ$ resonances for their decays into $pπ^0π^0$ via several intermediate states. Most prominent are decays proceeding via $Δ(1232)π$, $N(1440)1/2^+π$, $N(1520)3/2^-π$, $N(1680)5/2^+π$, but also $pf_0(500)$, $pf_0(980)$, and $pf_2(1270)$ contribute to the reaction.

nucl-ex↗

arXiv2015

Magnetism-induced massive Dirac spectra and topological defects in the surface state of Cr-doped Bi$_2$Se$_3$-bilayer topological insulators

Proximity-induced magnetic effects on the surface Dirac spectra of topological insulators are investigated by scanning tunneling spectroscopic (STS) studies of bilayer structures consisting of undoped Bi2Se3 thin films on top of Cr-doped Bi2Se3 layers. For thickness of the top Bi2Se3 layer equal to or smaller than 3 quintuple layers (QL), a spatially inhomogeneous surface spectral gap Δopens up below T_c^{2D}, which is much higher than the bulk Curie temperature T_c^{3D}. The mean value and spatial homogeneity of the gap Δgenerally increase with increasing c-axis magnetic field (H) and increasing Cr doping level (x), suggesting that the physical origin of this surface gap is associated with proximity-induced c-axis ferromagnetism. On the other hand, the temperature (T) dependence of Δis non-monotonic, showing an initial increase below T_c^{2D} followed by a dip and then reaching maximum at T << T_c^{3D}. These phenomena may be attributed to proximity magnetism induced by two types of contributions with different temperature dependence: a 3D contribution from the bulk magnetism that dominates at low T, and a 2D contribution associated with the RKKY interactions mediated by surface Dirac fermions, which dominates at T_c^{3D} << T < T_c^{2D}. Additionally, spatially localized sharp resonant spectra are found along the boundaries of gapped and gapless regions. These spectral resonances are long-lived at H = 0 and become suppressed under strong c-axis magnetic fields, and are attributed to magnetic impurity-induced topological defects in the spin texture of surface Dirac fermions.

cond-mat.mes-hall↗

arXiv2015

Measurement of double polarisation asymmetries in $ω$-photoproduction

The first measurements of the beam-target-helicity-asymmetries $E$ and $G$ in the photoproduction of $ω$-mesons off protons at the CBELSA/TAPS experiment are reported. $E$ ($G$) was measured using circularly (linearly) polarised photons and a longitudinally polarised target. $E$ was measured over the photon energy range from close to threshold ($E_γ= 1108$~MeV) to $E_γ= 2300$~MeV and $G$ at a single energy interval of $1108 < E_γ<1300$~MeV. Both measurements cover the full solid angle. The observables $E$ and $G$ are highly sensitive to the contribution of baryon resonances, with $E$ acting as a helicity filter in the $s$-channel. The new results indicate significant $s$-channel resonance contributions together with contributions from $t$-channel exchange processes. A partial wave analysis reveals strong contributions from the partial waves with spin-parity $J^P=3/2^+, 5/2^+$, and $3/2^-$.

nucl-ex↗

arXiv2015

Photoproduction of ω Mesons off the Proton

The differential cross sections and unpolarized spin-density matrix elements for the reaction $γp\to pω$ were measured using the CBELSA/TAPS experiment for initial photon energies ranging from the reaction threshold to 2.5 GeV. These observables were measured from the radiative decay of the $ω$ meson, $ω\toπ^0γ$. The cross sections cover the full angular range and show the full extent of the $t$-channel forward rise. The overall shape of the angular distributions in the differential cross sections and unpolarized spin-density matrix elements are in fair agreement with previous data. In addition, for the first time, a beam of linearly-polarized tagged photons in the energy range from 1150 MeV to 1650 MeV was used to extract polarized spin-density matrix elements. These data were included in the Bonn-Gatchina partial wave analysis (PWA). The dominant contribution to $ω$ photoproduction near threshold was found to be the $3/2^+$ partial wave, which is primarily due to the sub-threshold $N(1720)\,3/2^+$ resonance. At higher energies, pomeron-exchange was found to dominate whereas $π$-exchange remained small. These $t$-channel contributions as well as further contributions from nucleon resonances were necessary to describe the entire dataset: the $1/2^-$, $3/2^-$, and $5/2^+$ partial waves were also found to contribute significantly.

nucl-ex↗