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M. Li

Publications and source records attributed to M. Li.

At least 73 records · Page 4Linked to original sources
arXiv2020

Single-Atom Verification of the Information-Theoretical Bound of Irreversibility at the Quantum Level

Quantitative measure of disorder or randomness based on the entropy production characterizes thermodynamical irreversibility, which is relevant to the conventional second law of thermodynamics. Here we report, in a quantum mechanical fashion, the first theoretical prediction and experimental exploration of an information-theoretical bound on the entropy production. Our theoretical model consists of a simplest two-level dissipative system driven by a purely classical field, and under the Markovian dissipation, we find that such an information-theoretical bound, not fully validating quantum relaxation processes, strongly depends on the drive-to-decay ratio and the initial state. Furthermore, we carry out experimental verification of this information-theoretical bound by means of a single spin embedded in an ultracold trapped $^{40}$Ca$^{+}$ ion. Our finding, based on a two-level model, is fundamental to any quantum thermodynamical process and indicates much difference and complexity in quantum thermodynamics with respect to the conventionally classical counterpart.

quant-ph↗
arXiv2019

Observation of indirect ionization of W7+ in an electron-beam ion-trap plasma

In this work, visible and extreme ultraviolet spectra of W7+ are measured using the high-temperature superconducting electron-beam ion trap (EBIT) at the Shanghai EBIT Laboratory under extremely low-energy conditions (lower than the nominal electron-beam energy of 130 eV). The relevant atomic structure is calculated using the flexible atomic code package based on the relativistic configuration interaction method. The GRASP2K code, in the framework of the multiconfiguration Dirac-Hartree-Fock method, is employed as well for calculating the wavelength of the M1 transition in the ground configuration of W7+. A line from the W7+ ions is observed at a little higher electron-beam energy than the ionization potential for W4+, making this line appear to be from W5+. A hypothesis for the charge-state evolution of W7+ is proposed based on our experimental and theoretical results; that is, the occurrence of W7+ ions results from indirect ionization caused by stepwise excitation between some metastable states of lower-charge-state W ions, at the nominal electron-beam energy of 59 eV.

physics.atom-ph↗
arXiv2019

Observation of topological transition in high-T$_{c}$ superconductor FeTe$_{1-x}$Se$_{x}$/SrTiO$_{3}$(001) monolayers

Superconductors with topological surface or edge states have been intensively explored for the prospect of realizing Majorana bound states, which obey non-Abelian statistics and are crucial for topological quantum computation. The traditional routes for making topological insulator/superconductor and semiconductor/superconductor heterostructures suffer fabrication difficulties and can only work at low temperature. Here, we use angle-resolved photoemission spectroscopy to directly observe the evolution of a topological transition of band structure nearby the Fermi level in two-dimensional high-T$_{c}$ superconductor FeTe$_{1-x}$Se$_{x}$/SrTiO$_{3}$(001) monolayers, fully consistent with our theoretical calculations. Furthermore, evidence of edge states is revealed by scanning tunneling spectroscopy with assistance of theoretical calculations. Our study provides a simple and tunable platform for realizing and manipulating Majorana states at high temperature.

cond-mat.supr-con↗
arXiv2019

Tin+1Cn MXene with fully saturated and thermally stable Cl terminations

MXenes are a rapidly growing family of 2D materials that exhibit a highly versatile structure and composition, allowing for significant tuning of the material properties. These properties are, however, ultimately limited by the surface terminations, which are typically a mixture of species, including F and O that are inherent to the MXene processing. Other and robust terminations are lacking. Here, we apply high-resolution scanning transmission electron microscopy (STEM), corresponding image simulations and first-principles calculations to investigate the surface terminations on MXenes synthesized from MAX phases through Lewis acidic melts. The results show that atomic Cl terminates the synthesized MXenes, with mere residual presence of other termination species. Furthermore, in situ STEM-electron energy loss spectroscopy (EELS) heating experiments show that the Cl terminations are stable up to 750 °C. Thus, we present an attractive new termination that widely expands the MXenes functionalization space and enable new applications.

cond-mat.mtrl-sci↗
arXiv2018

Outstanding Radiation Resistance of Tungsten-based High Entropy Alloys

A novel W-based refractory high entropy alloy with outstanding radiation resistance has been developed. The alloy was grown as thin films showing a bimodal grain size distribution in the nanocrystalline and ultrafine regimes and a unique 4 nm lamella-like structure revealed by atom probe tomography (APT). Transmission electron microscopy (TEM) and X-ray diffraction show an underlying body-centered cubic crystalline structure with certain black spots appearing after thermal annealing at elevated temperatures. Thorough analysis based on TEM and APT correlated the black spots with second phase particles rich in Cr and V. After both in situ and ex situ irradiation, these precipitates evolve to quasi-spherical particles with no sign of irradiation-created dislocation loops even after 8 dpa at either room temperature or 1073 K. Furthermore, nanomechanical testing shows a large hardness of 14 GPa in the as-deposited samples, with a slight increase after thermal annealing and almost negligible irradiation hardening. Theoretical modeling based on ab initio methodologies combined with Monte Carlo techniques predicts the formation of Cr and V rich second phase particles and points at equal mobilities of point defects as the origin of the exceptional radiation tolerance. The fact that these alloys are suitable for bulk production coupled with the exceptional radiation and mechanical properties makes them ideal structural materials for applications requiring extreme conditions.

cond-mat.mtrl-sci↗
arXiv2018

Valley selective optical control of excitons in 2D semiconductors using Chiral metasurface

Recent advances in condensed matter physics have shown that the valley degree of freedom of electrons in 2D materials with hexagonal symmetry, such as graphene, h-BN, and TMDs, can be efficiently exploited, leading to the emergent field of valleytronics, which offers unique opportunities for efficient data transfer, computing and storage. The ability to couple the valley degree of freedom of electrons with light can further expand the ways one manipulate this degree of freedom, thus envisioning a new class of solid-state-photonic interfaces and devices. Besides this expansion of control of valley by light-waves, coupling of photons with valley-polarized electrons can dramatically expand the landscape of available optical responses, which may bring new means of controlling light in photonic devices. In this work we design such hybrid solid-state photonic metasurface integrating 2D TMD and photonic all-dielectric metasurface. While TMD is naturally endowed with the property of valley to optical-polarization coupling, the photonic metasurface is designed to produce chiral field which selectively couples to the valley degree of freedom of solid-state TMD component. We experimentally demonstrate that such coupling leads to controlled valley polarization due to the coupling of 2D materials with the chiral photonic metasurface. The measured emission from valley excitons in this hybrid system yields the preferential emission of specific helicity.

physics.optics↗
arXiv2018

Velocity-resolved reverberation mapping of five bright Seyfert 1 galaxies

We present the first results from a reverberation-mapping campaign undertaken during the first half of 2012, with additional data on one AGN (NGC 3227) from a 2014 campaign. Our main goals are (1) to determine the black hole masses from continuum-Hbeta reverberation signatures, and (2) to look for velocity-dependent time delays that might be indicators of the gross kinematics of the broad-line region. We successfully measure Hbeta time delays and black hole masses for five AGNs, four of which have previous reverberation mass measurements. The values measured here are in agreement with earlier estimates, though there is some intrinsic scatter beyond the formal measurement errors. We observe velocity dependent Hbeta lags in each case, and find that the patterns have changed in the intervening five years for three AGNs that were also observed in 2007.

astro-ph.GA↗
arXiv2018

Observation of a nodal chain with Dirac surface states in TiB2

Topological nodal-line semimetals (TNLSMs) are characterized by symmetry-protected band crossings extending along one-dimensional lines in momentum space. The nodal lines exhibit a variety of possible configurations, such as nodal ring, nodal link, nodal chain, and nodal knot. Here, using angle-resolved photoemission spectroscopy, we observe nodal rings in the orthogonal kz = 0 and kx = 0 planes of the Brillouin zone in TiB2. The nodal rings connect with each other on the intersecting line Γ-K of the orthogonal planes, forming a remarkable nodal-chain structure. Furthermore, we observe surface states (SSs) on the (001) cleaved surface, which are consistent with the calculated SSs considering the contribution from both Ti and B terminations. The calculated SSs have novel Dirac-cone-like band structures, which are distinct from the usual drumhead SSs with a single flat band proposed in other TNLSMs.

cond-mat.mtrl-sci↗
arXiv2017

Observation of Open-Orbit Fermi Surface Topology in Extremely Large Magnetoresistance Semimetal MoAs$_2$

While recent advances in band theory and sample growth have expanded the series of extremely large magnetoresistance (XMR) semimetals in transition metal dipnictides $TmPn_2$ ($Tm$ = Ta, Nb; $Pn$ = P, As, Sb), the experimental study on their electronic structure and the origin of XMR is still absent. Here, using angle-resolved photoemission spectroscopy combined with first-principles calculations and magnetotransport measurements, we performed a comprehensive investigation on MoAs$_2$, which is isostructural to the $TmPn_2$ family and also exhibits quadratic XMR. We resolve a clear band structure well agreeing with the predictions. Intriguingly, the unambiguously observed Fermi surfaces (FSs) are dominated by an open-orbit topology extending along both the [100] and [001] directions in the three-dimensional Brillouin zone. We further reveal the trivial topological nature of MoAs$_2$ by bulk parity analysis. Based on these results, we examine the proposed XMR mechanisms in other semimetals, and conclusively ascribe the origin of quadratic XMR in MoAs$_2$ to the carriers motion on the FSs with dominant open-orbit topology, innovating in the understanding of quadratic XMR in semimetals.

cond-mat.mtrl-sci↗
arXiv2017

Quantum Reactive Scattering of Ultracold Atoms and Molecules: Universality and Chaotic Dynamics

A fundamental question in the study of chemical reactions is how reactions proceed at a collision energy close to absolute zero. This question is no longer hypothetical: quantum degenerate gases of atoms and molecules can now be created at temperatures lower than a few tens of nanoKelvin. In this work we consider the benchmark ultracold reaction between, the most-celebrated ultracold molecule, KRb and K. For the first time we map out an accurate ab initio ground state potential energy surface of the KRbK complex in full dimensionality and report numerically exact quantum-mechanical reaction dynamics. The distribution of rotationally resolved rates is shown to be Poissonian. An analysis of the hyperspherical adiabatic potential curves explains this statistical character revealing a chaotic distribution for the short-range collision complex that plays a key role in governing the reaction outcome. We compare this with a lighter system with a smaller density of states (here the LiYbLi trimer) which displays random, and not chaotic, behavior.

physics.chem-ph↗
arXiv2017

A Likely Redback Millisecond Pulsar Counterpart of 3FGL J0838.8-2829

We obtained new optical observations of the X-ray source XMMU J083850.38-282756.8, the previously proposed counterpart of the gamma-ray source 3FGL J0838.8-2829. Time-series photometry in the $r'$ band reveals periodic modulation of $\approx1$ magnitude that is characteristic of the heating of the photosphere of a low-mass companion star by a compact object. The measured orbital period is 5.14817$\pm$0.00012 hr. The shape of the light curve is variable, evidently due to the effects of flaring and asymmetric heating. Spectroscopy reveals a companion of type M1 or later, having a radial velocity amplitude of 315$\pm$17 km/s, with period and phasing consistent with the heating interpretation. The mass function of the compact object is 0.69$\pm$0.11 $M_{\odot}$, which allows a neutron star in a high-inclination orbit. Variable, broad H$α$ emission is seen, which is probably associated with a wind from the companion. These properties, as well as the X-ray and gamma-ray luminosities at the inferred distance of <1.7 kpc, are consistent with a redback millisecond pulsar in its non-accreting state. A search for radio pulsations is needed to confirm this interpretation and derive complete system parameters for modeling, although absorption by the ionized wind could hinder such detection.

astro-ph.HE↗
arXiv2017

Space Telescope and Optical Reverberation Mapping Project. VII. Understanding the UV anomaly in NGC 5548 with X-Ray Spectroscopy

During the Space Telescope and Optical Reverberation Mapping Project (STORM) observations of NGC 5548, the continuum and emission-line variability became de-correlated during the second half of the 6-month long observing campaign. Here we present Swift and Chandra X-ray spectra of NGC 5548 obtained as a part of the campaign. The Swift spectra show that excess flux (relative to a power-law continuum) in the soft X-ray band appears before the start of the anomalous emission-line behavior, peaks during the period of the anomaly, and then declines. This is a model-independent result suggesting that the soft excess is related to the anomaly. We divide the Swift data into on- and off-anomaly spectra to characterize the soft excess via spectral fitting. The cause of the spectral differences is likely due to a change in the intrinsic spectrum rather than being due to variable obscuration or partial covering. The Chandra spectra have lower signal-to-noise ratios, but are consistent with Swift data. Our preferred model of the soft excess is emission from an optically thick, warm Comptonizing corona, the effective optical depth of which increases during the anomaly. This model simultaneously explains all the three observations: the UV emission line flux decrease, the soft-excess increase, and the emission line anomaly.

astro-ph.GA↗
arXiv2017

Formation of soap bubbles by gas jet

Soap bubbles can be easily generated by varies methods, while their formation process is complicated and still worth study. A model about the bubble formation process was proposed in Phys. Rev. Lett. 116, 077801 recently, and it was reported that the bubbles were formed when the gas blowing velocity was above one threshold. However, after repeating these experiments, we found the bubbles could be generated in two velocities ranges which corresponded to laminar and turbulent gas jet respectively, and the predicted threshold was only effective for turbulent gas flow. The study revealed that the bubble formation was mainly influenced by the aerodynamics of the gas jet blowing to the film, and these results will help to further understand the formation mechanism of the soap bubble as well as the interaction between gas jet and thin liquid film.

physics.flu-dyn↗
arXiv2017

Machine-to-Machine (M2M) Communications in Virtualized Cellular Networks with MEC

As an important part of the Internet-of-Things (IoT), machine-to-machine (M2M) communications have attracted great attention. In this paper, we introduce mobile edge computing (MEC) into virtualized cellular networks with M2M communications, to decrease the energy consumption and optimize the computing resource allocation as well as improve computing capability. Moreover, based on different functions and quality of service (QoS) requirements, the physical network can be virtualized into several virtual networks, and then each MTCD selects the corresponding virtual network to access. Meanwhile, the random access process of MTCDs is formulated as a partially observable Markov decision process (POMDP) to minimize the system cost, which consists of both the energy consumption and execution time of computing tasks. Furthermore, to facilitate the network architecture integration, software-defined networking (SDN) is introduced to deal with the diverse protocols and standards in the networks. Extensive simulation results with different system parameters reveal that the proposed scheme could significantly improve the system performance compared to the existing schemes.

cs.NI↗
arXiv2016

Suppression of magnetoresistance in thin $WTe_2$ flakes by surface oxidation

Recent renewed interest in layered transition metal dichalcogenides stems from the exotic electronic phases predicted and observed in the single- and few-layer limit. Realizing these electronic phases requires preserving the desired transport properties down to a monolayer, which is challenging. Here, using semimetallic $WTe_2$ that exhibits large magnetoresistance, we show that surface oxidation and Fermi level pinning degrade the transport properties of thin $WTe_2$ flakes significantly. With decreasing $WTe_2$ flake thickness, we observe a dramatic suppression of the large magnetoresistance. This is explained by fitting a two-band model to the transport data, which shows that mobility of the electron and hole carriers decreases significantly for thin flakes. The microscopic origin of this mobility decrease is attributed to a ~ 2 nm-thick amorphous surface oxide layer that introduces disorder. The oxide layer also shifts the Fermi level by ~ 300 meV at the $WTe_2$ surface. However, band bending due to this Fermi level shift is not the dominant cause for the suppression of magnetoresistance as the electron and hole carrier densities are balanced down to ~ 13 nm based on the two-band model. Our study highlights the critical need to investigate often unanticipated and sometimes unavoidable extrinsic surface effects on the transport properties of layered dichalcogenides and other 2D materials.

cond-mat.mtrl-sci↗
arXiv2014

Passive, Noiseless, Intensity Amplification of Repetitive Signals

Amplification of signal intensity is essential for initiating physical processes, diagnostics, sensing, communications, and scientific measurement. During traditional amplification, the signal is amplified by multiplying the signal carriers through an active gain process using an external power source. However, for repetitive waveforms, sufficient energy for amplification often resides in the signal itself. In such cases, the unneeded external power is wasted, and the signal is additionally degraded by noise and distortions that accompany active gain processes. We show noiseless, intensity amplification of repetitive optical pulse waveforms with a gain from 2 to ~20 without using active gain, by recycling energy already stored in the input repetitive signal. This "green" method uses dispersion-induced self-imaging (Talbot) effects to precisely re-distribute the original signal energy into fewer replica waveforms. This approach simply requires a suitable manipulation of the input signal's phase profile along the temporal and spectral domains. In addition, we show experimentally how our passive amplifier performs a real-time average of the wave train to reduce noise fluctuation present on the input pulse train, as well as enhances the extinction ratio of pulses to stand above the noise floor by approximately the passive gain factor. Finally, our technique is applicable to repetitive waveforms in any spectral region or wave system, including acoustic, mechanical, and quantum probability waveforms, for which active amplification methods are challenging to implement or nonexistent.

physics.optics↗
arXiv2014

Latent-heat and non-linear vortex liquid at the vicinity of the first-order phase transition in layered high-Tc superconductors

In this work we revisit the vortex matter phase diagram in layered superconductors solving still open questions by means of AC and DC local magnetic measurements in the paradigmatic Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8}$ compound. We show that measuring with AC magnetic techniques is mandatory in order to probe the bulk response of vortex matter, particularly at high-temperatures where surface barriers for vortex entrance dominate. From the $T_{\rm FOT}$-evolution of the enthalpy and latent-heat at the transition we find that, contrary to previous reports, the nature of the dominant interlayer coupling is electromagnetic in the whole temperature range. By studying the dynamic properties of the phase located at $T \gtrsim T_{\rm FOT}$, we reveal the spanning in a considerable fraction of the phase diagram of a non-linear vortex phase suggesting bulk pinning might play a role even in the liquid vortex phase.

cond-mat.supr-con↗