arXiv subjects

M. Orlita

Publications and source records attributed to M. Orlita.

At least 19 recordsLinked to original sources

arXiv2026

Spin-chiral electron-phonon coupling in metallic strontium titanate

Electron-phonon coupling (EPC) - the interaction between conduction electrons and quantized atomic vibrations - plays a central role in condensed matter physics and determines some of the most important properties of materials, such as electrical resistivity and superconductivity. Conventionally, EPC is assumed to be induced by the ionic electrostatic background, and electronic spin plays no role in the process. In stark contrast with this view, here we uncover a direct spin-mediated coupling mechanism between electrons and transverse polar phonons in a metal. Using far-infrared light absorption measurements of the model system SrTiO$_3$ in a magnetic field, we observe a strong spin-mediated EPC that is quantitatively consistent with recent theoretical predictions, and that generates chiral phonon modes with large effective magnetic moments. The extracted coupling strength is in good agreement with ab initio estimates and sufficiently high to explain superconductivity in SrTiO$_3$, thereby resolving a long-standing conundrum. Spin-chiral EPC should generically appear in all metals with polar phonons, and the present work could be of relevance to spintronics applications and to uncovering the origins of superconductivity in layered materials, metals with Dirac points in their electronic dispersions, and nearly ferroelectric superconductors.

cond-mat.str-el↗

arXiv2026

Magnetic-field-induced magnon portfolio in a van der Waals magnet

Magnonic excitations are investigated in chromium oxychloride (CrOCl), a van der Waal (vdW) antiferromagnet prone to a multitude of magnetic phase transitions, with absorption experiments in a broad continuous energy range. At low magnetic fields, the magnon spectra show a strong bi-axial anisotropy and inform on the relative weights of the effective exchange coupling and the system anisotropies. As the magnetic field increases, magnons characteristic of a canted phase are first observed, with peculiarities attributed to in-plane anisotropies and magnon-magnon coupling. Subsequently, a hysteretic magnon spectrum appears as the system transitions to a ferrimagnetic state, with two new magnon branches partly coexisting with the lower energy canted phase branch, indicating the formation of spatially separated magnetic phases. Further changes in the magnon spectrum in higher magnetic fields accompany transitions to the different canted magnetic phases previously reported. Our experiments show that competing exchange interactions and ground states broaden the options to generate different kinds of magnonic excitations in the same vdW material upon the variation of external parameters.

cond-mat.mtrl-sci↗

arXiv2026

Nonlinear Terahertz Electroluminescence from Dirac Landau Polaritons

We report Dirac Landau polaritons observed by terahertz (THz) magnetoreflectivity spectroscopy, demonstrating strong coupling between cyclotron transitions of two-dimensional (2D) Dirac fermions in HgTe quantum wells and optical cavity modes. Under pulsed electrical injection we observe efficient nonlinear electroluminescence, with a strongly out-of-equilibrium polariton distribution dominated by emission from the upper polariton branches. Model analysis of the bias-dependent emission intensity and spectral narrowing indicates a polariton occupancy per mode approaching unity, with a possible contribution from stimulated polariton emission in the spectral region of the upper anticrossing. These results open prospects toward Dirac Landau polariton condensates and low-threshold, tunable THz polariton lasers based on cyclotron emission.

cond-mat.mes-hall↗

arXiv2026

Dynamics of surface electrons in a topological insulator: cyclotron resonance at room temperature

The ability to manipulate the surface states of topological insulators using electric or magnetic fields under ambient conditions is a key step toward their integration into future electronic and optoelectronic devices. Here, we demonstrate - using cyclotron resonance measurements on a tin-doped BiSbTe$_2$S topological insulator - that moderate magnetic fields can quantize massless surface electrons into Landau levels even at room temperature. This finding suggests that surface-state electrons can behave as long-lived quasiparticles at unexpectedly high temperatures.

cond-mat.mes-hall↗

arXiv2025

Antiferromagnetic resonance in $α$-MnTe

Antiferromagnetic resonance in a bulk $α$-MnTe crystal is investigated using both frequency-domain and time-domain THz spectroscopy techniques. At low temperatures, an excitation at the photon energy of $(3.5\pm 0.1)$~meV is observed and identified as a magnon mode through its distinctive dependence on temperature and magnetic field. This behavior is reproduced using a simplified model for antiferromagnetic resonance in an easy-plane antiferromagnet. The results of our experiments, when compared to exchange constants established in the literature, allow us to extract the out-of-plane component of the single-ion magnetic anisotropy reaching $(40\pm10)$~$μ$eV.

cond-mat.mtrl-sci↗

arXiv2025

Magnetic phases and zone-folded phonons in a frustrated van der Waals magnet

2D magnetic materials have attracted extensive research interest due to their potential application in nanospintronics, optospintronics, and in magnonics. Ferromagnetic as well as antiferromagnetic layered materials have been demonstrated and successfully inserted into van der Waals heterostructures. However, the effects of magnetic frustration in van der Waals materials and the possibilities offered by spin configurations characterized by nonlinear spin arrangements have not been fully considered yet. Herein, we establish the magnetic phase diagram of bulk CrOCl, a frustrated van der Waals magnet, using magnetization and magneto-optical spectroscopy techniques. In particular, we use the magnetic superstructures relative to the crystallographic unit cell and the associated rich zone-folded phonon series to describe the magnetic field induced phases. Theoretical calculations taking into account the competing nearest neighbors magnetic exchange interactions provide a unique insight into the lattice vibrations of this class of magnetic system. This study expands the scope of 2D magnetic materials and provides a methodology to characterize frustrated van der Waals magnets.

cond-mat.mes-hall↗

arXiv2025

Generation of Weyl points and a nodal line by magnetization reorientation in Co$_3$Sn$_2$S$_2$

Topological magnets exhibit fascinating properties like topologically protected surface states or anomalous transport phenomena. While these properties can be significantly altered by manipulating the magnetic state, the experimental verification of such predictions remains challenging. Here, we demonstrate the efficient magnetic field control of the Weyl semimetallic state of the collinear ferromagnet Co$_3$Sn$_2$S$_2$ by magneto-optical spectroscopy. We resolve a redshift of the nodal loop resonance as the magnetization is rotated into the kagome plane by the magnetic field. Our material-specific theory, capturing the observed field-induced spectral reconstruction, shows the creation of 26 Weyl points for one in-plane magnetization direction and predicts the emergence of a gapless nodal loop for the orthogonal in-plane magnetization orientation. These findings demonstrate that while topological band structures are generally considered robust, breaking underlying crystal symmetries with external fields provides an efficient way to manipulate them, even in collinear magnets. This approach opens exciting avenues to control band topology also in materials with more complex magnetic structures and even to study the interplay of real- and momentum-space topological states, e.g. in skyrmion-lattice systems.

cond-mat.mtrl-sci↗

arXiv2025

Large magnetoreflectance and optical anisotropy due to $4f$ flat bands in the frustrated kagome magnet HoAgGe

We report peculiar optical properties of the frustrated itinerant magnet HoAgGe, which exhibits multiple magnetically ordered states obeying the kagome spin-ice rule. The optical conductivity is surprisingly higher for light polarization perpendicular to the kagome plane, both for the free carrier response and the interband transitions. The latter ones have strong contributions from Ho $4f$ flat bands located near the Fermi level, as revealed by our \textit{ab initio} calculations, explaining the unusual anisotropy of the optical properties and the pronounced temperature dependence of the interband transitions for out--of--plane light polarization. The key role of Ho $4f$ states is further supported by the large variation of the reflectivity upon the metamagnetic transitions, that follows the field dependence of the magnetization, in contrast to that of the dc magnetotransport data. Such heavy-electron bands near the Fermi level offer an efficient way to control transport and optical properties.

cond-mat.str-el↗

arXiv2025

Low-energy excitations in multiple modulation-doped CdTe/(CdMg)Te quantum wells

Low energy excitations of a two-dimensional electron gas (2DEG) in modulation-doped multiple (ten) quantum wells (QWs) was studied using far-infrared magneto-transmission technique at liquid helium temperatures. A large distance between neighbouring QWs of 54 nm excluded a direct interaction of electron wave functions confined in the wells. In four samples which differed in the spacer width and the level of doping with iodine donors, supplied with a metallic grid coupler, a uniform picture of exitations of the 2DEG was observed. These involved the cyclotron resonance (CR), its second harmonic (2CR) and magnetoplasmon modes (MPMs). MPMs with a small amplitude originated from excitations of the 2DEG in a single QW and these with a high amplitude resulted from a coherent excitation of the 2DEG in all wells. A polaron effect resulting from the interaction of the CR, 2CR and MPMs with an optical phonon was observed and discribed with appropriate models. Both types of MPMs exhibited gaps in the disperion relations at the frequency close to the 2CR, leading to Bernstein modes, which was discribed with an appropriate (non-local) theoretical model.

cond-mat.mes-hall↗

arXiv2024

Spin-Orbital-Lattice Coupling and the Phonon Zeeman Effect in the Dirac Honeycomb Magnet CoTiO$_3$

The entanglement of electronic spin and orbital degrees of freedom is often the precursor to emergent behaviors in condensed matter systems. With considerable spin-orbit coupling strength, the cobalt atom on a honeycomb lattice offers a platform that can make accessible the study of novel magnetic ground states. Using temperature-dependent Raman spectroscopy and high-magnetic field Raman and infrared (IR) spectroscopy, we studied the lattice and spin-orbital excitations in CoTiO$_3$, an antiferromagnetic material that exhibits topologically protected magnon Dirac crossings in the Brillouin zone. Under the application of an external magnetic field up to 22 T along the crystal's $c$-axis, we observed the splitting of both the spin-orbital excitations and a phonon nearby in energy. Using density functional theory (DFT), we identify a number of new modes that below the antiferromagnetic (AFM) transition become Raman-active due to the zone-folding of the Brillouin zone caused by the doubling of the magnetic unit cell. We use a model that includes both the spin and orbital degrees of freedom of the Co$^{2+}$ ions to explain the spin-orbital excitation energies and their behavior in an applied field. Our experimental observations along with several deviations from the model behavior point to significant coupling between the spin-orbital and the lattice excitations.

cond-mat.str-el↗

arXiv2024

Continuous-wave cryogenic optical absorption spectrometer for sub-THz frequencies

We present the design of a continuous-wave, highly sensitive optical spectrometer for millimeter-wave frequencies between 50 and 1000 GHz. The spectrometer uses photomixing of near-infrared light to generate radiation in a wide frequency range, and the absorbed optical power is determined directly through measurements of the sample temperature. This enables relative sensitivities of up to $10^6$ for the sample absorption coefficient below liquid-helium temperatures, suitable for measurements on highly reflective samples. The instrument is also compatible with high magnetic fields. In order to validate its performance, we measure the ferromagnetic resonance in the Mott insulator YTiO$_3$, the electron spin resonance in a standard free-radical reference compound, and the antiferromagnetic resonance in a van der Waals magnetic material.

physics.ins-det↗

arXiv2024

Tuning THz magnons in a mixed van-der-Waals antiferromagnet

Alloying stands out as a pivotal technological method employed across various compounds, be they metallic, magnetic, or semiconducting, serving to fine-tune their properties to meet specific requirements. Ternary semiconductors represent a prominent example of such alloys. They offer fine-tuning of electronic bands, the band gap in particular, thus granting the technology of semiconductor heterostructures devices, key elements in current electronics and optoelectronics. In the realm of magnetically ordered systems, akin to electronic bands in solids, spin waves exhibit characteristic dispersion relations, featuring sizeable magnon gaps in many antiferromagnets. The engineering of the magnon gap constitutes a relevant direction in current research on antiferromagnets, aiming to leverage their distinct properties for THz technologies, spintronics, or magnonics. In this study, we showcase the tunability of the magnon gap across the THz spectral range within an alloy comprising representative semiconducting van-der-Waals antiferromagnets FePS$_3$ and NiPS$_3$. These constituents share identical in-plane crystal structures, magnetic unit cells and the direction of the magnetic anisotropy, but differ in the amplitude and sign of the latter. Altogether these attributes result in the wide tunability of the magnon gap in the Fe$_{1-x}$Ni$_x$PS$_3$ alloy in which the magnetic order is imposed by stronger, perpendicular anisotropy of iron.

cond-mat.mtrl-sci↗

arXiv2024

Magneto-optical response of magnetic semiconductors EuCd2X2 (X= P, As, Sb)

In this study, we identify EuCd2X2 (for X = P, As, Sb) as a series of magnetic semiconductors. We examine how the band gap of the series responds to X changing from phosphorus (P), to arsenic (As), and finally antimony (Sb). We characterize the samples using electronic transport and magnetization measurements. Based on infrared spectroscopy, we find that the band gap reduces progressively from 1.23 eV in EuCd2P2, to 0.77 eV in EuCd2As2, and finally 0.52 eV in EuCd2Sb2. In a magnetic field, all three systems show a strong response and their band gaps decrease at 4 K. This decrease is non-monotonic as we change X. It is strongest in the phosphorous compound and weakest in the antimony compound. For all the three compositions, EuCd2X2 remains a semiconductor up to the highest magnetic field applied (16 T).

cond-mat.mtrl-sci↗

arXiv2024

Unique magnetic structure of the vdW antiferromagnet VBr$_3$

VBr$_3$ is a van der Waals antiferromagnet below the Néel temperature of 26.5 K with a saturation moment of 1.2 mB/f.u. above the metamagnetic transitions detected in the in-plane and out-of-plane directions. To reveal the AFM structure of VBr$_3$ experimentally, we performed a single-crystal neutron diffraction study on a large high-quality crystal. The collected data confirmed a slight monoclinic distortion of the high-temperature rhombohedral structure below 90 K. The magnetic structure was, nevertheless, investigated within the R-3 model. The antiferromagnetic structure propagation vector k = (1, 0, 0.5) was revealed. In an attempt to determine the magnetic structure, 72 non-equivalent magnetic reflections were recorded. The experimental data were confronted with the magnetic space groups dictated by the R-3 lattice symmetry and propagation vector. The best agreement between the experimental data and the magnetic structure model was obtained for the space group P-1.1'_c. The magnetic unit cell of the proposed unique antiferromagnetic structure with periodicity 6c is built from two identical triple layers antiferromagnetically coupled along the c axis. Each triple layer comprises a Néel antiferromagnetic monolayer sandwiched between two antiferromagnetically coupled ferromagnetic monolayers.

cond-mat.mtrl-sci↗

arXiv2024

Transverse and longitudinal magnons in strongly anisotropic antiferromagnet FePSe3

FePSe3 is a collinear honeycomb antiferromagnet with an easy-axis anisotropy and large spins S=2. It belongs to a family of magnetic van der Waals materials, which recently attracted a considerable attention. In this work we present an experimental magneto-optical study of the low-energy excitation spectrum in FePSe3, together with its theoretical description. The observed response contains several types of magnon excitations. Two of them are conventional transverse magnons described by a classical theory of antiferromagnetic resonance. Two other modes are identified as multimagnon hexadecapole excitations with an anomalous g factor approximately equal to four times the g factor of a single Fe^2+ ion. These quasiparticles correspond to full reversals of iron spins that coherently propagate in the up-down antiferromagnetic structure. They constitute a novel type of collective excitations in anisotropic magnetic solids, called longitudinal magnons. Comparison between theory and experiment allows us to estimate the microscopic parameters of FePSe3 including exchange coupling constants and the single-ion anisotropy.

cond-mat.str-el↗

arXiv2024

Electronic band structure of Sb2Te3

Here we report on Landau level spectroscopy of an epitaxially grown thin film of the topological insulator Sb2Te3, complemented by ellipsometry and magneto-transport measurements. The observed response suggests that Sb2Te3 is a direct-gap semiconductor with the fundamental band gap located at the Γpoint, or along the trigonal axis, and its width reaches Eg = 190 meV at low temperatures. Our data also indicate the presence of other low-energy extrema with a higher multiplicity in both the conduction and valence bands. The conclusions based on our experimental data are confronted with and to a great extent corroborated by the electronic band structure calculated using the GW method.

cond-mat.mtrl-sci↗

arXiv2023

Magneto-optical response of the Weyl semimetal NbAs: Experimental results and hyperbolic-band computations

The magneto-optical properties of (001)-oriented NbAs single crystals have been studied in the spectral range from 5 to 150 meV and in magnetic fields of up to 13 T. A rich spectrum of inter-Landau-level transitions is revealed by these measurements. The transitions follow a square-root-like dependence with magnetic field, but the simple linear-band approximation is unable to accurately reproduce the observed behavior of the transitions in applied fields. We argue that the detected magneto-optical spectra should be related to crossing hyperbolic bands, which form the W1 cones. We propose a model Hamiltonian, which describes coupled hyperbolic bands and reproduces the shape of the relevant bands in NbAs. The magneto-optical spectra computed from this Hamiltonian nicely reproduce our observations. We conclude that the hyperbolic-band approach is a minimal model to adequately describe the magneto-optical response of NbAs and that the chiral (conical) bands do not explicitly manifest themselves in the spectra.

cond-mat.mes-hall↗

arXiv2023

Exchange gap in GdPtBi probed by magneto-optics

We measured the magneto-reflectivity spectra (4 - 90 meV, 0 - 16 T) of the triple-point semimetal GdPtBi and found them to demonstrate two unusual broad features emerging in field. The electronic bands of GdPtBi are expected to experience large exchange-mediated shifts, which lends itself to a description via effective Zeeman splittings with a large g factor. Based on this approach, along with an ab initio band structure analysis, we propose a model Hamiltonian that describes our observations well and allows us to estimate the effective g factor, g* = 95. We conclude that we directly observe the exchange-induced $Γ_{8}$ band inversion in GdPtBi by means of infrared spectroscopy.

cond-mat.mes-hall↗