arXiv subjects

M. Poggio

Publications and source records attributed to M. Poggio.

At least 37 records · Page 2Linked to original sources

arXiv2016

Vectorial scanning force microscopy using a nanowire sensor

Self-assembled nanowire (NW) crystals can be grown into nearly defect-free nanomechanical resonators with exceptional properties, including small motional mass, high resonant frequency, and low dissipation. Furthermore, by virtue of slight asymmetries in geometry, a NW's flexural modes are split into doublets oscillating along orthogonal axes. These characteristics make bottom-up grown NWs extremely sensitive vectorial force sensors. Here, taking advantage of its adaptability as a scanning probe, we use a single NW to image a sample surface. By monitoring the frequency shift and direction of oscillation of both modes as we scan above the surface, we construct a map of all spatial tip-sample force derivatives in the plane. Finally, we use the NW to image electric force fields distinguishing between forces arising from the NW charge and polarizability. This universally applicable technique enables a form of atomic force microscopy particularly suited to mapping the size and direction of weak tip-sample forces.

cond-mat.mes-hall↗

arXiv2015

Dynamic cantilever magnetometry of individual CoFeB nanotubes

We investigate single CoFeB nanotubes with hexagonal cross-section using dynamic cantilever magnetometry (DCM). We develop both an analytical model based on the Stoner-Wohlfarth approximation and a broadly applicable numerical framework for analyzing DCM measurements of magnetic nanostructures. Magnetometry data show the presence of a uniformly magnetized configuration at high external fields with $μ_0 M_s =1.3 \pm 0.1$ T and non-uniform configurations at low fields. In this low-field regime, comparison between numerical simulations and DCM measurements supports the existence of flux-closure configurations. Crucially, evidence of such configurations is only apparent because of the sensitivity of DCM to single nanotubes, whereas conventional measurements of ensembles are often obscured by sample-to-sample inhomogeneities in size, shape, and orientation

cond-mat.mes-hall↗

arXiv2015

Magnetization reversal of an individual exchange biased permalloy nanotube

We investigate the magnetization reversal mechanism in an individual permalloy (Py) nanotube (NT) using a hybrid magnetometer consisting of a nanometer-scale SQUID (nanoSQUID) and a cantilever torque sensor. The Py NT is affixed to the tip of a Si cantilever and positioned in order to optimally couple its stray flux into a Nb nanoSQUID. We are thus able to measure both the NT's volume magnetization by dynamic cantilever magnetometry and its stray flux using the nanoSQUID. We observe a training effect and temperature dependence in the magnetic hysteresis, suggesting an exchange bias. We find a low blocking temperature $T_B = 18 \pm 2$ K, indicating the presence of a thin antiferromagnetic native oxide, as confirmed by X-ray absorption spectroscopy on similar samples. Furthermore, we measure changes in the shape of the magnetic hysteresis as a function of temperature and increased training. These observations show that the presence of a thin exchange-coupled native oxide modifies the magnetization reversal process at low temperatures. Complementary information obtained via cantilever and nanoSQUID magnetometry allows us to conclude that, in the absence of exchange coupling, this reversal process is nucleated at the NT's ends and propagates along its length as predicted by theory.

cond-mat.mes-hall↗

arXiv2014

Boundary between the thermal and statistical polarization regimes in a nuclear spin ensemble

As the number of spins in an ensemble is reduced, the statistical uctuations in its polarization eventually exceed the mean thermal polarization. This transition has now been surpassed in a number of recent nuclear magnetic resonance experiments, which achieve nanometer-scale detection volumes. Here, we measure nanometer- scale ensembles of nuclear spins in a KPF6 sample using magnetic resonance force microscopy. In particular, we investigate the transition between regimes dominated by thermal and statistical nuclear polarization. The ratio between the two types of polarization provides a measure of the number of spins in the detected ensemble.

cond-mat.mes-hall↗

arXiv2014

Nonlinear motion and mechanical mixing in as-grown GaAs nanowires

We report nonlinear behavior in the motion of driven nanowire cantilevers. The nonlinearity can be described by the Duffing equation and is used to demonstrate mechanical mixing of two distinct excitation frequencies. Furthermore, we demonstrate that the nonlinearity can be used to amplify a signal at a frequency close to the mechanical resonance of the nanowire oscillator. Up to 26 dB of amplitude gain are demonstrated in this way.

cond-mat.mes-hall↗

arXiv2014

Quantum dot opto-mechanics in a fully self-assembled nanowire

We show that fully self-assembled optically-active quantum dots (QDs) embedded in MBE-grown GaAs/AlGaAs core-shell nanowires (NWs) are coupled to the NW mechanical motion. Oscillations of the NW modulate the QD emission energy in a broad range exceeding 14 meV. Furthermore, this opto-mechanical interaction enables the dynamical tuning of two neighboring QDs into resonance, possibly allowing for emitter-emitter coupling. Both the QDs and the coupling mechanism -- material strain -- are intrinsic to the NW structure and do not depend on any functionalization or external field. Such systems open up the prospect of using QDs to probe and control the mechanical state of a NW, or conversely of making a quantum non-demolition readout of a QD state through a position measurement.

cond-mat.mes-hall↗

arXiv2014

Vortex Lattice Melting of a NbSe2 single grain probed by Ultrasensitive Cantilever Magnetometry

Using dynamic cantilever magnetometry, we study the vortex lattice and its corresponding melting transition in a micrometer-size crystallite of superconducting NbSe2. Measurements of the cantilever resonance frequency as a function of magnetic field and temperature respond to the magnetization of the vortex-lattice. The cantilever dissipation depends on thermally activated vortex creep motion, whose pinning energy barrier is found to be in good agreement with transport measurements on bulk samples. This approach reveals the phase diagram of the crystallite, and is applicable to other micro- or nanometer-scale superconducting samples.

cond-mat.supr-con↗

arXiv2013

Harnessing nuclear spin polarization fluctuations in a semiconductor nanowire

Soon after the first measurements of nuclear magnetic resonance (NMR) in a condensed matter system, Bloch predicted the presence of statistical fluctuations proportional to $1/\sqrt{N}$ in the polarization of an ensemble of $N$ spins. First observed by Sleator et al., so-called "spin noise" has recently emerged as a critical ingredient in nanometer-scale magnetic resonance imaging (nanoMRI). This prominence is a direct result of MRI resolution improving to better than 100 nm^3, a size-scale in which statistical spin fluctuations begin to dominate the polarization dynamics. We demonstrate a technique that creates spin order in nanometer-scale ensembles of nuclear spins by harnessing these fluctuations to produce polarizations both larger and narrower than the natural thermal distribution. We focus on ensembles containing ~10^6 phosphorus and hydrogen spins associated with single InP and GaP nanowires (NWs) and their hydrogen-containing adsorbate layers. We monitor, control, and capture fluctuations in the ensemble's spin polarization in real-time and store them for extended periods. This selective capture of large polarization fluctuations may provide a route for enhancing the weak magnetic signals produced by nanometer-scale volumes of nuclear spins. The scheme may also prove useful for initializing the nuclear hyperfine field of electron spin qubits in the solid-state.

cond-mat.mes-hall↗

arXiv2013

Reversal mechanism of an individual Ni nanotube simultaneously studied by torque and SQUID magnetometry

Using an optimally coupled nanometer-scale superconducting quantum interference device, we measure the magnetic flux originating from an individual ferromagnetic Ni nanotube attached to a Si cantilever. At the same time, we detect the nanotube's volume magnetization using torque magnetometry. We observe both the predicted reversible and irreversible reversal processes. A detailed comparison with micromagnetic simulations suggests that vortex-like states are formed in different segments of the individual nanotube. Such stray-field free states are interesting for memory applications and non-invasive sensing.

cond-mat.mes-hall↗

arXiv2013

Nanoscale multifunctional sensor formed by a Ni nanotube and a scanning Nb nanoSQUID

Nanoscale magnets might form the building blocks of next generation memories. To explore their functionality, magnetic sensing at the nanoscale is key. We present a multifunctional combination of a scanning nanometer-sized superconducting quantum interference device (nanoSQUID) and a Ni nanotube attached to an ultrasoft cantilever as a magnetic tip. We map out and analyze the magnetic coupling between the Ni tube and the Nb nanoSQUID, demonstrate imaging of an Abrikosov vortex trapped in the SQUID structure - which is important in ruling out spurious magnetic signals - and reveal the high potential of the nanoSQUID as an ultrasensitive displacement detector. Our results open a new avenue for fundamental studies of nanoscale magnetism and superconductivity.

cond-mat.supr-con↗

arXiv2012

Feedback cooling of cantilever motion using a quantum point contact transducer

We use a quantum point contact (QPC) as a displacement transducer to measure and control the low-temperature thermal motion of a nearby micromechanical cantilever. The QPC is included in an active feedback loop designed to cool the cantilever's fundamental mechanical mode, achieving a squashing of the QPC noise at high gain. The minimum achieved effective mode temperature of 0.2 K and the displacement resolution of 10^(-11) m/Hz^(1/2) are limited by the performance of the QPC as a one-dimensional conductor and by the cantilever-QPC capacitive coupling.

cond-mat.mes-hall↗

arXiv2011

Measurement of statistical nuclear spin polarization in a nanoscale GaAs sample

We measure the statistical polarization of quadrupolar nuclear spins in a sub-micrometer (0.6 um^3) particle of GaAs using magnetic resonance force microscopy. The crystalline sample is cut out of a GaAs wafer and attached to a micro-mechanical cantilever force sensor using a focused ion beam technique. Nuclear magnetic resonance is demonstrated on ensembles containing less than 5 x 10^8 nuclear spins and occupying a volume of around (300 nm)^3 in GaAs with reduced volumes possible in future experiments. We discuss how the further reduction of this detection volume will bring the spin ensemble into a regime where random spin fluctuations, rather than Boltzmann polarization, dominate its dynamics. The detection of statistical polarization in GaAs therefore represents an important first step toward 3D magnetic resonance imaging of III-V materials on the nanometer-scale.

cond-mat.mes-hall↗

arXiv2011

Probing single charge fluctuations in a semiconductor with laser spectroscopy on a quantum dot

We probe local charge fluctuations in a semiconductor via laser spectroscopy on a nearby self-assembled quantum dot. We demonstrate that the quantum dot is sensitive to changes in the local environment at the single charge level. By controlling the charge state of localized defects, we are able to infer the distance of the defects from the quantum dot with +-5 nm resolution. The results identify and quantify the main source of charge noise in the commonly-used optical field-effect devices. Based on this understanding we achieve routinely close-totransform-limited quantum dot optical linewidths.

cond-mat.mes-hall↗

arXiv2011

A geometry for optimizing nanoscale magnetic resonance force microscopy

We implement magnetic resonance force microscopy (MRFM) in an experimental geometry, where the long axis of the cantilever is normal to both the external magnetic field and the RF microwire source. Measurements are made of the statistical polarization of $^1$H in polystyrene with negligible magnetic dissipation, gradients greater than $10^5$ T/m within 100 nm of the magnetic tip, and rotating RF magnetic fields over 12 mT at 115 MHz. This geometry could facilitate the application of nanometer-scale MRFM to nuclear species with low gyro-magnetic ratios and samples with broadened resonances, such as In spins in quantum dots.

cond-mat.mes-hall↗

arXiv2010

Force-detected nuclear magnetic resonance: Recent advances and future challenges

We review recent efforts to detect small numbers of nuclear spins using magnetic resonance force microscopy. Magnetic resonance force microscopy (MRFM) is a scanning probe technique that relies on the mechanical measurement of the weak magnetic force between a microscopic magnet and the magnetic moments in a sample. Spurred by the recent progress in fabricating ultrasensitive force detectors, MRFM has rapidly improved its capability over the last decade. Today it boasts a spin sensitivity that surpasses conventional, inductive nuclear magnetic resonance detectors by about eight orders of magnitude. In this review we touch on the origins of this technique and focus on its recent application to nanoscale nuclear spin ensembles, in particular on the imaging of nanoscale objects with a three-dimensional (3D) spatial resolution better than 10 nm. We consider the experimental advances driving this work and highlight the underlying physical principles and limitations of the method. Finally, we discuss the challenges that must be met in order to advance the technique towards single nuclear spin sensitivity -- and perhaps -- to 3D microscopy of molecules with atomic resolution.

cond-mat.mes-hall↗

arXiv2008

Force-detected nuclear double resonance between statistical spin polarizations

We demonstrate nuclear double resonance for nanometer-scale volumes of spins where random fluctuations rather than Boltzmann polarization dominate. When the Hartmann-Hahn condition is met in a cross-polarization experiment, flip-flops occur between two species of spins and their fluctuations become coupled. We use magnetic resonance force microscopy to measure this effect between 1H and 13C spins in 13C-enriched stearic acid. The development of a cross-polarization technique for statistical ensembles adds an important tool for generating chemical contrast in nanometer-scale magnetic resonance.

cond-mat.stat-mech↗

arXiv2008

Overhauser frequency shifts in semiconductor nanostructures

We calculate the Overhauser frequency shifts in semiconductor nanostructures resulting from the hyperfine interaction between nonequilibrium electronic spins and nuclear spins. The frequency shifts depend on the electronic local density of states and spin polarization as well as the electronic and nuclear spin relaxation mechanisms. Unlike previous calculations, our method accounts for the electron confinement in low dimensional semiconductor nanostructures, resulting in both nuclear spin polarizations and Overhauser shifts that are strongly dependent on position. Our results explain previously puzzling measurements of Overhauser shifts in an Al$_x$Ga$_{1-x}$As parabolic quantum well by showing the connection between the electron spin lifetime and the frequency shifts.

cond-mat.mtrl-sci↗

arXiv2008

An off-board quantum point contact as a sensitive detector of cantilever motion

Recent advances in the fabrication of microelectromechanical systems (MEMS) and their evolution into nanoelectromechanical systems (NEMS) have allowed researchers to measure extremely small forces, masses, and displacements. In particular, researchers have developed position transducers with resolution approaching the uncertainty limit set by quantum mechanics. The achievement of such resolution has implications not only for the detection of quantum behavior in mechanical systems, but also for a variety of other precision experiments including the bounding of deviations from Newtonian gravity at short distances and the measurement of single spins. Here we demonstrate the use of a quantum point contact (QPC) as a sensitive displacement detector capable of sensing the low-temperature thermal motion of a nearby micromechanical cantilever. Advantages of this approach include versatility due to its off-board design, compatibility with nanoscale oscillators, and, with further development, the potential to achieve quantum limited displacement detection.

cond-mat.mes-hall↗