arXiv subjects

M. Poggio

Publications and source records attributed to M. Poggio.

48 records · Page 3Linked to original sources

arXiv2007

Nuclear spin relaxation induced by a mechanical resonator

We report on measurements of the spin lifetime of nuclear spins strongly coupled to a micromechanical cantilever as used in magnetic resonance force microscopy. We find that the rotating-frame correlation time of the statistical nuclear polarization is set by the magneto-mechanical noise originating from the thermal motion of the cantilever. Evidence is based on the effect of three parameters: (1) the magnetic field gradient (the coupling strength), (2) the Rabi frequency of the spins (the transition energy), and (3) the temperature of the low-frequency mechanical modes. Experimental results are compared to relaxation rates calculated from the spectral density of the magneto-mechanical noise.

cond-mat.mes-hall↗

arXiv2007

The role of spin noise in the detection of nanoscale ensembles of nuclear spins

When probing nuclear spins in materials on the nanometer scale, random fluctuations of the spin polarization will exceed the mean Boltzmann polarization for sample volumes below about (100nm)^3. In this work, we use magnetic resonance force microscopy to observe nuclear spin fluctuations in real time. We show how reproducible measurements of the polarization variance can be obtained by controlling the spin correlation time and rapidly sampling a large number of independent spin configurations. A protocol to periodically randomize the spin ensemble is demonstrated, allowing significant improvement in the signal-to-noise ratio for nanometer-scale magnetic resonance imaging.

cond-mat.mes-hall↗

arXiv2007

Nuclear magnetic resonance force microscopy with a microwire rf source

We use a 1.0-um-wide patterned Cu wire with an integrated nanomagnetic tip to measure the statistical nuclear polarization of 19F in CaF2 by magnetic resonance force microscopy (MRFM). With less than 350 uW of dissipated power, we achieve rf magnetic fields over 4 mT at 115 MHz for a sample positioned within 100 nm of the "microwire" rf source. A 200-nm diameter FeCo tip integrated onto the wire produces field gradients greater than 10^5 T/m at the same position. The large rf fields from the broadband microwire enable long rotating-frame spin lifetimes of up to 15 s at 4 K.

cond-mat.other↗

arXiv2007

Nuclear Magnetic Resonance Imaging with 90 nm Resolution

Magnetic resonance imaging, based on the manipulation and detection of nuclear spins, is a powerful imaging technique that typically operates on the scale of millimeters to microns. Using magnetic resonance force microscopy, we have demonstrated that magnetic resonance imaging of nuclear spins can be extended to a spatial resolution better than 100 nm. The two-dimensional imaging of 19F nuclei was done on a patterned CaF2 test object, and was enabled by a detection sensitivity of roughly 1200 nuclear spins. To achieve this sensitivity, we developed high-moment magnetic tips that produced field gradients up to 1.4x10^6 T/m, and implemented a measurement protocol based on force-gradient detection of naturally occurring spin fluctuations. The resulting detection volume of less than 650 zl represents 60,000x smaller volume than previous NMR microscopy and demonstrates the feasibility of pushing magnetic resonance imaging into the nanoscale regime.

cond-mat.other↗

arXiv2007

Feedback cooling of a cantilever's fundamental mode below 5 mK

We cool the fundamental mechanical mode of an ultrasoft silicon cantilever from a base temperature of 2.2 K to 2.9 +/- 0.3 mK using active optomechanical feedback. The lowest observed mode temperature is consistent with limits determined by the properties of the cantilever and by the measurement noise. For high feedback gain, the driven cantilever motion is found to suppress or "squash" the optical interferometer intensity noise below the shot noise level.

cond-mat.other↗

arXiv2006

Confinement engineering of s-d exchange interactions in GaMnAs quantum wells

Recent measurements of coherent electron spin dynamics reveal an antiferromagnetic s-d exchange coupling between conduction band electrons and electrons localized on Mn{2+} impurities in GaMnAs quantum wells. Here we discuss systematic measurements of the s-d exchange interaction in GaMnAs/AlGaAs quantum wells with different confinement potentials using time-resolved Kerr rotation. Extending previous investigations of the dependence of the s-d exchange, N{0}alpha, on well width, we find that its magnitude also depends on well depth. Both phenomena reduce to a general dependence on confinement energy, described by a band-mixing model of confinement-induced kinetic exchange in the conduction band.

cond-mat.mes-hall↗

arXiv2005

Structural, electrical, and magneto-optical characterization of paramagnetic GaMnAs quantum wells

Growth of GaMnAs by molecular beam epitaxy is typically performed at low substrate temperatures (250C) and high As overpressures leading to the incorporation of excess As and Mn interstitials, which quench optical signals such as photoluminescence (PL). We report on optical-quality Ga(1-x)Mn(x)As/Al(0.4)Ga(0.6)As quantum wells (QWs) with x < 0.2% grown at a substrate temperature of 400C. Electrical and structural measurements demonstrate that this elevated temperature reduces As defects while allowing the substitutional incorporation of Mn into Ga sites. From a combination of Hall and secondary ion mass spectroscopy measurements we estimate that at least 70-90% of the Mn incorporates substitutionally in all samples studied. The incorporation behavior shows both a substrate temperature and QW width dependence. The lower defect density of these heterostructures, compared to typical lower temperature grown GaMnAs, enables the observation of both polarization-resolved PL and coherent electron spin dynamics, from which the conduction band exchange parameter is extracted. No evidence of long-range Mn spin coupling is observed, whereas negative effective Curie temperatures indicate spin heating due to photoexcitation. The electron spin lifetime is maximized for light Mn doping and shows little magnetic field dependence indicating that the Dyakonov-Perel mechanism is dominant in these structures. PL spectra reveal a low energy peak from shallow donors, which because of the paramagnetic behavior of its PL polarization, we ascribe to Mn interstitials.

cond-mat.mtrl-sci↗

arXiv2005

Spin dynamics in electrochemically charged CdSe quantum dots

We use time-resolved Faraday rotation to measure coherent spin dynamics in colloidal CdSe quantum dots charged in an electrochemical cell at room temperature. Filling of the 1Se electron level is demonstrated by the bleaching of the 1Se-1S3/2 absorption peak. One of the two Lande g-factors observed in uncharged quantum dots disappears upon filling of the 1Se electron state. The transverse spin coherence time, which is over 1 ns and is limited by inhomogeneous dephasing, also appears to increase with charging voltage. The amplitude of the spin precession signal peaks near the half-filling potential. Its evolution at charging potentials without any observable bleaching of the 1Se-1S3/2 transition suggests that the spin dynamics are influenced by low-energy surface states.

cond-mat.other↗

arXiv2005

Antiferromagnetic s-d exchange coupling in GaMnAs

Measurements of coherent electron spin dynamics in Ga(1-x)Mn(x)As/Al(0.4)Ga(0.6)As quantum wells with 0.0006% < x < 0.03% show an antiferromagnetic (negative) exchange bewteen s-like conduction band electrons and electrons localized in the d-shell of the Mn2+ impurities. The magnitude of the s-d exchange parameter, N0 alpha, varies as a function of well width indicative of a large and negative contribution due to kinetic exchange. In the limit of no quantum confinement, N0 alpha extrapolates to -0.09 +/- 0.03 eV indicating that antiferromagnetic s-d exchange is a bulk property of GaMnAs. Measurements of the polarization-resolved photoluminescence show strong discrepancy from a simple model of the exchange enhanced Zeeman splitting, indicative of additional complexity in the exchange split valence band.

cond-mat.mtrl-sci↗

arXiv2005

High-field optically detected nuclear magnetic resonance in GaAs

A method for high-field optically detected nuclear magnetic resonance (ODNMR) is developed sensitive to 10**8 nuclei. Nuclear spin transitions are induced using a radio frequency coil and detected through Faraday rotation spectroscopy. Unlike conventional ODNMR, which is limited to low fields and relies on the measurement of time-averaged luminescence polarization, this technique monitors nuclear polarization through time-resolved measurements of electron spin dynamics. Measurements in a (110) GaAs quantum well reveal Ga-69, Ga-71, and As-75 resonances and their quadrupolar splittings while resolving changes in nuclear polarization of 0.02%.

cond-mat.mes-hall↗

arXiv2004

Spin transfer and coherence in coupled quantum wells

Spin dynamics of optically excited electrons confined in asymmetric coupled quantum wells are investigated through time resolved Faraday rotation experiments. The inter-well coupling is shown to depend on applied electric field and barrier thickness. We observe three coupling regimes: independent spin precession in isolated quantum wells, incoherent spin transfer between single-well states, and coherent spin transfer in a highly coupled system. Relative values of the inter-well tunneling time, the electron spin lifetime, and the Larmor precession period appear to govern this behavior.

cond-mat.mes-hall↗

arXiv2003

Local Manipulation of Nuclear Spin in a Semiconductor Quantum Well

The shaping of nuclear spin polarization profiles and the induction of nuclear resonances are demonstrated within a parabolic quantum well using an externally applied gate voltage. Voltage control of the electron and hole wave functions results in nanometer-scale sheets of polarized nuclei positioned along the growth direction of the well. RF voltages across the gates induce resonant spin transitions of selected isotopes. This depolarizing effect depends strongly on the separation of electrons and holes, suggesting that a highly localized mechanism accounts for the observed behavior.

cond-mat.mes-hall↗