arXiv subjects

M. R. Buitelaar

Publications and source records attributed to M. R. Buitelaar.

18 recordsLinked to original sources

arXiv2025

Synthetic spin-orbit coupling in superconductor-semiconductor hybrid nanowires with micromagnet arrays

Spin-orbit interaction accounts for the coupling of momentum and spin degrees of freedom of electrons and holes in semiconductor materials. In quantum information processing, it allows for electrical control of spin states and for the engineering of topologically protected Majorana zero modes. Although such functionalities were previously considered to be limited to semiconductor materials with strong intrinsic spin-orbit interactions only, recent theoretical work proposes using external rotating magnetic fields to engineer synthetic spin-orbit coupling. This would relax material constraints and open up new research directions for materials with low intrinsic spin-orbit interaction or augment existing spin-orbit interaction in materials in which this interaction is already strong. Here we demonstrate the feasibility of this approach and introduce rotating magnetic fields along an InAs/Al hybrid nanowire using permalloy micromagnet arrays which yields an estimated synthetic Rashba spin-orbit interaction coefficient of 0.022 eV nm. We use transport spectroscopy and the energy dependence of Andreev bound states in the nanowires as a probe of the magnetic field profiles of the micromagnets which are reconfigurably prepared in parallel or antiparallel magnetization configurations.

cond-mat.mes-hall↗

arXiv2020

Quantum paraelectric varactors for radio-frequency measurements at mK temperatures

Radio-frequency reflectometry allows for fast and sensitive electrical readout of charge and spin qubits hosted in quantum dot devices coupled to resonant circuits. Optimizing readout, however, requires frequency tuning of the resonators and impedance matching. This is difficult to achieve using conventional semiconductor or ferroelectric-based varactors in the detection circuit as their performance degrades significantly in the mK temperature range relevant for solid-state quantum devices. Here we explore a different type of material, strontium titanate, a quantum paraelectric with exceptionally large field-tunable permittivity at low temperatures. Using strontium titanate varactors we demonstrate perfect impedance matching and resonator frequency tuning at 6 mK and characterize the varactors at this temperature in terms of their capacitance tunability, dissipative losses and magnetic field sensitivity. We show that this allows us to optimize the radio-frequency readout signal-to-noise ratio of carbon nanotube quantum dot devices to achieve a charge sensitivity of 4.8 $μ$e/Hz$^{1/2}$ and capacitance sensitivity of 0.04 aF/Hz$^{1/2}$.

cond-mat.mes-hall↗

arXiv2017

Microwave spectroscopy of a carbon nanotube charge qubit

Carbon nanotube quantum dots allow accurate control of electron charge, spin and valley degrees of freedom in a material which is atomically perfect and can be grown isotopically pure. These properties underlie the unique potential of carbon nanotubes for quantum information processing, but developing nanotube charge, spin, or spin-valley qubits requires efficient readout techniques as well as understanding and extending quantum coherence in these devices. Here, we report on microwave spectroscopy of a carbon nanotube charge qubit in which quantum information is encoded in the spatial position of an electron. We combine radio-frequency reflectometry measurements of the quantum capacitance of the device with microwave manipulation to drive transitions between the qubit states. This approach simplifies charge-state readout and allows us to operate the device at an optimal point where the qubit is first-order insensitive to charge noise. From these measurements, we are able to quantify the degree of charge noise experienced by the qubit and obtain an inhomogeneous charge coherence of 5 ns. We use a chopped microwave signal whose duty-cycle period is varied to measure the decay of the qubit states, yielding a charge relaxation time of 48 ns.

cond-mat.mes-hall↗

arXiv2015

Vortex detection and quantum transport in mesoscopic graphene Josephson junction arrays

We investigate mesoscopic Josephson junction arrays created by patterning superconducting disks on monolayer graphene, concentrating on the high-$T/T_c$ regime of these devices and the phenomena which contribute to the superconducting glass state in diffusive arrays. We observe features in the magnetoconductance at rational fractions of flux quanta per array unit cell, which we attribute to the formation of flux-quantized vortices. The applied fields at which the features occur are well described by Ginzburg-Landau simulations that take into account the number of unit cells in the array. We find that the mean conductance and universal conductance fluctuations are both enhanced below the critical temperature and field of the superconductor, with greater enhancement away from the graphene Dirac point.

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arXiv2015

Radio-frequency capacitance spectroscopy of metallic nanoparticles

Recent years have seen great progress in our understanding of the electronic properties of nanomaterials in which at least one dimension measures less than 100 nm. However, contacting true nanometer scale materials such as individual molecules or nanoparticles remains a challenge as even state-of-the-art nanofabrication techniques such as electron-beam lithography have a resolution of a few nm at best. Here we present a fabrication and measurement technique that allows high sensitivity and high bandwidth readout of discrete quantum states of metallic nanoparticles which does not require nm resolution or precision. This is achieved by coupling the nanoparticles to resonant electrical circuits and measurement of the phase of a reflected radio-frequency signal. This requires only a single tunnel contact to the nanoparticles thus simplifying device fabrication and improving yield and reliability. The technique is demonstrated by measurements on 2.7 nm thiol coated gold nanoparticles which are shown to be in excellent quantitative agreement with theory.

cond-mat.mes-hall↗

arXiv2013

Transport Spectroscopy of a Graphene Quantum Dot Fabricated by Atomic Force Microscope Nanolithography

We report low-temperature transport spectroscopy of a graphene quantum dot fabricated by atomic force microscope nanolithography. The excellent spatial resolution of the atomic force microscope allows us to reliably fabricate quantum dots with short constrictions of less than 15 nm in length. Transport measurements demonstrate that the device is dominated by a single quantum dot over a wide gate range. The electron spin system of the quantum dot is investigated by applying an in-plane magnetic field. The results are consistent with a Lande g-factor of 2 but no regular spin filling sequence is observed, most likely due to disorder.

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arXiv2012

Tunable Kondo physics in a carbon nanotube double quantum dot

We investigate a tunable two-impurity Kondo system in a strongly correlated carbon nanotube double quantum dot, accessing the full range of charge regimes. In the regime where both dots contain an unpaired electron, the system approaches the two-impurity Kondo model. At zero magnetic field the interdot coupling disrupts the Kondo physics and a local singlet state arises, but we are able to tune the crossover to a Kondo screened phase by application of a magnetic field. All results show good agreement with a numerical renormalization group study of the device.

cond-mat.mes-hall↗

arXiv2012

Quantized Charge Pumping through a Carbon Nanotube Double Quantum Dot

We demonstrate single-electron pumping in a gate-defined carbon nanotube double quantum dot. By periodic modulation of the potentials of the two quantum dots we move the system around charge triple points and transport exactly one electron or hole per cycle. We investigate the pumping as a function of the modulation frequency and amplitude and observe good current quantization up to frequencies of 18 MHz where rectification effects cause the mechanism to break down.

cond-mat.mes-hall↗

arXiv2011

Measuring the complex admittance of a carbon nanotube double quantum dot

We investigate radio-frequency (rf) reflectometry in a tunable carbon nanotube double quantum dot coupled to a resonant circuit. By measuring the in-phase and quadrature components of the reflected rf signal, we are able to determine the complex admittance of the double quantum dot as a function of the energies of the single-electron states. The measurements are found to be in good agreement with a theoretical model of the device in the incoherent limit. Besides being of fundamental interest, our results present an important step forward towards non-invasive charge and spin state readout in carbon nanotube quantum dots.

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arXiv2011

Atomic force microscope nanolithography of graphene: cuts, pseudo-cuts and tip current measurements

We investigate atomic force microscope nanolithography of single and bilayer graphene. In situ tip current measurements show that cutting of graphene is not current driven. Using a combination of transport measurements and scanning electron microscopy we show that, while indentations accompanied by tip current appear in the graphene lattice for a range of tip voltages, real cuts are characterized by a strong reduction of the tip current above a threshold voltage. The reliability and flexibility of the technique is demonstrated by the fabrication, measurement, modification and re-measurement of graphene nanodevices with resolution down to 15 nm.

cond-mat.mes-hall↗

arXiv2010

Single Spin Detection with a Carbon Nanotube Double Quantum Dot

Spin qubits defined in carbon nanotube quantum dots are of considerable interest for encoding and manipulating quantum information because of the long electron spin coherence times expected. However, before carbon nanotubes can find applications in quantum information processing schemes, we need to understand and control the coupling between individual electron spins and the interaction between the electron spins and their environment. Here we make use of spin selection rules to directly measure - and demonstrate control of - the singlet-triplet exchange coupling between two carbon nanotube quantum dots. We furthermore elucidate the effects of spin-orbit interaction on the electron transitions and investigate the interaction of the quantum dot system with a single impurity spin - the ultimate limit in spin sensitivity.

cond-mat.mes-hall↗

arXiv2008

Pauli spin blockade in carbon nanotube double quantum dots

We report Pauli spin blockade in an impurity defined carbon nanotube double quantum dot. We observe a pronounced current suppression for negative source-drain bias voltages which is investigated for both symmetric and asymmetric coupling of the quantum dots to the leads. The measured differential conductance agrees well with a theoretical model of a double quantum dot system in the spin-blockade regime which allows us to estimate the occupation probabilities of the relevant singlet and triplet states. This work shows that effective spin-to-charge conversion in nanotube quantum dots is feasible and opens the possibility of single-spin readout in a material that is not limited by hyperfine interaction with nuclear spins.

cond-mat.mes-hall↗

arXiv2008

Charge pumping in carbon nanotube quantum dots

We investigate charge pumping in carbon nanotube quantum dots driven by the electric field of a surface acoustic wave. We find that at small driving amplitudes, the pumped current reverses polarity as the conductance is tuned through a Coulomb blockade peak using a gate electrode. We study the behavior as a function of wave amplitude, frequency and direction and develop a model in which our results can be understood as resulting from adiabatic charge redistribution between the leads and quantum dots on the nanotube.

cond-mat.mes-hall↗

arXiv2004

Conductance properties of nanotubes coupled to superconducting leads: signatures of Andreev states dynamics

We present a combined experimental and theoretical analysis of the low bias conductance properties of carbon nanotubes coupled to superconducting leads. In the Kondo regime the conductance exhibits a zero bias peak which can be several times larger than the unitary limit in the normal case. This zero bias peak can be understood by analyzing the dynamics of the subgap Andreev states under an applied bias voltage. It is shown that the existence of a linear regime is linked to the presence of a finite relaxation rate within the system. The theory provides a good fitting of the experimental results.

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arXiv2003

Multiple Andreev Reflections in a Carbon Nanotube Quantum Dot

We report resonant multiple Andreev relections in a multiwall carbon nanotube quantum dot coupled to superconducting leads. The position and magnitude of the subharmonic gap structure is found to depend strongly on the level positions of the single-electron states which are adjusted with a gate electrode. We discuss a theoretical model of the device and compare the calculated differential conductance with the experimental data. (pdf including figures, see: www.unibas.ch/phys-meso/Research/Papers/2003/MAR-MWNT.pdf)

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arXiv2002

A Quantum Dot in the Kondo Regime Coupled to Superconductors

The Kondo effect and superconductivity are both prime examples of many-body phenomena. Here we report transport measurements on a carbon nanotube quantum dot coupled to superconducting leads that show a delicate interplay between both effects. We demonstrate that the superconductivity of the leads does not destroy the Kondo correlations on the quantum dot when the Kondo temperature, which varies for different single-electron states, exceeds the superconducting gap energy.

cond-mat.mes-hall↗

arXiv2001

Multi-wall carbon nanotubes as quantum dots

We have measured the differential conductance dI/dV of individual multi-wall carbon nanotubes (MWNT) of different lengths. A cross-over from wire-like (long tubes) to dot-like (short tubes) behavior is observed. dI/dV is dominated by random conductance fluctuations (UCF) in long MWNT devices (L=2...7 $μm$), while Coulomb blockade and energy level quantization are observed in short ones (L=300 nm). The electron levels of short MWNT dots are nearly four-fold degenerate (including spin) and their evolution in magnetic field (Zeeman splitting) agrees with a g-factor of 2. In zero magnetic field the sequential filling of states evolves with spin S according to S=0 -> 1/2 -> 0... In addition, a Kondo enhancement of the conductance is observed when the number of electrons on the tube is odd.

cond-mat.mes-hall↗

arXiv2000

The Electrochemical Carbon Nanotube Field-Effect Transistor

We explore the electric-field effect of carbon nanotubes (NTs) in electrolytes. Due to the large gate capacitance, Fermi energy shifts of order +/- 1 V can be induced, enabling to tune NTs from p to n-type. Consequently, large resistance changes are measured. At zero gate voltage the NTs are hole doped in air with E_F ? 0.3-0.5 eV, corresponding to a doping level of ? 10^{13} cm^{-2}. Hole-doping increases in the electrolyte. This hole doping (oxidation) is most likely caused by the adsorption of oxygen in air and cations in the electrolyte.

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