arXiv subjects

M. Redshaw

Publications and source records attributed to M. Redshaw.

At least 19 recordsLinked to original sources

arXiv2026

First direct measurement of $^{48}$Ca single $\beta$-decay Q value with the TITAN Penning trap

Neutrinoless double $\beta$-decay (0$\nu\beta\beta$), if observed, would provide unequivocal evidence of physics beyond the Standard Model. $^{48}$Ca is an interesting candidate system to study because it has the largest Q value among all 2$\beta$ transitions and is also unstable against single $\beta$-decay. The observation of both $\beta$ and 2$\beta$-decay in the same isotope would provide a unique opportunity to benchmark theoretical calculations of $\beta$ and 2$\beta$-decay matrix elements and could provide insight on the quenching of the axial vector coupling constant, g$_A$. We performed a precise measurement of the $^{48}$Ca $\beta$-decay Q value using the TITAN Penning trap mass spectrometer at the TRIUMF facility. This was achieved through cyclotron frequency ratio measurements of $^{48}$Ca$^{+}$/$^{48}$Sc$^{+}$ and $^{48}$Sc$^{+}$/$^{48}$Ti$^{+}$ using the Time-of-Flight Ion Cyclotron Resonance technique. The $^{48}$Ca $\beta$-decay Q value was determined to be 279.14(50) keV, a factor of 10 more precise than the previous value given in the 2020 Atomic Mass Evaluation [Chin. Phys. C 45, 030003 (2021)]. This Q value was used to determine the $^{48}$Ca $\beta$-decay partial half-life, with the result $T_{1/2}^{\beta}$ = 5.09(5) x 10$^{20}$ ($g_{A}^{-2}$) y. Our $^{48}$Ca $\beta$-decay half-life was determined to a precision of 1%, a factor of 30 improvement compared to calculations with the previous Q value. Our result is marginally closer to the experimental lower limit $T_{1/2}^{\beta}$ > 1.1 x 10$^{20}$ y, but still a factor 5 longer. It is also a factor of 10 longer than the observed 2$\nu\beta\beta$ decay mode with $T_{1/2}^{2\nu\beta\beta} = 5.96^{+1.39}_{-1.08}$ x 10$^{19}$ y. Hence, it could be possible to observe $^{48}$Ca $\beta$-decay in future experiments, strengthening the potential importance of $^{48}$Ca to benchmark nuclear structure and 2$\beta$-decay studies.

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arXiv2024

High-precision mass measurement of $^{103}$Sn restores smoothness of the mass surface

As a step towards the ultimate goal of a high-precision mass measurement of doubly-magic $^{100}$Sn, the mass of $^{103}$Sn was measured at the Low Energy Beam and Ion Trap (LEBIT) located at the Facility for Rare Isotope Beams (FRIB). Utilizing the time-of-flight ion cyclotron resonance (ToF-ICR) technique, a mass uncertainty of 3.7~keV was achieved, an improvement by more than an order of magnitude compared to a recent measurement performed in 2023 at the Cooler Storage Ring (CSRe) in Lanzhou. Although the LEBIT and CSRe mass measurements of $^{103}$Sn are in agreement, they diverge from the experimental mass value reported in the 2016 version of the Atomic Mass Evaluation (AME2016), which was derived from the measured $Q_{\beta^+}$ value and the mass of $^{103}$In. In AME2020, this indirectly measured $^{103}$Sn mass was classified as a `seriously irregular mass' and replaced with an extrapolated value, which aligns with the most recent measured values from CSRe and LEBIT. As such, the smoothness of the mass surface is confidently reestablished for $^{103}$Sn. Furthermore, LEBIT's mass measurement of $^{103}$Sn enabled a significant reduction in the mass uncertainties of five parent isotopes which are now dominated by uncertainties in their respective $Q$-values.

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arXiv2023

First direct $^{7}$Be electron capture $Q$-value measurement towards high-precision BSM neutrino physics searches

We report the first direct measurement of the nuclear electron capture (EC) decay $Q$-value of $^{7}$Be $\rightarrow$ $^{7}$Li via high-precision Penning trap mass spectrometry (PTMS). This was performed using the LEBIT Penning trap located at the National Superconducting Cyclotron Laboratory/Facility for Rare Isotope Beams (NSCL/FRIB) using the newly commissioned Batch-Mode Ion-Source (BMIS) to deliver the unstable $^{7}$Be$^{+}$ samples. With a measured value of $Q_{EC}$ = 861.963(23) keV this result is also three times more precise than any previous determination of this quantity. This improved precision, and accuracy of the $^7$Be EC decay $Q$-value is critical for ongoing experiments that measure the recoiling nucleus in this system as a signature to search for beyond Standard Model (BSM) neutrino physics using $^7$Be-doped superconducting sensors.

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arXiv2023

Mass Measurement of $^{27}$P to Constrain Type-I X-ray Burst Models and Validate the IMME for the A=27, T=$\frac{3}{2}$ Isospin Quartet

Light curves are the primary observable of type-I x-ray bursts. Computational x-ray burst models must match simulations to observed light curves. Most of the error in simulated curves comes from uncertainties in $rp$ process reaction rates, which can be reduced via precision mass measurements of neutron-deficient isotopes in the $rp$ process path. We perform a precise Penning trap mass measurement of $^{27}$P utilizing the ToF-ICR technique. We use this measurement to calculate $rp$ process reaction rates and input these rates into an x-ray burst model to reduce simulated light curve uncertainty. We also use the mass measurement of $^{27}$P to validate the Isobaric Multiplet Mass Equation (IMME) for the A=27 T=$\frac{3}{2}$ isospin quartet which $^{27}$P belongs to. The mass excess of $^{27}$P was measured to be -670.7(6) keV, a fourteen-fold precision increase over the mass reported in the 2020 Atomic Mass Evaluation (AME2020). X-ray burst light curves were produced with the MESA (Modules for Experiments in Stellar Astrophysics) code using the new mass and associated reaction rates. Changes in the mass of $^{27}$P seem to have minimal effect on light curves, even in burster systems tailored to maximize impact. The mass of $^{27}$P does not play a significant role in x-ray burst light curves. It is important to understand that more advanced models do not just provide more precise results, but often qualitatively different ones. This result brings us a step closer to extracting stellar parameters from individual x-ray burst observations. The IMME has been validated for the $A=27, T=3/2$ quartet. The normal quadratic form of the IMME using the latest data yields a reduced $\chi^2$ of 2.9. The cubic term required to generate an exact fit to the latest data matches theoretical attempts to predict this term.

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arXiv2023

Nuclear $\beta$ decay as a probe for physics beyond the Standard Model

This white paper was submitted to the 2022 Fundamental Symmetries, Neutrons, and Neutrinos (FSNN) Town Hall Meeting in preparation for the next NSAC Long Range Plan. We advocate to support current and future theoretical and experimental searches for physics beyond the Standard Model using nuclear $\beta$ decay.

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arXiv2022

Identification of a potential ultra-low Q value electron capture decay branch in $^{75}$Se via a precise Penning trap measurement of the mass of $^{75}$As

Background: Low energy $\beta$ and electron capture (EC) decays are important systems in neutrino mass determination experiments. An isotope with an ultra-low Q value $\beta$-decay to an excited state in the daughter with Qes < 1 keV could provide a promising alternative candidate for future experiments. $^{75}$Se EC and $^{75}$Ge $\beta$-decay represent such candidates, but a more precise determination of the mass of the common daughter, $^{75}$As, is required to evaluate whether their potential decay branches are energetically allowed and ultra-low. Purpose: Perform a precise atomic mass measurement of $^{75}$As and combine the result with the precisely known atomic masses of $^{75}$Se and $^{75}$Ge, along with nuclear energy level data for $^{75}$As to evaluate potential ultra-low Q value decay branches in the EC decay of $^{75}$Se and the $\beta$-decay of $^{75}$Ge. Method: The LEBIT Penning trap mass spectrometer at the Facility for Rare Isotope Beams was used to perform a high-precision measurement of the atomic mass of $^{75}$As via cyclotron frequency ratio measurements of $^{75}$As$^{+}$ to a $^{12}$C$_{6}^{+}$ reference ion. Results: The $^{75}$As mass excess was determined to be ME($^{75}$As)= -73 035.98(43) keV, from which the ground-state to ground-state Q values for $^{75}$Se EC and $^{75}$Ge $\beta$-decay were determined to be 866.50(44) keV and 1179.01(44) keV, respectively. These results were compared to energies of excited states in $^{75}$As at 865.4(5) keV and 1172.0(6) keV to determine Q values of 1.1(7) keV and 7.0(7) keV for the potential ultra-low EC and $\beta$-decay branches of $^{75}$Se and $^{75}$Ge, respectively. Conclusion: The $^{75}$Se EC decay to the 865.4 keV excited state in $^{75}$As is potentially ultra-low with Qes $\approx$ 1 keV. However, a more precise determination of the 865.4(5) keV level in $^{75}$As is required.

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arXiv2022

Measurements and computational analysis on the natural decay of $^{176}$Lu

Mainly because of its long half-life and despite its scientific relevance, spectroscopic measurements of $^{176}$Lu forbidden $\beta$-decays are very limited and lack formulation of shape factors. A direct precise measurement of its $Q$ value is also presently unreported. In addition, the description of forbidden decays provides interesting challenges for nuclear theory. The comparison of precise experimental results with theoretical calculations for these decays can help to test underlying models and can aid the interpretation of data from other experiments.

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arXiv2022

High-precision mass measurement of $^{24}$Si and a refined determination of the $rp$ process at the $A=22$ waiting point

We report a high precision mass measurement of $^{24}{\rm Si}$, performed with the LEBIT facility at the National Superconducting Cyclotron Laboratory. The atomic mass excess, $10\;753.8$(37) keV, is a factor of 5 more precise than previous results. This substantially reduces the uncertainty of the $^{23}{\rm Al}(p,\gamma)^{24}{\rm Si}$ reaction rate, which is a key part of the rapid proton capture ($rp$) process powering Type I X-ray bursts. The updated rate constrains the onset temperature of the $(\alpha,p)$ process at the $^{22}{\rm Mg}$ waiting-point to a precision of 9%.

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arXiv2022

Investigating nuclear structure near $N = 32$ and $N = 34$: Precision mass measurements of neutron-rich Ca, Ti and V isotopes

Nuclear mass measurements of isotopes are key to improving our understanding of nuclear structure across the chart of nuclides, in particular for the determination of the appearance or disappearance of nuclear shell closures. We present high-precision mass measurements of neutron-rich Ca, Ti and V isotopes performed at the TITAN and LEBIT facilities. These measurements were made using the TITAN multiple-reflection time-of-flight mass spectrometer (MR-ToF-MS) and the LEBIT 9.4T Penning trap mass spectrometer. In total, 13 masses were measured, eight of which represent increases in precision over previous measurements. These measurements refine trends in the mass surface around $N = 32$ and $N = 34$, and support the disappearance of the $N = 32$ shell closure with increasing proton number. Additionally, our data does not support the presence of a shell closure at $N = 34$.

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arXiv2021

Improved Nuclear Physics Near $A=61$ Refines Urca Neutrino Luminosities in Accreted Neutron Star Crusts

We performed a Penning trap mass measurement of $^{61}{\rm Zn}$ at the National Superconducting Cyclotron Laboratory and NuShellX calculations of the $^{61}{\rm Zn}$ and $^{62}{\rm Ga}$ structure using the GXPF1A Hamiltonian to obtain improved estimates of the $^{61}{\rm Zn}(p,\gamma)^{62}{\rm Ga}$ and $^{60}{\rm Cu}(p,\gamma)^{61}{\rm Zn}$ reaction rates. Surveying astrophysical conditions for type-I X-ray bursts with the code MESA, implementing our improved reaction rates, and taking into account updated nuclear masses for $^{61}{\rm V}$ and $^{61}{\rm Cr}$ from the recent literature, we refine the neutrino luminosity from the important mass number $A=61$ urca cooling source in accreted neutron star crusts. This improves our understanding of the thermal barrier between deep heating in the crust and the shallow depths where extra heat is needed to explain X-ray superbursts, as well as the expected signature of crust urca neutrino emission in light curves of cooling transients.

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arXiv2020

Precision mass measurements of neutron-rich scandium isotopes refine the evolution of $N=32$ and $N=34$ shell closures

We report high-precision mass measurements of $^{50-55}$Sc isotopes performed at the LEBIT facility at NSCL and at the TITAN facility at TRIUMF. Our results provide a substantial reduction of their uncertainties and indicate significant deviations, up to 0.7 MeV, from the previously recommended mass values for $^{53-55}$Sc. The results of this work provide an important update to the description of emerging closed-shell phenomena at neutron numbers $N=32$ and $N=34$ above proton-magic $Z=20$. In particular, they finally enable a complete and precise characterization of the trends in ground state binding energies along the $N=32$ isotone, confirming that the empirical neutron shell gap energies peak at the doubly-magic $^{52}$Ca. Moreover, our data, combined with other recent measurements, does not support the existence of closed neutron shell in $^{55}$Sc at $N=34$. The results were compared to predictions from both \emph{ab initio} and phenomenological nuclear theories, which all had success describing $N=32$ neutron shell gap energies but were highly disparate in the description of the $N=34$ isotone.

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arXiv2020

First Penning trap mass measurement of $^{36}$Ca

Isobaric quintets provide the best test of the isobaric multiplet mass equation (IMME) and can uniquely identify higher order corrections suggestive of isospin symmetry breaking effects in the nuclear Hamiltonian. The Generalized IMME (GIMME) is a novel microscopic interaction theory that predicts an extension to the quadratic form of the IMME. Only the $A=20, 32$ $T=2$ quintets have the exotic $T_z = -2$ member ground state mass determined to high-precision by Penning trap mass spectrometry. In this work, we establish $A=36$ as the third high-precision $T=2$ isobaric quintet with the $T_z = -2$ member ground state mass measured by Penning trap mass spectrometry and provide the first test of the predictive power of the GIMME. A radioactive beam of neutron-deficient $^{36}$Ca was produced by projectile fragmentation at the National Superconducting Cyclotron Laboratory. The beam was thermalized and the mass of $^{36}$Ca$^+$ and $^{36}$Ca$^{2+}$ measured by the Time of Flight - Ion Cyclotron Resonance method in the LEBIT 9.4 T Penning trap. We measure the mass excess of $^{36}$Ca to be ME$ = -6483.6(56)$ keV, an improvement in precision by a factor of 6 over the literature value. The new datum is considered together with evaluated nuclear data on the $A=36$, $T=2$ quintet. We find agreement with the quadratic form of the IMME given by isospin symmetry, but only coarse qualitative agreement with predictions of the GIMME. A total of three isobaric quintets have their most exotic members measured by Penning trap mass spectrometry. The GIMME predictions in the $T = 2$ quintet appear to break down for $A = 32$ and greater.

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arXiv2020

A technique for the study of (p,n) reactions with unstable isotopes at energies relevant to astrophysics

We have developed and tested an experimental technique for the measurement of low-energy (p,n) reactions in inverse kinematics relevant to nuclear astrophysics. The proposed setup is located at the ReA3 facility at the National Superconducting Cyclotron Laboratory. In the current approach, we operate the beam-transport line in ReA3 as a recoil separator while tagging the outgoing neutrons from the (p,n) reactions with the low-energy neutron detector array (LENDA). The developed technique was verified by using the $^{40}$Ar(p,n)$^{40}$K reaction as a probe. The results of the proof-of-principle experiment with the $^{40}$Ar beam show that cross-section measurements within an uncertainty of $\sim$25\% are feasible with count rates up to 7 counts/mb/pnA/s. In this article, we give a detailed description of the experimental setup, and present the analysis method and results from the test experiment. Future plans on using the technique in experiments with the separator for capture reactions (SECAR) that is currently being commissioned are also discussed.

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arXiv2020

High precision mass measurements of the isomeric and ground states of $^{44}$V: improving constraints on the IMME parameters of the A=44, $\text{0}^{\text{+}}$ quintet

The Isobaric Multiplet Mass Equation (IMME) has been successful at predicting the masses of isobaric analogue states in the same multiplet, while its coefficients are known to follow trends as functions of mass number. The Atomic Mass Evaluation 2016 [Chin. Phys. C 41, 030003 (2017)] $^{44}$V mass value results in an negative $c$ coefficient for the IMME quadratic term. The $b$ and $c$ coefficients can provide constraints for construction of the isospin-nonconserving (INC) Hamiltonians for the $pf$ shell. The excitation energy of the $0^+, T=2$ level in $^{44}$V is currently unknown and can be used to constrain the $^{44}$Cr mass. The aim of the experiment was to perform high-precision mass measurements to resolve the difference between $^{44}$V isomeric and ground states, to test the IMME, and to provide ingredients for identifying the $0^+$, $T=2$ state in $^{44}$V. High-precision Penning trap mass spectrometry was performed at LEBIT, to measure the cyclotron frequency ratios of [$^{44g,m}$VO]$^+$ versus [$^{32}$SCO]$^+$, a reference mass, to extract both the isomeric and ground state masses of $^{44}$V. The mass excess of the ground and isomeric states in $^{44}$V were measured to be $-23\ 804.9(80)$ keV/$\text{c}^2$ and $-23\ 537.0(55)$ keV/$\text{c}^2$. This yielded a new proton separation energy of $S_p$ = 1\ 773(10) keV. The new mass values of $^{44}$V have been used to deduce the IMME $b$ and $c$ coefficients of the lowest $2^+$ and $6^+$ triplets in $A=44$. The $2^+$ $c$ coefficient is verified with the IMME trend and agrees with the shell-model predictions using charge-dependent Hamiltonians. The mirror energy differences were determined between $^{44}$V and $^{44}$Sc, in line with isospin-symmetry. The new value of the proton separation energy determined will be important for the determination of the $0^+$, $T=2$ state in $^{44}$V and for prediction of the mass of $^{44}$Cr.

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arXiv2019

Investigation of potential ultra-low $Q$-value $\beta$-decay candidates $^{89}$Sr and $^{139}$Ba using Penning trap mass spectrometry

Background: Ultra-low $Q$-value $\beta$-decays are interesting processes to study with potential applications to nuclear $\beta$-decay theory and neutrino physics. While a number of potential ultra-low $Q$-value $\beta$-decay candidates exist, improved mass measurements are necessary to determine which are energetically allowed. Method: Penning trap mass spectrometry was used to determine the atomic mass of $^{89}$Y and $^{139}$La, from which $\beta$-decay $Q$-values for $^{89}$Sr and $^{139}$Ba were obtained to determine if there could be an ultra-low $Q$-value decay branch in the $\beta$-decay of $^{89}$Sr $\rightarrow$ $^{89}$Y or $^{139}$Ba $\rightarrow$ $^{139}$La. Results: The $^{89}$Sr $\rightarrow$ $^{89}$Y and $^{139}$Ba $\rightarrow$ $^{139}$La $\beta$-decay $Q$-values were measured to be $Q_{\rm{Sr}}$ = 1502.20(0.35) keV and $Q_{\rm{Ba}}$ = 2308.37(68) keV. These were compared to energies of excited states in $^{89}$Y at 1507.4(1) keV, and in $^{139}$La at 2310(19) keV and 2313(1) keV to determine $Q$-values of -5.20(37) keV for the potential ultra-low $\beta$-decay branch of $^{89}$Sr and -1.6(19.0) keV and -4.6(1.2) keV for those of $^{139}$Ba. Conclusion: The potential ultra-low $Q$-value decay branch of $^{89}$Sr to the $^{89}$Y (3/2$^-$, 1507.4 keV) state is energetically forbidden and has been ruled out. The potential ultra-low $Q$-value decay branch of $^{139}$Ba to the 2313 keV state in $^{139}$La with unknown J$^{\pi}$ has also been ruled out at the 4$\sigma$ level, while more precise energy level data is needed for the $^{139}$La (1/2$^+$, 2310 keV) state to determine if an ultra-low $Q$-value $\beta$-decay branch to this state is energetically allowed.

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arXiv2019

Direct determination of the $^{138}$La $\beta$-decay $Q$ value using Penning trap mass spectrometry

Background: The understanding and description of forbidden decays provides interesting challenges for nuclear theory. These calculations could help to test underlying nuclear models and interpret experimental data. Purpose: Compare a direct measurement of the $^{138}$La $\beta$-decay $Q$ value with the $\beta$-decay spectrum end-point energy measured by Quarati et al. using LaBr$_3$ detectors [Appl. Radiat. Isot. 108, 30 (2016)]. Use new precise measurements of the $^{138}$La $\beta$-decay and electron capture (EC) $Q$ values to improve theoretical calculations of the $\beta$-decay spectrum and EC probabilities. Method: High-precision Penning trap mass spectrometry was used to measure cyclotron frequency ratios of $^{138}$La, $^{138}$Ce and $^{138}$Ba ions from which $\beta$-decay and EC $Q$ values for $^{138}$La were obtained. Results: The $^{138}$La $\beta$-decay and EC $Q$ values were measured to be $Q$ = 1052.42(41) keV and $Q_{EC}$ = 1748.41(34) keV, improving the precision compared to the values obtained in the most recent atomic mass evaluation [Wang, et al., Chin. Phys. C 41, 030003 (2017)] by an order of magnitude. These results are used for improved calculations of the $^{138}$La $\beta$-decay shape factor and EC probabilities. New determinations for the $^{138}$Ce 2EC $Q$ value and the atomic masses of $^{138}$La, $^{138}$Ce, and $^{138}$Ba are also reported. Conclusion: The $^{138}$La $\beta$-decay $Q$ value measured by Quarati et al. is in excellent agreement with our new result, which is an order of magnitude more precise. Uncertainties in the shape factor calculations for $^{138}$La beta-decay using our new $Q$ value are reduced by an order of magnitude. Uncertainties in the EC probability ratios are also reduced and show improved agreement with experimental data.

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arXiv2017

Precision Mass Measurements of Neutron-Rich Co Isotopes Beyond N=40

The region near Z=28, N=40 is a subject of great interest for nuclear structure studies due to spectroscopic signatures in $^{68}$Ni suggesting a subshell closure at N=40. Trends in nuclear masses and their derivatives provide a complementary approach to shell structure investigations via separation energies. Penning trap mass spectrometry has provided precise measurements for a number of nuclei in this region, however a complete picture of the mass surfaces has so far been limited by the large uncertainty remaining for nuclei with N > 40 along the iron and cobalt chains. Here we present the first Penning trap measurements of $^{68,69}$Co, performed at the Low-Energy Beam and Ion Trap facility at the National Superconducting Cyclotron Laboratory. In addition, we perform ab initio calculations of ground state and two-neutron separation energies of cobalt isotopes with the valence-space in-medium similarity renormalization group approach based on a particular set of two- and three-nucleon forces which predict saturation in infinite matter. We discuss the importance of these measurements and calculations for understanding the evolution of nuclear structure near $^{68}$Ni.

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arXiv2017

High-precision mass measurement of $^{56}$Cu and the redirection of the rp-process flow

We report the mass measurement of $^{56}$Cu, using the LEBIT 9.4T Penning trap mass spectrometer at the National Superconducting Cyclotron Laboratory at Michigan State University. The mass of $^{56}$Cu is critical for constraining the reaction rates of the $^{55}$Ni(p,$\gamma$)$^{56}$Cu(p,$\gamma$)$^{57}$Zn($\beta^+$)$^{57}$Cu bypass around the $^{56}$Ni waiting point. Previous recommended mass excess values have disagreed by several hundred keV. Our new value, ME=$-38 626.7(6.4)$ keV, is a factor of 30 more precise than the suggested value from the 2012 atomic mass evaluation [Chin. Phys. C {\bf{36}}, 1603 (2012)], and more than a factor of 12 more precise than values calculated using local mass extrapolations, while agreeing with the newest 2016 atomic mass evaluation value [Chin. Phys. C {\bf{41}}, 030003 (2017)]. The new experimental average was used to calculate the astrophysical $^{55}$Ni(p,$\gamma$) and $^{57}$Zn($\gamma$,p) reaction rates and perform reaction network calculations of the rp-process. These show that the rp-process flow redirects around the $^{56}$Ni waiting point through the $^{55}$Ni(p,$\gamma$) route, allowing it to proceed to higher masses more quickly and resulting in a reduction in ashes around this waiting point and an enhancement to higher-mass ashes.

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