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M. Rossi

Publications and source records attributed to M. Rossi.

At least 19 recordsLinked to original sources

Predicting coronal mass ejection travel times using enhanced model-guided machine learning

Coronal mass ejections (CMEs) are key drivers of space weather events, posing risks to both space-borne and ground-based systems. Accurate prediction of their arrival time at Earth is critical for impact mitigation. To this end, physics-informed artificial intelligence (AI) approaches have proven more effective than purely data-driven or physics-based methods, generally offering higher accuracy and better explainability than the former and lower computational cost than the latter. In this work, we propose a generalization of the physics-driven AI framework based on the classical drag-based model (DBM) by integrating the extended version of the drag-based model (EDBM). This enhancement allows us to include in the training process CME events whose interplanetary dynamics are incompatible with those assumed by the DBM. We achieve travel-time prediction accuracy comparable to state-of-the-art methods. We also perform a parametric robustness analysis, highlighting the stability of our approach under small variations in the drag coefficient. Furthermore, we propose a categorization of CMEs into speed regimes defined by the EDBM using a multiclass classification model based on logistic regression, which could be implemented in near-real-time operational space weather forecasting systems. The results show that the EDBM framework broadens the applicability of forecasting models while preserving good predictive accuracy.

astro-ph.SR

Capture and escape from the 2:1 resonance between Ariel and Umbriel in a fast-migration scenario of the Uranian system

Recent measurements suggest that Uranus may exhibit a higher tidal dissipation than previously assumed. This enhanced dissipation leads to a faster orbital migration of its five major moons: Miranda, Ariel, Umbriel, Titania, and Oberon. Consequently, resonant encounters that have always been discarded in previous works need to be included. In particular, Ariel's fast migration implies that the crossing of the 2:1 mean motion resonance with Umbriel is extremely likely and it could have occurred in recent times. Capture into this strong resonance would have induced significant tidal heating within Ariel, possibly explaining its resurfacing. Therefore, in this work, we aim to explore the orbital history of the Uranian moons in a context of fast tidal migration, including the crossing of the 2:1 mean motion resonance between Ariel and Umbriel. For small initial eccentricities, we confirm that the moons are always captured into this resonance. As the system is not currently involved in any mean motion resonance, we investigated possible dynamical mechanisms for exiting the 2:1 resonance. We show that the resonance could have been broken by a further resonant encounter with Titania. We analyzed the crossing of the 4:2:1 and 3:2:1 resonant chains, and looked for the parameter space where the probability of escaping the resonance is maximized. Taking a dissipative parameter of Ariel $k_{2,2}/Q_2<10^{-3}$, the passage through the 3:2:1 resonance succeeds in disrupting the 2:1 Ariel-Umbriel mean motion resonance in more than $60\%$ of our numerical experiments. A fraction of our simulations results in final low eccentricities and inclinations, which can eventually match the current orbital features of the system. As the proposed orbital history requires specific ranges of the dissipative parameters for the system, future Uranus mission data will validate (or disprove) this scenario.

astro-ph.EP

Improved direct measurement of low-energy resonances in the $^{21}$Ne(p,$\gamma$)$^{22}$Na reaction

In the nova temperature range, 0.1 GK $< T <$ 0.4 GK, several low-energy resonances dominate the $^{21}$Ne(p,$\gamma$)$^{22}$Na reaction rate, which is currently affected by large uncertainties. We present a high-precision study of the resonances at $E^{\rm{lab}}_{\rm{r}}$ = 127.3, 271.4, 272.3, 291.5, and 352.6 keV, measured directly at the Laboratory for Underground Nuclear Astrophysics in Italy. The strengths of the 127.3, 271.4, and 291.5 keV resonances are consistent with previous measurements within 1$\sigma$. However, for the 272.3 keV and 352.6 keV resonances, we report strength values of (129.9 $\pm$ 5.8) meV and (14.9 $\pm$ 0.8) meV, respectively, more than a factor of 1.5 higher than literature values. In addition, we report on new branching ratios for the 127.3, 272.3, and 352.6 keV resonances, leading to updated decay schemes. Finally, we present a revised thermonuclear reaction rate and investigate its impact on the NeNa nucleosynthesis.

nucl-ex

Characterization of avalanche photodiodes (APDs) for the CUbesat Solar Polarimeter (CUSP) mission

The CUbesat Solar Polarimeter (CUSP) project is a CubeSat mission orbiting the Earth aimed to measure the linear polarization of solar flares in the hard X-ray band by means of a Compton scattering polarimeter. CUSP will allow the study of the magnetic reconnection and particle acceleration in the flaring magnetic structures of our star. CUSP is a project in the framework of the Alcor Program of the Italian Space Agency aimed at developing new CubeSat missions. It is approved for a Phase B study. In this work, we report on the characterization of the Avalanche Photodiodes (APDs) that will be used as readout sensors of the absorption stage of the Compton polarimeter. We assessed the APDs gain and energy resolution as a function of temperature by irradiating the sensor with a \textsuperscript{55}Fe radioactive source. Moreover, the APDs were also characterized as being coupled to a GAGG scintillator.

astro-ph.IM

Universal orbital and magnetic structures in infinite-layer nickelates

We conducted a comparative study of the rare-earth infinite-layer nickelates films, RNiO2 (R = La, Pr, and Nd) using resonant inelastic X-ray scattering (RIXS). We found that the gross features of the orbital configurations are essentially the same, with minor variations in the detailed hybridization. For low-energy excitations, we unambiguously confirm the presence of damped magnetic excitations in all three compounds. By fitting to a linear spin-wave theory, comparable spin exchange coupling strengths and damping coefficients are extracted, indicating a universal magnetic structure in the infinite-layer nickelates. Interestingly, while signatures of a charge order are observed in LaNiO2 in the quasi-elastic region of the RIXS spectrum, it is absent in NdNiO2 and PrNiO2. This prompts further investigation into the universality and the origins of charge order within the infinite-layer inickelates.

cond-mat.str-el

The energy distribution of the first supernovae

The nature of the first Pop III stars is still a mystery and the energy distribution of the first supernovae is completely unexplored. For the first time we account simultaneously for the unknown initial mass function (IMF), stellar mixing, and energy distribution function (EDF) of Pop III stars in the context of a cosmological model for the formation of a MW-analogue. Our data-calibrated semi-analytic model is based on a N-body simulation and follows the formation and evolution of both Pop III and Pop II/I stars in their proper timescales. We discover degeneracies between the adopted Pop III unknowns, in the predicted metallicity and carbonicity distribution functions and the fraction of C-enhanced stars. Nonetheless, we are able to provide the first available constraints on the EDF, $dN/dE_\star \propto E_{\star}^{-\alpha_e}$ with $1\leq \alpha_e \leq2.5$. In addition, the characteristic mass of the Pop III IMF should be $m_{\rm ch}<100\:{\rm M_\odot}$, assuming a mass range consistent with hydrodynamical simulations (0.1-1000$\:{\rm M_\odot}$). Independent of the assumed Pop III properties, we find that all [C/Fe]>+0.7 stars (with [Fe/H]<-2.8) have been enriched by Pop III supernovae at a $>20\%$ level, and all [C/Fe]>+2 stars at a $>95\%$ level. All very metal-poor stars with $\rm [C/Fe]<0$ are predicted to be predominantly enriched by Pop III hypernovae and/or pair instabillity supernovae. To better constrain the primordial EDF, it is absolutely crucial to have a complete and accurate determination of the metallicity distribution function, and the properties of C-enhanced metal-poor stars (frequency and [C/Fe]) in the Galactic halo.

astro-ph.GA

First-Principles Simulations of Tip Enhanced Raman Scattering Reveal Active Role of Substrate on High-Resolution Images

Tip-enhanced Raman scattering (TERS) has emerged as a powerful tool to obtain subnanometer spatial resolution fingerprints of atomic motion. Theoretical calculations that can simulate the Raman scattering process and provide an unambiguous interpretation of TERS images often rely on crude approximations of the local electric field. In this work, we present a novel and first principles-based method to compute TERS images by combining Time-Dependent Density Functional Theory (TD-DFT) and Density Functional Perturbation Theory (DFPT) to calculate Raman cross sections with realistic local fields. We present TERS results on the benzene and TCNE molecule, the latter of which is adsorbed at Ag(110). We demonstrate that chemical effects on chemisorbed molecules, often ignored in TERS simulations of medium and large systems sizes, dramatically change TERS images. This calls for the inclusion of chemical effects for predictive theory-experiment comparisons and understanding of molecular motion at the nanoscale.

physics.chem-ph

Suppressing Recoil Heating in Levitated Optomechanics using Squeezed Light

We theoretically show that laser recoil heating in free-space levitated optomechanics can be arbitrarily suppressed by shining squeezed light onto an optically trapped nanoparticle. The presence of squeezing modifies the quantum electrodynamical light-matter interaction in a way that enables us to control the amount of information that the scattered light carries about a given mechanical degree of freedom. Moreover, we analyze the trade-off between measurement imprecision and back-action noise and show that optical detection beyond the standard quantum limit can be achieved. We predict that, with state-of-the-art squeezed light sources, laser recoil heating can be reduced by at least 60% by squeezing a single Gaussian mode with an appropriate incidence direction, and by 98% by squeezing a properly mode-matched mode. Our results, which are valid both for motional and librational degrees of freedom, will lead to improved feedback cooling schemes as well as boost the coherence time of optically levitated nanoparticles in the quantum regime.

quant-ph

Preoperative brain tumor imaging: models and software for segmentation and standardized reporting

For patients suffering from brain tumor, prognosis estimation and treatment decisions are made by a multidisciplinary team based on a set of preoperative MR scans. Currently, the lack of standardized and automatic methods for tumor detection and generation of clinical reports represents a major hurdle. In this study, we investigate glioblastomas, lower grade gliomas, meningiomas, and metastases, through four cohorts of up to 4000 patients. Tumor segmentation models were trained using the AGU-Net architecture with different preprocessing steps and protocols. Segmentation performances were assessed in-depth using a wide-range of voxel and patient-wise metrics covering volume, distance, and probabilistic aspects. Finally, two software solutions have been developed, enabling an easy use of the trained models and standardized generation of clinical reports: Raidionics and Raidionics-Slicer. Segmentation performances were quite homogeneous across the four different brain tumor types, with an average true positive Dice ranging between 80% and 90%, patient-wise recall between 88% and 98%, and patient-wise precision around 95%. With our Raidionics software, running on a desktop computer with CPU support, tumor segmentation can be performed in 16 to 54 seconds depending on the dimensions of the MRI volume. For the generation of a standardized clinical report, including the tumor segmentation and features computation, 5 to 15 minutes are necessary. All trained models have been made open-access together with the source code for both software solutions and validation metrics computation. In the future, an automatic classification of the brain tumor type would be necessary to replace manual user input. Finally, the inclusion of post-operative segmentation in both software solutions will be key for generating complete post-operative standardized clinical reports.

eess.IV

Dissipative Tunneling Rates through the Incorporation of First-Principles Electronic Friction in Instanton Rate Theory I: Theory

Reactions involving adsorbates on metallic surfaces and impurities in bulk metals are ubiquitous in a wide range of technological applications. The theoretical modelling of such reactions presents a formidable challenge for theory because nuclear quantum effects (NQEs) can play a prominent role and the coupling of the atomic motion with the electrons in the metal gives rise to important non-adiabatic effects (NAEs) that alter atomic dynamics. In this work, we derive a theoretical framework that captures both NQEs and NAEs and, due to its high efficiency, can be applied to first-principles calculations of reaction rates in high-dimensional realistic systems. In more detail, we develop a method that we coin ring polymer instanton with explicit friction (RPI-EF), starting from the ring-polymer instanton formalism applied to a system-bath model. We derive general equations that incorporate the spatial and frequency dependence of the friction tensor, and then combine this method with the \textit{ab initio} electronic friction formalism for the calculation of thermal reaction rates. We show that the connection between RPI-EF and the form of the electronic friction tensor presented in this work does not require any further approximations, and it is expected to be valid as long as the approximations of both underlying theories remain valid.

physics.chem-ph

Dissipative Tunneling Rates through the Incorporation of First-Principles Electronic Friction in Instanton Rate Theory II: Benchmarks and Applications

In part I, we presented the ring-polymer instanton with explicit friction (RPI-EF) method and showed how it can be connected to the \textit{ab initio} electronic friction formalism. This framework allows the calculation of tunneling reaction rates that incorporate the quantum nature of the nuclei and certain types of non-adiabatic effects (NAEs) present in metals. In this second part, we analyze the performance of RPI-EF on model potentials and apply it to realistic systems. For a 1D double-well model, we benchmark the method against numerically exact results obtained from multi-layer multi-configuration time-dependent Hartree calculations. We demonstrate that RPI-EF is accurate for medium and high friction strengths and less accurate for extremely low friction values. We also show quantitatively how the inclusion of NAEs lowers the cross-over temperature into the deep tunneling regime, reduces the tunneling rates, and in certain regimes, steers the quantum dynamics by modifying the tunneling pathways. As a showcase of the efficiency of this method, we present a study of hydrogen and deuterium hopping between neighboring interstitial sites in selected bulk metals. The results show that multidimensional vibrational coupling and nuclear quantum effects have a larger impact than NAEs on the tunneling rates of diffusion in metals. Together with part I, these results advance the calculations of dissipative tunneling rates from first principles.

physics.chem-ph

Restored strange metal phase through suppression of charge density waves in underdoped YBa$_2$Cu$_3$O$_{7-δ}$

The normal state of optimally doped cuprates is dominated by the "strange metal" phase that shows a linear temperature ($T$) dependence of the resistivity persisting down to the lowest $T$. For underdoped cuprates this behavior is lost below the pseudogap temperature $T^*$, where Charge Density Waves (CDW) together with other intertwined local orders characterize the ground state. Here we show that the $T$-linear resistivity of highly strained, ultrathin and underdoped YBa$_2$Cu$_3$O$_{7-δ}$ films is restored when the CDW amplitude, detected by Resonant Inelastic X-ray scattering, is suppressed. This observation points towards an intimate connection between the onset of CDW and the departure from $T$-linear resistivity in underdoped cuprates. Our results illustrate the potential of using strain control to manipulate the ground state of quantum materials.

cond-mat.supr-con

Magnetic excitations in infinite-layer nickelates

The discovery of superconductivity in infinite-layer nickelates brings us tantalizingly close to a new material class that mirrors the cuprate superconductors. Here, we report on magnetic excitations in these nickelates, measured using resonant inelastic x-ray scattering (RIXS) at the Ni L3-edge, to shed light on the material complexity and microscopic physics. Undoped NdNiO2 possesses a branch of dispersive excitations with a bandwidth of approximately 200 meV, reminiscent of strongly-coupled, antiferromagnetically aligned spins on a square lattice, despite a lack of evidence for long range magnetic order. The significant damping of these modes indicates the importance of coupling to rare-earth itinerant electrons. Upon doping, the spectral weight and energy decrease slightly, while the modes become overdamped. Our results highlight the role of Mottness in infinite-layer nickelates.

cond-mat.supr-con

Orbital and Spin Character of Doped Carriers in Infinite-Layer Nickelates

The recent discovery of superconductivity in Nd$_{1-x}$Sr$_{x}$NiO$_2$ has drawn significant attention in the field. A key open question regards the evolution of the electronic structure with respect to hole doping. Here, we exploit x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) to probe the doping dependent electronic structure of the NiO$_2$ planes. Upon doping, a higher energy feature in Ni $L_3$ edge XAS develops in addition to the main absorption peak. By comparing our data to atomic multiplet calculations including $D_{4h}$ crystal field, the doping induced feature is consistent with a $d^8$ spin singlet state, in which doped holes reside in the $d_{x^2-y^2}$ orbitals, similar to doped single band Hubbard models. This is further supported by orbital excitations observed in RIXS spectra, which soften upon doping, corroborating with Fermi level shift associated with increasing holes in the $d_{x^2-y^2}$ orbital.

cond-mat.str-el

Evolution of spin excitations from bulk to monolayer FeSe

The discovery of enhanced superconductivity (SC) in FeSe films grown on SrTiO3 (FeSe/STO) has revitalized the field of Fe-based superconductors. In the ultrathin limit, the superconducting transition temperature Tc is increased by almost an order of magnitude, raising new questions on the pairing mechanism. As in other unconventional superconductors, antiferromagnetic spin fluctuations have been proposed as a candidate to mediate SC in this system. Thus, it is essential to study the evolution of the spin dynamics of FeSe in the ultrathin limit to elucidate their relationship with superconductivity. Here, we investigate and compare the spin excitations in bulk and monolayer FeSe grown on STO using high-resolution resonant inelastic x-ray scattering (RIXS) and quantum Monte Carlo (QMC) calculations. Despite the absence of long-range magnetic order, bulk FeSe displays dispersive magnetic excitations reminiscent of other Fe-pnictides. Conversely, the spin excitations in FeSe/STO are gapped, dispersionless, and significantly hardened relative to the bulk counterpart. By comparing our RIXS results with simulations of a bilayer Hubbard model, we connect the evolution of the spin excitations to the Fermiology of the two systems. The present study reveals a remarkable reconfiguration of spin excitations in FeSe/STO, which is essential to understand the role of spin fluctuations in the pairing mechanism.

cond-mat.str-el

Cosmological constraints on post-Newtonian parameters in effectively massless scalar-tensor theories of gravity

We study the cosmological constraints on the variation of the Newton's constant and on post-Newtonian parameters for simple models of scalar-tensor theory of gravity beyond the extended Jordan-Brans-Dicke theory. We restrict ourselves to an effectively massless scalar field with a potential $V \propto F^2$, where $F(σ)=N_{pl}^2+ξσ^2$ is the coupling to the Ricci scalar considered. We derive the theoretical predictions for cosmic microwave background (CMB) anisotropies and matter power spectra by requiring that the effective gravitational strength at present is compatible with the one measured in a Cavendish-like experiment and by assuming adiabatic initial condition for scalar fluctuations. When comparing these models with $Planck$ 2015 and a compilation of baryonic acoustic oscilation (BAO) data, all these models accomodate a marginalized value for $H_0$ higher than in $Λ$CDM. We find no evidence for a statistically significant deviation from Einstein's general relativity. We find $ξ< 0.064$ ($|ξ| < 0.011$) at 95 % CL for $ξ> 0$ (for $ξ< 0$, $ξ\ne -1/6$). In terms of post-Newtonian parameters, we find $0.995 < γ_{\rm PN} < 1$ and $0.99987 < β_{\rm PN} < 1$ ($0.997 < γ_{\rm PN} < 1$ and $1 < β_{\rm PN} < 1.000011$) for $ξ>0$ (for $ξ< 0$). For the particular case of the conformal coupling, i.e. $ξ=-1/6$, we find constraints on the post-Newtonian parameters of similar precision to those within the Solar System.

astro-ph.CO

Electronic structure of the parent compound of superconducting infinite-layer nickelates

The search for oxide materials with physical properties similar to the cuprate high Tc superconductors, but based on alternative transition metals such as nickel, has grown and evolved over time. The recent discovery of superconductivity in doped infinite-layer nickelates RNiO2 (R = rare-earth element) further strengthens these efforts.With a crystal structure similar to the infinite-layer cuprates - transition metal oxide layers separated by a rare-earth spacer layer - formal valence counting suggests that these materials have monovalent Ni1+ cations with the same 3d electron count as Cu2+ in the cuprates. Here, we use x-ray spectroscopy in concert with density functional theory to show that the electronic structure of RNiO2 (R = La, Nd), while similar to the cuprates, includes significant distinctions. Unlike cuprates with insulating spacer layers between the CuO2 planes, the rare-earth spacer layer in the infinite-layer nickelate supports a weakly-interacting three-dimensional 5d metallic state. This three-dimensional metallic state hybridizes with a quasi-two-dimensional, strongly correlated state with 3dx2-y2 symmetry in the NiO2 layers. Thus, the infinite-layer nickelate can be regarded as a sibling of the rare earth intermetallics, well-known for heavy Fermion behavior, where the NiO2 correlated layers play an analogous role to the 4f states in rare-earth heavy Fermion compounds. This unique Kondo- or Anderson-lattice-like "oxide-intermetallic" replaces the Mott insulator as the reference state from which superconductivity emerges upon doping.

cond-mat.supr-con

Formation of Incommensurate Charge Density Waves in Cuprates

Although charge density waves (CDWs) are omnipresent in cuprate high-temperature superconductors, they occur at significantly different wavevectors, confounding efforts to understand their formation mechanism. Here, we use resonant inelastic x-ray scattering to investigate the doping- and temperature-dependent CDW evolution in La2-xBaxCuO4 (x=0.115-0.155). We discovered that the CDW develops in two stages with decreasing temperature. A precursor CDW with quasi-commensurate wavevector emerges first at high-temperature. This doping-independent precursor CDW correlation originates from the CDW phase mode coupled with a phonon and "seeds" the low-temperature CDW with strongly doping dependent wavevector. Our observation reveals the precursor CDW and its phase mode as the building blocks of the highly intertwined electronic ground state in the cuprates.

cond-mat.supr-con