arXiv subjects

M. Rossi

Publications and source records attributed to M. Rossi.

At least 37 records · Page 2Linked to original sources

arXiv2019

Polarization resolved Cu $L_3$-edge resonant inelastic x-ray scattering of orbital and spin excitations in NdBa$_{2}$Cu$_{3}$O$_{7-δ}$

High resolution resonant inelastic x-ray scattering (RIXS) has proven particularly effective in the determination of crystal field and spin excitations in cuprates. Its strength lies in the large Cu $L_{3}$ resonance and in the fact that the scattering cross section follows quite closely the single-ion model predictions, both in the insulating parent compounds and in the superconducting doped materials. However, the spectra become increasingly broader with (hole) doping, hence resolving and assigning spectral features has proven challenging even with the highest energy resolution experimentally achievable. Here we have overcome this limitation by measuring the complete polarization dependence of the RIXS spectra as function of momentum transfer and doping in thin films of NdBa$_{2}$Cu$_{3}$O$_{7-δ}$. Besides confirming the previous assignment of $dd$ and spin excitations (magnon, bimagnon) in the antiferromagnetic insulating parent compound, we unequivocally single out the actual spin-flip contribution at all dopings. We also demonstrate that the softening of $dd$ excitations is mainly attributed to the shift of the $xy$ peak to lower energy loss. These results provide a definitive assessment of the RIXS spectra of cuprates and demonstrate that RIXS measurements with full polarization control are practically feasible and highly informative.

cond-mat.supr-con↗

arXiv2017

Possibility to realize spin-orbit-induced correlated physics in iridium fluorides

Recent theoretical predictions of "unprecedented proximity" of the electronic ground state of iridium fluorides to the SU(2) symmetric $j_{\mathrm{eff}}=1/2$ limit, relevant for superconductivity in iridates, motivated us to investigate their crystal and electronic structure. To this aim, we performed high-resolution x-ray powder diffraction, Ir L$_3$-edge resonant inelastic x-ray scattering, and quantum chemical calculations on Rb$_2$[IrF$_6$] and other iridium fluorides. Our results are consistent with the Mott insulating scenario predicted by Birol and Haule [Phys. Rev. Lett. 114, 096403 (2015)], but we observe a sizable deviation of the $j_{\mathrm{eff}}=1/2$ state from the SU(2) symmetric limit. Interactions beyond the first coordination shell of iridium are negligible, hence the iridium fluorides do not show any magnetic ordering down to at least 20 K. A larger spin-orbit coupling in iridium fluorides compared to oxides is ascribed to a reduction of the degree of covalency, with consequences on the possibility to realize spin-orbit-induced strongly correlated physics in iridium fluorides.

cond-mat.str-el↗

arXiv2016

Long-range interactions in the effective low energy Hamiltonian of Sr2IrO4: a core level resonant inelastic x-ray scattering study

We have investigated the electronic structure of Sr2IrO4 using core level resonant inelastic x-ray scattering. The experimental spectra can be well reproduced using ab initio density functional theory based multiplet ligand field theory calculations, thereby validating these calculations. We found that the low-energy, effective Ir t2g orbitals are practically degenerate in energy. We uncovered that covalency in Sr2IrO4, and generally in iridates, is very large with substantial oxygen ligand hole character in the Ir t2g Wannier orbitals. This has far reaching consequences, as not only the onsite crystal-field energies are determined by the long range crystal-structure, but, more significantly, magnetic exchange interactions will have long range distance dependent anisotropies in the spin direction. These findings set constraints and show pathways for the design of d^5 materials that can host compass-like magnetic interactions.

cond-mat.str-el↗

arXiv2016

Linear response of one-dimensional liquid $^4$He to external perturbations

We study the response of one-dimensional liquid $^4$He to weak perturbations relying on the dynamical structure factor, $S(q,ω)$, recently obtained via ab-initio techniques [Phys. Rev. Lett. 116, 135302 (2016)]. We evaluate the drag force, $F_v$, experienced by an impurity moving along the system with velocity $v$ and the static response function, $χ(q)$, describing the density modulations induced by a periodic perturbation with wave vector $q$.

cond-mat.other↗

arXiv2016

Design and advancement status of the Beam Expander Testing X-ray facility (BEaTriX)

The BEaTriX (Beam Expander Testing X-ray facility) project is an X-ray apparatus under construction at INAF/OAB to generate a broad (200 x 60 mm2), uniform and low-divergent X-ray beam within a small lab (6 x 15 m2). BEaTriX will consist of an X-ray source in the focus a grazing incidence paraboloidal mirror to obtain a parallel beam, followed by a crystal monochromation system and by an asymmetrically-cut diffracting crystal to perform the beam expansion to the desired size. Once completed, BEaTriX will be used to directly perform the quality control of focusing modules of large X-ray optics such as those for the ATHENA X-ray observatory, based on either Silicon Pore Optics (baseline) or Slumped Glass Optics (alternative), and will thereby enable a direct quality control of angular resolution and effective area on a number of mirror modules in a short time, in full X-ray illumination and without being affected by the finite distance of the X-ray source. However, since the individual mirror modules for ATHENA will have an optical quality of 3-4 arcsec HEW or better, BEaTriX is required to produce a broad beam with divergence below 1-2 arcsec, and sufficient flux to quickly characterize the PSF of the module without being significantly affected by statistical uncertainties. Therefore, the optical components of BEaTriX have to be selected and/or manufactured with excellent optical properties in order to guarantee the final performance of the system. In this paper we report the final design of the facility and a detailed performance simulation.

astro-ph.IM↗

arXiv2016

Dynamical structure factor of one-dimensional hard rods

The zero-temperature dynamical structure factor $S(q,ω)$ of one-dimensional hard rods is computed using state-of-the-art quantum Monte Carlo and analytic continuation techniques, complemented by a Bethe Ansatz analysis. As the density increases, $S(q,ω)$ reveals a crossover from the Tonks-Girardeau gas to a quasi-solid regime, along which the low-energy properties are found in agreement with the nonlinear Luttinger liquid theory. Our quantitative estimate of $S(q,ω)$ extends beyond the low-energy limit and confirms a theoretical prediction regarding the behavior of $S(q,ω)$ at specific wavevectors $\mathcal{Q}_n=n 2 π/a$, where $a$ is the core radius, resulting from the interplay of the particle-hole boundaries of suitably rescaled ideal Fermi gases. We observe significant similarities between hard rods and one-dimensional $^4$He at high density, suggesting that the hard-rods model may provide an accurate description of dense one-dimensional liquids of quantum particles interacting through a strongly repulsive, finite-range potential.

cond-mat.other↗

arXiv2016

One-dimensional liquid $^4$He: dynamical properties beyond Luttinger liquid theory

We compute the zero-temperature dynamical structure factor of one-dimensional liquid $^4$He by means of state-of-the-art Quantum Monte Carlo and analytic continuation techniques. By increasing the density, the dynamical structure factor reveals a transition from a highly compressible critical liquid to a quasi-solid regime. In the low-energy limit, the dynamical structure factor can be described by the quantum hydrodynamic Luttinger liquid theory, with a Luttinger parameter spanning all possible values by increasing the density. At higher energies, our approach provides quantitative results beyond the Luttinger liquid theory. In particular, as the density increases, the interplay between dimensionality and interaction makes the dynamical structure factor manifest a pseudo {\it{particle-hole}} continuum typical of fermionic systems. At the low-energy boundary of such region and moderate densities, we find consistency, within statistical uncertainties, with predictions of a power-law structure by the recently-developed non-linear Luttinger liquid theory. In the quasi-solid regime we observe a novel behavior at intermediate momenta, which can be described by new analytical relations that we derive for the hard-rods model.

cond-mat.other↗

arXiv2015

Microfabrication of large area high-stress silicon nitride membranes for optomechanical devices

In view of the integration of membrane resonators with more complex MEMS structures, we developed a general fabrication procedure for circular shape SiN$_x$ membranes using Deep Reactive Ion Etching (DRIE). Large area and high-stress SiN$_x$ membranes were fabricated and used as optomechanical resonators in a Michelson interferometer and in a Fabry-Pérot cavity. The measurements show that the fabrication process preserves both the optical quality and the mechanical quality factor of the membrane.

quant-ph↗

arXiv2014

Entanglement and nonclassical properties of hypergraph states

Hypergraph states are multi-qubit states that form a subset of the locally maximally entangleable states and a generalization of the well--established notion of graph states. Mathematically, they can conveniently be described by a hypergraph that indicates a possible generation procedure of these states; alternatively, they can also be phrased in terms of a non-local stabilizer formalism. In this paper, we explore the entanglement properties and nonclassical features of hypergraph states. First, we identify the equivalence classes under local unitary transformations for up to four qubits, as well as important classes of five- and six-qubit states, and determine various entanglement properties of these classes. Second, we present general conditions under which the local unitary equivalence of hypergraph states can simply be decided by considering a finite set of transformations with a clear graph-theoretical interpretation. Finally, we consider the question whether hypergraph states and their correlations can be used to reveal contradictions with classical hidden variable theories. We demonstrate that various noncontextuality inequalities and Bell inequalities can be derived for hypergraph states.

quant-ph↗

arXiv2014

Crystal field splitting in Sr$_{n+1}$Ir$_n$O$_{3n+1}$ ($n$ = 1, 2) iridates probed by x-ray Raman spectroscopy

Non-resonant Raman spectroscopy in the hard X-ray regime has been used to explore the electronic structure of the first two members of the Ruddlesden-Popper series Sr$_{n+1}$Ir$_n$O$_{3n+1}$ of iridates. By tuning the photon energy transfer around 530 eV we have been able to explore the oxygen K near edge structure with bulk sensitivity. The angular dependence of the spectra has been exploited to assign features in the 528-535 eV energy range to specific transitions involving the Ir 5d orbitals. This has allowed us to extract reliable values for both the t2g-eg splitting arising from the cubic component of the crystal field (10Dq), in addition to the splitting of the eg orbitals due to tetragonal distortions. The values we obtain are (3.8, 1.6) eV and (3.55, 1.9) eV for Sr$_2$IrO$_4$ and Sr$_3$Ir$_2$O$_7$, respectively.

cond-mat.str-el↗

arXiv2014

Hypergraph states in Grover's quantum search algorithm

We study the entanglement content of the states employed in the Grover algorithm after the first oracle call when a few searched items are concerned. We then construct a link between these initial states and hypergraphs, which provides an illustration of their entanglement properties.

quant-ph↗

arXiv2014

Scaling Properties of Rainfall-Induced Landslides Predicted by a Physically Based Model

Natural landslides exhibit scaling properties revealed by power law relationships. These relationships include the frequency of the size (e.g., area, volume) of the landslides, and the rainfall conditions responsible for slope failures in a region. Reasons for the scaling behavior of landslides are poorly known. We investigate the possibility of using the Transient Rainfall Infiltration and Grid-Based Regional Slope-Stability analysis code (TRIGRS), a consolidated, physically-based, numerical model that describes the stability/instability conditions of natural slopes forced by rainfall, to determine the frequency statistics of the area of the unstable slopes and the rainfall intensity (I) - duration (D) conditions that result in landslides in a region. We apply TRIGRS in a portion of the Upper Tiber River Basin, Central Italy. The spatially distributed model predicts the stability/instability conditions of individual grid cells, given the local terrain and rainfall conditions. We run TRIGRS using multiple, synthetic rainfall histories, and we compare the modeling results with empirical evidences of the area of landslides and of the rainfall conditions that have caused landslides in the study area. Our findings revealed that TRIGRS is capable of reproducing the frequency of the size of the patches of terrain predicted as unstable by the model, which match the frequency size statistics of landslides in the study area, and the mean rainfall D, I conditions that result in unstable slopes in the study area, which match rainfall I-D thresholds for possible landslide occurrence. Our results are a step towards understanding the mechanisms that give rise to landslide scaling properties.

physics.geo-ph↗

arXiv2014

Improving predictive power of physically based rainfall-induced shallow landslide models: a probabilistic approach

Distributed models to forecast the spatial and temporal occurrence of rainfall-induced shallow landslides are based on deterministic laws. These models extend spatially the static stability models adopted in geotechnical engineering, and adopt an infinite-slope geometry to balance the resisting and the driving forces acting on the sliding mass. An infiltration model is used to determine how rainfall changes pore-water conditions, modulating the local stability/instability conditions. A problem with the operation of the existing models lays in the difficulty in obtaining accurate values for the several variables that describe the material properties of the slopes. The problem is particularly severe when the models are applied over large areas, for which sufficient information on the geotechnical and hydrological conditions of the slopes is not generally available. To help solve the problem, we propose a probabilistic Monte Carlo approach to the distributed modeling of rainfall-induced shallow landslides. For the purpose, we have modified the Transient Rainfall Infiltration and Grid-Based Regional Slope-Stability Analysis (TRIGRS) code. The new code (TRIGRS-P) adopts a probabilistic approach to compute, on a cell-by-cell basis, transient pore-pressure changes and related changes in the factor of safety due to rainfall infiltration. Infiltration is modeled using analytical solutions of partial differential equations describing one-dimensional vertical flow in isotropic, homogeneous materials. Both saturated and unsaturated soil conditions can be considered. TRIGRS-P copes with the natural variability inherent to the mechanical and hydrological properties of the slope materials by allowing values of the TRIGRS model input parameters to be sampled randomly from a given probability distribution. [..]

physics.geo-ph↗

arXiv2013

Detection methods to rule out completely co-positive and bi-entangling operations

In this work we extend the quantum channel detection method developed in [Phys. Rev. A 88, 042335 (2013)] and [Phys. Script. T153, 014044 (2013)] in order to detect other interesting convex sets of quantum channels. First we work out a procedure to detect non completely co-positive maps. Then we focus on the set of so-called bi-entangling operations and show how a map outside this set can be revealed. In both cases we provide explicit examples showing the theoretical technique and the corresponding experimental procedure.

quant-ph↗

arXiv2013

Orbital occupancies and the putative jeff = 1/2 groundstate in Ba2IrO4: a combined oxygen K edge XAS and RIXS study

The nature of the electronic groundstate of Ba2IrO4 has been addressed using soft X-ray absorption and inelastic scattering techniques in the vicinity of the oxygen K edge. From the polarization and angular dependence of XAS we deduce an approximately equal superposition of xy, yz and zx Ir4+ 5d orbitals. By combining the measured orbital occupancies, with the value of the spin-orbit coupling provided by RIXS, we estimate the crystal field splitting associated with the tetragonal distortion of the IrO6 octahedra to be small, Δ=50(50) meV. We thus conclude definitively that Ba2IrO4 is a close realization of a spin-orbit Mott insulator with a jeff = 1/2 groundstate, thereby overcoming ambiguities in this assignment associated with the interpretation of X-ray resonant scattering experiments.

cond-mat.str-el↗

arXiv2013

Quantum Hypergraph States

We introduce a class of multiqubit quantum states which generalizes graph states. These states correspond to an underlying mathematical hypergraph, i.e. a graph where edges connecting more than two vertices are considered. We derive a generalised stabilizer formalism to describe this class of states. We introduce the notion of k-uniformity and show that this gives rise to classes of states which are inequivalent under the action of the local Pauli group. Finally we disclose a one-to-one correspondence with states employed in quantum algorithms, such as Deutsch-Jozsa's and Grover's.

quant-ph↗

arXiv2013

Noise robustness in the detection of non separable random unitary maps

We briefly review a recently proposed method to detect properties of quantum noise processes and quantum channels. We illustrate in detail the method for detecting non separable random unitary channels and consider in particular the explicit examples of the CNOT and CZ gates. We analyse their robustness in the presence of noise for several quantum noise models.

quant-ph↗

arXiv2013

Quantum channel detection

We present a method to detect properties of quantum channels, assuming that some a priori information about the form of the channel is available. The method is based on a correspondence with entanglement detection methods for multipartite density matrices based on witness operators. We first illustrate the method in the case of entanglement breaking channels and non separable random unitary channels, and show how it can be implemented experimentally by means of local measurements. We then study the detection of non separable maps and show that for pairs of systems of dimension higher than two the detection operators are not the same as in the random unitary case, highlighting a richer separability structure of quantum channels with respect to quantum states. Finally we consider the set of PPT maps, developing a technique to reveal NPT maps.

quant-ph↗