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M. Schmidt

Publications and source records attributed to M. Schmidt.

At least 109 records · Page 6Linked to original sources

Spin-orbiton and quantum criticality in FeSc2S4

In FeSc2S4 spin-orbital exchange competes with strong spin-orbit coupling, suppressing long-range spin and orbital order and, hence, this material represents one of the rare examples of a spin-orbital liquid ground state. Moreover, it is close to a quantum-critical point separating the ordered and disordered regimes. Using THz and FIR spectroscopy we study low-lying excitations in FeSc2S4 and provide clear evidence for a spin-orbiton, an excitation of strongly entangled spins and orbitals. It becomes particularly well pronounced upon cooling, when advancing deep into the quantum-critical regime. Moreover, indications of an underlying structureless excitation continuum are found, a possible signature of quantum criticality.

cond-mat.str-el↗

Microscopic magnetic modeling for the $S$=1/2 alternating chain compounds Na$_3$Cu$_2$SbO$_6$ and Na$_2$Cu$_2$TeO$_6$

The spin-1/2 alternating Heisenberg chain system Na$_3$Cu$_2$SbO$_6$ features two relevant exchange couplings: $J_{1a}$ within the structural Cu$_2$O$_6$ dimers and $J_{1b}$ between the dimers. Motivated by the controversially discussed nature of $J_{1a}$, we perform extensive density-functional-theory (DFT) calculations, including DFT+$U$ and hybrid functionals. Fits to the experimental magnetic susceptibility using high-temperature series expansions and quantum Monte Carlo simulations yield the optimal parameters $J_{1a}$ = $-$217 K and $J_{1b}$ = 174 K with the alternation ratio $α= J_{1a}/J_{1b} \simeq$ $-$1.25. For the closely related system Na$_2$Cu$_2$TeO$_6$, DFT yields substantially enhanced $J_{1b}$, but weaker $J_{1a}$. The comparative analysis renders the buckling of the chains as the key parameter altering the magnetic coupling regime. Numerical simulation of the dispersion relations of the alternating chain model clarify why both antiferromagnetic and ferrromagnetic $J_{1a}$ can reproduce the experimental magnetic susceptibility data.

cond-mat.str-el↗

Optomechanical Dirac Physics

Recent progress in optomechanical systems may soon allow the realization of optomechanical arrays, i.e. periodic arrangements of interacting optical and vibrational modes. We show that photons and phonons on a honeycomb lattice will produce an optically tunable Dirac-type band structure. Transport in such a system can exhibit transmission through an optically created barrier, similar to Klein tunneling, but with interconversion between light and sound. In addition, edge states at the sample boundaries are dispersive and enable controlled propagation of photon-phonon polaritons.

cond-mat.mes-hall↗

Electron Beam Ion Sources

Electron beam ion sources (EBISs) are ion sources that work based on the principle of electron impact ionization, allowing the production of very highly charged ions. The ions produced can be extracted as a DC ion beam as well as ion pulses of different time structures. In comparison to most of the other known ion sources, EBISs feature ion beams with very good beam emittances and a low energy spread. Furthermore, EBISs are excellent sources of photons (X-rays, ultraviolet, extreme ultraviolet, visible light) from highly charged ions. This chapter gives an overview of EBIS physics, the principle of operation, and the known technical solutions. Using examples, the performance of EBISs as well as their applications in various fields of basic research, technology and medicine are discussed.

physics.acc-ph↗

Coplanar waveguide based ferromagnetic resonance in ultrathin film magnetic nanostructures: impact of conducting layers

We report broadband ferromagnetic resonance (FMR) measurements based on a coplanar waveguide (CPW) of ultrathin magnetic film structures that comprise in-plane/out-of-plane decoupled layers deposited on nonmagnetic buffer layers of various thickness or other buffer structures with a diverse sheet resistance. We show that the excitation of the fundamental mode can be substantially (up to 10 times) enhanced in the structures deposited on buffer layers with a low sheet resistance in comparison to the structures deposited on thin or weakly conducting buffer layers. The results are analyzed in terms of shielding of the electromagnetic field of CPW by the conducting buffer layers. The effect of enhancement of FMR absorption can be attractive for applications in spintronic devices that utilize magnetization dynamics of ultrathin ferromagnetic layers.

cond-mat.mes-hall↗

The wind of W Hya as seen by Herschel - I. The CO envelope

Asymptotic giant branch (AGB) stars lose their envelopes by means of a stellar wind whose driving mechanism is not understood well. Characterizing the composition and thermal and dynamical structure of the outflow provides constraints that are essential for understanding AGB evolution, including the rate of mass loss and isotopic ratios. We modeled the CO emission from the wind of the low mass-loss rate oxygen-rich AGB star W Hya using data obtained by the HIFI, PACS, and SPIRE instruments onboard the Herschel Space Observatory and ground-based telescopes. $^{12}$CO and $^{13}$CO lines are used to constrain the intrinsic $^{12}$C/$^{13}$C ratio from resolved HIFI lines. The acceleration of the outflow up to about 5.5 km/s is quite slow and can be represented by a beta-type velocity law with index 5. Beyond this point, acceleration up the terminal velocity of 7 km/s is faster. Using the J=10-9, 9-8, and 6-5 transitions, we find an intrinsic $^{12}$C/$^{13}$C ratio of $18\pm10$ for W Hya, where the error bar is mostly due to uncertainties in the $^{12}$CO abundance and the stellar flux around 4.6 $μ$m. To match the low-excitation CO lines, these molecules need to be photo-dissociated at about 500 stellar radii. The radial dust emission intensity profile measured by PACS images at 70 $μ$m shows substantially stronger emission than our model predicts beyond 20 arcsec. The initial slow acceleration of the wind implies inefficient wind driving in the lower part of the envelope. The final injection of momentum in the wind might be the result of an increase in the opacity thanks to the late condensation of dust species. The derived intrinsic isotopologue ratio for W Hya is consistent with values set by the first dredge-up and suggestive of an initial mass of 2 M$_\odot$ or more. However, the uncertainty in the main-sequence mass derived based on this isotopologic ratio is large.

astro-ph.SR↗

High-field spectroscopy of singlet-triplet transitions in the spin-dimer systems Sr3Cr2O8 and Ba3Cr2O8

Magnetic excitations in the isostructural spin-dimer systems Sr3Cr2O8 and Ba3Cr2O8 are probed by means of high-field electron spin resonance at sub-terahertz frequencies. Three types of magnetic modes were observed. One mode is gapless and corresponds to transitions within excited states, while two other sets of modes are gapped and correspond to transitions from the ground to the first excited states. The selection rules of the gapped modes are analyzed in terms of a dynamical Dzyaloshinskii-Moriya interaction, suggesting the presence of phonon-assisted effects in the low-temperature spin dynamics of Sr3Cr2O8 and Ba3Cr2O8

cond-mat.str-el↗

HIFISTARS Herschel/HIFI observations of VY Canis Majoris. Molecular-line inventory of the envelope around the largest known star

To gain insight into the physical conditions and kinematics of the warm (100-1000 K) gas around the red hyper-giant VY CMa, we performed sensitive high spectral resolution observations of molecular lines in the sub-mm/FIR using the HIFI instrument of the Herschel Space Observatory. We observed CO, H2O, and other molecular species, sampling excitation energies from a few tens to a few thousand K. These observations are part of the Herschel Guaranteed Time Key Program HIFISTARS. We detected the J=6-5, J=10-9, and J=16-15 lines of 12CO and 13CO at about 100, 300, and 750K above the ground state (and the 13CO J=9-8 line). These lines are crucial for improving the modelling of the internal layers of the envelope around VY CMa. We also detected 27 lines of H2O and its isotopomers, and 96 lines of species such as NH3, SiO, SO, SO2 HCN, OH and others, some of them originating from vibrationally excited levels. Three lines were not unambiguously assigned. Our observations confirm that VY CMa's envelope must consist of two or more detached components. The molecular excitation in the outer layers is significantly lower than in the inner ones, resulting in strong self-absorbed profiles in molecular lines that are optically thick in this outer envelope, for instance, low-lying lines of H2O. Except for the most abundant species, CO and H2O, most of the molecular emission detected at these sub-mm/FIR wavelengths arise from the central parts of the envelope. The spectrum of VY CMa is very prominent in vibrationally excited lines, which are caused by the strong IR pumping present in the central regions. Compared with envelopes of other massive evolved stars, VY CMa's emission is particularly strong in these vibrationally excited lines, as well as in the emission from less abundant species such as H13CN, SO, and NH3.

astro-ph.SR↗

Orbital-selective metal-insulator transition and gap formation above Tc in superconducting Rb1-xFe2-ySe2

We report on a hierarchy of temperatures Tc < Tgap < Tmet in superconducting Rb1-xFe2-ySe2 observed by THz spectroscopy. Above Tmet = 90 K the material reveals semiconducting characteristics. Below Tmet a coherent metallic THz response emerges. This metal-to-insulator type, orbital selective transition is clearly indicated by an isosbestic point in the temperature dependence of the optical conductivity and dielectric constant at THz-frequencies. At Tgap = 61 K a gap opens in the THz regime and then the superconducting transition occurs at Tc = 32 K. This sequence of temperatures seems to reflect a corresponding hierarchy of the electronic correlations in the different bands.

cond-mat.supr-con↗

Next generation KATRIN high precision voltage divider for voltages up to 65kV

The KATRIN (KArlsruhe TRItium Neutrino) experiment aims to determine the mass of the electron antineutrino with a sensitivity of 200meV by precisely measuring the electron spectrum of the tritium beta decay. This will be done by the use of a retarding spectrometer of the MAC-E-Filter type. To achieve the desired sensitivity the stability of the retarding potential of -18.6kV has to be monitored with a precision of 3ppm over at least two months. Since this is not feasible with commercial devices, two ppm-class high voltage dividers were developed, following the concept of the standard divider for DC voltages of up to 100kV of the Physikalisch-Technische Bundesanstalt (PTB). In order to reach such high accuracies different effects have to be considered. The two most important ones are the temperature dependence of resistance and leakage currents, caused by insulators or corona discharges. For the second divider improvements were made concerning the high-precision resistors and the thermal design of the divider. The improved resistors are the result of a cooperation with the manufacturer. The design improvements, the investigation and the selection of the resistors, the built-in ripple probe and the calibrations at PTB will be reported here. The latter demonstrated a stability of about 0.1ppm/month over a period of two years.

physics.ins-det↗

Spectroscopic evidence for giant orbital moment and magnetic anisotropy induced by local distortions in alpha-CoV2O6

We present a combined experimental and theoretical study on the local magnetism of the Co ions in the spin-chain compound CoV2O6, which crystallizes in two different allotropic phases, alpha- and gamma-CoV2O6. Using x-ray magnetic circular dichroism, we have found a very large and a moderate orbital contribution to the magnetism in alpha- and gamma-CoV2O6, respectively. Full-multiplet calculations indicate that the differences in the magnetic behavior of alpha- and gamma-CoV2O6 phases originate from different local distortions of the CoO6 octahedra. In particular, the strong compression of the CoO6 octahedra in alpha-CoV2O6 lead to a strong mixture of t2g and eg orbitals which, via the local atomic Coulomb and exchange interactions, results in an exceptionally large orbital moment.

cond-mat.str-el↗

Exciton-magnon transitions in the frustrated chromium antiferromagnets CuCrO2, alpha-CaCr2O4, CdCr2O4, and ZnCr2O4

We report on optical transmission spectroscopy of the Cr-based frustrated triangular antiferromagnets CuCrO2 and alpha-CaCr2O4, and the spinels CdCr2O4 and ZnCr2O4 in the near-infrared to visible-light frequency range. We explore the possibility to search for spin correlations far above the magnetic ordering temperature and for anomalies in the magnon lifetime in the magnetically ordered state by probing exciton-magnon sidebands of the spin-forbidden crystal-field transitions of the Cr3+ ions (spin S = 3/2). In CuCrO2 and alpha-CaCr2O4 the appearance of fine structures below T_N is assigned to magnon sidebands by comparison with neutron scattering results. The temperature dependence of the line width of the most intense sidebands in both compounds can be described by an Arrhenius law. For CuCrO2 the sideband associated with the 4A2 -> 2T2 transition can be observed even above T_N. Its line width does not show a kink at the magnetic ordering temperature and can alternatively be described by a Z2 vortex scenario proposed previously for similar materials. The exciton-magnon features in alpha-CaCr2O4 are more complex due to the orthorhombic distortion. While for CdCr2O4 magnon sidebands are identified below T_N and one sideband excitation is found to persist across the magnetic ordering transition, only a weak fine structure related to magnetic ordering has been observed in ZnCr2O4.

cond-mat.str-el↗

Low-energy magnetic excitations in the quasi-one-dimensional spin-1 chain compound SrNi2V2O8

Multi-frequency electron spin resonance (ESR) transmission spectra have been measured as function of temperature and magnetic field on single crystals of the quasi-one-dimensional spin-1 chain compound SrNi2V2O8 in the GHz frequency range. Magnetic resonance modes above 50 K have been observed with an effective g-factor of 2.24 at 100 K. Below 30 K, intra-triplet excitations have been observed in the ESR spectra, which reveal the presence of single-ion anisotropy with D = -0.29 meV.

cond-mat.str-el↗

Complex Chiral Modulations in FeGe close to Magnetic Ordering

We report on detailed polarized small-angle neutron scattering on cubic FeGe in magnetic fields applied either along (transverse) the scattering vector or parallel (longitudinal)to the neutron beam. The ($H,T$) phase diagrams for all principal axes contain a segmented $A$-phase region just below the onset of magnetic order. Hexagonal Bragg-spot patterns were observed across the entire $A$-phase region for the longitudinal geometry. Scattering intensity was observed in parts of the A phase for both scattering configurations. Only in a distinct pocket ($A_1$) vanishing scattering intensity was found in the transverse geometry.

cond-mat.mtrl-sci↗

Recent developments in classical density functional theory: Internal energy functional and diagrammatic structure of fundamental measure theory

An overview of several recent developments in density functional theory for classical inhomogeneous liquids is given. We show how Levy's constrained search method can be used to derive the variational principle that underlies density functional theory. An advantage of the method is that the Helmholtz free energy as a functional of a trial one-body density is given as an explicit expression, without reference to an external potential as is the case in the standard Mermin-Evans proof by reductio ad absurdum. We show how to generalize the approach in order to express the internal energy as a functional of the one-body density distribution and of the local entropy distribution. Here the local chemical potential and the bulk temperature play the role of Lagrange multipliers in the Euler-Lagrange equations for minimiziation of the functional. As an explicit approximation for the free-energy functional for hard sphere mixtures, the diagrammatic structure of Rosenfeld's fundamental measure density unctional is laid out. Recent extensions, based on the Kierlik-Rosinberg scalar weight functions, to binary and ternary non-additive hard sphere mixtures are described.

cond-mat.soft↗

THz spectroscopy in the pseudo-Kagome system Cu3Bi(SeO3)2O2Br

Terahertz (THz) transmission spectra have been measured as function of temperature and magnetic field on single crystals of Cu3Bi(SeO3)2O2Br. In the time-domain THz spectra without magnetic field, two resonance absorptions are observed below the magnetic ordering temperature T_N~27.4 K. The corresponding resonance frequencies increase with decreasing temperature and reach energies of 1.28 and 1.23 meV at 3.5 K. Multi-frequency electron spin resonance transmission spectra as a function of applied magnetic field show the field dependence of four magnetic resonance modes, which can be modeled as a ferromagnetic resonance including demagnetization and anisotropy effects.

cond-mat.str-el↗

Thermodynamic investigations in the precursor region of FeGe

High-resolution DC magnetization and AC-specific heat data of the cubic helimagnet FeGe have been measured as function of temperature and magnetic field. The magnetization data as well as the isothermal susceptibility data confirm the complexity of the magnetic phase diagram in the vicinity of the onset of long-rang magnetic order (Tc = 278.5 K) and the existence of a segmented A-phase region. Moreover, these data revealed independent and clear indications of phase boundaries and crossovers within the A-phase region. Together with the anomalies in the specific-heat data around Tc and at small magnetic fields (H < 600 Oe) a complex magnetic phase diagram of FeGe is obtained.

cond-mat.str-el↗

Herschel/HIFI observations of red supergiants and yellow hypergiants: I. Molecular inventory

Red supergiant stars (RSGs) and yellow hypergiant stars (YHGs) are believed to be the high-mass counterparts of stars in the AGB and early post-AGB phases. We study the mass-loss in the post main-sequence evolution of massive stars, through the properties of their envelopes in the intermediate and warm gas layers. These are the regions where the acceleration of the gas takes place and the most recent mass-loss episodes can be seen. We used the HIFI instrument on-board the Herschel Space Observatory to observe sub-mm and FIR transitions of CO, water, and their isotopologues in a sample of two RSGs (NML Cyg and Betelgeuse) and two YHGs (IRC+10420 and AFGL 2343) stars. We present an inventory of the detected lines and analyse the information revealed by their spectral profiles. On the basis of the results presented in an earlier study, we model the CO and 13CO emission in IRC+10420 and compare it to a set of lines ranging from the mm, to the FIR. Red supergiants have stronger high-excitation lines than the YHGs, indicating that they harbour dense and hot inner shells contributing to these transitions. Consequently, these high-J lines in RSGs originate from acceleration layers that have not yet reached the circumstellar terminal velocity and have narrower profiles than their flat-topped lower-J counterparts. The YHGs tend to lack this inner component, in line with the picture of detached, hollow envelopes derived from studies at longer wavelengths. NH3 is only detected in two sources (NML Cyg, IRC+10420), which are also observed to be the strongest water-line emitters of the studied sample. In contrast, OH is detected in all sources and does not seem to correlate with the water line intensities. We show that the IRC+10420 model derived solely from mm low-J CO transitions is capable of reproducing the high-J transitions when the temperature in the inner shell is simply lowered by about 30%.

astro-ph.GA↗