arXiv subjects

M. V. Milosevic

Publications and source records attributed to M. V. Milosevic.

At least 19 recordsLinked to original sources

arXiv2025

Plasmonic detection of Rashba spin-orbit coupling in monolayer transition-metal dichalcogenides

Rashba spin-orbit coupling (RSOC) induces strong momentum-dependent spin splitting and plays a crucial role in fields like spintronics and topological photonics. We here theoretically investigate the collective excitations in monolayer transition metal dichalcogenides (ML-TMDs) hosting RSOC, and conceive an approach to precisely quantify the strength of RSOC using plasmons. We determine the electron energy loss function (EELF) and plasmon dispersions for n-type ML-TMD from the dynamic dielectric function in the framework of the standard random phase approximation (RPA). In this system, both optical and acoustic plasmon modes are observed in the EELF and plasmon dispersions. Moreover, the plasmonic and spectral properties are tunable by electron density and dependent on RSOC. Crucially, we identify a minimum energy gap between the two plasmon modes to serve as a direct spectral signature of the RSOC strength. These results establish plasmons as a non-invasive, precise, and broadly tunable technique for determining RSOC in TMD van der Waals heterostructures and devices.

cond-mat.mes-hall↗

arXiv2025

Skyrmion Lattice Manipulation with Electric Currents and Thermal Gradients in MnSi

The skyrmion lattice (SkL) in MnSi was studied using small-angle neutron scattering and under the influence of a radial electric current in a Corbino geometry. In response to the applied current, the SkL undergoes an angular reorientation with respect to the MnSi crystal lattice. The reorientation is non-monotonic with increasing current, with the SkL rotating first in one direction and then the other. The SkL reorientation was studied at different sample locations and found to depend on the local current density as inferred from a finite element analysis. The non-monotonic response indicates the presence of two competing effects on the SkL, most likely due to the presence of both radial electric and thermal currents. Such a scenario is supported by micromagnetic simulations, which show how these effects can act constructively or destructively to drive the SkL rotation, depending on the direction of the electric current. In addition, the simulations also suggest how the direction of the skyrmion flow may affect the SkL orientation.

cond-mat.mes-hall↗

arXiv2024

Characteristic times for gap relaxation and heat escape in nanothin NbTi superconducting filaments: thickness dependence and effect of substrate

We measured the temporal voltage response of NbTi superconducting filaments with varied nanoscale thicknesses to step current pulses that induce non-equilibrium superconducting states governed by a hot-spot mechanism. Such detected voltage emerges after a delay time td, which is intimately connected to the gap relaxation and heat escape times. By employing time-dependent Ginzburg-Landau theory to link the delay time to the applied current, we determined that the gap relaxation time depends linearly on film thickness, aligning with the acoustic mismatch theory for phonon transmission at the superconductor-substrate interface. We thereby find a gap relaxation time of 104 ps per nm of thickness for NbTi films on polished sapphire. We further show that interfacial interaction with the substrate significantly impacts the gap relaxation time, with observed values of 9 ns on SiOx, 6.8 ns on fused silica, and 5.2 ns on sapphire for a 50 nm thick NbTi strip at T = 5.75 K. These insights are valuable for optimizing superconducting sensing technologies, particularly the single-photon detectors that operate in the transient regime of nanothin superconducting bridges and filaments

cond-mat.supr-con↗

arXiv2023

Tunable magnon topology in monolayer CrI$_\mathbf{3}$ under external stimuli

Two-dimensional (2D) honeycomb ferromagnets, such as monolayer chromium-trihalides, are predicted to behave as topological magnon insulators - characterized by an insulating bulk and topologically protected edge states, giving rise to a thermal magnon Hall effect. Here we report the behavior of the topological magnons in monolayer CrI$_3$ under external stimuli, including biaxial and uniaxial strain, electric gating, as well as in-plane and out-of-plane magnetic field, revealing that one can thereby tailor the magnetic states as well as the size and the topology of the magnonic bandgap. These findings broaden the perspective of using 2D magnetic materials to design topological magnonic devices.

cond-mat.mes-hall↗

arXiv2023

Stacking-dependent topological magnons in bilayer CrI$_3$

Motivated by the potential of atomically-thin magnets towards tunable high-frequency magnonics, we detail the spin-wave dispersion of bilayer CrI$_3$. We demonstrate that the magnonic behavior of the bilayer strongly depends on its stacking configuration and the interlayer magnetic ordering, where a topological bandgap opens in the dispersion caused by the Dzyaloshinskii-Moriya and Kitaev interactions, classifying bilayer CrI$_3$ as a topological magnon insulator. We further reveal that both size and topology of the bandgap in a CrI$_3$ bilayer with an antiferromagnetic interlayer ordering are tunable by an external magnetic field.

cond-mat.mtrl-sci↗

arXiv2022

Electronic and valleytronic properties of crystalline boron-arsenide tuned by strain and disorder

Ab initio density functional theory (DFT) and DFT plus coherent potential approximation (DFT+CPA) are employed to reveal, respectively, the effect of in-plane strain and site-diagonal disorder on the electronic structure of cubic boron arsenide (BAs). It is demonstrated that tensile strain and static diagonal disorder both reduce the semiconducting one-particle band gap of BAs, and a V-shaped p-band electronic state emerges -- enabling advanced valleytronics based on strained and disordered semiconducting bulk crystals. At biaxial tensile strains close to 15% the valence band lineshape relevant for optoelectronics is shown to coincide with one reported for GaAs at low energies. The role played by static disorder on the As sites is to promote p-type conductivity in the unstrained BAs bulk crystal, consistent with experimental observations. These findings illuminate the intricate and interdependent changes in crystal structure and lattice disorder on the electronic degrees of freedom of semiconductors and semimetals.

cond-mat.mtrl-sci↗

arXiv2022

Alternating superconducting and charge density wave monolayers within bulk 6R-TaS2

Van der Waals (vdW) heterostructures continue to attract intense interest as a route of designing materials with novel properties that cannot be found in naturally occurring materials. Unfortunately, this approach is currently limited to only a few layers that can be stacked on top of each other. Here we report a bulk material consisting of superconducting monolayers interlayered with monolayers displaying charge density waves (CDW). This bulk vdW heterostructure is created by phase transition of 1T-TaS2 to 6R at 800 °C in an inert atmosphere. Electron microscopy analysis directly shows the presence of alternating 1T and 1H monolayers within the resulting bulk 6R phase. Its superconducting transition (Tc) is found at 2.6 K, exceeding the Tc of the bulk 2H phase of TaS2. The superconducting temperature can be further increased to 3.6 K by exfoliating 6R-TaS2 and then restacking its layers. Using first-principles calculations, we argue that the coexistence of superconductivity and CDW within 6R-TaS2 stems from amalgamation of the properties of adjacent 1H and 1T monolayers, where the former dominates the superconducting state and the latter the CDW behavior.

cond-mat.supr-con↗

arXiv2022

Soliton Motion in Skyrmion Chains

Using a particle-based model we examine the depinning motion of solitons in skyrmion chains in quasi-one dimensional (1D) and two-dimensional (2D) systems containing embedded 1D interfaces. The solitons take the form of a particle or hole in a commensurate chain of skyrmions. Under an applied drive, just above a critical depinning threshold the soliton moves with a skyrmion Hall angle of zero. For higher drives, the entire chain depins, and in a 2D system we observe that both the solitons and chain move at zero skyrmion Hall angle and then transition to a finite skyrmion Hall angle as the drive increases. In a 2D system with a 1D interface that is at an angle to the driving direction, there can be a reversal of the sign of the skyrmion Hall angle from positive to negative. Our results suggest that solitons in skyrmion systems could be used as information carriers in racetrack geometries that would avoid the drawbacks of finite skyrmion Hall angles. The soliton states become mobile at significantly lower drives than the depinning transition of the skyrmion chains themselves.

cond-mat.mes-hall↗

arXiv2022

Evolution of lattice, spin, and charge properties across the phase diagram of FeSe$_{1-x}$S$_x$

A Raman scattering study covering the entire substitution range of the FeSe$_{1-x}$S$_x$ solid solution is presented. Data were taken as a function of sulfur concentration $x$ for $0\le x \le 1$, of temperature and of scattering symmetry. All type of excitations including phonons, spins and charges are analyzed in detail. It is observed that the energy and width of iron-related B$_{1g}$ phonon mode vary continuously across the entire range of sulfur substitution. The A$_{1g}$ chalcogenide mode disappears above $x=0.23$ and reappears at a much higher energy for $x=0.69$. In a similar way the spectral features appearing at finite doping in A$_{1g}$ symmetry vary discontinuously. The magnetic excitation centered at approximately 500 cm$^{-1}$ disappears above $x=0.23$ where the A$_{1g}$ lattice excitations exhibit a discontinuous change in energy. The low-energy mode associated with fluctuations displays maximal intensity at the nemato-structural transition and thus tracks the phase boundary.

cond-mat.supr-con↗

arXiv2021

Statics and Dynamics of Skyrmions Interacting with Pinning: A Review

Magnetic skyrmions are topologically stable nanoscale particle-like objects that were discovered in 2009. Since that time, intense research interest has led to the identification of numerous compounds that support skyrmions over a range of conditions spanning cryogenic to room temperatures. Skyrmions can be set into motion under various types of driving, and the combination of their size, stability, and dynamics makes them ideal candidates for numerous applications. Skyrmions represent a new class of system in which the energy scales of the skyrmion-skyrmion interactions, sample disorder, temperature, and drive can compete. A growing body of work indicates that the static and dynamic states of skyrmions can be influenced strongly by pinning or disorder in the sample; thus, an understanding of such effects is essential for the eventual use of skyrmions in applications. In this article we review the current state of knowledge regarding individual skyrmions and skyrmion assemblies interacting with quenched disorder or pinning. We outline the microscopic mechanisms for skyrmion pinning, including the repulsive and attractive interactions that can arise from impurities, grain boundaries, or nanostructures. This is followed by descriptions of depinning phenomena, sliding states over disorder, the effect of pinning on the skyrmion Hall angle, the competition between thermal and pinning effects, the control of skyrmion motion using ordered potential landscapes such as one- or two-dimensional periodic asymmetric substrates, the creation of skyrmion diodes, and skyrmion ratchet effects. We highlight the distinctions arising from internal modes and the strong gyroscopic or Magnus forces that cause the dynamical states of skyrmions to differ from those of other systems with pinning. We also discuss future directions and open questions related to the pinning and dynamics in skyrmion systems.

cond-mat.mes-hall↗

arXiv2020

Topological energy barrier for skyrmion lattice formation in MnSi

We report the direct measurement of the topological skyrmion energy barrier through a hysteresis of the skyrmion lattice in the chiral magnet MnSi. Measurements were made using small-angle neutron scattering with a custom-built resistive coil to allow for high-precision minor hysteresis loops. The experimental data was analyzed using an adapted Preisach model to quantify the energy barrier for skyrmion formation and corroborated by the minimum-energy path analysis based on atomistic spin simulations. We reveal that the skyrmion lattice in MnSi forms from the conical phase progressively in small domains, each of which consisting of hundreds of skyrmions, and with an activation barrier of several eV.

cond-mat.mes-hall↗

arXiv2017

Evolution of multi-gap superconductivity in the atomically thin limit: Strain-enhanced three-gap superconductivity in monolayer MgB$_2$

Starting from first principles, we show the formation and evolution of superconducting gaps in MgB$_2$ at its ultrathin limit. Atomically thin MgB$_2$ is distinctly different from bulk MgB$_2$ in that surface states become comparable in electronic density to the bulk-like $σ$- and $π$-bands. Combining the ab initio electron-phonon coupling with the anisotropic Eliashberg equations, we show that monolayer MgB$_2$ develops three distinct superconducting gaps, on completely separate parts of the Fermi surface due to the emergent surface contribution. These gaps hybridize nontrivially with every extra monolayer added to the film, owing to the opening of additional coupling channels. Furthermore, we reveal that the three-gap superconductivity in monolayer MgB$_2$ is robust over the entire temperature range that stretches up to a considerably high critical temperature of 20 K. The latter can be boosted to $>$50 K under biaxial tensile strain of $\sim$ 4\%, which is an enhancement stronger than in any other graphene-related superconductor known to date.

cond-mat.supr-con↗

arXiv2015

Giant paramagnetic Meissner effect in multiband superconductors

Superconductors, ideally diamagnetic when in the Meissner state, can also exhibit paramagnetic behavior due to trapped magnetic flux. In the absence of pinning such paramagnetic response is weak, and ceases with increasing sample thickness. Here we show that in multiband superconductors paramagnetic response can be observed even in slab geometries, and can be far larger than any previous estimate - even multiply larger than the diamagnetic Meissner response for the same applied magnetic field. We link the appearance of this giant paramagnetic response to the broad crossover between conventional Type-I and Type-II superconductors, where Abrikosov vortices interact non-monotonically and multibody effects become important, causing unique flux configurations and their locking in the presence of surfaces.

cond-mat.supr-con↗

arXiv2009

Second generation of vortex-antivortex states in mesoscopic superconductors: stabilization by artificial pinning

Antagonistic symmetries of superconducting polygons and their induced multi-vortex states in a homogeneous magnetic field may lead to appearance of antivortices in the vicinity of the superconducting/normal state boundary (where mesoscopic confinement is particularly strong). Resulting vortex-antivortex (V-Av) molecules match the sample symmetry, but are extremely sensitive to defects and fluctuations and remain undetected experimentally. Here we show that V-Av states can re-appear deep in the superconducting state due to an array of perforations in a polygonal setting, surrounding a central hole. Such states are no longer caused by the symmetry of the sample but rather by pinning itself, which prevents the vortex-antivortex annihilation. As a result, even micron-size, clearly spaced V-Av molecules can be stabilized in large mesoscopic samples.

cond-mat.supr-con↗

arXiv2008

Continuum versus discrete flux behaviour in large mesoscopic Bi(2)Sr(2)CaCu(2)O(8+delta) disks

Scanning Hall probe and local Hall magnetometry measurements have been used to investigate flux distributions in large mesoscopic superconducting disks with sizes that lie near the crossover between the bulk and mesoscopic vortex regimes. Results obtained by directly mapping the magnetic induction profiles of the disks at different applied fields can be quite successfully fitted to analytic models which assume a continuous distribution of flux in the sample. At low fields, however, we do observe clear signatures of the underlying discrete vortex structure and can resolve the characteristic mesoscopic compression of vortex clusters in increasing magnetic fields. Even at higher fields, where single vortex resolution is lost, we are still able to track configurational changes in the vortex patterns, since competing vortex orders impose unmistakable signatures on "local" magnetisation curves as a function of the applied field. Our observations are in excellent agreement with molecular dynamics numerical simulations which lead us to a natural definition of the lengthscale for the crossover between discrete and continuum behaviours in our system.

cond-mat.supr-con↗

arXiv2008

Fluxonic Cellular Automata

We formulate a new concept for computing with quantum cellular automata composed of arrays of nanostructured superconducting devices. The logic states are defined by the position of two trapped flux quanta (vortices) in a 2x2 blind-hole-matrix etched on a mesoscopic superconducting square. Such small computational unit-cells are well within reach of current fabrication technology. In an array of unit-cells, the vortex configuration of one cell influences the penetrating flux lines in the neighboring cell through the screening currents. Alternatively, in conjoined cells, the information transfer can be strengthened by the interactions between the supercurrents in adjacent cells. Here we present the functioning logic gates based on this fluxonic cellular automata (FCA), where the logic operations are verified through theoretical simulations performed in the framework of the time-dependent Ginzburg-Landau theory. The input signals are defined by current loops placed on top of the two diagonal blind holes of the input cell. For given current-polarization, external flux lines are attracted or repelled by the loops, forming the '0' or '1' configuration. The read-out technology may be chosen from a large variety of modern vortex imaging methods, transport and LDOS measurements.

cond-mat.supr-con↗

arXiv2005

Mesoscopic field and current compensator based on a hybrid superconductor-ferromagnet structure

A rather general enhancement of superconductivity is demonstrated in a hybrid structure consisting of submicron superconducting (SC) sample combined with an in-plane ferromagnet (FM). The superconducting state resists much higher applied magnetic fields for both perpendicular polarities, as applied field is screened by the FM. In addition, FM induces (in the perpendicular direction to its moment) two opposite current-flows in the SC plane, under and aside the magnet, respectively. Due to the compensation effects, superconductivity persists up to higher applied currents. With increasing current, the sample undergoes SC-"resistive"-normal state transitions through a mixture of vortex-antivortex and phase-slip phenomena.

cond-mat.supr-con↗

arXiv2005

Vortex-Antivortex Lattices in Superconducting Films with Magnetic Pinning Arrays

Novel vortex structures are found when a thin superconducting film (SC) is covered with a lattice of out-of-plane magnetized magnetic dots (MDs). The stray magnetic field of the dots confines the vortices to the MD regions, surrounded by antivortices which "crystallize" into regular lattices. First and second order transitions are found as magnetic array is made sparser or MD-magnetization larger. For sparse MD-arrays fractional vortex-antivortex states are formed, where the crystal-symmetry is combined with a non-uniform "charge" distribution. We demonstrate that due to the (anti)vortices and the supercurrents induced by the MDs, the critical current of the sample actually increases if exposed to a homogeneous external magnetic field, contrary to conventional SC behavior.

cond-mat.supr-con↗