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M. W. Wu

Publications and source records attributed to M. W. Wu.

At least 19 recordsLinked to original sources
arXiv2023

Diamagnetic property and optical absorption in conventional superconductors with magnetic impurities

By solving the renormalization of the $s$-$d$ interaction from magnetic impurities embeded in conventional superconductors at low concentration, we derive the macroscopic superconducting phase fluctuation and electromagnetic properties within the path-integral approach. It is found that there exist two superconducting phase modes, both exhibiting similar behaviors of the Nambu-Goldstone mode. The existence of two phase modes suggests that in addition to the conventional free Cooper pairs as in the BCS case, there emerges a small part of the localized Cooper pairs around magnetic impurities due to the quantum correlation by the $s$-$d$ interaction, acting as Josephson islands. The emerging impurity Shiba bands inside the superconducting gap then correspond to the excitations of the ground state of the localized Cooper pairs, associated with the breaking of these Cooper pairs. In the diamagnetic response, the state of the free Cooper pairs gives rise to the conventional real contribution in the generated supercurrent, whereas the one of the localized Cooper pairs results in an imaginary contribution, leading to the superconducting Friedel oscillation, i.e., oscillation in the decay of the vector potential in the Meissner effect. As for the optical absorption of a conventional superconductor lying in the anomalous-skin-effect region, it is found that besides the conventional interband transition of Bogoliubov quasiparticles as revealed by Mattis-Bardeen theory, there also exist the interband transition between the impurity Shiba bands as well as all interband transitions between Bogoliubov quasiparticle and impurity Shiba bands. These transitions exhibit clear and separate resonance characters, providing a feasible scheme for the experimental detection.

cond-mat.supr-con↗
arXiv2023

Optical response of Higgs mode in superconductors at clean limit: formulation through Eilenberger equation and Ginzburg-Landau Lagrangian

Both macroscopic Ginzburg-Landau Lagrangian and microscopic gauge-invariant kinetic equation suggest a finite Higgs-mode generation in the second-order optical response of superconductors at clean limit, whereas the previous derivations through the path-integral approach and Eilenberger equation within the Matsubara formalism failed to give such generation. The crucial treatment leading to this controversy lies at an artificial scheme that whether the external optical frequency is taken as continuous variable or bosonic Matsubara frequency to handle the gap dynamics within the Matsubara formalism. To resolve this issue, we derive the effective action of the superconducting gap near $T_c$ in the presence of the vector potential through the path-integral approach, to fill the long missing blank of the microscopic derivation of the Ginzburg-Landau Lagrangian in superconductors. It is shown that only by taking optical frequency as continuous variable within the Matsubara formalism, can one achieve the fundamental Ginzburg-Landau Lagrangian, and in particular, the finite Ginzburg-Landau kinetic term leads to a finite Higgs-mode generation at clean limit. To further eliminate the confusion of the Matsubara frequency through a separate framework, we apply the Eilenberger equation within the Keldysh formalism, which is totally irrelevant to the Matsubara space. By calculating the gap dynamics in the second-order response, it is analytically proved that the involved optical frequency is a continuous variable rather than bosonic Matsubara frequency, causing a finite Higgs-mode generation at clean limit.

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arXiv2022

Optical response of Higgs mode in superconductors at clean limit

The phenomenological Ginzburg-Landau theory and the charge conservation directly lead to the finite Higgs-mode generation and vanishing charge-density fluctuation in the second-order optical response of superconductors at clean limit. Nevertheless, recent microscopic theoretical studies of the second-order optical response, apart from the one through the gauge-invariant kinetic equation [Yang and Wu, Phys. Rev. B {\bf 100}, 104513 (2019)], have derived a vanishing Higgs-mode generation but finite charge-density fluctuation at clean limit. We resolve this controversy by re-examining the previous derivations with the vector potential alone within the path-integral and Eilenberger-equation approaches, and show that both previous derivations contain mathematical flaws. After fixing these flaws, a finite Higgs-mode generation through the drive effect of vector potential is derived at clean limit, exactly recovering the previous result from the gauge-invariant kinetic equation as well as Ginzburg-Landau theory. By further extending the path-integral approach to include electromagnetic effects from the scalar potential and phase mode, in the second-order response, a finite contribution from the drive effect of scalar potential to the Higgs-mode generation at clean limit as well as the vanishing charge-density fluctuation are derived, also recovering the results from the gauge-invariant kinetic equation. Particularly, we show that the phase mode is excited in the second-order response, and exactly cancels the previously reported unphysical excitation of the charge-density fluctuation, guaranteeing the charge conservation.

cond-mat.supr-con↗
arXiv2022

Impurity scattering in superconductors revisited

The diagrammatic formalism and transport equation are conventionally considered as separate but complementary techniques to tackle the impurity scattering effect. To compare with the previous studies from the gauge-invariant kinetic equation approach [F. Yang and M. W. Wu, Phys. Rev. B 98, 094507 (2018); 102, 144508 (2020)], we analytically perform a diagrammatic formulation of the impurity scattering in superconductors, with both transport and collective Higgs mode studied, in order to fill the long missing calculation of the Kubo current-current correlation in superconductors with impurity scattering and resolve the controversy (whether the impurity scattering can lead to the damping of Higgs mode) between gauge-invariant kinetic equation and Eilenberger equation. For transport behavior, through a special unitary transformation that is equivalent to the Wilson-line technique for the diamagnetic response, we derive the Meissner-supercurrent vertex. Then, by formulating the supercurrent-supercurrent correlation with Born and vertex corrections from impurity scattering, we recover the previously revealed microscopic momentum-relaxation rate of superfluid by gauge-invariant kinetic equation. This rate is finite only when the superconducting velocity is larger than a threshold, at which the normal fluid emerges and causes the friction with the superfluid current, similar to the Landau's superfluid theory of liquid helium. This derivation also provides a physical understanding of the relaxation-time approximation in the previous diagrammatic formulation in the literature, which leads to the friction resistance of the Meissner supercurrent. For the collective Higgs mode, we calculate the amplitude-amplitude correlation with Born and vertex corrections from impurity scattering. The vertex correction, which only emerges at nonequilibrium case, leads to a Higgs-mode damping, ......

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arXiv2021

A theory of coupled dual dynamics of macroscopic phase coherence and microscopic electronic fluids: effect of dephasing on cuprate superconductivity

By using the gauge-invariant kinetic equation approach [Yang and Wu, Phys. Rev. B {\bf 98}, 094507 (2018); {\bf 100}, 104513 (2019)], we construct the coupled dual dynamics of macroscopic phase coherence and microscopic electronic fluids in cuprate superconductors. We prove that the developed dual dynamics provides an efficient and simplified approach to formulate the dephasing process of macroscopic superconducting phase coherence, as well as its influence on microscopic electronic fluids (including gap, densities of superfluid and normal fluid, and in particular, the transport property to determine superconducting transition temperature $T_c$). We then present theoretical description of the preformed Cooper pairs in pseudogap state. The key origin of pseudogap state comes from the quantum effect of disorder, which excites the macroscopic inhomogeneous phase fluctuation through Josephson effect. Influenced by this phase fluctuation, there exist normal fluid and viscous superfluid below $T_c$ in cuprate superconductors, in addition to conventional non-viscous superfluid. The normal fluid always emerges around nodal points even at zero temperature, whereas the viscous superfluid emerges due to the friction between superfluid and normal fluid. Particularly, the non-viscous superfluid gets suppressed when the phase fluctuation is enhanced by increasing temperature, until vanishes at $T_c$. Then, the system enters the pseudogap state, showing the nonzero resistivity as well as the finite gap from the viscous superfluid. By further increasing temperature to $T^{\rm os}$, the viscous superfluid and hence gap vanish. An experimental scheme to distinguish the densities of normal fluid as well as viscous and non-viscous superfluids is proposed. Finally, this theory is also applied to low-dimensional disordered $s$-wave superconductors.

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arXiv2020

Theory of Higgs Modes in $d$-Wave Superconductors

By applying a microscopic gauge-invariant kinetic theory in $d$-wave superconductors, we analytically derive the energy spectra of the breathing Higgs mode and, in particular, rotating Higgs mode that is unique for the $d$-wave order parameter. Analytical investigation on their dynamic properties is also revealed. We show that the breathing Higgs mode is optically visible in the second-order regime. Whereas the rotating Higgs mode is optically inactive, we show that this mode can be detected in the pseudogap phase by magnetic resonance experiment. It is interesting to find that with a longitudinal temperature gradient, the charge-neutral rotating Higgs mode generates a thermal Hall current by magnetic field in the pseudogap phase, providing a unique scheme for its detection.

cond-mat.supr-con↗
arXiv2019

Influence of scattering on optical response of superconductivity

By using the gauge-invariant kinetic equation, we analytically investigate the influence of the scattering on the optical properties of superconductors in the normal-skin-effect region. Both linear and second-order responses are studied under a multi-cycle terahertz pulse. In the linear regime, we reveal that the optical absorption $σ_{1s}(ω)$, which origins from the scattering, exhibits a crossover point at $ω=2|Δ|$. Particularly, it is further shown that when $ω<2|Δ|$, $σ_{1s}(ω)$ from the scattering always exhibits a finite value even at low temperature, in contrast to the vanishing $σ_{1s}(ω)$ in the anomalous-skin-effect region as the Mattis-Bardeen theory revealed. In the second-order regime, responses of the Higgs mode during and after the optical pulse are studied. During the pulse, we show that the scattering causes a phase shift in the second-order response of the Higgs mode. Particularly, this phase shift exhibits a significant $π$-jump at $ω=|Δ|$, which provides a very clear feature for the experimental detection. After the pulse, by studying the damping of the Higgs-mode excitation, we reveal a relaxation mechanism from the elastic scattering, which shows a monotonic enhancement with the increase of the impurity density.

cond-mat.supr-con↗
arXiv2018

Gauge-invariant microscopic kinetic theory of superconductivity: application to electromagnetic response of Nambu-Goldstone and Higgs modes

We show that the gauge-invariant kinetic equation of superconductivity provides an efficient approach to study the electromagnetic response of the gapless Nambu-Goldstone and gapful Higgs modes on an equal footing. We prove that the Fock energy in the kinetic equation is equivalent to the generalized Ward's identity. Hence, the gauge invariance directly leads to the charge conservation. Both linear and second-order responses are investigated. The linear response of the Higgs mode vanishes in the long-wave limit. Whereas the linear response of the Nambu-Goldstone mode interacts with the long-range Coulomb interaction, causing the original gapless spectrum lifted up to the plasma frequency as a result of the Anderson-Higgs mechanism, in consistency with the previous works. The second-order response exhibits interesting physics. On one hand, a finite second-order response of the Higgs mode is obtained in the long-wave limit. We reveal that this response, which has been experimentally observed, is attributed solely to the drive effect rather than the widely considered Anderson-pump effect. On the other hand, the second-order response of the Nambu-Goldstone mode, free from the influence of the long-range Coulomb interaction and hence the Anderson-Higgs mechanism, is predicted. We find that both Anderson-pump and drive effects play important role in this response. A tentative scheme to detect this second-order response is proposed.

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arXiv2018

Gauge-invariant microscopic kinetic theory of superconductivity in response to electromagnetic fields

Within a gauge-invariant microscopic kinetic theory, we study the electromagnetic response in the superconducting states. Both superfluid and normal-fluid dynamics are involved. We predict that the normal fluid is present only when the excited superconducting velocity $v_s$ is larger than a threshold $v_L=|Δ|/k_F$. Interestingly, with the normal fluid, we find that there exists friction between the normal-fluid and superfluid currents. Due to this friction, part of the superfluid becomes viscous. Therefore, a three-fluid model: normal fluid, non-viscous and viscous superfluids, is proposed. For the stationary magnetic response, at $v_s<v_L$ with only the non-viscous superfluid, the Meissner supercurrent is excited and the gap equation can reduce to Ginzburg-Landau equation. At $v_s{\ge}v_L$, with the normal fluid, non-viscous and viscous superfluids, in addition to the directly excited Meissner supercurrent in the superfluid, normal-fluid current is also induced through the friction drag with the viscous superfluid current. Due to the normal-fluid and viscous superfluid currents, the penetration depth is influenced by the scattering effect. In addition, a modified Ginzburg-Landau equation is proposed. We predict an exotic phase in which both the resistivity and superconducting gap are {\em finite}. As for the optical response, the excited ${v_s}$ oscillates with time. When $v_s<v_L$, only the non-viscous superfluid is present whereas at $v_s{\ge}v_L$, normal fluid, non-viscous and viscous superfluids are present. We show that the excited normal-fluid current exhibits the Drude-model behavior while the superfluid current consists of the Meissner supercurrent and Bogoliubov quasiparticle current. Due to the friction between the superfluid and normal-fluid currents, the optical conductivity is captured by the three-fluid model. ......

cond-mat.supr-con↗
arXiv2018

Anomalous Hall effect in semiconductor quantum wells in proximity to chiral p-wave superconductors

By using the gauge-invariant optical Bloch equation, we perform a microscopic kinetic investigation on the anomalous Hall effect in chiral p-wave superconducting states. Specifically, the intrinsic anomalous Hall conductivity in the absence of the magnetic field is zero as a consequence of Galilean invariance in our description. As for the extrinsic channel, a finite anomalous Hall current is obtained from the impurity scattering with the optically excited normal quasiparticle current even at zero temperature. From our kinetic description, it can be clearly seen that the excited normal quasiparticle current is due to an induced center-of-mass momentum of Cooper pairs through the acceleration driven by ac electric field. For the induced anomalous Hall current, we show that the conventional skew-scattering channel in the linear response makes the dominant contribution in the strong impurity interaction. In this case, our kinetic description as a supplementary viewpoint mostly confirms the results of Kubo formalism in the literature. Nevertheless, in the weak impurity interaction, this skew-scattering channel becomes marginal and we reveal that a novel induction channel from the Born contribution dominates the anomalous Hall current. This novel channel, which has long been overlooked in the literature, is due to the particle-hole asymmetry by nonlinear optical excitation. Finally, we study the case in the chiral p-wave superconducting state with a transverse conical magnetization, which breaks the Galilean invariance. In this situation, the intrinsic anomalous Hall conductivity is no longer zero. Comparison of this intrinsic channel with the extrinsic one from impurity scattering is addressed.

cond-mat.supr-con↗
arXiv2017

Gauge-invariant theory of optical response to THz pulses in s-wave and ($s$+$p$)-wave superconducting semiconductor quantum wells

We investigate the optical response to the THz pulses in the s-wave and ($s$+$p$)-wave superconducting semiconductor quantum wells by using the gauge-invariant optical Bloch equations, in which the gauge structure in the superconductivity is explicitly retained. By using the gauge transformation, not only can the microscopic description for the quasiparticle dynamics be realized, but also the dynamics of the condensate is included, with the superfluid velocity and the effective chemical potential naturally incorporated. We reveal that the superfluid velocity itself can contribute to the pump of quasiparticles (pump effect), with its rate of change acting as the drive field to drive the quasiparticles (drive effect). Specifically, the drive effect can contribute to the formation of the blocking region for the quasiparticle, which directly suppresses the anomalous correlation of the Cooper pairs. We find that both the pump and drive effects contribute to the oscillations of the Higgs mode with twice the frequency of the optical field. However, it is shown that the contribution from the drive effect to the excitation of Higgs mode is dominant as long as the driven superconducting momentum is less than the Fermi momentum. This is in contrast to the conclusion from the Liouville or Bloch equations in the literature, in which the drive effect on the anomalous correlation is overlooked with only the pump effect considered.Furthermore, in the gauge-invariant optical Bloch equations, the charge neutrality condition is {\em consistently} considered based on the two-component model for the charge, in which the charge imbalance of quasiparticles can cause the fluctuation of the effective chemical potential. ......

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arXiv2017

Fulde-Ferrell-Larkin-Ovchinnikov state in spin-orbit-coupled superconductors

We show that in the presence of magnetic field, two superconducting phases with the center-of-mass momentum of Cooper pair parallel to the magnetic field are induced in spin-orbit-coupled superconductor Li$_2$Pd$_3$B. Specifically, at small magnetic field, the center-of-mass momentum is induced due to the energy-spectrum distortion and no unpairing region with vanishing singlet correlation appears. We refer to this superconducting state as the drift-BCS state. By further increasing the magnetic field, the superconducting state falls into the Fulde-Ferrell-Larkin-Ovchinnikov state with the emergence of the unpairing regions. The observed abrupt enhancement of the center-of-mass momenta and suppression on the order parameters during the crossover indicate the first-order phase transition. Enhanced Pauli limit and hence enlarged magnetic-field regime of the Fulde-Ferrell-Larkin-Ovchinnikov state, due to the spin-flip terms of the spin-orbit coupling, are revealed. We also address the triplet correlations induced by the spin-orbit coupling, and show that the Cooper-pair spin polarizations, generated by the magnetic field and center-of-mass momentum with the triplet correlations, exhibit totally different magnetic-field dependences between the drift-BCS and Fulde-Ferrell-Larkin-Ovchinnikov states.

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arXiv2017

Gapped superconductivity with all symmetries in InSb (110) quantum wells in proximity to s-wave superconductor in Fulde-Ferrell-Larkin-Ovchinnikov phase or with a supercurrent

We show that all the singlet even-frequency, singlet odd-frequency, triplet even-frequency and triplet odd-frequency pairings, and together with the corresponding order parameters (gaps) can be realized in InSb (110) spin-orbit-coupled quantum well in proximity to s-wave superconductor in Fulde-Ferrell-Larkin-Ovchinnikov phase or with a supercurrent. It is revealed that with the singlet even-frequency order parameter induced by the proximity effect, triplet even-frequency pairing is induced due to the broken spin-rotational symmetry by the spin-orbit coupling. Since the translational symmetry is broken by the center-of-mass momentum of Cooper pair in the Fulde-Ferrell-Larkin-Ovchinnikov phase or with a supercurrent, the singlet odd-frequency pairing can be induced. With the translational and spin-rotational asymmetries, the triplet odd-frequency pairing is also realized. Then, we show that the corresponding order parameters can be obtained from the self-energy of the electron-electron Coulomb interaction with the dynamic screening. The singlet and the induced triplet even-frequency order parameters are found to exhibit the conventional s-wave and p-wave characters in the momentum space, respectively. Whereas for the induced odd-frequency order parameters in quantum well, the singlet and triplet ones show the p-wave and d-wave characters, respectively. Moreover, the p-wave character of the singlet odd-frequency order parameter exhibits anisotropy with respect to the direction of the center-of-mass momentum. While for the triplet one, we find that $d_{x^2}$-wave and $d_{xy}$-wave characters can be obtained with respect to the direction of the center-of-mass momentum. ......

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arXiv2016

A novel superconducting-velocity--tunable quasiparticle state and spin relaxation in GaAs (100) quantum wells in proximity to $s$-wave superconductor

We present a novel quasiparticle state driven by a supercurrent in GaAs (100) quantum wells in proximity to an $s$-wave superconductor, which can be tuned by the superconducting velocity. Rich features such as the suppressed Cooper pairings, large quasiparticle density and non-monotonically tunable momentum current can be realized by varying the superconducting velocity. In the degenerate regime, the quasiparticle Fermi surface is composed by two arcs, referred to as Fermi arcs, which are contributed by the electron- and hole-like branches. The D'yakonov-Perel' spin relaxation is explored, and intriguing physics is revealed when the Fermi arc emerges. Specifically, when the order parameter tends to zero, it is found that the branch-mixing scattering is forbidden in the quasi-electron band. When the condensation process associated with the annihilation of the quasi-electron and quasi-hole is {\em slow}, this indicates that the electron- and hole-like Fermi arcs in the quasi-electron band are independent. The open structure of the Fermi arc leads to the nonzero angular-average of the effective magnetic field due to the spin-orbit coupling, which acts as an effective Zeeman field. This Zeeman field leads to the spin oscillations even in the strong scattering regime. Moreover, in the strong scattering regime, we show that the open structure of the Fermi arc also leads to the insensitiveness of the spin relaxation to the momentum scattering, in contrast to the conventional motional narrowing situation. Nevertheless, with a {\em finite} order parameter, the branch-mixing scattering can be triggered, opening the inter-branch spin relaxation channel, which is dominant in the strong scattering regime. In contrast to the situation with an extremely small order parameter,....(omitted due to the limit of space)

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arXiv2016

Spin diffusion in p-type bilayer WSe$_2$

We investigate the steady-state out-of-plane spin diffusion in p-type bilayer WSe2 in the presence of the Rashba spin-orbit coupling and Hartree-Fock effective magnetic field. The out-of-plane components of the Rashba spin-orbit coupling serve as the opposite Zeeman-like fields in the two valleys. Together with the identical Hartree-Fock effective magnetic fields, different total effective magnetic field strengths in the two valleys are obtained. It is further revealed that due to the valley-dependent total effective magnetic field strength, similar (different) spin-diffusion lengths in the two valleys are observed at small (large) spin injection. Nevertheless, it is shown that the intervalley hole-phonon scattering can suppress the difference in the spin-diffusion lengths at large spin injection due to the spin-conserving intervalley charge transfers with the opposite transfer directions between spin-up and -down holes. Moreover, with a fixed large pure spin injection, we predict the build-up of a steady-state valley polarization during the spin diffusion with the maximum along the diffusion direction being capable of exceeding 1 %. It is revealed that the valley polarization arises from the induced quasi hot-hole Fermi distributions with different effective hot-hole temperatures between spin-up and -down holes during the spin diffusion, leading to the different intervalley charge transfer rates in the opposite transfer directions. Additionally, it is also shown that by increasing the injected spin polarization, the hole density or the impurity density, the larger valley polarization can be obtained.

cond-mat.mes-hall↗
arXiv2016

Gapped triplet $p$-wave superconductivity in strong spin-orbit-coupled semiconductor quantum wells in proximity to $s$-wave superconductor

We show that the {\it gapped} triplet superconductivity, i.e., a triplet superconductor with triplet order parameter, can be realized in strong spin-orbit-coupled quantum wells in proximity to $s$-wave superconductor. It is revealed that with the singlet order parameter induced from the superconducting proximity effect, in quantum wells, not only can the triplet pairings arise due to the spin-orbit coupling, but also the triplet order parameter can be induced due to the repulsive effective electron-electron interaction, including the electron-electron Coulomb and electron-phonon interactions. This is a natural extension of the work of de Gennes, in which the repulsive-interaction-induced singlet order parameter arises in the normal metal in proximity to $s$-wave superconductor [Rev. Mod. Phys. {\bf 36}, 225 (1964)]. Specifically, we derive the effective Bogoliubov-de Gennes equation, in which the self-energies due to the effective electron-electron interactions contribute to the singlet and triplet order parameters. It is further shown that for the singlet order parameter, it is efficiently suppressed due to this self-energy renormalization; whereas for the triplet order parameter, it is the $p$-wave ($p_x\pm ip_y$) one with the ${\bf d}$-vector parallel to the effective magnetic field due to the spin-orbit coupling. Finally, we perform the numerical calculation in InSb (100) quantum wells. Specifically, we reveal that the Coulomb interaction is much more important than the electron-phonon interaction at low temperature. Moreover, it shows that with proper electron density, the minimum of the renormalized singlet and the maximum of the induced triplet order parameters are comparable, and hence can be experimentally distinguished.

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arXiv2016

Topological superconductor with a large Chern number and a large bulk excitation gap in single layer graphene

We show that a two-dimensional topological superconductor (TSC) can be realized in a hybrid system with a conventional $s$-wave superconductor proximity-coupled to a quantum anomalous Hall (QAH) state from the Rashba and exchange effects in single layer graphene. With very low or even zero doping near the Dirac points, i.e., two inequivalent valleys, this TSC has a Chern number as large as four, which supports four Majorana edge modes. More importantly, we show that this TSC has a robust topologically nontrivial bulk excitation gap, which can be larger or even one order of magnitude larger than the proximity-induced superconducting gap. This unique property paves a way for the application of QAH insulators as seed materials to realize robust TSCs and Majorana modes.

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