arXiv subjects

M. Wada

Publications and source records attributed to M. Wada.

At least 19 recordsLinked to original sources

arXiv2026

A diagnostic system of 5.7 keV muon beam for muon accelerator

Realization of a low-emittance muon beam through the acceleration of keV-scale muons requires the injection of a suitably matched beam into an accelerator, since beam mismatch can lead to emittance growth and reduced acceleration efficiency. In one such scheme, muons are first thermalized to room temperature and then injected into a linear accelerator. Non-destructive diagnostics are challenging because of the low energy and low intensity. We developed a compact low-energy muon diagnostic system compatible with the accelerator under construction at J-PARC. The system is designed to evaluate beam conditions required for precise tuning prior to acceleration. Commissioning with low-energy muon sources shows the system's capability to identify low-energy muon signals and measure beam profiles.

physics.acc-ph↗

arXiv2026

Search for two-neutrino double electron capture in $^{36}$Ar with the DarkSide-50 detector

Two-neutrino double electron capture is a rare nuclear decay where two electrons are simultaneously captured from the atomic shells and two neutrinos are emitted. We report on the first search for two-neutrino double electron capture in the $\textit{KK}$- and $\textit{KL}$-shells of $^{36}$Ar using the low-radioactivity liquid argon target from underground sources in the DarkSide-50 experiment. No statistically significant excess was observed with approximately 12 ton-day exposure of underground argon (UAr) and, taking into account the $^{36}$Ar isotopic abundance in UAr (0.007%), we set a limit on the half-life of the two-electron capture process in $^{36}$Ar of $T_{1/2} > 9.2 \times 10^{19}$ yr at 90% C.L. The sensitivity of the DarkSide-20k experiment, which will become operational in the next few years, was also evaluated and is expected to increase by a factor $\sim$100 with 10 years of expected operation and assuming the same $^{36}$Ar abundance as in the DarkSide-50 underground argon target.

nucl-ex↗

arXiv2026

High-Precision Mass Measurements of Proton-Rich Rh, Pd, Cd isotopes in the vicinity of 100Sn and Impact on X-Ray Burst and Supernova Nucleosynthesis

Using the ZeroDegree multi-reflection time-of-flight mass spectrograph of the CRISMASS project at RIKEN Radioactive Isotope Beam Factory, we performed high-precision mass measurements of proton-rich nuclei near the doubly magic nucleus 100Sn, achieving uncertainties on the order of 10 keV. The masses of 91Rh, 92Pd, and 96Cd were determined for the first time with high precision, and the accuracy of several additional masses was substantially improved. Incorporating the new data into X-ray burst simulations significantly reduces the abundance uncertainties in the $A$ = 90-100 region, shifting the reaction flow toward $A$ = 90 production and suppressing the synthesis of heavier nuclei. Further investigation of the $\nu p$-process indicates that 99Rh plays a significant role in the reaction flow within the mass region studied. These high-precision mass measurements refine the mass surface near 100Sn and provide critical constraints on models of proton-rich nucleosynthesis.

nucl-ex↗

arXiv2026

Characterization of argon recoils at the keV scale with ReD and ReD+

The ReD experiment measured the ionization yield Qy of argon for nuclear recoils in the 2-10 keV range using a dual-phase Time Projection Chamber irradiated with neutrons from a Cf-252 fission source. The measurement extends coverage below 7 keV, confirms consistency with previous data above 7 keV, and indicates a higher Qy at lower energies. These results are relevant for argon-based experiments searching for dark matter in the form of low-mass Weakly Interacting Massive Particles, which are very sensitive to the modeling of the detector response in this energy range.

hep-ex↗

arXiv2025

New Ground State in ${}^{149}$La Removes Two-Neutron-Separation-Energy Anomaly in Lanthanum Isotopes

Nuclear mass is a key indicator of how the nuclear shell structure evolves. The recent mass measurement study of neutron-rich lanthanum isotopes [A. Jaries, $et~al$., Phys. Rev. Lett. {\bf 134}, 042501(2025)] reveals the presence of a distinct prominence in their two-neutron separation energies. However, its presence has been called into question based on the results of another mass determination [B. Liu, Ph.D. thesis, University of Notre Dame (2025)]. In this letter, we report an effort to clarify these contradictory results through the use of the simultaneous mass-lifetime measurement of the neutron-rich lanthanum isotope ${}^{149}$La using a multi-reflection time-of-flight mass spectrograph combined with a $\beta$-TOF detector. The peak corresponding to a $\beta$-decaying state was observed in the time-of-flight spectra at a position of $221(6)~{\rm keV/c^2}$ lighter than the reported ${}^{149}$La mass in A. Jaries, $et~al$., but our measured result is in excellent agreement with the mass value reported in B. Liu. We have concluded that this peak is the ground state of ${}^{149}$La. With this, the previously reported distinct prominence in the two-neutron separation energies disappears, while a new kink structure, similar to that in the cerium isotopes, appears. Comparison with theoretical models suggests that a nuclear shape transition from octupole deformation to another type of deformation occurs around $N=91$ and is likely the cause of this kink structure.

nucl-ex↗

arXiv2025

Characterization of the ionization response of argon to nuclear recoils at the keV scale with the ReD experiment

In the recent years, argon-based experiments looking for Dark Matter in the Universe have explored the non-standard scenario in which Dark Matter is made by low-mass Weakly Interacting Massive Particles, of mass in the range of 1-10 GeV instead of the canonical hundreds of GeV. Detecting such particles is challenging, as their expected signatures are nuclear recoils with energies below 10 keV, observable solely via ionization. This necessitates a precise understanding of the detector response in this energy regime, which remains incomplete for argon. To address this, the ReD experiment was developed within the framework of the DarkSide-20k Collaboration to produce and characterize few-keV nuclear recoils. A compact dual-phase argon Time Projection Chamber (TPC) was irradiated with neutrons from a Cf252 source, to produce Ar recoils in the energy range of interest via (n,n') elastic scattering. A downstream spectrometer composed of 18 plastic scintillators detected the neutrons scattered off Ar nuclei, enabling recoil energy reconstruction via two-body kinematics. The ionization yield Qy of argon, defined as the number of electrons produced per unit energy deposit, was measured in a model-independent way between 2 and 10 keV. These measurements extend direct experimental coverage well below the previous limit of approximately 7 keV. The results are consistent with existing data above 7 keV, while they indicate a higher Qy at lower energies.

nucl-ex↗

arXiv2025

Precision mass measurements around ${}^{84}$Mo rule out ZrNb cycle formation in the rapid proton-capture process at type I X-ray bursts

The rapid proton-capture ($rp$-) process is one of the primary, explosive thermonuclear burning processes that drive type I X-ray bursts. A possible termination of the $rp$-process at around ${}^{84}$Mo was previously suggested by the formation of a ZrNb cycle. We report here precision mass measurements at around ${}^{84}$Mo, which have concluded the possibility of the cycle. The experiment was conducted using the multi-reflection time-of-flight spectrograph at RIKEN RI Beam Factory, and the masses of ${}^{79}$Y, ${}^{83}$Nb, ${}^{84}$Mo, ${}^{88}$Ru, and an isomer in ${}^{78}$Y were measured. For ${}^{84}$Mo, and ${}^{88}$Ru, and the isomeric state of ${}^{78}$Y, their masses are experimentally determined for the first time with uncertainties of $\delta m \approx 20~{\rm keV/c^2}$. The mass precision of ${}^{79}$Y and ${}^{83}$Nb is improved to $13~{\rm keV/c^2}$ and $9.6~{\rm keV/c^2}$, respectively. The new $\alpha$-separation energy of ${}^{84}$Mo, 1.434(83) MeV, unambiguously rules out the possibility of forming the ZrNb cycle. The X-ray burst simulation with the new masses shows that our measurements effectively remove the large final abundance uncertainties in the $A=80-90$ mass region. The new mass values improve the prediction power for the composition of the nuclear ashes in X-ray bursts.

nucl-ex↗

arXiv2025

Direct observation of $\beta$ and $\gamma$ decay from a high-spin long-lived isomer in $^{187}$Ta

$^{187}$Ta ($Z=73$, $N=114$) is located in the neutron-rich $A \approx 190$ region where a prolate-to-oblate shape transition via triaxial softness is predicted to take place. A preceding work on the $K^{\pi} = (25/2^-)$ isomer and a rotational band to which the isomer decays carried out by the same collaboration revealed that axial symmetry is slightly violated in this nucleus. This paper focuses on a higher-lying isomer, which was previously identified at 2933(14) keV by mass measurements with the Experimental Storage Ring at GSI. The isomer of interest has been populated by a multi-nucleon transfer reaction with a $^{136}$Xe primary beam incident on a natural tungsten target, using the KEK Isotope Separation System at RIKEN. New experimental findings obtained in the present paper include the internal and external $\beta$-decay branches from the high-spin isomer and a revised half-life of 136(24) s. The evaluated hindrances for $K$-forbidden transitions put constraints on the spin-parity assignment, which can be interpreted as being ascribed to a prolate shape with a five-quasiparticle configuration by model calculations.

nucl-ex↗

arXiv2024

Impact of extreme ultraviolet radiation on the scintillation of pure and xenon-doped liquid argon

The Xenon-Argon Technology (X-ArT) collaboration presents a study on the dynamics of pure and xenon-doped liquid argon (LAr) scintillation. Using two types of silicon photomultipliers sensitive to different wavelength ranges, we provide evidence in favor of a contribution from long-lived (>10 $\mu$s) extreme ultraviolet (EUV) lines emitted from argon atomic states, which enhances the light yield. This component is present in both pure and xenon-doped LAr, becoming more pronounced at higher xenon concentrations, where it complements the traditional collisional energy transfer process. To explain this mechanism, we develop a comprehensive model of the Xe-doped LAr scintillation process that integrates both collisional and radiative contributions. Additionally, we investigate how xenon doping affects LAr scintillation light yield and pulse shape discrimination. Finally, we hypothesize that the EUV component may explain the emission of spurious electrons, a known challenge in light dark matter searches using noble liquids. By characterizing the scintillation dynamics in Xe-doped LAr, identifying the long-lived EUV component, and exploring the potential origin of spurious electrons, this work lays the groundwork for optimizing detector performance and advancing the design and sensitivity of future noble liquid particle detectors.

hep-ex↗

arXiv2023

Increasing the rate capability for the cryogenic stopping cell of the FRS Ion Catcher

At the FRS Ion Catcher (FRS-IC), projectile and fission fragments are produced at relativistic energies, separated in-flight, energy-bunched, slowed down, and thermalized in the ultra-pure helium gas-filled cryogenic stopping cell (CSC). Thermalized nuclei are extracted from the CSC using a combination of DC and RF electric fields and gas flow. This CSC also serves as the prototype CSC for the Super-FRS, where exotic nuclei will be produced at unprecedented rates making it possible to go towards the extremes of the nuclear chart. Therefore, it is essential to efficiently extract thermalized exotic nuclei from the CSC under high beam rate conditions, in order to use the rare exotic nuclei which come as cocktail beams. The extraction efficiency dependence on the intensity of the impinging beam into the CSC was studied with a primary beam of 238U and its fragments. Tests were done with two different versions of the DC electrode structure inside the cryogenic chamber, the standard 1 m long and a short 0.5 m long DC electrode. In contrast to the rate capability of 10^4 ions/s with the long DC electrode, results show no extraction efficiency loss up to the rate of 2x10^5 ions/s with the new short DC electrode. This order of magnitude increase of the rate capability paves the way for new experiments at the FRS-IC, including exotic nuclei studies with in-cell multi-nucleon transfer reactions. The results further validate the design concept of the CSC for the Super-FRS, which was developed to effectively manage beams of even higher intensities.

physics.ins-det↗

arXiv2022

A new study of the $N=32$ and $N=34$ shell gap for Ti and V by the first high-precision MRTOF mass measurements at BigRIPS-SLOWRI

The atomic masses of $^{55}$Sc, $^{56,58}$Ti, and $^{56-59}$V have been determined using the high-precision multi-reflection time-of-flight technique. The radioisotopes have been produced at RIKEN's RIBF facility and delivered to the novel designed gas cell and multi-reflection system (ZD MRTOF), which has been recently commissioned downstream of the ZeroDegree spectrometer following the BigRIPS separator. For $^{56,58}$Ti and $^{56-59}$V the mass uncertainties have been reduced down to the order of $10\,\mathrm{keV}$, shedding new light on the $N=34$ shell effect in Ti and V isotopes by the first high-precision mass measurements of the critical species $^{58}$Ti and $^{59}$V. With the new precision achieved, we reveal the non-existence of the $N=34$ empirical two-neutron shell gaps for Ti and V, and the enhanced energy gap above the occupied $\nu p_{3/2}$ orbit is identified as a feature unique to Ca. We perform new Monte Carlo shell model calculations including the $\nu d_{5/2}$ and $\nu g_{9/2}$ orbits and compare the results with conventional shell model calculations, which exclude the $\nu g_{9/2}$ and the $\nu d_{5/2}$ orbits. The comparison indicates that the shell gap reduction in Ti is related to a partial occupation of the higher orbitals for the outer two valence neutrons at $N=34$.

nucl-ex↗

arXiv2021

The new MRTOF mass spectrograph following the ZeroDegree spectrometer at RIKEN's RIBF facility

A newly assembled multi-reflection time-of-flight mass spectrograph (MRTOF-MS) at RIKEN's RIBF facility became operational for the first time in spring 2020; further modifications and performance tests using stable ions were completed in early 2021. By using a pulsed-drift-tube technique to modify the ions' kinetic energy in a wide range, we directly characterize the dispersion function of the system for use in a new procedure for optimizing the voltages applied to the electrostatic mirrors. Thus far, a mass resolving power of $R_m > 1\,000\,000$ is reached within a total time-of-flight of only $12.5\,\mathrm{ms}$, making the spectrometer capable of studying short-lived nuclei possessing low-lying isomers. Detailed information about the setup and measurement procedure is reported, and an alternative in-MRTOF ion selection scheme to remove molecular contaminants in the absence of a dedicated deflection device is introduced. The setup underwent an initial on-line commissioning at the BigRIPS facility at the end of 2020, where more than 70 nuclear masses have been measured. A summary of the commissioning experiments and results from a test of mass accuracy will be presented.

physics.ins-det↗

arXiv2021

First direct observation of isomeric decay in neutron-rich odd-odd $^{186}$Ta

De-excitation $\gamma $ rays associated with an isomeric state of $^{186}$Ta were investigated. The isomers were produced in multinucleon transfer reactions between a $^{136}$Xe beam and a natural W target, and were collected and separated by the KEK Isotope Separation System. Two $\gamma $ transitions with energies of 161.1(2) and 186.8(1) keV associated with an isomeric decay were observed for the first time. The half-life of the isomeric state of the neutral atom $^{186 \rm m}$Ta was deduced as 17(2) s. Based on the comparison with the previous measurements of the isomeric state using the ESR storage ring at GSI Darmstadt and the coupling of angular momenta of individual particle orbitals in odd-odd nuclei, a decay scheme of $^{186 \rm m}$Ta was proposed.

nucl-ex↗

arXiv2021

Alpha-decay-correlated mass measurement of 206,207Ra using an $\alpha$-TOF detector equipped MRTOF-MS system

The atomic masses of the isotopes $^{206,207}$Ra have been measured via decay-correlated mass spectroscopy using a multi-reflection time-of-flight mass spectrograph equipped with an $\alpha$-TOF detector. The Ra isotopes were produced as fusion-evaporation products in the $^{51}$V+$^{159}$Tb reaction system and delivered by the gas-filled recoil ion separator GARIS-II at RIKEN. The $\alpha$-TOF detector provides for high-accuracy mass measurements by correlating time-of-flight signals with subsequent $\alpha$-decay events. The masses of $^{206}$Ra and $^{207g,m}$Ra were directly measured using a multi-reflection time-of-flight mass spectrograph equipped with an $\alpha$-TOF detector. A mass excess of ME = 3538(15) keV/c$^2$ and an excitation energy of E$_{\rm ex}$ = 552(42) keV were determined. The $\alpha$-decay branching ratio of $^{207m}$Ra, b$\alpha$ = 0.26(20), was directly determined from decay-correlated time-of-flight signals, and the reduced alpha width of $^{207m}$Ra was calculated to be $\delta^2$ = 50+62-41 keV from the branching ratio. The spin-parity of $^{207m}$Ra was confirmed to be $J^\pi$ = 13/2$^-$ from decay correlated mass measurement results.

nucl-ex↗

arXiv2021

Performance of the ReD TPC, a novel double-phase LAr detector with Silicon Photomultiplier Readout

A double-phase argon Time Projection Chamber (TPC), with an active mass of 185 g, has been designed and constructed for the Recoil Directionality (ReD) experiment. The aim of the ReD project is to investigate the directional sensitivity of argon-based TPCs via columnar recombination to nuclear recoils in the energy range of interest (20-200 keV$_{nr}$) for direct dark matter searches. The key novel feature of the ReD TPC is a readout system based on cryogenic Silicon Photomultipliers, which are employed and operated continuously for the first time in an argon TPC. Over the course of six months, the ReD TPC was commissioned and characterised under various operating conditions using $\gamma$-ray and neutron sources, demonstrating remarkable stability of the optical sensors and reproducibility of the results. The scintillation gain and ionisation amplification of the TPC were measured to be $g_1 = (0.194 \pm 0.013)$ PE/photon and $g_2 = (20.0 \pm 0.9)$ PE/electron, respectively. The ratio of the ionisation to scintillation signals (S2/S1), instrumental for the positive identification of a candidate directional signal induced by WIMPs, has been investigated for both nuclear and electron recoils. At a drift field of 183 V/cm, an S2/S1 dispersion of 12% was measured for nuclear recoils of approximately 60-90 keV$_{nr}$, as compared to 18% for electron recoils depositing 60 keV of energy. The detector performance reported here meets the requirements needed to achieve the principal scientific goals of the ReD experiment in the search for a directional effect due to columnar recombination. A phenomenological parameterisation of the recombination probability in LAr is presented and employed for modeling the dependence of scintillation quenching and charge yield on the drift field for electron recoils between 50-500 keV and fields up to 1000 V/cm.

physics.ins-det↗

arXiv2021

High sensitivity characterization of an ultra-high purity NaI(Tl) crystal scintillator with the SABRE proof-of-principle detector

We present new results on the radiopurity of a 3.4-kg NaI(Tl) crystal scintillator operated in the SABRE proof-of-principle detector setup. The amount of potassium contamination, determined by the direct counting of radioactive $^{40}$K, is found to be $2.2\pm1.5$ ppb, lowest ever achieved for NaI(Tl) crystals. With the active veto, the average background rate in the crystal in the 1-6 keV energy region-of-interest (ROI) is $1.20\pm0.05$ counts/day/kg/keV, which is a breakthrough since the DAMA/LIBRA experiment. Our background model indicates that the rate is dominated by $^{210}$Pb and that about half of this contamination is located in the PTFE reflector. We discuss ongoing developments of the crystal manufacture aimed at the further reduction of the background, including data from purification by zone refining. A projected background rate lower than $\sim$0.2 counts/day/kg/keV in the ROI is within reach. These results represent a benchmark for the development of next-generation NaI(Tl) detector arrays for the direct detection of dark matter particles.

physics.ins-det↗

arXiv2020

Characterization of SABRE crystal NaI-33 with direct underground counting

Ultra-pure NaI(Tl) crystals are the key element for a model-independent verification of the long standing DAMA result and a powerful means to search for the annual modulation signature of dark matter interactions. The SABRE collaboration has been developing cutting-edge techniques for the reduction of intrinsic backgrounds over several years. In this paper we report the first characterization of a 3.4 kg crystal, named NaI-33, performed in an underground passive shielding setup at LNGS. NaI-33 has a record low $^{39}$K contamination of 4.3$\pm$0.2 ppb as determined by mass spectrometry. We measured a light yield of 11.1$\pm$0.2 photoelectrons/keV and an energy resolution of 13.2% (FWHM/E) at 59.5 keV. We evaluated the activities of $^{226}$Ra and $^{228}$Th inside the crystal to be $5.9\pm0.6 \mu$Bq/kg and $1.6\pm0.3 \mu$Bq/kg, respectively, which would indicate a contamination from $^{238}$U and $^{232}$Th at part-per-trillion level. We measured an activity of 0.51$\pm$0.02 mBq/kg due to $^{210}$Pb out of equilibrium and a $\alpha$ quenching factor of 0.63$\pm$0.01 at 5304 keV. We illustrate the analyses techniques developed to reject electronic noise in the lower part of the energy spectrum. A cut-based strategy and a multivariate approach indicated a rate, attributed to the intrinsic radioactivity of the crystal, of $\sim$1 count/day/kg/keV in the [5-20] keV region.

physics.ins-det↗

arXiv2020

Properties of 187Ta revealed through isomeric decay

Mass-separated 187Ta in a high-spin isomeric state has been produced for the first time by multi-nucleon transfer reactions, employing an argon gas stopping cell and laser ionisation. Internal gamma rays revealed a 7.3 s isomer at 1778 keV, which decays through a rotational band with perturbations associated with the approach to a prolate-oblate shape transition. Model calculations show less influence from triaxiality compared to heavier elements in the same mass region. The isomer decay reduced E2 hindrance factor of 27 supports the interpretation that axial symmetry is approximately conserved.

nucl-ex↗