arXiv subjects

Marc Aßmann

Publications and source records attributed to Marc Aßmann.

36 records · Page 2Linked to original sources

arXiv2020

Formation dynamics of exciton polariton vortices created by non-resonant annular pumping

We study the spontaneous formation of exciton polariton vortices in an all-optical non-resonantly excited annular trap, which is formed by ring-shaped subpicosecond laser pulses. Since the light emitted by these vortices carries orbital angular momentum (OAM) corresponding to their topological charge, we apply a dedicated OAM spectroscopy technique to detect the OAM of the measurement signal with picosecond time resolution. This allows us to identify the formation of OAM modes and investigate the dynamics of the vortex formation process. We also study the power dependence of this process and how the ring diameter influences the formation of OAM modes.

physics.optics↗

arXiv2020

Conditional Spectroscopy via Non-Stationary Optical Homodyne Quantum State Tomography

Continuous variable quantum state tomography is one of the most powerful techniques to study the properties of light fields in quantum optics. However, the need for a fixed phase reference has so far prevented widespread usage in other fields such as semiconductor spectroscopy. Here, we introduce non-stationary quantum state tomography, which adapts the technique to the special requirements of ultrafast spectroscopy. In detail, we gain access to the amplitude and phase of light fields with a temporal resolution of about 100\,fs without the need for a fixed phase reference. Further, we show how our technique allows us to perform conditional studies of stochastic dynamics that are inaccessible experimentally by conventional means, and demonstrate the capabilities experimentally by monitoring the stochastic dynamics of a thermal light field on the sub-ps scale. Finally, we discuss differences and similarities to more standard Hanbury Brown-Twiss photon correlation experiments, which may be considered as the discrete variable analogues of our technique.

physics.optics↗

arXiv2019

An eavesdropping attack on a trusted continuous-variable quantum random number generator

Harnessing quantum processes is an efficient method to generate truly indeterministic random numbers, which are of fundamental importance for cryptographic protocols, security applications or Monte-Carlo simulations. Recently, quantum random number generators based on continuous variables have gathered a lot of attention due to the potentially high bit rates they can deliver. Especially quadrature measurements on shot-noise limited states have been studied in detail as they do not offer any side information to potential adversaries under ideal experimental conditions. However, they may be subject to additional classical noise beyond the quantum limit, which may become a source of side information for eavesdroppers. While such eavesdropping attacks have been investigated in theory in some detail, experimental studies are still rare. We experimentally realize a continuous variable eavesdropping attack, based on heterodyne detection, on a trusted quantum random number generator and discuss the limitations for secure random number generation that arise.

quant-ph↗

arXiv2019

Tracking Dark Excitons with Exciton Polaritons in Semiconductor Microcavities

Dark excitons are of fundamental importance for a wide variety of processes in semiconductors, but are difficult to investigate using optical techniques due to their weak interaction with light fields. We reveal and characterize dark excitons injected by non-resonant pulsed excitation in a semiconductor microcavity structure containing InGaAs/GaAs quantum wells by monitoring their interactions with the bright lower polariton mode. We find a surprisingly long dark exciton lifetime of more than 20 ns which is longer than the time delay between two consecutive pulses. This creates a memory effect that we clearly observe through the variation of the time-resolved transmission signal. We propose a rate equation model that provides a quantitative agreement with the experimental data.

cond-mat.mes-hall↗

arXiv2018

Spectroscopy of fractional orbital angular momentum states

We present an approach for measuring the orbital angular momentum (OAM) of light tailored towards applications in spectroscopy and non-integer OAM values. It is based on the OAM sorting method (Berkhout et al., Phys. Rev. Lett. 105, 153601 (2010)). We demonstrate that mixed OAM states and fractional OAM states can be identified using moments of the sorted output intensity distribution and OAM states with integer and non-integer topological charge can be clearly distinguished. Furthermore the difference between intrinsic OAM and total OAM for fractional OAM states is highlighted and the importance of the orientation of the fractional OAM beam is shown. All experimental results show good agreement with simulations. Finally we discuss possible applications of this method for spectroscopy of semiconductor systems such as exciton-polaritons in microcavities.

physics.optics↗

arXiv2018

Magneto-Stark-effect of yellow excitons in cuprous oxide

We investigate and compare experimental and numerical excitonic spectra of the yellow series in cuprous oxide Cu$_2$O in the Voigt configuration and thus partially extend the results from Schweiner et al. [Phys. Rev. B 95, 035202 (2017)], who only considered the Faraday configuration. The main difference between the configurations is given by an additional effective electric field in the Voigt configuration, caused by the motion of the exciton through the magnetic field. This Magneto-Stark effect was already postulated by Gross et al. and Thomas et al. in 1961 [Sov. Phys. Solid State 3, 221 (1961); Phys. Rev. 124, 657 (1961)]. Group theoretical considerations show that the field most of all significantly increases the number of allowed lines by decreasing the symmetry of the system. This conclusion is supported by both the experimental and numerical data.

cond-mat.mtrl-sci↗

arXiv2018

Dephasing of InAs quantum dot p-shell excitons using two-dimensional coherent spectroscopy

The dephasing mechanisms of p-shell and s-shell excitons in an InAs self-assembled quantum dot ensemble are examined using two-dimensional coherent spectroscopy (2DCS). 2DCS provides a comprehensive picture of how the energy level structure of dots affects the exciton dephasing rates and recombination lifetimes. We find that at low temperatures, dephasing of s-shell excitons is lifetime limited, whereas p-shell excitons exhibit significant pure dephasing due to scattering between degenerate spin states. At elevated temperatures, quadratic exciton-phonon coupling plays an important role in both s-shell and p-shell exciton dephasing. We show that multiple p-shell states are also responsible for stronger phonon dephasing for these transitions

cond-mat.mes-hall↗

arXiv2018

Real time $g^{(2)}$ monitoring at 100 kHz

We introduce a technique to determine photon correlations of optical light fields in real time. The method is based on ultrafast phase-randomized homodyne detection and allows us to follow the temporal evolution of the second-order correlation function $g^{(2)}(0)$ of a light field. We demonstrate the capabilities of our approach by applying it to a laser diode operated in the threshold region. In particular, we are able to monitor the emission dynamics of the diode switching back and forth between lasing and spontaneous emission with a $g^{(2)}(0)$-sampling rate of 100 kHz.

physics.ins-det↗

arXiv2017

Dynamics of the Optical Spin Hall Effect

We study the time evolution of the Optical Spin Hall Effect (OSHE), which occurs when exciton-polaritons undergo resonant Rayleigh scattering. The resulting spin pattern in momentum space is quantified by calculating the degree of circular polarization of the momentum space image for each point in time. We find the degree of circular polarization performing oscillations, which can be described within the framework of the pseudospin model by Kavokin et al. (Ref. 1).

cond-mat.mes-hall↗

arXiv2017

Streak-camera measurements of single photons at telecom wavelength

Up to this point streak-cameras have been a powerful tool for temporal characterization of ultrafast light pulses even at the single photon level. However, the low signal-to-noise ratio in the infrared range prevents measurement on weak light sources in the telecom regime. We present an approach to circumvent this problem. The method utilizes an up-conversion process in periodically poled waveguides in Lithium Niobate. We convert single photons from a parametric down-conversion source in order to reach the point of maximum detection efficiency of commercially available streak-cameras. We explore phase-matching configurations to investigate the up-conversion scheme in real-world applications.

quant-ph↗

arXiv2016

Magnetoexcitons in cuprous oxide

Two of the most striking experimental findings when investigating exciton spectra in cuprous oxide using high-resolution spectroscopy are the observability and the fine structure splitting of $F$ excitons reported by J. Thewes et al. [Phys. Rev. Lett. 115, 027402 (2015)]. These findings show that it is indispensable to account for the complex valence band structure and the cubic symmetry of the solid in the theory of excitons. This is all the more important for magnetoexcitons, where the external magnetic field reduces the symmetry of the system even further. We present the theory of excitons in $\mathrm{Cu_{2}O}$ in an external magnetic field and especially discuss the dependence of the spectra on the direction of the external magnetic field, which cannot be understood from a simple hydrogen-like model. Using high-resolution spectroscopy, we also present the corresponding experimental spectra for cuprous oxide in Faraday configuration. The theoretical results and experimental spectra are in excellent agreement as regards not only the energies but also the relative oscillator strengths. Furthermore, this comparison allows for the determination of the fourth Luttinger parameter $κ$ of this semiconductor.

cond-mat.mtrl-sci↗

arXiv2016

Deviations of the exciton level spectrum in cuprous oxide from the hydrogen series

Recent high-resolution absorption spectroscopy on excited excitons in cuprous oxide [Nature (London) 514, 343 (2014)] has revealed significant deviations of their spectrum from that of the ideal hydrogen-like series. Here we show that the complex band dispersion of the crystal, which determines the kinetic energy of electrons and holes, strongly affects the exciton binding energy. Specifically, we show that the nonparabolicity of the band dispersion is the main cause of the deviation from the hydrogen series. Experimental data collected from high-resolution absorption spectroscopy in electric fields validate the assignment of the deviation to the nonparabolicity of the band dispersion.

cond-mat.mes-hall↗

arXiv2016

Experimental realization of a polariton beam amplifier

In this report we demonstrate a novel concept for a planar cavity polariton beam amplifier using non-resonant excitation. In contrast to resonant excitation schemes, background carriers are injected which form excitons, providing both gain and a repulsive potential for a polariton condensate. Using an attractive potential environment induced by a locally elongated cavity layer, the repulsive potential of the injected background carriers is compensated and a significant amplification of polariton beams is achieved without beam distortion.

cond-mat.mes-hall↗

arXiv2015

All-optical flow control of a polariton condensate using non-resonant excitation

The precise adjustment of the polariton condensate flow under incoherent excitation conditions is an indispensable prerequisite for polariton-based logic gate operations. In this report, an all-optical approach for steering the motion of a polariton condensate using only non-resonant excitation is demonstrated. We create arbitrarily shaped functional potentials by means of a spatial light modulator, which allow for tailoring the condensate state and guiding a propagating condensate along reconfigurable pathways. Additional numerical simulations confirm the experimental observations and elucidate the interaction effects between background carriers and polariton condensates.

cond-mat.mes-hall↗

arXiv2014

Nonlinear spectroscopy of exciton-polaritons in a GaAs-based microcavity

We present a systematic investigation of two-photon excitation processes in a GaAs-based microcavity in the strong-coupling regime. We observe second harmonic generation resonant to the upper and lower polariton level, which exhibits a strong dependence on the photonic fraction of the corresponding polariton. In addition we have performed two-photon excitation spectroscopy to identify $2p$ exciton states which are crucial for the operation as a terahertz lasing device, which was suggested recently [A. V. Kavokin et al., Phys. Rev. Lett. \textbf{108}, 197401 (2012)]. However, no distinct signatures of a $2p$ exciton state could be identified, which indicates a low two-photon pumping efficiency.

cond-mat.mes-hall↗

arXiv2014

Influence of interactions with non-condensed particles on the coherence of a 1D polariton condensate

One-dimensional polariton condensates (PoCos) in a photonic wire are generated through non-resonant laser excitation, by which also a reservoir of background carriers is created. Interaction with this reservoir may affect the coherence of the PoCo, which is studied here by injecting a condensate locally and monitoring the coherence along the wire. While the incoherent reservoir is mostly present within the excitation laser spot, the condensate can propagate ballistically through the wire. Photon correlation measurements show that far from the laser spot the second order correlation function approaches unity value, as expected for the coherent condensed state. When approaching the spot, however, the correlation function increases up to values of 1.2 showing the addition of noise to the emission due to interaction with the reservoir. This finding is substantiated by measuring the first order coherence by a double slit experiment, which shows a reduced visibility of interference at the excitation laser spot.

cond-mat.mes-hall↗

arXiv2013

Compressive adaptive computational ghost imaging

Compressive sensing is considered a huge breakthrough in signal acquisition. It allows recording an image consisting of $N^2$ pixels using much fewer than $N^2$ measurements if it can be transformed to a basis where most pixels take on negligibly small values. Standard compressive sensing techniques suffer from the computational overhead needed to reconstruct an image with typical computation times between hours and days and are thus not optimal for applications in physics and spectroscopy. We demonstrate an adaptive compressive sampling technique that performs measurements directly in a sparse basis. It needs much fewer than $N^2$ measurements without any computational overhead, so the result is available instantly.

physics.optics↗

arXiv2011

Distinguishing photon and polariton lasing from GaAs microcavities by spectral and temporal analysis of the two-threshold behavior

We compare polariton lasing with photon lasing of a planar GaAs/GaAlAs microcavity with zero detuning between the bare cavity mode and the bare exciton mode. For the emission from the lower energy-momentum dispersion branch we find a two-threshold behavior of the ground state in the input-output curve where each transition is accompanied by characteristic changes of the in-plane mode dispersion. In particular, we show that the thresholds are unambiguously evidenced in the photon statistics of the emission based on the second-order correlation function. Moreover, the distinct two-threshold behavior is confirmed in the evolution of the emission pulse duration.

cond-mat.quant-gas↗