arXiv subjects

Marco Polini

Publications and source records attributed to Marco Polini.

At least 73 records · Page 4Linked to original sources

arXiv2020

Phonon-mediated superconductivity in strongly correlated electron systems: a Luttinger-Ward functional approach

We use a Luttinger-Ward functional approach to study the problem of phonon-mediated superconductivity in electron systems with strong electron-electron interactions (EEIs). Our derivation does not rely on an expansion in skeleton diagrams for the EEI and the resulting theory is therefore nonperturbative in the strength of the latter. We show that one of the building blocks of the theory is the irreducible six-leg vertex related to EEIs. Diagrammatically, this implies five contributions (one of the Fock and four of the Hartree type) to the electronic self-energy, which, to the best of our knowledge, have never been discussed in the literature. Our approach is applicable to (and in fact designed to tackle superconductivity in) strongly correlated electron systems described by generic lattice models, as long as the glue for electron pairing is provided by phonons.

cond-mat.supr-con↗

arXiv2019

Collective excitations in twisted bilayer graphene close to the magic angle

The electronic properties of twisted bilayer graphene (TBG) can be dramatically different from those of a single graphene layer, in particular when the two layers are rotated relative to each other by a small angle. TBG has recently attracted a great deal of interest, sparked by the discovery of correlated insulating and superconducting states, for twist angle $θ$ close to a so-called 'magic angle' $\approx 1.1°$. In this work, we unveil, via near-field optical microscopy, a collective plasmon mode in charge-neutral TBG near the magic angle, which is dramatically different from the ordinary single-layer graphene intraband plasmon. In selected regions of our samples, we find a gapped collective mode with linear dispersion, akin to the bulk magnetoplasmons of a two-dimensional (2D) electron gas. We interpret these as interband plasmons and associate those with the optical transitions between quasi-localized states originating from the moiré superlattice. Surprisingly, we find a higher plasmon group velocity than expected, which implies an enhanced strength of the corresponding optical transition. This points to a weaker interlayer coupling in the AA regions. These intriguing optical properties offer new insights, complementary to other techniques, on the carrier dynamics in this novel quantum electron system.

cond-mat.str-el↗

arXiv2019

Dielectric function and plasmons of doped three-dimensional Luttinger semimetals

Luttinger semimetals are three-dimensional electron systems with a parabolic band touching and an effective total spin $J=3/2$. In this paper, we present an analytical theory of dielectric screening of inversion-symmetric Luttinger semimetals with an arbitrary carrier density and conduction-valence effective mass asymmetry. Assuming a spherical approximation for the single-particle Luttinger Hamiltonian, we determine analytically the dielectric screening function in the random phase approximation for arbitrary values of the wave vector and frequency, the latter in the complex plane. We use this analytical expression to calculate the dispersion relation and Landau damping of the collective modes in the charge sector (i.e., plasmons).

cond-mat.str-el↗

arXiv2019

Viscous electron fluids

Recent advances in materials science have made it possible to achieve conditions under which electrons in metals start behaving as highly viscous fluids, "thicker than honey", and exhibit fascinating hydrodynamic effects. In this short review we provide a popular introduction to the emerging field of electron hydrodynamics.

cond-mat.str-el↗

arXiv2019

Many-body localized quantum batteries

The collective and quantum behavior of many-body systems may be harnessed to achieve fast charging of energy storage devices, which have been recently dubbed quantum batteries. In this paper, we present an extensive numerical analysis of energy flow in a quantum battery described by a disordered quantum Ising chain Hamiltonian, whose equilibrium phase diagram presents many-body localized (MBL), Anderson localized (AL), and ergodic phases. We demonstrate that i) the low amount of entanglement of the MBL phase guarantees much better work extraction capabilities than the ergodic phase and ii) interactions suppress temporal energy fluctuations in comparison with those of the non-interacting AL phase. Finally, we show that the statistical distribution of values of the optimal charging time is a clear-cut diagnostic tool of the MBL phase.

cond-mat.mes-hall↗

arXiv2019

Discrete-time construction of nonequilibrium path integrals on the Kostantinov-Perel' time contour

Rigorous nonequilibrium actions for the many-body problem are usually derived by means of path integrals combined with a discrete temporal mesh on the Schwinger-Keldysh time contour. The latter suffers from a fundamental limitation: the initial state on this contour cannot be arbitrary, but necessarily needs to be described by a non-interacting density matrix, while interactions are switched on adiabatically. The Kostantinov-Perel' contour overcomes these and other limitations, allowing generic initial-state preparations. In this Article, we apply the technique of the discrete temporal mesh to rigorously build the nonequilibrium path integral on the Kostantinov-Perel' time contour.

cond-mat.str-el↗

arXiv2019

Electronic structure and magnetic properties of few-layer Cr$_2$Ge$_2$Te$_6$: the key role of nonlocal electron-electron interaction effects

Atomically-thin magnetic crystals have been recently isolated experimentally, greatly expanding the family of two-dimensional materials. In this Article we present an extensive comparative analysis of the electronic and magnetic properties of ${\rm Cr}_2{\rm Ge}_2{\rm Te}_6$, based on density functional theory (DFT). We first show that the often-used ${\rm DFT}+U$ approaches fail in predicting the ground-state properties of this material in both its monolayer and bilayer forms, and even more spectacularly in its bulk form. In the latter case, the fundamental gap {\it decreases} by increasing the Hubbard-$U$ parameter, eventually leading to a metallic ground state for physically relevant values of $U$, in stark contrast with experimental data. On the contrary, the use of hybrid functionals, which naturally take into account nonlocal exchange interactions between all orbitals, yields good account of the available ARPES experimental data. We then calculate all the relevant exchange couplings (and the magneto-crystalline anisotropy energy) for monolayer, bilayer, and bulk ${\rm Cr}_2{\rm Ge}_2{\rm Te}_6$ with a hybrid functional, with super-cells containing up to $270$ atoms, commenting on existing calculations with much smaller super-cell sizes. In the case of bilayer ${\rm Cr}_2{\rm Ge}_2{\rm Te}_6$, we show that two distinct intra-layer second-neighbor exchange couplings emerge, a result which, to the best of our knowledge, has not been noticed in the literature.

cond-mat.str-el↗

arXiv2019

Quantum supercapacitors

Recently there has been a great deal of interest on the possibility to exploit quantum-mechanical effects to increase the performance of energy storage systems. Here we introduce and solve a model of a quantum supercapacitor. This consists of two chains, one containing electrons and the other one holes, hosted by arrays of double quantum dots, the latter being a building block of experimental architectures for realizing charge and spin qubits. The two chains are in close proximity and embedded in the same photonic cavity, which is responsible for long-range coupling between all the qubits, in the same spirit of the Dicke model. By employing a variational approach, we find the phase diagram of the model, which displays ferromagnetic and antiferromagnetic phases for suitable pseudospin degrees of freedom, together with phases characterized by collective superradiant behavior. Importantly, we show that when transitioning from the ferro/antiferromagnetic to the superradiant phase, the quantum capacitance of the model is greatly enhanced. Our work offers opportunities for the experimental realization of a novel class of quantum supercapacitors with an enhanced storing power stemming from exquisite quantum mechanical effects.

cond-mat.mes-hall↗

arXiv2019

Extractable work, the role of correlations, and asymptotic freedom in quantum batteries

We investigate a quantum battery made of N two-level systems, which is charged by an optical mode via an energy-conserving interaction. We quantify the fraction E(N) of energy stored in the B battery that can be extracted in order to perform thermodynamic work. We first demonstrate that E(N) is highly reduced by the presence of correlations between the charger and the battery or B between the two-level systems composing the battery. We then show that the correlation-induced suppression of extractable energy, however, can be mitigated by preparing the charger in a coherent optical state. We conclude by proving that the charger-battery system is asymptotically free of such locking correlations in the N \to \infty limit.

quant-ph↗

arXiv2019

Magnetic hallmarks of viscous electron flow in graphene

We propose a protocol to identify spatial hallmarks of viscous electron flow in graphene and other two-dimensional viscous electron fluids. We predict that the profile of the magnetic field generated by hydrodynamic electron currents flowing in confined geometries displays unambiguous features linked to whirlpools and backflow near current injectors. We also show that the same profile sheds light on the nature of the boundary conditions describing friction exerted on the electron fluid by the edges of the sample. Our predictions are within reach of vector magnetometry based on nitrogen-vacancy centers embedded in a diamond slab mounted onto a graphene layer.

cond-mat.mes-hall↗

arXiv2019

Pseudo-Euler equations from nonlinear optics: plasmon-assisted photodetection beyond hydrodynamics

A great deal of theoretical and experimental efforts have been devoted in the last decades to the study of long-wavelength photodetection mechanisms in field-effect transistors hosting two-dimensional (2D) electron systems. A particularly interesting subclass of these mechanisms is intrinsic and based on the conversion of the incoming electromagnetic radiation into plasmons, which resonantly enhance the photoresponse, and subsequent rectification via hydrodynamic nonlinearities. In this Article we show that such conversion and subsequent rectification occur well beyond the frequency regime in which hydrodynamic theory applies. We consider the nonlinear optical response of generic 2D electron systems and derive pseudo-Euler equations of motion for suitable collective variables. These are solved in one- and two-dimensional geometries for the case of graphene and the results are compared with those of hydrodynamic theory. Significant qualitative differences are found, which are amenable to experimental studies. Our theory expands the knowledge of the fundamental physics behind long-wavelength photodetection.

cond-mat.mes-hall↗

arXiv2019

Failure of conductance quantization in two-dimensional topological insulators due to non-magnetic impurities

Despite topological protection and the absence of magnetic impurities, two-dimensional topological insulators display quantized conductance only in surprisingly short channels, which can be as short as 100 nm for atomically thin materials. We show that the combined action of short-range nonmagnetic impurities located near the edges and on site electron-electron interactions effectively creates noncollinear magnetic scatterers, and, hence, results in strong backscattering. The mechanism causes deviations from quantization even at zero temperature and for a modest strength of electron-electron interactions. Our theory provides a straightforward conceptual framework to explain experimental results, especially those in atomically thin crystals, plagued with short-range edge disorder.

cond-mat.mes-hall↗

arXiv2018

Acoustic plasmons at the crossover between the collisionless and hydrodynamic regimes in two-dimensional electron liquids

Hydrodynamic flow in two-dimensional electron systems has so far been probed only by dc transport and scanning gate microscopy measurements. In this work we discuss theoretically signatures of the hydrodynamic regime in near-field optical microscopy. We analyze the dispersion of acoustic plasmon modes in two-dimensional electron liquids using a non-local conductivity that takes into account the effects of (momentum-conserving) electron-electron collisions, (momentum-relaxing) electron-phonon and electron-impurity collisions, and many-body interactions beyond the celebrated Random Phase Approximation. We derive the dispersion and, most importantly, the damping of acoustic plasmon modes and their coupling to a near-field probe, identifying key experimental signatures of the crossover between collisionless and hydrodynamic regimes.

cond-mat.mes-hall↗

arXiv2018

Scanning Gate Microscopy in a Viscous Electron Fluid

We measure transport through a Ga[Al]As heterostructure at temperatures between 0.1 K and 30 K. Increasing the temperature enhances the electron-electron scattering rate and viscous effects in the two-dimensional electron gas arise. To probe this regime we measure so-called vicinity voltages and use a voltage-biased scanning tip to induce a movable local perturbation. We find that the scanning gate images differentiate reliably between the different regimes of electron transport. Our data are in good agreement with recent theories for interacting electron liquids in the ballistic and viscous regimes stimulated by measurements in graphene. However, the range of temperatures and densities where viscous effects are observable in Ga[Al]As are very distinct from the graphene material system.

cond-mat.mes-hall↗

arXiv2018

Quantum versus classical many-body batteries

Quantum batteries are quantum mechanical systems with many degrees of freedom which can be used to store energy and that display fast charging. The physics behind fast charging is still unclear. Is this just due to the collective behavior of the underlying interacting many-body system or does it have its roots in the quantum mechanical nature of the system itself? In this work we address these questions by studying three examples of quantum-mechanical many-body batteries with rigorous classical analogs. We find that the answer is model dependent and, even within the same model, depends on the value of the coupling constant that controls the interaction between the charger and the battery itself.

quant-ph↗

arXiv2018

Charger-mediated energy transfer in exactly-solvable models for quantum batteries

We present a systematic analysis and classification of several models of quantum batteries involving different combinations of two level systems and quantum harmonic oscillators. In particular, we study energy transfer processes from a given quantum system, termed charger, to another one, i.e. the proper battery. In this setting, we analyze different figures of merit, including the charging time, the maximum energy transfer, and the average charging power. The role of coupling Hamiltonians which do not preserve the number of local excitations in the charger-battery system is clarified by properly accounting them in the global energy balance of the model.

quant-ph↗

arXiv2018

Electrical plasmon injection in double-layer graphene heterostructures

It is by now well established that high-quality graphene enables a gate-tunable low-loss plasmonic platform for the efficient confinement, enhancement, and manipulation of optical fields spanning a broad range of frequencies, from the mid infrared to the Terahertz domain. While all-electrical detection of graphene plasmons has been demonstrated, electrical plasmon injection (EPI), which is crucial to operate nanoplasmonic devices without the encumbrance of a far-field optical apparatus, remains elusive. In this work, we present a theory of EPI in double-layer graphene, where a vertical tunnel current excites acoustic and optical plasmon modes. We first calculate the power delivered by the applied inter-layer voltage bias into these collective modes. We then show that this system works also as a spectrally-resolved molecular sensor.

cond-mat.mes-hall↗

arXiv2018

Charger-mediated energy transfer for quantum batteries: an open system approach

The energy charging of a quantum battery is analyzed in an open quantum setting, where the interaction between the battery element and the external power source is mediated by an ancilla system (the quantum charger) that acts as a controllable switch. Different implementations are analyzed putting emphasis on the interplay between coherent energy pumping mechanisms and thermalization.

cond-mat.mes-hall↗